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| Open AccessDual-comb optomechanical spectroscopy
Spectroscopic gas sensing with high sensitivity and selectivity finds an increasing number of applications. Here, the authors report an approach to ultrasensitive multiplexed gas sensing by integrating dual-comb spectroscopy with cavity optomechanics.
- Xinyi Ren
- , Jin Pan
- & Heping Zeng
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| Open AccessDeep optoacoustic localization microangiography of ischemic stroke in mice
Optoacoustic super-resolution at millimeter-scale depths has been impeded by the strong background absorption from blood cells. Here, the authors use dichloromethane microdroplets with high optical absorption and demonstrate 3D microangiography of the mouse brain via optoacoustic localization.
- Xosé Luís Deán-Ben
- , Justine Robin
- & Daniel Razansky
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| Open AccessParallel interrogation of the chalcogenide-based micro-ring sensor array for photoacoustic tomography
The authors report a highly sensitive chalcogenide-based micro-ring sensor array for photoacoustic tomography and develops a compatible parallel interrogation means by synthesizing a digital optical frequency comb. Imaging is demonstrated on fast-moving objects, leaf veins, and live zebrafish.
- Jingshun Pan
- , Qiang Li
- & Zhaohui Li
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| Open AccessA photoacoustic patch for three-dimensional imaging of hemoglobin and core temperature
The authors present a wearable photoacoustic patch, which integrates laser diodes and piezoelectric transducers for three-dimensional imaging of hemoglobin and temperature in deep tissues.
- Xiaoxiang Gao
- , Xiangjun Chen
- & Sheng Xu
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| Open AccessOptical-resolution functional gastrointestinal photoacoustic endoscopy based on optical heterodyne detection of ultrasound
The authors developed an optical-fiber-based photoacoustic endoscope for gastroenterology. It can noninvasively view the internal vascular structures and visualize the hemodynamic response in a lesion.
- Yizhi Liang
- , Wubing Fu
- & Bai-Ou Guan
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| Open AccessFrequency wavelength multiplexed optoacoustic tomography
Optoacoustic imaging is mostly performed in the time domain. Here the authors demonstrate frequency wavelength multiplexed optoacoustic tomography that can operate at multiple wavelengths simultaneously and offers signal-to-noise ratio advantages over time domain methods.
- Antonios Stylogiannis
- , Ludwig Prade
- & Vasilis Ntziachristos
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| Open AccessOptomechanical crystal with bound states in the continuum
Unsuspended optomechanical systems might enable unique applications for quantum sensing and transduction. Here, the authors demonstrate a two-dimensional slab-on-substrate optomechanical crystal empowered by mechanical bound states in the continuum.
- Shengyan Liu
- , Hao Tong
- & Kejie Fang
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| Open AccessSilicon-photonics acoustic detector for optoacoustic micro-tomography
High-resolution photoacoustic tomography is challenging due to reduced efficiency of miniaturized piezoelectric elements. Here, the authors fabricate a miniaturized silicon-photonics acoustic detector coated with a sensitivity-enhancing elastomer, and demonstrate high-resolution in vivo imaging.
- Yoav Hazan
- , Ahiad Levi
- & Amir Rosenthal
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| Open AccessA H2O2-activatable nanoprobe for diagnosing interstitial cystitis and liver ischemia-reperfusion injury via multispectral optoacoustic tomography and NIR-II fluorescent imaging
Fluorescent imaging in the second biological window has advantages for in vivo applications. Here, the authors synthesise a molecular nanoprobe which activates upon binding H2O2, generating both strong fluorescent NIR-II emission and ultrasound signal for multi-mode imaging of inflammatory diseases.
- Junjie Chen
- , Longqi Chen
- & Yanli Zhao
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| Open AccessHigh spatiotemporal resolution optoacoustic sensing with photothermally induced acoustic vibrations in optical fibres
Optoacoustic sensing applications are limited by weak electrostrictive force. Here, the authors induce photothermally acoustic vibrations with a focused pulsed laser, and via scanning demonstrate sensing of acoustic impedance at 10 µm spatial resolution, allowing for visualisation of diffusion dynamics.
- Yizhi Liang
- , Huojiao Sun
- & Bai-Ou Guan
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| Open AccessPhoto-acoustic dual-frequency comb spectroscopy
Here, the authors show that the resolution and speed limitations in broadband photo-acoustic spectroscopy can be overcome by combining dual-comb spectroscopy with photo-acoustic detection. This enables broadband detection and allows for rapid and sensitive multi-species molecular analysis across all wavelengths of light.
- Thibault Wildi
- , Thibault Voumard
- & Tobias Herr
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Article
| Open AccessHybrid integrated photonics using bulk acoustic resonators
Here, the authors demonstrate acousto-optic modulation of silicon nitride microring resonators using high-overtone bulk acoustic wave resonances, allowing modulation in the GHz range via acoustic waves. As an application, an optical isolator is demonstrated with 17 dB non-reciprocity.
- Hao Tian
- , Junqiu Liu
- & Sunil A. Bhave
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Article
| Open AccessPushing the boundaries of optoacoustic microscopy by total impulse response characterization
Characterizing the total impulse response (TIR) of photoacoustic microscopes has been challenging due to difficulties distributing appropriate point sources. Here, the authors present a method for 3D generation of spatially-distributed optoacoustic point sources and show that subsequent TIR correction results in improved image quality.
- Markus Seeger
- , Dominik Soliman
- & Vasilis Ntziachristos
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Article
| Open AccessLarge non-thermal contribution to picosecond strain pulse generation using the photo-induced phase transition in VO2
Ultrafast driving of vanadium dioxide can induce a large structural phase transition, which can be used to generate picosecond strain pulses. Here the authors show that the photo-induced phase transition can contribute 0.45% strain without causing undesirable heating.
- Iaroslav A. Mogunov
- , Sergiy Lysenko
- & Alexandra M. Kalashnikova
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| Open AccessHigh-speed modulation of a terahertz quantum cascade laser by coherent acoustic phonon pulses
The typical electronic modulation of terahertz quantum cascade lasers is fundamentally limited at fast timescales by device properties. Here the authors propose and study an alternative, acoustic mechanism for modulating such THz QCLs at high speed.
- Aniela Dunn
- , Caroline Poyser
- & Anthony Kent
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| Open AccessActivatable probes for diagnosing and positioning liver injury and metastatic tumors by multispectral optoacoustic tomography
Optoacoustic tomography has great potential for medical diagnosis and preclinical research. Here they develop near infrared activatable xanthene-based optoacoustic probes for diagnosing and localizing drug-induced liver injury and metastasis in mouse models.
- Yinglong Wu
- , Shuailing Huang
- & Shuizhu Wu
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| Open AccessIsolated detection of elastic waves driven by the momentum of light
The exact mechanism of momentum conversion from light to an object has varied descriptions in the literature and experimental verifications are difficult. Here the authors do an in-depth experimental and numerical study of the momentum dynamics of elastic waves in a dielectric mirror hit by a pulsed laser beam.
- Tomaž Požar
- , Jernej Laloš
- & Nelson G. C. Astrath
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| Open AccessDistributed forward Brillouin sensor based on local light phase recovery
Conventional distributed Brillouin sensing allows real-time sampling at high spatial resolution, but is so far restricted to measuring quantities inside the fibre core. Here, Chow et al. demonstrate a distributed forward Brillouin sensor that is sensitive to quantities outside the fibre bulk.
- Desmond M. Chow
- , Zhisheng Yang
- & Luc Thévenaz
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| Open AccessDynamically induced robust phonon transport and chiral cooling in an optomechanical system
Chiral transport can provide robustness against disorder, resulting in improved resonant modes for sensing and metrology. Here, Kim et al. demonstrate chiral phonon transport, disorder suppression and anomalous cooling without damping in an asymmetrically-pumped optomechanical system.
- Seunghwi Kim
- , Xunnong Xu
- & Gaurav Bahl
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| Open AccessBeat frequency quartz-enhanced photoacoustic spectroscopy for fast and calibration-free continuous trace-gas monitoring
Quartz-enhanced photoacoustic spectroscopy is a sensitive gas detection method whereby radiation-induced sound waves from gas absorption are detected. Here, Wuet al. use the beat frequency between a modulated laser and a tuning fork resonance to increase sensitivity and avoid frequent calibrations.
- Hongpeng Wu
- , Lei Dong
- & Frank K. Tittel
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| Open AccessObservation of optomechanical buckling transitions
Optomechanical systems could form logic gates, but key requirements are two stable static states and the ability to switch between them. Here, the authors observe radiation-pressure induced buckling transitions in an optomechanical system, and control this transition by varying laser power and detuning.
- H. Xu
- , U. Kemiktarak
- & J. M. Taylor
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| Open AccessUltrafast acousto-optic mode conversion in optically birefringent ferroelectrics
Electrically driven acousto-optic light modulators are limited to frequencies of a few hundred megahertz and are typically no smaller than a few micrometres. Here, the authors demonstrate gigahertz acousto-optic conversion of light polarization in a region of a few nanometres using pulsed laser stimulation of a ferroelectric.
- Mariusz Lejman
- , Gwenaelle Vaudel
- & Pascal Ruello
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| Open AccessBrillouin scattering self-cancellation
The interaction between light and acoustic phonons is radically modified in sub-wavelength photonic structures. Here, the authors engineer the optical and acoustic modes to perfectly cancel the two interaction mechanisms—the photo-elastic and moving-boundary effects—which leads to Brillouin self-cancellation.
- O. Florez
- , P. F. Jarschel
- & P. Dainese
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| Open AccessFemtosecond electron imaging of defect-modulated phonon dynamics
Phonons—crystal lattice vibrations—interact with crystal defects on the nanometre spatial scale and femtosecond timescale. Here, the authors demonstrate direct, real-space imaging of the nucleation, emergence and dispersion of single-phonon wavefronts at individual atomic-scale defects in semiconductors.
- Daniel R. Cremons
- , Dayne A. Plemmons
- & David J. Flannigan
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| Open AccessPhotoacoustics of single laser-trapped nanodroplets for the direct observation of nanofocusing in aerosol photokinetics
Aerosol droplets have significant effects on atmospheric photochemistry, however measuring absorption from single droplets is a challenge. Here, the authors report a method to measure absorption of nanodroplets with attolitre sensitivity, showing rate enhancements for light focusing in photolysis reactions.
- Johannes W. Cremer
- , Klemens M. Thaler
- & Ruth Signorell
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| Open AccessDynamic acousto-optic control of a strongly coupled photonic molecule
Dynamic control of components is required for large-scale quantum photonic networks. Here, Kapfingeret al. show dynamic control of the interaction between two coupled photonic crystal nanocavities forming a photonic molecule. Tuning is achieved by using an electrically generated radio frequency surface acoustic wave.
- Stephan Kapfinger
- , Thorsten Reichert
- & Hubert J. Krenner
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Super-resolution photoacoustic imaging through a scattering wall
With wavefront shaping, imaging through scattering walls is possible, but this technique requires generating feedback from behind the wall. Here, Conkeyet al. use photoacoustic feedback for wavefront optimization for sub-acoustic resolution imaging behind a scattering wall with an improved signal-to-noise ratio.
- Donald B. Conkey
- , Antonio M. Caravaca-Aguirre
- & Rafael Piestun
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Tuning the acoustic frequency of a gold nanodisk through its adhesion layer
The mechanical properties of metal nanostructures depend on nature of the adhesion layer attaching it to a substrate. Chang et al.find that the properties of phonons in gold nanodisks vary with adhesion layer thickness, and that this response can act as a probe of the metallic composition of the disk.
- Wei-Shun Chang
- , Fangfang Wen
- & Stephan Link
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| Open AccessBrillouin-scattering-induced transparency and non-reciprocal light storage
Stimulated Brillouin scattering is a non-linear interaction that allows light to be stored as coherent acoustic waves. Here, the authors report on Brillouin scattering-induced transparency in an optical microresonator whose high quality allows for long-lifetime non-reciprocal light storage.
- Chun-Hua Dong
- , Zhen Shen
- & Guang-Can Guo
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Sub-optical wavelength acoustic wave modulation of integrated photonic resonators at microwave frequencies
Acousto-optic modulators use acoustic waves to control light on a chip. Here, the authors achieve modulation in nanophotonic resonators using microwave frequency surface acoustic waves with wavelength smaller than the optical wavelength towards highly integrated devices on silicon.
- Semere Ayalew Tadesse
- & Mo Li
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Giant ultrafast photo-induced shear strain in ferroelectric BiFeO3
The generation of strain in a material using light is of relevance for ultrasonic devices. Here, the authors observe a large, ultrafast photo-induced shear strain in BiFeO3at room temperature, suggesting promising uses of such oxides for high-frequency acoustic devices.
- Mariusz Lejman
- , Gwenaelle Vaudel
- & Pascal Ruello
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Ultrafast acousto-plasmonic control and sensing in complex nanostructures
The nanometre length scale of plasmonic structures leads to vibrational dynamics at high frequencies, which could be exploited for sensitive optical detectors. O'Brien et al. show that they can detect spatial properties of phonon modes in multimodal plasmonic structures, revealing complex nanomechanical dynamics.
- Kevin O’Brien
- , N. D. Lanzillotti-Kimura
- & Xiang Zhang
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| Open AccessPhotonic Aharonov–Bohm effect in photon–phonon interactions
The Aharonov–Bohm effect describes the influence of an electromagnetic vector potential on the phase of a charged particle. Here, Li et al.demonstrate that photon–phonon interactions can lead to the Aharonov–Bohm effect also for the electrically neutral photons.
- Enbang Li
- , Benjamin J. Eggleton
- & Shanhui Fan
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| Open AccessDynamics of a vertical cavity quantum cascade phonon laser structure
Phonon lasers are the acoustic equivalent to optical lasers. Here Maryam and colleagues study the dynamics of semiconductor phonon lasers operating in the terahertz frequency regime, and show that these dynamics are similar to that of comparable optical lasers.
- W. Maryam
- , A. V. Akimov
- & A. J. Kent
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Biomedical photoacoustics beyond thermal expansion using triggered nanodroplet vaporization for contrast-enhanced imaging
A dual-contrast agent has been developed for combined ultrasound and photoacoustic imaging. This agent uses vaporization for ultrasound contrast enhancement and photoacoustic signal generation, providing significantly higher signals than thermal expansion, the most commonly used photoacoustic mechanism.
- Katheryne Wilson
- , Kimberly Homan
- & Stanislav Emelianov