Featured
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Time-resolved compression of a capsule with a cone to high density for fast-ignition laser fusion
One of the challenges in fast-ignition fusion is to laser-compress an asymmetric cone-in-shell target to a density at which it can be ignited by a second laser. Theobald et al. report the achievement of areal densities in excess of 300 mg cm−2, to a point at which ignition might soon be possible.
- W. Theobald
- , A. A. Solodov
- & M. S. Wei
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Laser-induced porous graphene films from commercial polymers
The straightforward and scalable synthesis and patterning of graphene-based nanomaterials remains a technological challenge. Here, the authors use a CO2infrared laser, under ambient conditions, to directly produce and pattern porous graphene films with three-dimensional networks from commercial polymer films.
- Jian Lin
- , Zhiwei Peng
- & James M. Tour
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Bio-optimized energy transfer in densely packed fluorescent protein enables near-maximal luminescence and solid-state lasers
Mammalian and bacteria cells producing fluorescent proteins (FP) have been recently proposed as living sources of laser light. Here, Gather and Yun demonstrate efficient lasing in the solid state form of FPs and observed Förster resonance energy transfer between molecules in blends of different FPs.
- Malte C. Gather
- & Seok Hyun Yun
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Efficient and tuneable photoluminescent boehmite hybrid nanoplates lacking metal activator centres for single-phase white LEDs
One approach to making white light LEDs is to combine a phosphor material that emits light over a wide spectrum with a ultraviolet LED. Xue Bai et al.demonstrate an inexpensive boehmite hybrid phosphor that produces high-quality white light with high efficiency.
- Xue Bai
- , Gianvito Caputo
- & Nicola Pinna
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Wave–matter interactions in epsilon-and-mu-near-zero structures
Unusual effects arise when a material’s permittivity or permeability approach zero, a scenario that can be readily engineered in metamaterials. This study explores the regime wherein both these quantities go to zero and the electric and magnetic fields effectively decouple while remaining temporally dynamic.
- Ahmed M. Mahmoud
- & Nader Engheta
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Wavefront modulation and subwavelength diffractive acoustics with an acoustic metasurface
Metasurfaces are subwavelength structures that manipulate impinging waves into desired output waveforms, but building them for acoustic applications remains challenging. Exploiting tapered labyrinthine structures, Xie et al.present an acoustic metasurface that manipulates sound waves in a variety of ways.
- Yangbo Xie
- , Wenqi Wang
- & Steven A. Cummer
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Negative refraction of elastic waves at the deep-subwavelength scale in a single-phase metamaterial
Acoustic metamaterials passively manipulate sound waves propagating through them, which is attractive for applications. Zhu et al.present a single-phase metamaterial based on a microstructure with simultaneous translational and rotational resonances, enabling negative refraction at deep-subwavelength scales.
- R. Zhu
- , X. N. Liu
- & G. L. Huang
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Nondispersive optical activity of meshed helical metamaterials
Metamaterials manipulate light to deliver tailored optical functionalities, like nonlinearity and optical activity. By exploiting the Drude response and four-fold rotational symmetries, Park et al. show that meshed helical metallic structures can produce a strong and broadband nondispersive optical activity.
- Hyun Sung Park
- , Teun-Teun Kim
- & Bumki Min
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Silicon nanofin grating as a miniature chirality-distinguishing beam-splitter
There is a need for micro- and nanostructures capable of polarization control to cope with the increasing miniaturization of optics devices. Here, the authors propose a beam-splitter consisting of amorphous silicon nanofins on glass that reflect left- and right-circularly polarized light in different directions.
- Mohammadreza Khorasaninejad
- & Kenneth B. Crozier
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Electrically controlled one-way photon flow in plasmonic nanostructures
If photonics and electronics are to form hybrid information processing systems, it will be necessary to manipulate and isolate light electrically, over short distances. Davoyan and Engheta propose a route to achieve this in plasmonic waveguides by exploiting the magnetic field induced by a direct current.
- Artur Davoyan
- & Nader Engheta
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Enhanced acoustic sensing through wave compression and pressure amplification in anisotropic metamaterials
Acoustic sensors have myriad important applications, but they are limited by their pressure sensitivity. Chen et al.show how the use of graded anisotropic acoustic metamaterial structures can help overcome this by amplifying the acoustic waves via compression effects.
- Yongyao Chen
- , Haijun Liu
- & Miao Yu
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Highly efficient inverted polymer light-emitting diodes using surface modifications of ZnO layer
Light trapped in the active polymeric layer limits the total efficiency of polymer light-emitting diodes. Here, Lee et al.get round this bottleneck by enhancing light extraction in waveguide optical modes via ripple-shaped nanostructures that spontaneously form on ZnO electrode surfaces.
- Bo Ram Lee
- , Eui Dae Jung
- & Myoung Hoon Song
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Phosphorescent dye-based supramolecules for high-efficiency organic light-emitting diodes
The limit external quantum efficiency of organic LEDs based on isotropically oriented iridium complexes is believed to be around 30%. But Kim et al. show that the emission from these complexes is in fact anisotropic, enabling them to increase the external quantum efficiency of these devices to 36%.
- Kwon-Hyeon Kim
- , Sunghun Lee
- & Jang-Joo Kim
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| Open AccessMultiple intrinsically identical single-photon emitters in the solid state
In quantum optical technologies, identical emitters of indistinguishable single photons are difficult to realize due to the inherent dissimilarity of each emitting device. Here, Rogers et al.demonstrate a solid-state uniform single-photon source, which does not require external tuning of optical properties.
- L.J. Rogers
- , K.D. Jahnke
- & F. Jelezko
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Mechano-actuated ultrafast full-colour switching in layered photonic hydrogels
Photonic crystals used for many optical devices are the materials made of nanoscaled periodic structures that diffract light. Yue et al. design and fabricate a soft mechanochromic hydrogel that exhibits a fast colour switching rate at 0.1 ms in a full-colour band.
- Youfeng Yue
- , Takayuki Kurokawa
- & Jian Ping Gong
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Single-molecule electroluminescence and photoluminescence of polyfluorene unveils the photophysics behind the green emission band
Polyfluorenes emit blue light in organic light-emitting diodes, but their colour purity is always degraded by accompanied green emission band. Here, the authors investigate the physical origin of the green emission using electroluminescence and photoluminescence spectroscopy on a single-molecular level.
- Yoshihiro Honmou
- , Shuzo Hirata
- & Martin Vacha
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Efficient optical extraction of hot-carrier energy
The thermalization of high-energy photons limits the efficient conversion of photon energy in photovoltaic applications. Here, Saeed et al. consider optical extraction of the excess energy of hot carriers by emission of infrared photons, using erbium ions in combination with silicon nanocrystals.
- S. Saeed
- , E. M. L. D. de Jong
- & T. Gregorkiewicz
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Electrifying photonic metamaterials for tunable nonlinear optics
Active metamaterials provide tailored optical properties that can be tuned on-demand by an external stimulus. Kang et al. present a nonlinear metamaterial, based on a nanostructured metal film, exhibiting second harmonic generation and optical rectification that can be electrically controlled.
- Lei Kang
- , Yonghao Cui
- & Wenshan Cai
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Spontaneous chiral symmetry breaking in metamaterials
Spontaneous symmetry breaking is one of the unusual effects offered by nonlinear metamaterials. Here, the authors study this effect in chiral magnetoelastic metamaterials where the meta-molecules of opposite handedness are both electromagnetically and mechanically coupled.
- Mingkai Liu
- , David A. Powell
- & Yuri S. Kivshar
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Highly efficient non-rare-earth red emitting phosphor for warm white light-emitting diodes
Manganese-activated fluoride phosphors for high-efficacy warm white light-emitting diodes have been limited by low photoluminescence quantum yields. Here, Zhu et al.use an efficient cation exchange reaction to synthesize manganese phosphors with photoluminescence quantum yields as high as 98%.
- Haomiao Zhu
- , Chun Che Lin
- & Xueyuan Chen
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Ultrafast fluorescence imaging in vivo with conjugated polymer fluorophores in the second near-infrared window
In vivofluorescence imaging in the second near-infrared window allows high resolution and tissue penetration. Here, using conjugated polymers, the authors achieve imaging with high spatial and time resolutions capable of resolving mouse femoral artery blood-flow variations within a single cardiac cycle.
- Guosong Hong
- , Yingping Zou
- & Hongjie Dai
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Single-shot three-dimensional structure determination of nanocrystals with femtosecond X-ray free-electron laser pulses
Three-dimensional imaging is typically complex and time consuming. Here, the authors report the use of X-ray free-electron laser pulses for single-shot three-dimensional imaging of nanocrystals at ~5.5 nm resolution, using the symmetry in the nanocrystal and the curvature of the Ewald sphere.
- Rui Xu
- , Huaidong Jiang
- & Jianwei Miao
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Design amphiphilic dipolar π-systems for stimuli-responsive luminescent materials using metastable states
Some π-conjugated molecules exhibit tunable luminescence—a property that is useful for the next generation of optical devices. Yagai et al. propose a strategy to design these materials on a molecular level, which tailors the emission colour via structural changes in response to mechanical stimuli.
- Shiki Yagai
- , Satoru Okamura
- & Hajime Ito
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High-efficiency organic light-emitting diodes with fluorescent emitters
Fluorescent organic light-emitting diodes hold promise for next-generation full-colour displays, but are currently limited by the internal electroluminescence quantum efficiency. Nakanotani et al.break this limit and demonstrate nearly 100% efficiency in a double-dopant system without a rare metal.
- Hajime Nakanotani
- , Takahiro Higuchi
- & Chihaya Adachi
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Beryllium-free Li4Sr(BO3)2 for deep-ultraviolet nonlinear optical applications
Deep-ultraviolet nonlinear optical materials can generate laser light below 200 nm, which is crucial to solid-state deep-ultraviolet lasers. Here, the authors find that Li4Sr(BO3)2shows advantageous properties as a deep-ultraviolet nonlinear optical material, where alternatives are rare.
- Sangen Zhao
- , Pifu Gong
- & Junhua Luo
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| Open AccessOn-the-fly decoding luminescence lifetimes in the microsecond region for lanthanide-encoded suspension arrays
Accurately determining luminescence lifetimes for slow-decaying signals can be challenging. Here, the authors report a fitting algorithm and subsequently experimentally show a method for the rapid measurement of luminescence lifetimes in the microsecond region.
- Yiqing Lu
- , Jie Lu
- & Dayong Jin
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Multistability and switching in a superconducting metamaterial
Metamaterials are artificial media with tailored optical properties that can ideally be altered at will. Jung et al.use superconducting quantum interference devices as switchable meta-atoms to build a metamaterial that can be rapidly controlled by microwave-probe signals.
- P. Jung
- , S. Butz
- & A. V. Ustinov
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Double-heterojunction nanorods
Introducing active hetrojunctions could improve the capabilities of devices based on colloidal quantum dots. Here, the authors develop nanorods with double heterojunctions and show that they can provide independent control over the electron and hole processes, demonstrating their potential in light-emitting diodes.
- Nuri Oh
- , Sooji Nam
- & Moonsub Shim
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Smart responsive phosphorescent materials for data recording and security protection
Smart luminescent materials have many potential applications. Here, the authors synthesize a series of responsive iridium complexes, with tunable emission colours, and use their mechano-, vapo- and electrochromic phosphorescence properties to construct a proof of concept data recording device.
- Huibin Sun
- , Shujuan Liu
- & Wei Huang
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Two-photon polarization-selective etching of emergent nano-structures on diamond surfaces
Using light to manipulate matter on scales smaller than its wavelength presents a major challenge. Here, the authors show that two-photon surface excitation of diamond surfaces etches a variety of nano-scale patterns, comprising evidence for carbon ejection via a highly localized photon interaction with the crystal bonds.
- A. Lehmann
- , C. Bradac
- & R. P. Mildren
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Heterogeneous stacking of nanodot monolayers by dry pick-and-place transfer and its applications in quantum dot light-emitting diodes
Several techniques exist for patterning a single densely packed layer of quantum dots onto a surface. Kim et al.now demonstrate a simple and reliable technique for transferring multiple monolayers, one-by-one, to form stacked multilayers of quantum dots of different types and sizes on a surface.
- Tae-Ho Kim
- , Dae-Young Chung
- & Kinam Kim
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| Open AccessSolar spectral conversion for improving the photosynthetic activity in algae reactors
Algae beds are a promising resource for bio-energy and gas production, but their productivity is often limited by solar energy harvesting efficiency. Wondraczek et al. promote algal growth by using photoluminescent phosphor, which shifts the light spectrum to better match the algal adsorption band.
- Lothar Wondraczek
- , Miroslaw Batentschuk
- & Christoph J. Brabec
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All-solution processed polymer light-emitting diode displays
Polymer light-emitting diodes promise cheap and flexible lighting and displays, but their fabrication is hindered by high-vacuum methods for creating cathodes. Zheng et al.show an all-solution processing approach to polymer diodes that removes this obstacle, offering roll-to-roll fabrication of devices.
- Hua Zheng
- , Yina Zheng
- & Yong Cao
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Photoconductive response in organic charge transfer interfaces with high quantum efficiency
Single-crystal organic semiconductors are potential materials for electronic applications, for example, as field-effect transistors. Here, the authors demonstrate photoconductivity of single-crystal charge-transfer interfaces, suggesting that they may also be used for photonic applications.
- Helena Alves
- , Rui M. Pinto
- & Ermelinda S. Maçôas
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Switching and amplification in disordered lasing resonators
Information transport and control of the energy flow in a disordered system is difficult to achieve. Here Leonetti et al. demonstrate that the transmission of one laser mode in a random medium can be switched and amplified by exciting a second mode.
- Marco Leonetti
- , Claudio Conti
- & Cefe Lopez
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Diamond-integrated optomechanical circuits
Diamond is of interest for optical and electronic applications owing to its unique mechanical and optical properties. Here, Rath et al. demonstrate the use of small nanometre-sized beams etched from diamond thin films for integrated photonic circuits.
- Patrik Rath
- , Svetlana Khasminskaya
- & Wolfram H.P. Pernice
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Athermal photofluidization of glasses
Glasses are solid when cold, but when mixed with the correct dye can be fluidized by light. Fang et al.show that each photon absorbed in an azobenzen-based molecule layer produces an efficient local heating up to 800 K to melt the glass but without altering the average temperature.
- G.J. Fang
- , J.E. Maclennan
- & N.A. Clark
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| Open AccessFemtosecond nonlinear ultrasonics in gold probed with ultrashort surface plasmons
Measuring acoustic phonons across the Brillouin zone reveals important information on electrical and thermal transport in materials. Temnov et al.generate giant acoustic strain pulses in gold/cobalt bilayers and monitor their nonlinear reshaping in the gold layer with plasmonic interferometry.
- Vasily V. Temnov
- , Christoph Klieber
- & Rudolf Bratschitsch
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Improved heat dissipation in gallium nitride light-emitting diodes with embedded graphene oxide pattern
High-brightness light-emitting diodes require high operating currents, which generate significant Joule heating and subsequent heat dissipation is an issue. This work demonstrates the growth of GaN-based light-emitting diodes directly on graphene oxide with a low thermal resistance for efficient heat removal.
- Nam Han
- , Tran Viet Cuong
- & Chang-Hee Hong
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| Open AccessMicroelectromechanical Maltese-cross metamaterial with tunable terahertz anisotropy
Metamaterials can be designed with anisotropy, which tailors their optical properties to enable interesting functionalities. Here, the anisotropy of a Maltese-cross metamaterial is actively controlled by an actuator, allowing for tunable birefringence and dichroism in the terahertz frequency region.
- W.M. Zhu
- , A.Q. Liu
- & N.I. Zheludev
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Single-particle structure determination by correlations of snapshot X-ray diffraction patterns
Free-electron lasers enable diffractive imaging of single nanostructures, but algorithms, such as correlation analyses, are needed to determine their diffraction volume from accumulated data. Starodub et al.present such a method for X-ray diffractive imaging of nanometre-scale polystyrene dimers.
- D. Starodub
- , A. Aquila
- & M.J. Bogan
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Broadband electromagnetic cloaking with smart metamaterials
Metamaterial cloaks can manipulate light to effectively hide objects from view, but they mostly rely on rigid structures that are tailored specifically for the chosen object. Shin et al.demonstrate an elastic, smart metamaterial cloak that can adapt to a range of deformations and object sizes.
- Dongheok Shin
- , Yaroslav Urzhumov
- & David R. Smith
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Review Article |
Hyperlenses and metalenses for far-field super-resolution imaging
The diffraction limit of light constrains the achievable resolution of conventional optical systems, but metamaterials provide numerous avenues to beat it. Lu and Liu review recent advances in super-resolution imaging with hyperlenses and metalenses, and discuss future directions and hurdles for the field.
- Dylan Lu
- & Zhaowei Liu
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Magnetic and electric coherence in forward- and back-scattered electromagnetic waves by a single dielectric subwavelength sphere
The absence of forward or backward scattered radiation by magnetodielectric spheres was predicted decades ago, yet direct measurements have remained elusive. Geffrin et al. present unambiguous evidence of such scattering effects in the gigahertz range for a sub-wavelength dielectric sphere.
- J.M. Geffrin
- , B. García-Cámara
- & F. Moreno
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Active control of electromagnetically induced transparency analogue in terahertz metamaterials
Metamaterial analogues of electromagnetically-induced transparency provide interesting optical components and applications. By actively tuning the dark mode of a metamaterial, Guet al. optically control its electromagnetically-induced transparency, showing tunable group delay of terahertz light.
- Jianqiang Gu
- , Ranjan Singh
- & Weili Zhang
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A novel phosphor for glareless white light-emitting diodes
Light-emitting diodes are attractive sources of light used in an increasing range of applications. This study presents a novel europium-based phosphor that gives rise to a substantial reduction in the glare that often makes LEDs uncomfortable to the human eye.
- Hisayoshi Daicho
- , Takeshi Iwasaki
- & Hideo Hosono
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Article
| Open AccessAmbient fabrication of flexible and large-area organic light-emitting devices using slot-die coating
Light-emitting electrochromic cells are a promising alternative to organic light-emitting diodes, as their performance is less sensitive to fabrication conditions. Here, a roll-to-roll compatible fabrication of such devices is presented, demonstrating large-area continuous production in ambient conditions.
- Andreas Sandström
- , Henrik F. Dam
- & Ludvig Edman
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Laser-induced ultrafast demagnetization in the presence of a nanoscale magnetic domain network
Understanding ultrafast demagnetisation is key to manipulating magnetic structures on fast timescales, yet laser sources limit the attainable spatial resolution. Here, a soft X-ray high harmonic source enables a high temporal and spatial resolution study of domain demagnetisation in [Co/Pt]30multilayer films.
- Boris Vodungbo
- , Julien Gautier
- & Jan Lüning
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| Open AccessStructural correlations in the generation of polaron pairs in low-bandgap polymers for photovoltaics
The electronic and optical properties of polymer semiconductors are largely dictated by their chemical structure. This study examines the nature of the photoexcited states generated in donor–acceptor polymers, and uncovers the dynamics of polaron pairs generation and recombination.
- Raphael Tautz
- , Enrico Da Como
- & Ullrich Scherf