Abstract
Quantum processors use the native interactions between effective spins to simulate Hamiltonians or execute quantum gates. In most processors, the native interactions are pairwise, limiting the efficiency of controlling entanglement between many qubits. The capability of manipulating entanglement generated by higher-order interactions is a key challenge for the simulation of many Hamiltonian models appearing in various fields, including high-energy and nuclear physics, as well as quantum chemistry and error correction applications. Here we experimentally demonstrate control over a class of native interactions between trapped-ion qubits, extending conventional pairwise interactions to a higher order. By exploiting state-dependent squeezing operations, we realize and characterize high-fidelity gates and spin Hamiltonians comprising three- and four-body spin interactions. Our results demonstrate the potential of high-order spin interactions as a toolbox for quantum information applications.
This is a preview of subscription content, access via your institution
Access options
Access Nature and 54 other Nature Portfolio journals
Get Nature+, our best-value online-access subscription
$29.99 / 30 days
cancel any time
Subscribe to this journal
Receive 12 print issues and online access
$209.00 per year
only $17.42 per issue
Buy this article
- Purchase on Springer Link
- Instant access to full article PDF
Prices may be subject to local taxes which are calculated during checkout
Similar content being viewed by others
Data availability
Source data are provided with this paper. Other data that support the findings of this study are available from the corresponding authors on reasonable request.
References
Nielsen, M. A. & Chuang, I. L. Quantum Computation and Quantum Information (Cambridge Univ. Press, 2000).
Monroe, C. et al. Programmable quantum simulations of spin systems with trapped ions. Rev. Mod. Phys. 93, 025001 (2021).
Feng, L. et al. Continuous symmetry breaking in a trapped-ion spin chain. Preprint at arXiv https://doi.org/10.48550/arXiv.2211.01275 (2022).
Mølmer, K. & Sørensen, A. Multiparticle entanglement of hot trapped ions. Phys. Rev. Lett. 82, 1835 (1999).
Kjaergaard, M. et al. Superconducting qubits: current state of play. Annu. Rev. Condens. Matter Phys. 11, 369–395 (2020).
Gross, C. & Bloch, I. Quantum simulations with ultracold atoms in optical lattices. Science 357, 995–1001 (2017).
Banuls, M. C. et al. Simulating lattice gauge theories within quantum technologies. Eur. Phys. J. D 74, 165 (2020).
Ciavarella, A., Klco, N. & Savage, M. J. Trailhead for quantum simulation of SU(3) Yang-Mills lattice gauge theory in the local multiplet basis. Phys. Rev. D 103, 094501 (2021).
Hauke, P., Marcos, D., Dalmonte, M. & Zoller, P. Quantum simulation of a lattice Schwinger model in a chain of trapped ions. Phys. Rev. X 3, 041018 (2013).
Farrell, R. C. et al. Preparations for quantum simulations of quantum chromodynamics in 1+1 dimensions: (I) axial gauge. Phys. Rev. D 107, 054512 (2023).
Pachos, J. K. & Plenio, M. B. Three-spin interactions in optical lattices and criticality in cluster Hamiltonians. Phys. Rev. Lett. 93, 056402 (2004).
Müller, M., Hammerer, K., Zhou, Y., Roos, C. F. & Zoller, P. Simulating open quantum systems: from many-body interactions to stabilizer pumping. New J. Phys. 13, 085007 (2011).
Motrunich, O. I. Variational study of triangular lattice spin-1/2 model with ring exchanges and spin liquid state in κ-(ET)2Cu2(CN)3. Phys. Rev. B 72, 045105 (2005).
Andrade, B. et al. Engineering an effective three-spin Hamiltonian in trapped-ion systems for applications in quantum simulation. Quantum Sci. Technol. 7, 034001 (2022).
Bermudez, A., Porras, D. & Martin-Delgado, M. Competing many-body interactions in systems of trapped ions. Phys. Rev. A 79, 060303 (2009).
Seeley, J. T., Richard, M. J. & Love, P. J. The Bravyi-Kitaev transformation for quantum computation of electronic structure. J. Chem. Phys. 137, 224109 (2012).
O’Malley, P. J. J. et al. Scalable quantum simulation of molecular energies. Phys. Rev. X 6, 031007 (2016).
Nam, Y. et al. Ground-state energy estimation of the water molecule on a trapped-ion quantum computer. NPJ Quantum Inf. 6, 33 (2020).
Aspuru-Guzik, A., Dutoi, A. D., Love, P. J. & Head-Gordon, M. Simulated quantum computation of molecular energies. Science 309, 1704–1707 (2005).
Hempel, C. et al. Quantum chemistry calculations on a trapped-ion quantum simulator. Phys. Rev. X 8, 031022 (2018).
Paetznick, A. & Reichardt, B. W. Universal fault-tolerant quantum computation with only transversal gates and error correction. Phys. Rev. Lett. 111, 090505 (2013).
Kitaev, A. Y. Fault-tolerant quantum computation by anyons. Ann. Phys. 303, 2–30 (2003).
Vedral, V., Barenco, A. & Ekert, A. Quantum networks for elementary arithmetic operations. Phys. Rev. A 54, 147 (1996).
Grover, L. K. A fast quantum mechanical algorithm for database search. In Proc. Twenty-Eighth Annual ACM Symposium on Theory of Computing 212–219 (ACM, 1996).
Wang, X., Sørensen, A. & Mølmer, K. Multibit gates for quantum computing. Phys. Rev. Lett. 86, 3907–3910 (2001).
Monz, T. et al. Realization of the quantum Toffoli gate with trapped ions. Phys. Rev. Lett. 102, 040501 (2009).
Arias Espinoza, J. D., Groenland, K., Mazzanti, M., Schoutens, K. & Gerritsma, R. High-fidelity method for a single-step N-bit Toffoli gate in trapped ions. Phys. Rev. A 103, 052437 (2021).
Figgatt, C. et al. Complete 3-qubit Grover search on a programmable quantum computer. Nat. Commun. 8, 1918 (2017).
Marvian, I. Restrictions on realizable unitary operations imposed by symmetry and locality. Nat. Phys. 18, 283–289 (2022).
Lloyd, S. Universal quantum simulators. Science 273, 1073–1078 (1996).
Bullock, S. S. & Markov, I. L. Asymptotically optimal circuits for arbitrary n-qubit diagonal comutations. Quantum Inf. Comput. 4, 27–47 (2004).
Efimov, V. Energy levels arising from resonant two-body forces in a three-body system. Phys. Lett. B 33, 563–564 (1970).
Kraemer, T. et al. Evidence for Efimov quantum states in an ultracold gas of caesium atoms. Nature 440, 315–318 (2006).
Aaij, R. et al. Observation of J/ψp resonances consistent with pentaquark states in Λb0→J/ψk–p decays. Phys. Rev. Lett. 115, 072001 (2015).
Weimer, H., Müller, M., Lesanovsky, I., Zoller, P. & Büchler, H. P. A Rydberg quantum simulator. Nat. Phys. 6, 382–388 (2010).
Isenhower, L., Saffman, M. & Mølmer, K. Multibit Ck NOT quantum gates via Rydberg blockade. Quantum Inf. Process. 10, 755–770 (2011).
Levine, H. et al. Parallel implementation of high-fidelity multiqubit gates with neutral atoms. Phys. Rev. Lett. 123, 170503 (2019).
Xing, T. H., Zhao, P. Z. & Tong, D. M. Realization of nonadiabatic holonomic multiqubit controlled gates with Rydberg atoms. Phys. Rev. A 104, 012618 (2021).
Khazali, M. & Mølmer, K. Fast multiqubit gates by adiabatic evolution in interacting excited-state manifolds of Rydberg atoms and superconducting circuits. Phys. Rev. X 10, 021054 (2020).
Naidon, P. & Endo, S. Efimov physics: a review. Rep. Prog. Phys. 80, 056001 (2017).
Zahedinejad, E., Ghosh, J. & Sanders, B. C. High-fidelity single-shot Toffoli gate via quantum control. Phys. Rev. Lett. 114, 200502 (2015).
Hill, A. D., Hodson, M. J., Didier, N. & Reagor, M. J. Realization of arbitrary doubly-controlled quantum phase gates. Preprint at arXiv https://doi.org/10.48550/arXiv.2108.01652 (2021).
Kim, Y. et al. High-fidelity three-qubit iToffoli gate for fixed-frequency superconducting qubits. Nat. Phys. 18, 783–788 (2022).
Menke, T. et al. Demonstration of tunable three-body interactions between superconducting qubits. Phys. Rev. Lett. 129, 220501 (2022).
Cirac, J. I. & Zoller, P. Quantum computation with cold trapped ions. Phys. Rev. Lett. 74, 4091–4094 (1995).
Monz, T. et al. Realization of the quantum Toffoli gate with trapped ions. Phys. Rev. Lett. 102, 040501 (2009).
Goto, H. & Ichimura, K. Multiqubit controlled unitary gate by adiabatic passage with an optical cavity. Phys. Rev. A 70, 012305 (2004).
Gambetta, F. M., Zhang, C., Hennrich, M., Lesanovsky, I. & Li, W. Long-range multibody interactions and three-body antiblockade in a trapped Rydberg ion chain. Phys. Rev. Lett. 125, 133602 (2020).
Milburn, G., Schneider, S. & James, D. Ion trap quantum computing with warm ions. Fortschr. Phys. 48, 801–810 (2000).
Solano, E., de Matos Filho, R. L. & Zagury, N. Deterministic Bell states and measurement of the motional state of two trapped ions. Phys. Rev. A 59, R2539–R2543 (1999).
Burd, S. et al. Quantum amplification of boson-mediated interactions. Nat. Phys. 17, 898–902 (2021).
Shapira, Y., Cohen, S., Akerman, N., Stern, A. & Ozeri, R. Robust two-qubit gates for trapped ions using spin-dependent squeezing. Phys. Rev. Lett. 130, 030602 (2023).
Katz, O., Cetina, M. & Monroe, C. N-body interactions between trapped ion qubits via spin-dependent squeezing. Phys. Rev. Lett. 129, 063603 (2022).
Katz, O., Cetina, M. & Monroe, C. Programmable N-body interactions with trapped ions. Preprint at arXiv https://doi.org/10.48550/arXiv.2207.10550 (2022).
Maunz, P. L. W. High Optical Access Trap 2.0. Technical Report (Sandia National Lab, 2016).
Egan, L. et al. Fault-tolerant control of an error-corrected qubit. Nature 598, 281–286 (2021).
Cetina, M. et al. Control of transverse motion for quantum gates on individually addressed atomic qubits. PRX Quantum 3, 010334 (2022).
Olmschenk, S. et al. Manipulation and detection of a trapped Yb+ hyperfine qubit. Phys. Rev. A 76, 052314 (2007).
Egan, L. N. Scaling Quantum Computers with Long Chains of Trapped Ions. PhD thesis, Univ. Maryland (2021).
Sørensen, A. & Mølmer, K. Entanglement and quantum computation with ions in thermal motion. Phys. Rev. A 62, 022311 (2000).
Zhu, S.-L., Monroe, C. & Duan, L.-M. Trapped ion quantum computation with transverse phonon modes. Phys. Rev. Lett. 97, 050505 (2006).
Sackett, C. A. et al. Experimental entanglement of four particles. Nature 404, 256–259 (2000).
Lu, Y. et al. Global entangling gates on arbitrary ion qubits. Nature 572, 363–367 (2019).
Pogorelov, I. et al. Compact ion-trap quantum computing demonstrator. PRX Quantum 2, 020343 (2021).
Figgatt, C. et al. Parallel entangling operations on a universal ion-trap quantum computer. Nature 572, 368–372 (2019).
Shapira, Y., Shaniv, R., Manovitz, T., Akerman, N. & Ozeri, R. Robust entanglement gates for trapped-ion qubits. Phys. Rev. Lett. 121, 180502 (2018).
Wang, Y. et al. High-fidelity two-qubit gates using a microelectromechanical-system-based beam steering system for individual qubit addressing. Phys. Rev. Lett. 125, 150505 (2020).
Leung, P. H. et al. Robust 2-qubit gates in a linear ion crystal using a frequency-modulated driving force. Phys. Rev. Lett. 120, 020501 (2018).
Webb, A. E. et al. Resilient entangling gates for trapped ions. Phys. Rev. Lett. 121, 180501 (2018).
Biamonte, J. et al. Quantum machine learning. Nature 549, 195–202 (2017).
Zhou, L., Wang, S.-T., Choi, S., Pichler, H. & Lukin, M. D. Quantum approximate optimization algorithm: performance, mechanism, and implementation on near-term devices. Phys. Rev. X 10, 021067 (2020).
Cerezo, M. et al. Variational quantum algorithms. Nat. Rev. Phys. 3, 625–644 (2021).
Kandala, A. et al. Hardware-efficient variational quantum eigensolver for small molecules and quantum magnets. Nature 549, 242–246 (2017).
Brown, K. R., Harrow, A. W. & Chuang, I. L. Arbitrarily accurate composite pulse sequences. Phys. Rev. A 70, 052318 (2004).
Acknowledgements
We thank A. Schuckert for useful comments. This work is supported by the ARO through the IARPA LogiQ program; the NSF STAQ and QLCI programs; the DOE QSA program; the AFOSR MURIs on Dissipation Engineering in Open Quantum Systems, Quantum Measurement/Verification and Quantum Interactive Protocols; the ARO MURI on Modular Quantum Circuits; and the DOE HEP QuantISED Program.
Author information
Authors and Affiliations
Contributions
All authors contributed to the experimental design, construction and discussions and wrote the manuscript. O.K. collected the data, and O.K. and L.F. analysed the results. L.F. produced Fig. 1. O.K. produced Figs. 2–4.
Corresponding authors
Ethics declarations
Competing interests
O.K., L.F. and A.R. declare that they have no competing interests. M.C. is a co-inventor of the intellectual property that is licensed by the University of Maryland to IonQ, Inc. C.M. is a co-founder and chief scientist at IonQ, Inc.
Peer review
Peer review information
Nature Physics thanks Christian Schmiegelow and the other, anonymous, reviewer(s) for their contribution to the peer review of this work.
Additional information
Publisher’s note Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Extended data
Extended Data Fig. 1 Experimental sequences.
a, Sequence of displacement operations acting on the two edge ions and composing the MS interaction, enclosing a closed rectangular loop in phase-space and generating the evolution in Fig. 2a. b, Superimposing spin-dependent squeezing operations on the second spin scales the displacement generated by the third spin by a factor \(\exp ({\hat{\sigma }}_{x}^{(2)}\xi )\) and consequently also the enclosed phase-space area. This sequence was applied to the configurations in Fig. 2b–c and in Fig. 3 and Fig. 4a. c, Displacement of the edge two spins and simultaneous squeezing of the middle spins for the four ions configuration presented in Fig. 4b. The simultaneous squeezing scales the displacement generated by the fourth spin by a spin-dependent factor \(\exp ({\hat{\sigma }}_{x}^{(2)}\xi +{\hat{\sigma }}_{x}^{(3)}\zeta\,\, )\) as seen from the identity \({S}^{(m)}(-\xi ){D}_{p}^{(n)}(\pm \alpha ){S}^{(m)}(\xi )={D}_{p}^{(n)}(\pm {e}^{{\hat{\sigma }}_{x}^{(m)}\xi }\alpha )\). The operators \({D}_{p}^{(n)}(\pm \alpha )\) and \({D}_{q}^{(n)}(\pm \alpha )\) denote displacement of the target phonon mode via the nth ion by ± α along the p and q coordinates respectively. S(m)( ± ξ) denotes the squeezing operator acting on ion m and \({R}_{\theta }^{(n)}(\pm \pi )\) denotes short single-qubit π-pulses acting on the n th ion, which commute with the spin-dependent displacement operations and which correct for slowly-varying uncompensated Stark shifts without altering the target state. See Methods for further details.
Supplementary information
Supplementary Information
Supplementary Note 1 and Figs. 1–4.
Source data
Source Data Fig. 2
Data for Fig. 2a–c.
Source Data Fig. 3
Data for Fig. 3a,b.
Source Data Fig. 4
Data for Fig. 4a,b.
Rights and permissions
Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.
About this article
Cite this article
Katz, O., Feng, L., Risinger, A. et al. Demonstration of three- and four-body interactions between trapped-ion spins. Nat. Phys. 19, 1452–1458 (2023). https://doi.org/10.1038/s41567-023-02102-7
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1038/s41567-023-02102-7
This article is cited by
-
Continuous symmetry breaking in a trapped-ion spin chain
Nature (2023)