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| Open AccessMeasuring long-range carrier diffusion across multiple grains in polycrystalline semiconductors by photoluminescence imaging
Understanding the role of defects on semiconductor carrier transport should help improve their performance in devices. Using photoluminescence techniques, Alberi et al. image the carrier diffusion in polycrystalline CdTe and find that long-range transport is mediated by the distribution of defect states.
- K. Alberi
- , B. Fluegel
- & A. Mascarenhas
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Hopping transport through defect-induced localized states in molybdenum disulphide
There is great interest in molybdenum disulphide for electronic devices but the mechanism of charge transport remains elusive. Qiu et al. find that sulphur vacancies introduce localized donor states within the bandgap, enabling low-carrier-density transport via hopping.
- Hao Qiu
- , Tao Xu
- & Xinran Wang
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A plasma-treated chalcogenide switch device for stackable scalable 3D nanoscale memory
To reach terabit density in random access memory devices, the select switching and storage components need to be improved. Here, the authors fabricate a fully stackable switching device based on chalcogenides, which reaches an exceptional performance following reactive nitrogen and nitrogen plasma treatments.
- Myoung-Jae Lee
- , Dongsoo Lee
- & In-Kyeong Yoo
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Mobility transition from ballistic to diffusive transport in non-Hermitian lattices
Transport of particles in the presence of disorder is of interest for applications in electronics as well as photonics. Here the authors show theoretically and experimentally that based on dissipation alone, transport of light undergoes a change from ballistic to diffusive transport even in the absence of disorder.
- T. Eichelkraut
- , R. Heilmann
- & A. Szameit
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Article
| Open AccessPhotonic polarization gears for ultra-sensitive angular measurements
Beating the standard measurement limits is a goal of metrology, as it would allow for more precise estimation of physical quantities. Borrowing concepts from NOON-state quantum metrology, this work presents a single-photon scheme to measure rotation angles of light with super-resolution precision.
- Vincenzo D'Ambrosio
- , Nicolò Spagnolo
- & Fabio Sciarrino
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| Open AccessGenetic design of enhanced valley splitting towards a spin qubit in silicon
Electronic spins in Si are potentially useful in the development of solid-state quantum devices, but its degenerate valley states limits this potential. Zhang et al.use a genetic algorithm to identify a Ge/Si-multilayer-clad Si quantum structure whose valley splitting is increased by an order of magnitude.
- Lijun Zhang
- , Jun-Wei Luo
- & Alex Zunger
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Microwave magnetoelectric effect via skyrmion resonance modes in a helimagnetic multiferroic
Magnetic skyrmions are topologically stable swirls in a spin structure. Here, the authors demonstrate new ways of controlling them by showing that the absorption of an electromagnetic wave by a skyrmion depends on the direction of incidence and that the resonance modes respond to a magnetic field.
- Y. Okamura
- , F. Kagawa
- & Y. Tokura
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Plasmonic gold mushroom arrays with refractive index sensing figures of merit approaching the theoretical limit
Plasmonic resonances in nanostructures are useful for high-performance biosensors. Shen et al. build arrays of nanoscale gold mushrooms with a high figure of merit close to the predicted upper limit and show their use for detecting low concentrations of cytochrome cand alpha-fetoprotein.
- Yang Shen
- , Jianhua Zhou
- & Jianfang Wang
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LaAlO3 stoichiometry is key to electron liquid formation at LaAlO3/SrTiO3 interfaces
The origin of the two-dimensional electron liquid between LaAlO3 and SrTiO3 has been a matter of debate. The authors’ investigation of stoichiometry reveals that only Al-rich LaAlO3leads to electron liquid formation, which points to the much discussed polar catastrophe mechanism as its origin.
- M. P. Warusawithana
- , C. Richter
- & D. G. Schlom
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Tetragonal phase of epitaxial room-temperature antiferromagnet CuMnAs
The use of antiferromagnetic materials in spintronic devices has been proposed as an attractive alternative to ferromagnets, but only a few suitable materials are known. Here, the authors synthesize a new antiferromagnet (AFM)—tetragonal epitaxial CuMnAs—and show that it is ideal for spintronic applications.
- P. Wadley
- , V. Novák
- & T. Jungwirth
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Efficient and bright organic light-emitting diodes on single-layer graphene electrodes
Indium tin oxide, the predominant material used as transparent electrodes in organic LEDs, is expensive and brittle. Ning Li and colleagues form transparent electrodes using single-layer graphene to construct organic LEDs with unprecedented performance that are suitable for both displays and lighting.
- Ning Li
- , Satoshi Oida
- & Tze-Chiang Chen
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Article
| Open AccessA chiral-based magnetic memory device without a permanent magnet
Most new device concepts for random-access memory are based on inorganic spin filters, which need a permanent magnet to operate. Here, the authors exploit the chiral-induced spin selectivity effect in an organic spin filter to construct a novel type of memory device, which works without a permanent magnet.
- Oren Ben Dor
- , Shira Yochelis
- & Yossi Paltiel
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Article
| Open AccessMouldable all-carbon integrated circuits
The incorporation of electronic circuits into various plastic products and devices is limited by the brittle nature of silicon wafers. Here, Sun et al.demonstrate flexible and high-performance all-carbon-based transistor circuits that can be thermo-moulded into various shapes.
- Dong-Ming Sun
- , Marina Y. Timmermans
- & Yutaka Ohno
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| Open AccessNoise-resilient quantum evolution steered by dynamical decoupling
Realistic quantum computers require a high degree of qubit control and must also be resilient to noise. Using dynamical decoupling control techniques, Liuet al.implement a self-protected controlled-NOT gate for electron and nuclear spins that retains a high final state fidelity.
- Gang-Qin Liu
- , Hoi Chun Po
- & Xin-Yu Pan
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Mechanism of carrier accumulation in perovskite thin-absorber solar cells
Understanding the accumulation of photogenerated charges in photovoltaics is crucial to developing more efficient structures. Kim et al.use impedence spectroscopy to observe charge accumulation in thin lead halide perovskite solar cells, finding a high density of states that differs from other types of cells.
- Hui-Seon Kim
- , Ivan Mora-Sero
- & Juan Bisquert
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| Open AccessHigh transconductance organic electrochemical transistors
Although organic transistors have many advantages, they are not typically known for their high performance. Khodagholy et al. report the fabrication of organic electrochemical transistors that combine high transconductance with mechanical flexibility, and are attractive for biosensor applications.
- Dion Khodagholy
- , Jonathan Rivnay
- & George G. Malliaras
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Pattern classification by memristive crossbar circuits using ex situ and in situ training
Experimental demonstration of memristor circuits in artificial neural networks is challenging. Here, pattern classification by a single-layer perceptron network is realised with a memristive crossbar circuit, and both in situ and ex situtraining are applied.
- Fabien Alibart
- , Elham Zamanidoost
- & Dmitri B. Strukov
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| Open AccessTailorable stimulated Brillouin scattering in nanoscale silicon waveguides
Exploiting photon–phonon coupling in nanoscale silicon waveguides could enable a host of powerful features in photonic devices. Using a hybrid photonic–phononic waveguide structure, Shin et al. show stimulated Brillouin scattering nonlinearities and gain, which offers new on-chip signal-processing abilities.
- Heedeuk Shin
- , Wenjun Qiu
- & Peter T. Rakich
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Photocurrent in graphene harnessed by tunable intrinsic plasmons
By patterning graphene with sub-wavelength features to introduce plasmonic modes, its optical properties can be tailored. Freitag et al. show how tunable plasmons in graphene nanoribbons can be exploited to form polarization-sensitive graphene photodetectors in the mid-infrared spectral region.
- Marcus Freitag
- , Tony Low
- & Phaedon Avouris
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| Open AccessMillisecond charge-parity fluctuations and induced decoherence in a superconducting transmon qubit
Superconducting circuits are promising for quantum computing, but quasiparticle tunnelling across Josephson junctions introduces qubit decoherence. Ristè et al. convert a transmon qubit into its own real-time quasiparticle tunnelling detector and accurately measure induced decoherence in the millisecond range.
- D. Ristè
- , C. C. Bultink
- & L. DiCarlo
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Picosecond pulses from wavelength-swept continuous-wave Fourier domain mode-locked lasers
Ultrafast lasers are important in many fields of science, but they typically have high power consumption. Here Eigenwillig et al.realize picosecond laser pulses directly from a semiconductor-based laser. Due to the low repetition rate, high-energy pulses are generated at low average power.
- Christoph M. Eigenwillig
- , Wolfgang Wieser
- & Robert Huber
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Stepwise self-assembly of C60 mediated by atomic scale moiré magnifiers
A promising route towards molecular devices is the self-assembly of atoms or molecules on a surface. Here, Gruznev et al. show that the synthesis of unique geometries of C60molecules on gold–indium-covered crystalline silicon is governed by moiré interference.
- D.V. Gruznev
- , A.V. Matetskiy
- & Y.L. Wang
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Controlled charge trapping by molybdenum disulphide and graphene in ultrathin heterostructured memory devices
Two-dimensional materials such as graphene and molybdenum disulphide are promising for ultrathin electronic devices. Here Choi et al. realize a non-volatile memory device from stacked graphene, boron nitride and molybdenum disulphide films.
- Min Sup Choi
- , Gwan-Hyoung Lee
- & Won Jong Yoo
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Article
| Open AccessThree-photon bosonic coalescence in an integrated tritter
For the development and application of quantum technologies, devices capable of implementing more than two-photon processes are vital. Towards this aim, Spagnolo et al.build a three-port beam splitter and demonstrate mutual interference between the three photons.
- Nicolò Spagnolo
- , Chiara Vitelli
- & Roberto Osellame
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Magnetic spin imaging under ambient conditions with sub-cellular resolution
Detecting the magnetic spins of a small number of atoms is important for applications such as magnetic resonance imaging. Here, Steinert et al.demonstrate that nitrogen-vacancy defect centres in diamond allow spin detection at room temperature at length scales smaller than human cells.
- S. Steinert
- , F. Ziem
- & J. Wrachtrup
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Epitaxial lift-off process for gallium arsenide substrate reuse and flexible electronics
The fabrication of electronic devices depends on semiconductor substrates for device growth. The etching technique implemented here by Cheng et al. allows the reuse of these substrates and suggests a more economic fabrication of electronic devices.
- Cheng-Wei Cheng
- , Kuen-Ting Shiu
- & Devendra K. Sadana
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Article
| Open AccessA magnetic non-reciprocal isolator for broadband terahertz operation
Faraday isolators prevent back reflection of light through photonic systems, and are widespread at optical frequencies. Shalaby et al. show that the permanent magnet SrFe12O19can be used to generate a broadband rotation with low dispersion, and build an isolator suitable for short terahertz pulses.
- Mostafa Shalaby
- , Marco Peccianti
- & Roberto Morandotti
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Stretchable batteries with self-similar serpentine interconnects and integrated wireless recharging systems
Components for flexible electronics capable of both bending and stretching have been reported but the fabrication of similarly pliable power sources remains challenging. Here, the authors present stretchable lithium ion batteries exploiting segmented layouts and deformable electrical interconnects.
- Sheng Xu
- , Yihui Zhang
- & John A. Rogers
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Surface-passivated GaAsP single-nanowire solar cells exceeding 10% efficiency grown on silicon
The use of III-V semiconductor nanowires can overcome the need for lattice matching in multi-junction solar cells, which restricts the choice of materials and their bandgaps. This work demonstrates efficient solar cells with GaAsP single nanowires with tunable bandgap and grown on low-cost Si substrates.
- Jeppe V. Holm
- , Henrik I. Jørgensen
- & Martin Aagesen
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| Open AccessGaAs nanopillar-array solar cells employing in situ surface passivation
Arrays of III–V semiconductor nanopillars are promising photovoltaic materials due to their favourable optical properties, however, they show low power conversion efficiencies. Mariani et al. fabricate a GaAs nanopillar solar cell achieving an efficiency of 6.63% owing to surface passivation.
- Giacomo Mariani
- , Adam C. Scofield
- & Diana L. Huffaker
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Electrical control of neutral and charged excitons in a monolayer semiconductor
Single layers of group-VI transition metal dichalcogenides have emerged as direct bandgap semiconductors in the two-dimensional limit. The authors show that monolayer molybdenum diselenide is an ideal system enabling electrostatic tunability of charging effects in neutral and charged electron-hole pairs, so-called excitons.
- Jason S. Ross
- , Sanfeng Wu
- & Xiaodong Xu
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| Open AccessA polymer tandem solar cell with 10.6% power conversion efficiency
Tandem solar cell structures combine high- and low-bandgap materials, allowing a broader spectral absorption of solar radiation. The authors report the synthesis of a high performance low-bandgap polymer which enables fabrication of a tandem solar cell with a certified power conversion efficiency of 10.6%.
- Jingbi You
- , Letian Dou
- & Yang Yang
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The random mass Dirac model and long-range correlations on an integrated optical platform
Photonic lattices provide a useful platform for simulating quantum dynamics and systems. Keil et al.fabricate coupled waveguides on-chip and use them to simulate the one-dimensional random mass Dirac model, a test-bed for both Dirac fermions and antiferromagnetic spin systems.
- Robert Keil
- , Julia M. Zeuner
- & Alexander Szameit
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Interaction imaging with amplitude-dependence force spectroscopy
Atomic force microscopy provides surface topography images with atomic resolution, but a quantitative measurement of the force while imaging has been missing. Now, Platzet al. present a method based on modulating the cantilever oscillation amplitude to rapidly measure the interaction between tip and surface.
- Daniel Platz
- , Daniel Forchheimer
- & David B. Haviland
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| Open AccessOvercurvature describes the buckling and folding of rings from curved origami to foldable tents
Although foldable structures have found a widespread use in daily life, for example as popup tents, their mathematical properties have been difficult to describe. Mouthuyet al. here present an analytical model that reproduces quantitatively the shape and buckling behaviour of foldable items.
- Pierre-Olivier Mouthuy
- , Michael Coulombier
- & Alain M. Jonas
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Bright e-Paper by transport of ink through a white electrofluidic imaging film
Electronic paper technology is used in displays of portable electronic devices for its low-power consumption; however, it suffers from a sub-optimal reflectance. Hagedon et al.fabricate an electrofluidic film that allows video-rate switching and magazine-quality reflectance in electronic paper.
- M. Hagedon
- , S. Yang
- & J. Heikenfeld
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Bursting drops in solid dielectrics caused by high voltages
Bursting of electrified drops is a fundamental physical process and important for diverse technical applications. Wanget al. find that bursting of electrified drops in polymers is sensitive to the shape of the drops, which in turn is determined by the polymer's elasticity
- Qiming Wang
- , Zhigang Suo
- & Xuanhe Zhao
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| Open AccessLinear magnetoresistance due to multiple-electron scattering by low-mobility islands in an inhomogeneous conductor
Linear magnetoresistance is a phenomenon observed in many material systems and could be used in magnetic field sensors. This paper uncovers its microscopic origin showing how it arises from multiple scattering of electrons by low-mobility islands within an inhomogeneous high-mobility semiconductor.
- N.V. Kozlova
- , N. Mori
- & A. Patanè
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| Open AccessObservation of Landau levels in potassium-intercalated graphite under a zero magnetic field
A signature of the Dirac-like physics of charge carriers in graphene is the occurrence of an anomalous Hall effect, resulting in a quantization of the Landau levels. Guoet al. observe Landau levels of Dirac fermions in potassium-intercalated graphite arising in the absence of an applied magnetic field.
- Donghui Guo
- , Takahiro Kondo
- & Junji Nakamura
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Tunable ferroelectricity in artificial tri-layer superlattices comprised of non-ferroic components
Ferroelectric materials are appealing for use in a range of technological applications. This study demonstrates the onset of ferroelectric behaviour in a superlattice structure that consists of three non-ferroelectric layers, suggesting ferroelectricity can also be induced by interface effects.
- K. Rogdakis
- , J.W. Seo
- & C. Panagopoulos
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Phase-locking to a free-space terahertz comb for metrological-grade terahertz lasers
Frequency comb synthesizers are important for metrology, but they have been difficult to use as frequency rulers in the terahertz region due to their low power. Consolinoet al. phase-lock a quantum cascade laser to a free-space-propagating terahertz comb, demonstrating that they can overcome this limitation.
- L. Consolino
- , A. Taschin
- & P. De Natale
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Spin-enhanced organic bulk heterojunction photovoltaic solar cells
One of the obstacles to improving the efficiency of organic photovoltaic solar cells is the recombination of polaron pairs at the interface between donor and acceptor molecules. By doping cells with galvinoxyl radicals, Zhanget al. demonstrate a mechanism that overcomes this problem via a spin-flip process.
- Ye Zhang
- , Tek P. Basel
- & Z. Valy Vardeny
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Antenna electrodes for controlling electroluminescence
Metallic nanoantennas can be used to enhance and tailor the photoluminescence effects in small-scale devices. Huanget al.design combined nanoantenna electrodes for quantum well nanoscale light-emitting diodes, to both inject charge and control the electroluminescence properties.
- Kevin C.Y. Huang
- , Min-Kyo Seo
- & Mark L. Brongersma
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Article
| Open AccessAmbient fabrication of flexible and large-area organic light-emitting devices using slot-die coating
Light-emitting electrochromic cells are a promising alternative to organic light-emitting diodes, as their performance is less sensitive to fabrication conditions. Here, a roll-to-roll compatible fabrication of such devices is presented, demonstrating large-area continuous production in ambient conditions.
- Andreas Sandström
- , Henrik F. Dam
- & Ludvig Edman
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| Open AccessObservation of resistively detected hole spin resonance and zero-field pseudo-spin splitting in epitaxial graphene
Along with its electronic characteristics, the spin properties of graphene have recently received increasing attention in the context of spintronic applications. Using microwave radiation, Maniet al. identify resistively detected spin resonance in monolayer and trilayer graphene sheets and extract the value for the Landé g-factor.
- Ramesh G. Mani
- , John Hankinson
- & Walter A. de Heer
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Symmetry breaking in the formation of magnetic vortex states in a permalloy nanodisk
Vortex states in magnetic nanoislands are characterized by a curling of the magnetization in the plane of the disk. This study demonstrates experimentally that vortices tend to form with a preferred handedness that is dictated by the Dzyaloshinskii–Moriya interaction.
- Mi-Young Im
- , Peter Fischer
- & Teruo Ono
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Gate-defined quantum confinement in suspended bilayer graphene
The ability to manipulate single charges is a key requisite for novel nanoelectronic devices. Allenet al. show how to electrostatically confine electrons in suspended bilayer graphene quantum dots by local control of the graphene band structure.
- M. T. Allen
- , J. Martin
- & A. Yacoby
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Field-directed sputter sharpening for tailored probe materials and atomic-scale lithography
Scanning probe microscopy and related techniques rely on the availability of very sharp tips. Here, a sharpening technique based on field-directed sputtering is demonstrated, resulting in ultrasharp metallic tips for use in scanning tunnelling microscopy as well as atomic-scale lithographic experiments.
- S.W. Schmucker
- , N. Kumar
- & J.W. Lyding
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Robust classification of salient links in complex networks
Methods to study the structure of complex networks often rely on case-sensitive parameters that have limited applications. In this study, a new method—link salience—is used to classify network elements based on a consensus estimate of all nodes, finding generic topological features in many empirical networks.
- Daniel Grady
- , Christian Thiemann
- & Dirk Brockmann