Abstract
The search for novel topological quantum states has recently moved beyond naturally occurring crystalline materials to complex and engineered systems. In this work we generalize the notion of topological electronic states to random lattices in non-integer dimensions. By considering a class D tight-binding model on critical clusters resulting from a two-dimensional site percolation process, we demonstrate that these topological random fractals exhibit the hallmarks of topological insulators. Specifically, our large-scale numerical studies reveal that topological random fractals display a robust mobility gap, support quantized conductance and represent a well-defined thermodynamic phase of matter. The finite-size scaling analysis further suggests that the critical properties are not consistent with the expectations of class D systems in two dimensions, hinting to the nontrivial relationship between fractal and integer-dimensional topological states. Our results establish topological random fractals as the most complex systems known to support nontrivial band topology with their distinct unique properties.
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Introduction
Since the discovery of the quantum Hall effect, the quantized conductance, dissipationless currents and unconventional edge excitations have captured the fascination of generations of physicists1,2,3,4. These remarkable properties, unlikely from the point of view of traditional solid-state physics, ultimately result from the topology of the electronic spectrum5. Recent efforts have revealed that topological states in naturally occurring materials are ubiquitous in nature6,7,8.
Currently, the research of topological states of matter has moved beyond crystalline solids to amorphous and quasicrystalline systems9,10,11,12,13,14,15,16,17,18,19,20,21,22,23,24,25,26,27,28,29,30,31,32,33,34,35,36,36,37,38,39,40,41,42. While it is not yet clear whether these states of matter exist in nature, they can be realized in artificial designer systems43,44,45,46,46,47,48,49. Besides offering new avenues for functional devices, these systems open a new chapter in the physics of topological matter and the theory of Anderson localization. In this vein, the possibility of topological states in fractals has stirred a new research direction. Despite reported signatures of topology in a number of fractal lattices, many aspect of these systems remains unclear or controversial50,51,52,53,54,55,56,57,58,59,60,61,62. The existence of the spectral gap, possibility of supporting quantized responses and anomalous dependence on system details, such as the coordination number and connectivity of lattice sites, remain under debate. Furthermore, since the studies are mostly restricted to modest-size structures without systematic finite-size scaling analysis, it is not clear whether the finite samples actually represent a well-defined thermodynamic phase of matter.
The research on topological fractals so far has been limited to deterministic self-similar structures. The organization principle of these structures, as of quasicrystals, is completely deterministic without any element of randomness. In contrast, in this work we demonstrate a topological phase on fundamentally more complex self-similar random lattices depicted in Fig. 1. These random fractals are statistically self-similar, i.e. generated from a probability distribution, and characterized by a non-integer spatial dimension63,64. Specifically, we study a symmetry class D Hamiltonian on critical clusters of 2d square lattice percolation. The geometry of the critical percolating cluster is characterized by the fractal dimension \({d}_{{{{{{{{\rm{f}}}}}}}}}=\frac{91}{48}\, < \,2\) (the number of sites within a circle of radius r scales as \({r}^{{d}_{{{{{{{{\rm{f}}}}}}}}}}\) for large r) and a set of standard critical exponents. Our main findings are summarized in the following discoveries: (I) the studied topological random fractals have in general a gapless energy spectrum but exhibit a well-defined mobility gap protecting the topological phase, (II) the studied system supports robust quantized conductance, (III) finite-size scaling analysis show that topological random fractals represent a well-defined thermodynamic phase of matter, (IV) the localization exponent for class D random fractals is incompatible with the universal value ν = 1 in two dimensions. The last property suggests that, despite similarities with topological insulators in integer dimensions where they are embedded, topological random fractals represent a distinct state of matter.
Results
Percolation-generated random fractal lattices
Percolation theory provides a paradigmatic framework to study complex systems in physics and many related fields65,66,67. In this work we consider random lattices arising from a site percolation process on a square lattice where each site is randomly occupied by probability p. There exists a critical concentration 0 < pc < 1, known as the percolation threshold, above which the random lattice has an infinite nearest-neighbour-connected cluster in the thermodynamic limit. Below the threshold, the system consists of disconnected finite clusters. When approaching the percolation threshold, the characteristic length scale of the lattice ξ(p) (the statistical correlation length) diverges as ξ(p) ∝ ∣p − pc∣−4/3, signifying that the percolating critical cluster becomes a scale-free random fractal. The fractal dimension \({d}_{{{{{{{{\rm{f}}}}}}}}}=\frac{91}{48}\) is universal for both site and bond percolation in two dimensions and it can be derived, for example, from a set of other universal critical exponents67. A finite snapshot of a percolating network at p ≠ pc appears indistinguishable from an infinite random fractal up to the correlation length ξ(p).
On a square lattice, the percolation transition takes place at pc ≈ 0.59365,68. In Fig. 1 we have illustrated three finite-size realizations of the random fractals generated by the percolation process (see “Methods” for details). The properties of the critical percolation clusters have been studied in great detail in various contexts65. In striking contrast to all 2d lattices, the fractal spatial dimension of a critical cluster df < 2 means that they do not have a well-separated bulk interior and boundary. As the topological phases typically manifest in protected edge modes, the absence of clear distinction between the interior and the boundary appears disconcerting. Moreover, despite the statistical self-similarity, random fractals exhibit wild sample-to-sample fluctuations. The complexity of random fractals is underlined by the fact that random fractals differ from deterministic fractals in much the same way as amorphous lattices differ from regular lattices. Remarkably, despite the controversial present understanding of topology in deterministic fractals, our results establish that random fractals can support robust topological states.
Model and phase diagram
Next we define a two-band tight-binding model69,70,71 on critical square lattice percolation clusters. The model is determined by the Hamiltonian
where M is the onsite mass parameter and t and t2 represent the hopping amplitudes between the nearest- and second-nearest-neighbour sites on a square lattice provided those sites are present in a given random realization. The matrix \({\eta }_{ij}={\sigma }_{z}+i\cos {\theta }_{ij}{\sigma }_{x}+i\sin {\theta }_{ij}{\sigma }_{y}\) is determined by θij, which denotes the angle between the x axis and the bond vector from site i to site j. The two-component operators \({{{{{{{{\boldsymbol{c}}}}}}}}}_{i}^{{{{\dagger}}} }=({c}_{i,1}^{{{{\dagger}}} },{c}_{i,2}^{{{{\dagger}}} })\) create fermions at site i, and σx,y,z are the Pauli matrices operating in the two-orbital space. The model (1) breaks time-reversal symmetry and satisfies particle-hole symmetry as \({\sigma }_{x}{{\mathbb{H}}}^{* }{\sigma }_{x}=-{\mathbb{H}}\), hence belonging to the symmetry class D71,72,73. On a square lattice in the clean limit, the model supports topological phases with nonzero Chern number. Potentially other symmetry classes may support topology on random fractals as well; the choice to study class D here was made to simplify the large-scale computing efforts, as a minimal model proof-of-concept already poses a substantial computational challenge. In the remainder of this paper, we set t = 1 and express the other parameters in units of t. On a regular lattice, a disordered class D model is known to host a metallic phase which separates the two insulating topological phases. In the case of anisotropic models, an intervening localized phase appears. The localization exponents at metal-insulator and insulator-insulator transitions are known to be νMI ≈ 1.4 and νII = 1, respectively74,75,76,77,78,79,80.
Defining a topological phase on a random fractal poses conceptual challenges. While real-space methods for calculating topological invariants exist, the fractal does not lend itself well to these methods. A more critical issue is the fact that the known methods are defined for integer dimensions, and there are indications that they may not carry the same physical consequences on a fractal of dimension 1 < df < 253,55,81,82. It is even unclear presently whether the mathematical structures that underline the topological classification in integer dimensions can be generalized to fractal dimensions. We bypass these delicate issues by focusing on the possibility of quantized two-terminal conductance G, which we adopt as an operational criterion of nontrivial fractal topology. This is physically motivated by the fact that, irrespective of mathematical definitions, a quantized two-terminal conductance carries direct observational relevance. Furthermore, the only mechanism known to result in robust quantized nonzero conductance plateaus in disordered systems is nontrivial topology.
To numerically evaluate G we employ the KWANT software83, which implements transport calculations using scattering theory84 (see “Methods”). The resulting conductances are calculated at the half-filling E = 0 when not stated otherwise. Figure 2 displays the phase diagram in the (t2, M) plane obtained by calculation of the configuration-averaged conductance. This reveals the existence of a topological phase, which is characterized by quantized conductance G = 1 in the thermodynamic limit, and trivial, insulating regions. As discussed below in the context of finite-size scaling, the topological phase is separated from the trivial phases by a critical line which corresponds to critical conductance Gc ≈ 0.65. The critical point at \(({t}_{2}^{{{{{{{{\rm{c}}}}}}}}},{M}^{{{{{{{{\rm{c}}}}}}}}})\,\approx \,(0,1.1)\) signifies a meeting of three distinct phases, the topological phase, a trivial spectral insulator and a trivial Anderson insulator. A finite second-nearest-neighbour hopping ∣t2∣ > 0 opens up a robust topological phase studied in detail below. In contrast to the sharp spectral insulator-topological fractal phase boundary, identifying the topological fractal-Anderson insulator phase boundary is complicated in finite-size systems due to the fact that both phases are gapless as seen below. The nature of the transition between the trivial spectral and Anderson insulator phases at the t2 = 0 line is illustrated in Fig. 3. In Fig. 3(a), the mid-spectrum density of states indicates the formation of a spectral gap for M < 1.1, while for 1.1 < M < 2.9 the system is in a gapless Anderson-localized phase. However, both phases separated by the tricritical metallic point \(({t}_{2}^{{{{{{{{\rm{c}}}}}}}}},{M}^{{{{{{{{\rm{c}}}}}}}}})\,\approx \,(0,1.1)\) are insulating, as seen in Fig. 3(b). The localization of states in the Anderson insulating phase is further analyzed by the configuration-averaged inverse participation ratio \(\,{{\mbox{IPR}}}\,(E)={\sum }_{i\alpha }| {{{\Psi }}}_{i\alpha }^{E}{| }^{4}\). As can be seen from the inset of the Fig. 3(b), the inverse participation ratio in the region 1.1 < M < 2.9 shows great enhancement around E = 0 everywhere in the Anderson-localized regime, indicating that the spectrum is gapless but consists of trivial localized states.
Topological random fractal phase
Having established the global features of the phase diagram, we now study the properties of the topological random fractal phase in detail. As seen in Fig. 4(a), at the transition point between the spectral insulator and topological random fractal phase, the energy gap closes and remains closed in the topological and Anderson insulator phases. Despite being gapless, and in contrast to the studies of deterministic fractals50,55,57, we uncover unambiguous and robust quantization of conductance in the topological random fractal phase. The formation of the quantized plateau as a function of finite t2 is demonstrated in Fig. 4(b). At the tricritical point \(({t}_{2}^{{{{{{{{\rm{c}}}}}}}}},{M}^{{{{{{{{\rm{c}}}}}}}}})\,\approx \,(0,1.1)\), even a marginal increase of t2 leads to formation of the topological phase with robust conductance quantization. In Fig. 4(c), we have plotted the conductance as a function of the energy (or the chemical potential of the leads) for a number of individual random fractal realizations. All the samples exhibit a finite quantized plateau around E = 0. While the topological random fractal phase is gapless, the topology is protected by a mobility gap. The width of the plateaus in Fig. 4(c), which show sample-to-sample fluctuations, corresponds to the value of the mobility gap. As long as the energy is located in the mobility gap, the conductance (for samples larger than the localization length) remains quantized.
As a testament to the remarkable robustness of the topological states, as the system size grows, the conductance quantization becomes accurate despite the great complexity and variation of different random fractal realizations. As illustrated by histograms in Fig. 4(d), well inside the topological regime, over 90% of configurations with the linear size L = 1600 display conductance quantization with 1% accuracy or better. As seen in Fig. 4(e), the quantization develops rapidly when moving from the tricritical point towards the topological phase. Larger systems exhibit on average more precise quantization, indicating that the random fractal phase is a well-defined thermodynamic phase of matter.
To illustrate that topological random fractals constitute a well-defined thermodynamic phase of matter, we carry out a finite-size scaling study. According to the theory of topological localization transitions, near the transition one expects that the configuration-averaged conductance obeys a single-parameter scaling hypothesis in the large system limit. This hypothesis predicts that the conductance curves for different system sizes collapse to a universal curve \(G=f\left[{L}^{1/\nu }\zeta \right]\), where ζ represents a parameter that drives the transition85. The scaling function f approaches 0 (1) at large negative (positive) arguments. The scaling behaviour indicates that the system undergoes a sharply-defined topological phase transition at ζ = 0 in the thermodynamic limit, separating two distinct phases of matter. The localization length critical exponent ν is expected to be universal for all systems with the same spatial dimension and symmetry class. In particular, for symmetry class D in two dimensions the exponent is ν = 179,80. A high-precision determination of the critical exponents in the topological random fractal is beyond the scope of the present work. However, by calculating the conductance as a function of the second-nearest-neighbour hopping, to explore the validity of the scaling hypothesis \(G=f\left[{L}^{1/\nu }({t}_{2}-{t}_{2}^{{{{{{{{\rm{c}}}}}}}}})\right]\), we can show that the standard two-dimensional class D scaling does not match the numerical evidence. In Fig. 5(a), we employ the value ν = 1 expected for the insulator-insulator phase transition for class D systems in two dimensions. The curves do accurately cross in a single point, indicating that sufficiently close to the critical point, the system sizes L = 300 − 1100 are in the single-parameter scaling regime, but the data clearly do not follow a single curve. As a contrast, as seen in Fig. 5(b) for a higher value exponent ν = 2.4, the curves collapse to a single curve near the critical point. While not yielding a high-precision numerical value for the exponent, the data supports the conclusion that the transition obeys scaling behaviour. The observed substantial departure of the critical exponent from its universal 2d value further suggests that, despite bearing similarities to its integer-dimensional counterpart, the random fractal phase is a genuinely distinct phase of matter with unique critical properties. Additionally, as the curves are accurate near the critical point we can extract the critical conductance Gc ≈ 0.65, which provides the basis for the white dashed line as an approximate phase boundary in Fig. 2.
Discussion
In this work we introduced an electronic state of matter, topological random fractals, and established its central properties. The studied system, supporting robust quantized conductance protected by a mobility gap, constitutes of the first example of a non-integer-dimensional system defined on a random lattice and, in this sense, is the most complex realization of nontrivial band topology known to date. The finite-size scaling results suggest that the topological random fractals belong to a different universality class than their integer-dimensional parent states, calling for further studies on topological fractals. Besides the fundamental interest, there is reason for optimism that such systems will become available for experimental studies in the near future. Technological advances have enabled fabrication of artificial and quantum simulator systems realizing quasicrystalline and fractal electronic structures46,48,49. These advances suggest that experimental realization of topological random fractals may not be far behind.
Methods
Generating random fractals
We construct the studied random lattices by starting with an L × L square lattice, and independently associating a probability p = pc ≈ 0.5927 for each site being populated. After drawing the random populations of all sites from a uniform distribution, we keep a single remaining cluster which connects the left and right edges of the lattice (statistically present in half of the end configurations). To this cluster we associate the Hamiltonian of Eq. (1), modified appropriately by the missing sites and hoppings; in the clean limit this would be a topologically nontrivial system as seen in Fig. 6. Repeating this process many times provides us with a statistical sample of 103 − 104 finite snapshots of infinite random fractal lattices.
Calculation of two-terminal conductance
We employ the KWANT software83 to extract the two-terminal conductances. The obtained L × L random fractal configurations are attached to two identical semi-infinite metallic leads, represented by a set of parallel decoupled 1d chains. As seen in Fig. 7 for a square lattice with leads attached in y-direction, the repeating unit cell is a vertical line of points, such that the open tight-binding chain along y gets repeated in x-direction. We employ large-scale parallel computing to carry out the calculation of the configuration-averaged conductance of up to 104 different random configurations per parameter point for linear system sizes L = 120−1600.
Data availability
The data supporting the findings of this work are available upon reasonable request.
Code availability
The codes implementing the calculations in this work are available upon reasonable request.
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Acknowledgements
The authors acknowledge the Academy of Finland project 331094 for support.
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Authors and Affiliations
Contributions
The project was planned jointly by M.I., I.S., K.P., and T.O. The numerical calculations were carried out by M.I. with some assistance from I.S. All the authors participated in analyzing the results, discussing their interpretation and writing the manuscript.
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Ivaki, M.N., Sahlberg, I., Pöyhönen, K. et al. Topological random fractals. Commun Phys 5, 327 (2022). https://doi.org/10.1038/s42005-022-01101-z
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DOI: https://doi.org/10.1038/s42005-022-01101-z
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