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| Open AccessQuantum phase transitions in highly crystalline two-dimensional superconductors
Superconductor-insulator transitions predominantly occur in highly disordered thin films. Here, Saito et al. report that a quantum metallic state transforms via the quantum Griffiths state to a weakly localized metal at high magnetic fields in a crystalline two-dimensional superconductor.
- Yu Saito
- , Tsutomu Nojima
- & Yoshihiro Iwasa
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Article
| Open AccessEvidence of a one-dimensional thermodynamic phase diagram for simple glass-formers
Glass formers show dynamics over a broad range of timescales, presenting a hurdle to understanding the glass transition. Here, the authors find that the dynamics of glass-forming liquids are governed by the same mechanisms over different timescales, effectively reducing the phase diagram from two to one dimension.
- H. W. Hansen
- , A. Sanz
- & K. Niss
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Article
| Open AccessAmorphous martensite in β-Ti alloys
Displacive martensitic transformations through lattice distortion usually involve a change from one crystal structure to another. Here however, the authors “melt” metastable Ti alloys during cooling and show that a martensitic transformation can lead to the formation of an intragranular amorphous phase.
- Long Zhang
- , Haifeng Zhang
- & Simon Pauly
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Article
| Open AccessMatched asymptotic solution for crease nucleation in soft solids
Our understanding of material instabilities in soft solids remains elusive mainly due to the mathematical challenges in capturing localised phenomena within nonlinear elastic materials. Ciarletta develops an analytical theory to describe the nucleation threshold of creases in agreement with experiments.
- P. Ciarletta
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Article
| Open AccessGeometric isotope effect of deuteration in a hydrogen-bonded host–guest crystal
Deuterating a hydrogen bond can change the bond’s geometry, a phenomenon known as the geometric isotope effect (GIE). Here, the authors find that a hydrogen-bonded host–guest crystal, imidazolium hydrogen terephthalate, exhibits significant GIE on its hydrogen bonds, changing its crystal phases and bulk dielectric properties.
- Chao Shi
- , Xi Zhang
- & Wen Zhang
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Article
| Open AccessMeasurements of growing surface tension of amorphous–amorphous interfaces on approaching the colloidal glass transition
The existence of interfaces, separating distinct relaxing regions, has been predicted in glass theory, but a direct proof remains challenging due to the amorphous nature of glasses. Ganapathi et al. identify and measure the surface tension of these interfaces in bulk supercooled colloidal liquids.
- Divya Ganapathi
- , K. Hima Nagamanasa
- & Rajesh Ganapathy
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Article
| Open AccessQuasi-continuous transition from a Fermi liquid to a spin liquid in κ-(ET)2Cu2(CN)3
Several organic materials exhibit spin liquid phases, which are predicted to host exotic spinon excitations that emerge from non-local quantum effects. Here, the authors identify a quasi-continuous phase transition in κ-(ET)2Cu2(CN)3 that may be associated with the presence of spinons.
- Tetsuya Furukawa
- , Kazuhiko Kobashi
- & Kazushi Kanoda
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| Open AccessAbnormal phase transition between two-dimensional high-density liquid crystal and low-density crystalline solid phases
Intermolecular interactions have a crucial role in the adsorption of molecules on a surface, however their role in promoting phase transitions is less well known. Here, the authors report an abnormal phase transition between a high-density liquid crystal and low-density solid in the case of carbon monoxide on Cu(111), driven by intermolecular interactions and entropy.
- Wenbin Li
- , Longjuan Kong
- & Lan Chen
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Article
| Open AccessExperimental evidence for bipolaron condensation as a mechanism for the metal-insulator transition in rare-earth nickelates
Rare-earth nickelates undergo a metal-to-insulator transition accompanied by the formation of ordered lattice distortions, but the role of the lattice in the metallic phase remains unclear. Here the authors provide evidence that the metal is a polaronic liquid that freezes into the insulating state.
- Jacob Shamblin
- , Maximilian Heres
- & Steven Johnston
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Article
| Open AccessMomentum-resolved observations of the phonon instability driving geometric improper ferroelectricity in yttrium manganite
The improper ferroelectric mechanism of YMnO3 has been difficult to observe directly but is important for understanding its other interesting properties such as multiferroicity. Bansal et al. use neutron scattering and ab initio calculations to show that phonons drive the transition, confirming earlier theories.
- Dipanshu Bansal
- , Jennifer L. Niedziela
- & Olivier Delaire
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Article
| Open AccessNear-field spectroscopic investigation of dual-band heavy fermion metamaterials
Understanding the electromagnetic responses at subwavelength scales is important for achieving tunability. Using a combination of the near-field and far-field spectroscopy, the authors demonstrate a heavy fermion metamaterial with tunable dual-band optical responses by selectively and separately modifying the 4f and 5d band electrons.
- Stephanie N. Gilbert Corder
- , Xinzhong Chen
- & Mengkun Liu
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Article
| Open AccessPre-critical fluctuations and what they disclose about heterogeneous crystal nucleation
Heterogeneous nucleation is a process that mediates the birth of many crystalline materials, but is not fully understood. Here, the authors show that the study of precritical cluster fluctuations paves new ways for the identification of polymorphism, polymorphic control and theoretical modeling.
- Martin Fitzner
- , Gabriele C. Sosso
- & Angelos Michaelides
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| Open AccessFrustration-driven C 4 symmetric order in a naturally-heterostructured superconductor Sr2VO3FeAs
Iron-based superconductors exhibit complex couplings between different electronic degrees of freedom, leading to unusual correlated phases. Ok et al. show that Sr2VO3FeAs develops a hidden order state due to frustrated interactions between the magnetic fluctuations of its SrVO3 and SrFeAs layers.
- Jong Mok Ok
- , S.-H. Baek
- & Jun Sung Kim
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Article
| Open AccessTailoring crystallization phases in metallic glass nanorods via nucleus starvation
Crystallising a bulk metallic glass usually results in separate phases. Here, the authors use metallic glass nanorods to show that as the sample size approaches the nucleation scale lengths, the crystallization behavior is dictated by the lack of nuclei and nanorods crystallise into a single phase.
- Sungwoo Sohn
- , Yujun Xie
- & Judy J. Cha
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Article
| Open AccessBending and breaking of stripes in a charge ordered manganite
Charge-lattice coupling plays a central role in the exotic behaviors of multiferroic complex oxides, such as manganites, however, obtaining a microscopic picture is challenging. Here, Savitzky et al. map periodic lattice displacement fields at the picometer scale to study local order-disorder competition.
- Benjamin H. Savitzky
- , Ismail El Baggari
- & Lena F. Kourkoutis
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Article
| Open AccessGiant barocaloric effects over a wide temperature range in superionic conductor AgI
Barocaloric materials offer promise in solid-state cooling devices, but few materials have been show to display giant barocaloric effects near room temperature. Here, the authors demonstrate that solid electrolyte AgI displays giant inverse barocaloric effects near its superionic phase transition at ~420 K.
- Araceli Aznar
- , Pol Lloveras
- & Lluís Mañosa
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Article
| Open AccessStructurally triggered metal-insulator transition in rare-earth nickelates
Applications of rare-earth nickelates are hampered by lack of global understanding of the interplay among various degrees of freedom. Here, Mercy et al. propose that the metal-insulator transition of nickelates arises from the softening of an oxygen breathing distortion, providing a united picture of electronic, structural and magnetic properties.
- Alain Mercy
- , Jordan Bieder
- & Philippe Ghosez
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Article
| Open AccessOptimal percolation on multiplex networks
Multiplex networks consist of a collection of interacting layers and occur in social and technological systems. Here Osat et al. investigate optimal percolation which relates to the process of optimally dismantling multiplex networks and show that simplified versions of this problem lead to error.
- Saeed Osat
- , Ali Faqeeh
- & Filippo Radicchi
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| Open AccessObservation of replica symmetry breaking in disordered nonlinear wave propagation
Replica symmetry breaking describes identical copies of a randomly interacting system exhibiting different dynamics. Here, Pierangeli et al. observe this critical phenomenon in the optical wave propagation inside a disordered nonlinear waveguide.
- Davide Pierangeli
- , Andrea Tavani
- & Eugenio DelRe
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| Open AccessOscillators that sync and swarm
Collective self-organized behavior can be observed in a variety of systems such as colloids and microswimmers. Here O’Keeffe et al. propose a model of oscillators which move in space and tend to synchronize with neighboring oscillators and outline five types of collective self-organized states.
- Kevin P. O’Keeffe
- , Hyunsuk Hong
- & Steven H. Strogatz
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Article
| Open AccessTime-resolved diffraction of shock-released SiO2 and diaplectic glass formation
Our understanding of shock metamorphism and thus the collision of planetary bodies is limited by a dependence on ex situ analyses. Here, the authors perform in situ analysis on shocked-produced densified glass and show that estimates of impactor size based on traditional techniques are likely inflated.
- A. E. Gleason
- , C. A. Bolme
- & W. L. Mao
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Article
| Open AccessGiant thermal expansion and α-precipitation pathways in Ti-alloys
Complex phase transformations in β-stabilised titanium alloys can dramatically change their α and β microstructures, providing tailorability for aerospace or biomaterial applications. Here the authors show that Ti-Nb alloys exhibit giant thermal expansions and identify two new pathways that lead to α phase formation.
- Matthias Bönisch
- , Ajit Panigrahi
- & Jürgen Eckert
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Article
| Open AccessThermodynamic signatures of the field-induced states of graphite
Previous transport studies of graphite in strong magnetic fields have found a sequence of phase transitions with a still unresolved microscopic origin. Here the authors present ultrasound measurements enabling sharper resolution and demonstrating the thermodynamic nature of these transitions.
- D. LeBoeuf
- , C. W. Rischau
- & B. Fauqué
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Article
| Open AccessCharge-density-wave order takes over antiferromagnetism in Bi2Sr2−x La x CuO6 superconductors
Whilst superconductivity usually appears when magnetic order is suppressed, the role of charge is less known. Here, Kawasaki et al. report a charge density wave (CDW) above the superconducting transition induced by an in-plane magnetic field in Bi2Sr2-x La x CuO6, with the CDW onset temperature scaling with the pseudogap temperature.
- S. Kawasaki
- , Z. Li
- & Guo-qing Zheng
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Article
| Open AccessTemporal profiles of avalanches on networks
Cascade propagation models represent a range of processes on networks, such as power-grid blackouts and epidemic outbreaks. Here the authors investigate temporal profiles of avalanches and show how nonsymmetric average avalanche shapes can occur at criticality.
- James P. Gleeson
- & Rick Durrett
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Article
| Open AccessAnomalous elastic properties across the γ to α volume collapse in cerium
The origin of the volume collapse of cerium, the only elemental metal with a critical point in the solid phase, remains elusive. Here the authors show that, near the critical point, the f-electrons make cerium lose its compressive strength while maintaining a finite shear strength—which makes cerium unexpectedly auxetic.
- Magnus J. Lipp
- , Zs. Jenei
- & W. J. Evans
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| Open AccessMaximizing T c by tuning nematicity and magnetism in FeSe1−x S x superconductors
The overlap between different phases has hindered the understanding of how each phase affects superconductivity in FeSe. Here, Matsuura et al. achieve a complete separation of non-magnetic nematic and antiferromagnetic phases for FeSe1-x S x , observing a tetragonal phase in between with a strikingly enhanced T c.
- K. Matsuura
- , Y. Mizukami
- & T. Shibauchi
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Article
| Open AccessTopologically frustrated ionisation in a water-ammonia ice mixture
Water and ammonia are major constituents of icy planet interiors, however their phase behaviour under extreme conditions remain relatively unknown. Here, the authors show that ammonia monohydrate transforms under pressure into an alloy composed of molecules as well as ions, owing to a topological frustration.
- C. Liu
- , A. Mafety
- & S. Ninet
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Article
| Open AccessRobust Bain distortion in the premartensite phase of a platinum-substituted Ni2MnGa magnetic shape memory alloy
In magnetic shape memory Heusler alloys, the premartensite phase is believed to be a precursor state of the martensite phase with preserved austenite phase symmetry. Here, the authors show that the premartensite is a stable phase with its own crystallographic symmetry resulting from the stepped growth of Bain distortions in the lattice.
- Sanjay Singh
- , B. Dutta
- & D. Pandey
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Article
| Open AccessTopological quantum phase transition from mirror to time reversal symmetry protected topological insulator
Transitions between topological phases of matter protected by different symmetries remain rare. Here, Mandal et al. report a quantum phase transition from a topological crystalline insulator to a Z2 topological insulator by doping Bi into Pb1-x Sn x Se (111) thin films.
- Partha S. Mandal
- , Gunther Springholz
- & Jaime Sánchez-Barriga
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Article
| Open AccessNanoscale control of competing interactions and geometrical frustration in a dipolar trident lattice
Artificial magnetic nanostructures enable the study of competing frustrated interactions with more control over the system parameters than is possible in magnetic materials. Farhan et al. present a two-dimensional lattice geometry where the frustration can be controlled by tuning the unit cell parameters.
- Alan Farhan
- , Charlotte F. Petersen
- & Sebastiaan van Dijken
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Article
| Open AccessCorrelated states in β-Li2IrO3 driven by applied magnetic fields
Materials with a Kitaev spin liquid ground state are sought after as models of quantum phases but candidates so far form either zig-zag or incommensurate magnetic order. Ruiz et al. find a crossover between these states in β-Li2IrO3 under weak magnetic fields, indicating strongly frustrated spin interactions.
- Alejandro Ruiz
- , Alex Frano
- & James G. Analytis
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Article
| Open AccessElectrical magnetochiral effect induced by chiral spin fluctuations
The magnetism-induced chirality in electron transportation is of fundamental importantance in condensed matter physics but the origin is still unclear. Here the authors demonstrate that the asymmetric electron scattering by chiral spin fluctuations can be the key to the electrical magnetochiral effect in MnSi.
- T. Yokouchi
- , N. Kanazawa
- & Y. Tokura
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| Open AccessAnalog quantum simulation of the Rabi model in the ultra-strong coupling regime
An analog quantum simulation scheme has been explored with a quantum hardware based on a superconducting circuit. Here the authors investigate the time evolution of the quantum Rabi model at ultra-strong coupling conditions, which is synthesized by slowing down the system dynamics in an effective frame.
- Jochen Braumüller
- , Michael Marthaler
- & Alexey V. Ustinov
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Article
| Open AccessAnomalous metallic behaviour in the doped spin liquid candidate κ-(ET)4Hg2.89Br8
It is expected that introducing charge carriers into an exotic quantum spin liquid state may lead to an unconventional metal but there are no clear realizations of a metallic spin liquid. Here, the authors present a spin liquid candidate that also shows evidence of strange metal behavior.
- Hiroshi Oike
- , Yuji Suzuki
- & Kazushi Kanoda
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Article
| Open AccessTricritical wings and modulated magnetic phases in LaCrGe3 under pressure
The study of phase transitions in quantum ferromagnets has shown that the approach to a continuous quantum ferromagnetic transition is typically interrupted by either a tricritical point or a new magnetic phase. Here the authors show that LaCrGe3 exhibits both these features in its phase diagram.
- Udhara S. Kaluarachchi
- , Sergey L. Bud’ko
- & Valentin Taufour
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Article
| Open AccessEmergence of charge density waves and a pseudogap in single-layer TiTe2
Due to reduced dimensionality, the properties of 2D materials are often different from their 3D counterparts. Here, the authors identify the emergence of a unique charge density wave (CDW) order in monolayer TiTe2 that challenges the current understanding of CDW formation.
- P. Chen
- , Woei Wu Pai
- & T.-C. Chiang
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Article
| Open AccessTunneling anisotropic magnetoresistance driven by magnetic phase transition
Tunneling anisotropic magnetoresistance is promising for next generation memory devices but limited by the low efficiency and functioning temperature. Here the authors achieved 20% tunneling anisotropic magnetoresistance at room temperature in magnetic tunnel junctions with one α′-FeRh magnetic electrode.
- X. Z. Chen
- , J. F. Feng
- & F. Pan
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Article
| Open AccessFermion-induced quantum critical points
Quantum phase transitions are governed by Landau-Ginzburg theory and the exceptions are rare. Here, Li et al. propose a type of Landau-forbidden quantum critical points induced by gapless fermions in two-dimensional Dirac semimetals.
- Zi-Xiang Li
- , Yi-Fan Jiang
- & Hong Yao
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Article
| Open AccessThree-dimensional imaging of vortex structure in a ferroelectric nanoparticle driven by an electric field
Imaging of topological states of matter such as vortex configurations has generally been limited to 2D surface effects. Here Karpov et al. study the volumetric structure and dynamics of a vortex core mediated by electric-field induced structural phase transition in a ferroelectric BaTiO3 nanoparticle.
- D. Karpov
- , Z. Liu
- & E. Fohtung
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Article
| Open AccessAtomic-resolution imaging of electrically induced oxygen vacancy migration and phase transformation in SrCoO2.5-σ
Information on how oxygen ions transport is crucial to understanding field-induced phase transformations in materials. Here, Zhang et al. directly image atomic-scale oxygen migration and the subsequent structural reconstruction in a SrCoO2.5-σ film in the presence of an electric field.
- Qinghua Zhang
- , Xu He
- & Ce-Wen Nan
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Article
| Open AccessPiezomagnetism and magnetoelastic memory in uranium dioxide
The nuclear fuel uranium dioxide is of intrinsic interest due to its industrial applications but it also exhibits intriguing electronic and magnetic properties. Here, the authors demonstrate how its complex magnetic structure and interactions give rise to a strong piezomagnetic effect.
- M. Jaime
- , A. Saul
- & K. Gofryk
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Article
| Open AccessUniversal features of amorphous plasticity
The universality class for plastic yield in amorphous materials remains controversial. Here authors present a tensorial mesoscale model that captures both complex shear patterns and avalanche scaling behaviour, which differs from mean-field models and suggests a distinct type of critical phenomenon.
- Zoe Budrikis
- , David Fernandez Castellanos
- & Stefano Zapperi
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Article
| Open AccessMicroscopic origins of the large piezoelectricity of leadfree (Ba,Ca)(Zr,Ti)O3
(Ba,Ca)(Zr,Ti)O3ceramics have attracted interest as lead-free materials with large piezoelectric responses. Here, the authors use an atomistic model to show the electromechanical properties are due to a complex microstructure and polarization fluctuations in the narrowly stable orthorhombic phase.
- Yousra Nahas
- , Alireza Akbarzadeh
- & L. Bellaiche
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Article
| Open AccessGroup additivity-Pourbaix diagrams advocate thermodynamically stable nanoscale clusters in aqueous environments
Aqueous clusters are important in a variety of biological and materials systems. Here Willset al. develop a theoretical approach based on a group additivity relationship which allows the evaluation of a wide range of clusters without the need of cumbersome ab initiocalculations.
- Lindsay A. Wills
- , Xiaohui Qu
- & Paul Ha-Yeon Cheong
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Article
| Open AccessImaging metal-like monoclinic phase stabilized by surface coordination effect in vanadium dioxide nanobeam
Identifying intermediates during phase transitions is critical for our understanding of correlated materials, but difficult to achieve experimentally. Here, the authors report a surface coordination route to stabilize and directly image a phase-transition intermediate during the metal-insulator transition in vanadium dioxide.
- Zejun Li
- , Jiajing Wu
- & Yi Xie
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Article
| Open AccessExperimental neutron scattering evidence for proton polaron in hydrated metal oxide proton conductors
Hydration of oxygen vacancies could form hydroxyl groups with interstitial structural protons. Here a quasi-elastic neutron scattering study reveals proton polarons in proton-conducting ceramic electrolytes, and the proton transport turns out to be a cooperative process.
- Artur Braun
- & Qianli Chen
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Article
| Open AccessParity-time-symmetric quantum critical phenomena
Parity-time (PT) symmetry has been mainly studied in optical and weakly interacting open quantum systems without many-body correlations. Here the authors show that in a strongly correlated many-body system the interplay between correlations and PT symmetry leads to the emergence of new critical phenomena.
- Yuto Ashida
- , Shunsuke Furukawa
- & Masahito Ueda
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| Open AccessInhomogeneous spatial distribution of the magnetic transition in an iron-rhodium thin film
Films of iron-rhodium alloy undergo a magnetic transition at 100°C, and so are attractive for applications, but a detailed understanding of the transition mechanism has not been achieved. Here, the authors use electron holography to quantitatively map the transition’s progress through the film depth.
- C. Gatel
- , B. Warot-Fonrose
- & M.J. Casanove