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| Open AccessDepletable peroxidase-like activity of Fe3O4 nanozymes accompanied with separate migration of electrons and iron ions
The mechanism of peroxidase-like Fe3O4 nanozymes remains elusive. Here, the authors show the electron transfer mechanism of Fe(II) ions to regenerate surface Fe(II) and the related phase transformation and depletion of activity.
- Haijiao Dong
- , Wei Du
- & Yu Zhang
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Article
| Open AccessGate-controlled skyrmion and domain wall chirality
A major feature defining the motion of magnetic spin textures is the chirality or ’handedness’ of the spin texture, which in turn depends on the underlying material. Normally it is considered as fixed, but in this article Fillion et al demonstrate control of the chirality of skyrmions in a ferromagnetic multilayer, switching the chirality back and forth using an applied gate voltage.
- Charles-Elie Fillion
- , Johanna Fischer
- & Hélène Béa
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Article
| Open AccessUltrathin ferrite nanosheets for room-temperature two-dimensional magnetic semiconductors
Van der Waals crystals allow for magnetism down to the monolayer limit, however, this magnetism, and frequently the material itself, is fragile. Ferrites, conversely, have robust material stability and magnetic order, but are three dimensional. Here the authors succeed in creating a single unit cell thickness of Cobalt Ferrite via chemical vapour deposition, with hard magnetic properties, and curie temperature exceeding room temperature.
- Ruiqing Cheng
- , Lei Yin
- & Jun He
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Comment
| Open AccessChirality dependence of spin current in spin pumping
Chirality of magnons is an intrinsic degree of freedom that characterizes the handedness of spin precession around its equilibrium direction. This commentary summarizes recent progress on spin pumping by ferromagnetic resonance in magnetic heterostructures. In particular, the commentary highlights one fundamental issue in spin pumping: the chirality dependence of the spin current.
- Z. Q. Qiu
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Article
| Open AccessSpin-selected electron transfer in liquid–solid contact electrification
Electron transfer has been shown to contribute to contact electrification at liquid–solid interface. Here, authors investigate the magnetic field effect on the liquid–solid electron transfer and propose a spin conversion model for the liquid–solid contact electrification.
- Shiquan Lin
- , Laipan Zhu
- & Zhong Lin Wang
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Article
| Open AccessProximity-magnetized quantum spin Hall insulator: monolayer 1 T’ WTe2/Cr2Ge2Te6
Van der Waals heterostructures allow for the integration of several materials with different properties in the one heterostructure. Here, Li et al combine a quantum spin hall insulator, WTe2, with an insulating ferromagnet, Cr2Ge2Te6, in a van der Waals heterostructure, with resulting proximity-induced magnetism in the WTe2 layer leading to an anomalous Hall and Nernst effect.
- Junxue Li
- , Mina Rashetnia
- & Jing Shi
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Article
| Open AccessImaging and phase-locking of non-linear spin waves
Many proposed spin-wave based devices make use of non-linear behaviour of spin-waves. Here, Dreyer et al show the emergence of non-linear spin waves oscillating at half-integer harmonics in the strong modulation regime. By applying super-Nyquist sampling Kerr microscopy they directly image these non-linear spin waves and demonstrate their phase-locking to an external frequency source.
- Rouven Dreyer
- , Alexander F. Schäffer
- & Georg Woltersdorf
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Article
| Open AccessSkyrmions in synthetic antiferromagnets and their nucleation via electrical current and ultra-fast laser illumination
Skyrmions in synthetic antiferromagnets are appealing for use in future memory and computing devices, combining small size and fast motion, but creating, stabilizing, and observing them remains a challenge. Here, Juge et al demonstrate the stabilization and current and light induced nucleation of skyrmions in a synthetic antiferromagnet, observing the magnetization texture in each layer using X-ray magnetic microscopy.
- Roméo Juge
- , Naveen Sisodia
- & Olivier Boulle
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Article
| Open AccessDynamic magnetic crossover at the origin of the hidden-order in van der Waals antiferromagnet CrSBr
A 2D magnet CrSBr has attracted interest for applications in spintronics due to its high critical temperature and interesting magneto-electrical properties. Here the authors report a detailed study of its magnetic and structural phases and uncover a hidden magnetic order inside the magnetically-ordered phase.
- Sara A. López-Paz
- , Zurab Guguchia
- & Fabian O. von Rohr
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Article
| Open AccessAnomalous Ferromagnetism of quasiparticle doped holes in cuprate heterostructures revealed using resonant soft X-ray magnetic scattering
Long-range magnetic order of quasiparticle doped holes is important for understanding the physics of cuprate superconductors, albeit difficult to probe in experiments. Ong et al. observe ferromagnetism of quasiparticle doped holes in a cuprate heterostructure and discuss implications for cuprates in the ground state.
- B. L. Ong
- , K. Jayaraman
- & A. Rusydi
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Article
| Open AccessPhonon thermal Hall effect in a metallic spin ice
The thermal Hall effect, or a temperature gradient transverse to a heat current and a magnetic field, has been observed in many materials, but its mechanism is not fully understood. Uehara et al. demonstrate the dominant phonon contribution to both longitudinal and transverse thermal response in a metallic spin ice Pr2Ir2O7.
- Taiki Uehara
- , Takumi Ohtsuki
- & Yo Machida
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Article
| Open AccessExchange-induced spin polarization in a single magnetic molecule junction
The spin exchange, which is central to spintronics, has been restricted to devices with long-range magnetic ordering to date. Here, Pei et al. design a single-molecule-magnet and utilize its internal spin exchange to control the current through a single-molecule junction with high spin polarization (>95%).
- Tian Pei
- , James O. Thomas
- & Lapo Bogani
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Article
| Open AccessCoherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3
CrI3 is a van der Waals material which exhibits magnetic ordering down to the monolayer limit. Here, using ultrafast optical spectroscopy, Padmanabhan and Buessen et al. investigate the coupling between the magnetically ordered spins and lattice distortions, finding a coherent spin-coupled phonon mode.
- P. Padmanabhan
- , F. L. Buessen
- & R. P. Prasankumar
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Article
| Open AccessEfficient perpendicular magnetization switching by a magnetic spin Hall effect in a noncollinear antiferromagnet
Spin-orbit torques driven by the conventional spin Hall effect are widely used to switch magnetization, but this approach is nondeterministic and inefficient for magnets with perpendicular magnetic anisotropy. Here, the authors demonstrate deterministic, field-free switching in a Ni/Co multilayer by exploiting the magnetic spin Hall effect in adjacent Mn3Sn.
- Shuai Hu
- , Ding-Fu Shao
- & Xuepeng Qiu
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Article
| Open AccessA reconfigurable and magnetically responsive assembly for dynamic solar steam generation
Despite a promising water harvesting approach solar steam generation low efficiency remains a challenging obstacle. Here, authors present a macro- and microscopically reconfigurable and magnetically responsive assembly towards a dynamic evaporation system with improved performance and salt resistance.
- Yajie Hu
- , Hongyun Ma
- & Liangti Qu
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Article
| Open AccessMagnetic control over the fundamental structure of atomic wires
Magnetic effects can emerge due to structural variations when the size of materials is reduced towards the nanoscale. Here, Chakrabarti et al demonstrates the opposite effect, showing that the interatomic distance in atomic wires changes by up to 20% depending on the orientation of an applied magnetic field.
- Sudipto Chakrabarti
- , Ayelet Vilan
- & Oren Tal
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Article
| Open AccessAnisotropic magnon damping by zero-temperature quantum fluctuations in ferromagnetic CrGeTe3
CrGeTe3 is a van der Waals honeycomb ferromagnet, known for exhibiting strong coupling between lattice and spin degrees of freedom. Here, Chen et al perform neutron scattering on CrGeTe3, find a broadened spin-wave excitation resulting from zero-temperature motion of the atoms in the lattice.
- Lebing Chen
- , Chengjie Mao
- & Pengcheng Dai
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Article
| Open AccessMagnetic molecules as local sensors of topological hysteresis of superconductors
Magnetic molecules have long been seen to hold promise in magnetic sensing applications. In this paper, Serrano et al show that a single layer of a magnetic molecule, a terbium based complex, is sensitive to the local magnetic field variation of a superconducting surface on which it is deposited.
- Giulia Serrano
- , Lorenzo Poggini
- & Roberta Sessoli
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Article
| Open AccessInvestigation of the monopole magneto-chemical potential in spin ices using capacitive torque magnetometry
Magnetic-field induced phase transitions in spin-ice materials have been investigated with various experimental techniques. Here, the authors demonstrate the capability of capacitive torque magnetometry in probing magnetic interaction energies and establishing magnetic phase boundaries in Ho2Ti2O7.
- Naween Anand
- , Kevin Barry
- & Christianne Beekman
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Article
| Open AccessUnveiling the S=3/2 Kitaev honeycomb spin liquids
Recently, material realizations of the spin 3/2 Kitaev honeycomb model have been proposed, but the model has not been solved by either analytical or numerical methods. Here the authors report exact results for the spin 3/2 model consistent with numerical simulations, and find gapped and gapless quantum spin liquids.
- Hui-Ke Jin
- , W. M. H. Natori
- & J. Knolle
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Article
| Open AccessScanning gradiometry with a single spin quantum magnetometer
Scanning NV center magnetometry enables imaging of weak magnetic fields at the nanoscale. Huxter et al. achieve an order-of-magnitude improvement in sensitivity by converting a spatial field gradient into an AC field by mechanical oscillations of the sensor, and image stray fields from atomic steps in an antiferromagnet.
- W. S. Huxter
- , M. L. Palm
- & C. L. Degen
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Article
| Open AccessDefect-induced monopole injection and manipulation in artificial spin ice
Artificial spin ice systems offer a promising platform to study the motion of emergent magnetic monopoles, but controlled nucleation of monopoles is challenging. Here the authors demonstrate controlled injection and propagation of emergent monopoles in an artificial spin ice utilizing ferromagnetic defects.
- Robert Puttock
- , Ingrid M. Andersen
- & Olga Kazakova
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Article
| Open AccessAnderson transition in stoichiometric Fe2VAl: high thermoelectric performance from impurity bands
The mathematical conditions for the best thermoelectric is well known but never realised in real materials. Here, the authors propose the Anderson transition in a narrow impurity band as a physical realisation of this seemingly unrealisable scenario.
- Fabian Garmroudi
- , Michael Parzer
- & Ernst Bauer
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Article
| Open AccessCurrent-induced self-switching of perpendicular magnetization in CoPt single layer
One challenge for spin-based electronics is the controlled and reliable switching of magnetization without magnetic fields. Here, Liu et al investigate a variety of compositions of CoPt, and determine the specific composition to maximize switching performance, potentially simplifying device design.
- Liang Liu
- , Chenghang Zhou
- & Jingsheng Chen
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Article
| Open AccessDirect investigation of the atomic structure and decreased magnetism of antiphase boundaries in garnet
Iron garnets are widely used in magneto-optical devices, but knowledge of the effects of common defects on performance is limited. Here, using high-resolution microscopy and spectroscopy, the authors find that magnetism is weakened near these defects causing reduced performance, but can be avoided by tuning the growth rate.
- Kun Xu
- , Ting Lin
- & Jing Zhu
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Article
| Open AccessSlowdown of photoexcited spin dynamics in the non-collinear spin-ordered phases in skyrmion host GaV4S8
Skyrmions are a topological magnetic texture that have garnered considerable interest for various technological applications. Here, Sekiguchi et al. investigate the ultrafast optical response of GaV4S6, and find a significant reduction in the thermal conductivity in the skyrmion phase.
- Fumiya Sekiguchi
- , Kestutis Budzinauskas
- & Paul H. M. van Loosdrecht
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Article
| Open AccessDeciphering quantum fingerprints in electric conductance
Scattering of electrons from defects and boundaries in mesoscopic samples is encoded in quantum interference patterns of magneto-conductance, but these patterns are difficult to interpret. Here the authors use machine learning to reconstruct electron wavefunction intensities and sample geometry from magneto-conductance data.
- Shunsuke Daimon
- , Kakeru Tsunekawa
- & Eiji Saitoh
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Article
| Open AccessParamagnons and high-temperature superconductivity in a model family of cuprates
Finding a parameter that limits the critical temperature of cuprate superconductors can provide crucial insight on the superconducting mechanism. Here, the authors use inelastic photon scattering on two Ruddlesden-Popper members of the model Hg-family of cuprates to reveal that the energy of magnetic fluctuations may play such a role, and suggest that the Cooper pairing is mediated by paramagnons.
- Lichen Wang
- , Guanhong He
- & Yuan Li
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Article
| Open AccessSkyrmion pinning energetics in thin film systems
Skyrmions, topological spin textures, can be pinned by defects present in the material that hosts them, influencing their motion. Here, Gruber et al show that the skyrmions are pinned at their boundary where the finite size of the skyrmions governs their pinning, and they demonstrate that certain pinning sites can switched on and off in-situ.
- Raphael Gruber
- , Jakub Zázvorka
- & Mathias Kläui
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Article
| Open AccessNonlinear two-level dynamics of quantum time crystals
Recent work has reported a realization of a time crystal in the form of the Bose-Einstein condensate of magnons in superfluid 3He. Here, the authors study the dynamics of a pair of such quantum time crystals and show that it closely resembles the evolution of a two-level system, modified by nonlinear feedback.
- S. Autti
- , P. J. Heikkinen
- & V. B. Eltsov
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Article
| Open AccessEvidence for pressure induced unconventional quantum criticality in the coupled spin ladder antiferromagnet C9H18N2CuBr4
There is a class of quantum phase transitions that do not fit into the traditional Landau paradigm, but are described in terms of fractionalized degrees of freedom and emergent gauge fields. Hong et al. find evidence of such a transition in a molecular spin-1/2 antiferromagnetic ladder compound under hydrostatic pressure.
- Tao Hong
- , Tao Ying
- & Stefan Wessel
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Article
| Open AccessStructural independence of hydrogen-bond symmetrisation dynamics at extreme pressure conditions
The authors use in-situ high pressure nuclear magnetic resonance spectroscopy in diamond anvil cells to show that at all observed H-bond environments undergo a distinct maximum in hydrogen mobility regardless of the structure of the compounds.
- Thomas Meier
- , Florian Trybel
- & Leonid Dubrovinsky
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Article
| Open AccessHistory-dependent domain and skyrmion formation in 2D van der Waals magnet Fe3GeTe2
Fe3GeTe2, known as FGT, is a van der Waals magnetic material that was recently shown to host magnetic skyrmions. Here, Birch et al using both X-ray and electron microscopy to study the stability of skyrmions in FGT, revealing how the sample history can influence skyrmion formation
- M. T. Birch
- , L. Powalla
- & G. Schütz
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Article
| Open AccessObservation of a phase transition within the domain walls of ferromagnetic Co3Sn2S2
In the Bloch or Neel domain walls in ferromagnets, the magnetization rotates smoothly from up to down, preserving its magnitude. Here, Lee et al show that Co3Sn2S2 exhibits a phase transition within its domain walls to a state in which the magnetization passes through zero rather than rotating as the wall is traversed.
- Changmin Lee
- , Praveen Vir
- & Joseph Orenstein
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Article
| Open AccessEminuscent phase in frustrated magnets: a challenge to quantum spin liquids
A spin-glass forms in frustrated magnetic systems when at low temperatures impurity sites “freeze” into a random spin configuration. Here, by looking back at previous experimental results, Syzranov and Ramirez show that the glass-transition temperature grows with decreasing impurity concentration.
- S. V. Syzranov
- & A. P. Ramirez
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Article
| Open AccessUltrafast kinetics of the antiferromagnetic-ferromagnetic phase transition in FeRh
Using ultrashort laser pulses it is possible to induce ferromagnetic ordering in otherwise anti-ferromagnetic FeRh. Here, Li et al. use THz emission spectroscopy with double pump to probe the transient dynamics of this transition, showing the insusceptibility of the ferromagnetic order to applied magnetic fields at picosecond timescales.
- G. Li
- , R. Medapalli
- & A. V. Kimel
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Article
| Open AccessZrTe2/CrTe2: an epitaxial van der Waals platform for spintronics
Van der Waals heterostructures offer the potential of integrating multiple material layers into a single device to achieve new functionalities. Here, Ou et al combine ZrTe2, a topological semimetal, with CrTe2, a 2D ferromagnet, in a single heterostructure and demonstrate spin-orbit torque switching of the 2D ferromagnet by current in the topological semimetal.
- Yongxi Ou
- , Wilson Yanez
- & Nitin Samarth
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Article
| Open AccessGeometric transformation and three-dimensional hopping of Hopf solitons
Hopf solitons are three-dimensional particle-like field distortions with nontrivial topology. Tai et al. show stable Hopf solitons in a liquid crystal material in the absence of an electric field or geometric confinement, their transformation and hopping-like dynamics in response to electric pulses.
- Jung-Shen B. Tai
- , Jin-Sheng Wu
- & Ivan I. Smalyukh
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Article
| Open AccessPressured-induced superconducting phase with large upper critical field and concomitant enhancement of antiferromagnetic transition in EuTe2
Here, the authors report pressure-induced superconductivity with concomitant enhancement of antiferromagnetic transition in layered EuTe2. The superconductivity is distinctly characterized by the high upper critical fields exceeding the Pauli limit among binary tellurides, a prerequisite of the coexistence of ferromagnetism with superconductivity.
- P. T. Yang
- , Z. Y. Liu
- & J.-G. Cheng
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Article
| Open AccessMagnetic Bloch oscillations and domain wall dynamics in a near-Ising ferromagnetic chain
An electron subject to a periodic potential and a constant electric field exhibit oscillatory dynamics, known as Bloch oscillations. Here, the authors demonstrate a magnetic analogue of Bloch oscillations in a ferromagnetic near-Ising chain, where magnetic excitations oscillate in response to a magnetic field.
- Ursula B. Hansen
- , Olav F. Syljuåsen
- & Kim Lefmann
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Article
| Open AccessMagnons and magnetic fluctuations in atomically thin MnBi2Te4
MnBi2Te4, referred to as MBT, is a van der Waals material combining topological electron bands with magnetic order. Here, Lujan et al study collective spin excitations in MBT, and show that magnetic fluctuations increase as samples reduce in thickness, implying less robust magnetic order.
- David Lujan
- , Jeongheon Choe
- & Xiaoqin Li
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Article
| Open AccessPhysical realization of topological Roman surface by spin-induced ferroelectric polarization in cubic lattice
A non-orientable surface can mirror reflecting the man travelling on it. Realizing such topological object is fascinating. Here, the authors discover that antiferromagnetic-induced polarization in a solid can realize a non-orientable Roman surface.
- Guangxiu Liu
- , Maocai Pi
- & Youwen Long
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Article
| Open AccessEmergent multiferroism with magnetodielectric coupling in EuTiO3 created by a negative pressure control of strong spin-phonon coupling
Negative pressure tailors the physical properties of functional oxide materials. Here, the authors demonstrate an emergent multiferroism with magnetodielectric coupling in EuTiO3 created by a negative pressure control of strong spin-phonon coupling.
- Run Zhao
- , Chao Yang
- & Hao Yang
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Article
| Open AccessObservation of fractional spin textures in a Heusler material
Skyrmions and anti-skyrmions are magnetic textures that have garnered much interest due to their stability. Here, Jena et al demonstrate the existence of fractional spin textures at the edges of Heusler alloy sample, which can have continuous variable topological charges.
- Jagannath Jena
- , Börge Göbel
- & Stuart S. P. Parkin
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Article
| Open AccessQuadrupolar magnetic excitations in an isotropic spin-1 antiferromagnet
Multipolar magnetic excitations are challenging to measure as most experimental probes are sensitive to dipolar processes. Here, Nag et al. show the existence of dispersing quadrupolar components to the spin excitations in an antiferromagnet, highlighting the importance of higher order magnetic excitations.
- A. Nag
- , A. Nocera
- & Ke-Jin Zhou
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Article
| Open AccessDiscovery of quantum phases in the Shastry-Sutherland compound SrCu2(BO3)2 under extreme conditions of field and pressure
SrCu2(BO3)2 is a 2D quantum antiferromagnet on a particular frustrated lattice showing multiple magnetization plateaus and quantum phase transitions under high pressure. Here the authors uncover novel magnetic phases in this material under combined effects of extreme magnetic field and pressure.
- Zhenzhong Shi
- , Sachith Dissanayake
- & Sara Haravifard
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Article
| Open AccessAnisotropy-driven quantum criticality in an intermediate valence system
The nature of quantum criticality in intermetallic f-electron compounds exhibiting valence fluctuations is not well understood. Here, using a combination of experimental techniques, the authors attribute quantum criticality in YbAlB4 to the anisotropic hybridization between the conduction and f-electrons.
- Mihael S. Grbić
- , Eoin C. T. O’Farrell
- & Satoru Nakatsuji
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Article
| Open AccessNon-metallic T2-MRI agents based on conjugated polymers
The toxicity of heavy metals for MRI contrast agents is an issue. Here, the authors report on the development of conjugated polymers nanoparticles based on paramagnetic polypyrrole to generate T2 MRI contrast effects by changing the interactions between polarons and water protons.
- Qinrui Lin
- , Yuhong Yang
- & Zhengzhong Shao
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Article
| Open AccessInterlayer magnetophononic coupling in MnBi2Te4
Tunable coupling between magnetism and the lattice is important for on-demand manipulation of magnetic phases. Here, the authors demonstrate that lattice vibrations can coherently modulate the interlayer magnetic exchange coupling in the magnetic topological insulator MnBi2Te4.
- Hari Padmanabhan
- , Maxwell Poore
- & Venkatraman Gopalan