Abstract
The Pancharatnam–Berry phase is a geometric phase acquired over a cycle of parameters in the Hamiltonian governing the evolution of the system. Here, we report on the observation of the Pancharatnam–Berry phase in a condensate of indirect excitons (IXs) in a GaAscoupled quantum well structure. The Pancharatnam–Berry phase is directly measured by detecting phase shifts of interference fringes in IX interference patterns. Correlations are found between the phase shifts, polarization pattern of IX emission, and onset of IX spontaneous coherence. The evolving Pancharatnam–Berry phase is acquired due to coherent spin precession in IX condensate and is observed with no decay over lengths exceeding 10 μm indicating longrange coherent spin transport.
Introduction
The Pancharatnam–Berry phase was discovered by Pancharatnam in studies of polarized light^{1} and introduced by Berry as a topological phase for matter wave functions^{2}. For light, the Pancharatnam–Berry phase is measured in laser interferometers^{3,4} and exploited in optical elements^{5,6}. Excitons are matter waves that directly transform to photons inheriting their coherence and polarization. This makes excitons a unique interface between matter and light and a unique system for exploring the Pancharatnam–Berry phase for matter waves by light interference experiments.
Recent studies led to the discovery of polarization textures in light emission of indirect excitons (IXs)^{7,8,9,10,11,12,13,14,15,16} and exciton–polaritons^{17,18,19}. The Pancharatnam–Berry phase appears when the polarization state of light changes^{1}. This connection of the Pancharatnam–Berry phase to polarization makes it an intrinsic phenomenon for polarization textures.
An IX is a bound pair of an electron and a hole confined in spatially separated layers. IXs are realized in coupled quantum well (CQW) structures. Due to their long lifetimes IXs can cool below the temperature of quantum degeneracy and form a condensate in momentum (k) space^{7}. IX condensation is detected by measurement of IX spontaneous coherence with a coherence length much larger than in a classical gas^{7}. The large coherence length observed in an IX condensate, reaching ~10 μm, indicates coherent IX transport with suppressed scattering^{7}, in agreement with theory^{20}.
A cold IX gas is realized in the regions of the external ring and localized bright spot (LBS) rings in the IX emission^{7,8}. These rings form on the boundaries of electronrich and holerich regions created by current through the structure and optical excitation, respectively; see ref. ^{21} and references therein. An LBS is a stable, well defined, and tunable source of cold IXs^{21}, thus an ideal system for studying coherence and polarization phenomena. Different LBS offer IX sources of different strength and spatial extension; furthermore, these parameters can be controlled by optical excitation and voltage^{21}. This variability gives the opportunity to measure correlations between coherence and polarization. Here, we explore LBS to uncover the Pancharatnam–Berry phase in a condensate of IXs.
Results
Experiment
Figure 1b shows the interference pattern of IX emission measured by shiftinterferometry: The emission images produced by each of the two arms of the Mach–Zehnder interferometer are shifted with respect to each other to measure the interference between the emission of IXs separated by δr in the CQW plane (Supplementary Note 3).
Spontaneous coherence of matter waves is equivalent to condensation of particles in kspace. The Fourier transform of the firstorder coherence function g_{1}(δx) gives the particle distribution n_{ k }. The width of g_{1}(δx), the coherence length ξ, is inversely proportional to the width of n_{ k }. In a classical gas, ξ is close to the thermal de Broglie wavelength λ_{dB} = (2πħ^{2}/mT)^{1/2} and is small (λ_{dB} ~ 0.5 μm for IXs with m = 0.22m_{0} at T = 0.1 K). The measurement of spontaneous coherence with \(\xi \gg \lambda _{{\mathrm{dB}}}\) is a direct measurement of Bose–Einstein condensation.
The measured amplitude of interference fringes A_{interf}(δx) is given by the convolution of g_{1}(δx) with the pointspread function (PSF) of the optical system^{22}. The PSF width corresponds to the spatial resolution (~1.5 μm in this experiment). For a classical IX gas, g_{1}(δx) is narrow and A_{interf}(δx) fits well to the PSF, while for the IX condensate, g_{1}(δx) and, in turn, A_{interf}(δx) extend to large δx^{7}. While a more detailed picture is obtained by measuring g_{1}(δx) as in ref. ^{7}, mapping IX condensate can be done by measuring A_{interf}(x, y) at one value of δx chosen to exceed both λ_{dB} and the PSF width. For such δx, a low A_{interf} is observed for a classical gas and a high A_{interf} for the condensate. For the parameters of our system, δx = 2 μm is optimal for this experiment.
The IX gas is classical close to the heating sources in the LBS central region (this heating is due to the current filament at the LBS centre and the binding energy released at IX formation^{21}). This is revealed by the small amplitude of the interference fringes A_{interf} at r < r_{coh} (Fig. 1c). Away from the heating sources, IXs cool down and approach the condensation temperature. At r = r_{coh}, A_{interf} sharply rises, indicating the condensation.
Figure 1b, d shows that the phase of interference fringes sharply changes at the distance from the LBS centre r = r_{phase}. The comparison of Fig. 1b–d shows that the phase shifts occur at the same location as condensation, r_{phase} = r_{coh}.
The phase shifts are sharp in the circular region around each LBS. However smoother phase shifts can be followed further (as shown by dashed magenta lines in Fig. 1b). The lines embracing the phase domains of interference fringes end by left and rightforks of interference fringes at the opposite ends of the domain (the forks are shown by circles in Fig. 1b), indicating that the forks originate from the phase domains.
To uncover the origin of the phase shifts and associated phase domains of interference fringes, we compare their locations with the pattern of linear polarization of IX emission (Fig. 1e). A ring of linear polarization is seen for each LBS in the region r < r_{linear} where the IX gas is classical, r_{linear} = r_{coh} (compare Fig. 1c, e). This linear polarization originates from the distribution of IXs over the linearly polarized IX states^{8}. A helical IX polarization texture winding by 2π around the origin, i.e. a vortex of linear polarization, emerges at r > r_{linear} where the IX condensate forms (Fig. 1e).
The comparison of Fig. 1b–e shows that for all LBS sources, the phase shifts of interference fringes are observed when the polarization state of IX emission sharply changes. To examine this relationship, we measured IX coherence and polarization patterns at different laser exciation powers P. As in ref. ^{21}, we also adjusted the applied voltage V keeping the external ring radius constant. The simultaneous increase of P and V leads to the enhancement of both electron and hole sources and, as a result, the exciton source at each LBS.
Increasing the excitation power increases r_{phase} (Fig. 2a, b), r_{linear} (Fig. 2c, d), and r_{coh} (Fig. 2e, f). The increase of r_{coh} with P follows an enhanced heating at the LBS central region due to the enhanced electron and hole sources. Figure 2 shows that r_{linear} stays equal to r_{coh} with increasing P, confirming that the polarization textures appear in the IX condensate, in agreement with theory^{7,8}. Remarkably, Fig. 2 shows that r_{phase} also keeps equal to r_{linear} with increasing P.
We found a universal relationship between r_{phase} and r_{linear} measured for many LBS over a broad range of P. Large variations of both r_{phase} and r_{linear} are observed for different LBS and P (Fig. 3a, b). However, all data collapse on a universal line r_{phase} = r_{linear} (Fig. 3c). Slight deviation of the slope of the line r_{phase}(r_{linear}) from 1 may be related to the calibration accuracy (Supplementary Note 3).
The phase of IX wave function ψ(r) acquired as IXs propagate from the origin can be derived from the interference pattern simulated using I_{interf}(r) = \(\left {\psi ({\bf{r}}  \delta {\bf{r}}{\mathrm{/}}2) + {\mathrm {e}}^{{\mathrm {i}}q_ty}\psi ({\bf{r}} + \delta {\bf{r}}{\mathrm{/}}2)} \right^2\), where q_{ t } = 2πα/λ sets the period of the interference fringes, α is a small tilt angle between the image planes of the interferometer arms, and λ is the emission wavelength. Figure 4a–c show the simulated I_{interf}(x, y) for ψ(r) = e^{ik·r} and the shift δx = 2 μm for IXs radially propagating from the origin with a small k (Fig. 4a), with a larger k (Fig. 4b), and with the small k at r < r_{ k } and larger k at r > r_{ k } (Fig. 4c). For k = 0, the interference fringes are parallel lines separated by D = λ/α. A deviation of the Nth fringe from its zerok position is given by δy_{ N } = −D/(2π)·k_{ x }δx. Phase shifts of interference fringes, i.e., jumps in δy_{ N }, correspond to jumps in k (Fig. 4c). The values of k at r < r_{k} and r > r_{k} in Fig. 4c were selected to qualitatively reproduce the measured I_{interf} in Fig. 1 and illustrate a jump in k at r = r_{phase}.
The x and y components of k were derived by fitting the patterns of interference fringes measured for shifts in the x and y directions using k_{ x }(x, y) = −2π/D · δy_{ N }(x, y)/δx and k_{ y }(x, y) = −2π/D · δy_{ N }(x, y)/δy, respectively. The positions of faint interference fringes at r < r_{coh} and pronounced interference fringes at r > r_{coh} were used in the estimate of k. This allowed obtaining a map of IX momentum k describing the evolving IX phase (Fig. 4d). This map shows that IXs propagate away from the LBS source and sharply acquire an additional evolving phase ϕ = kr at r = r_{phase}. This phase is revealed in Fig. 4d by a jump in associated momentum k.
The experiment shows that the phase shifts correlate with the polarization pattern of IX emission and onset of IX spontaneous coherence. The correlation between the phase shift and the polarization change identifies the phase as the Pancharatnam–Berry phase acquired in a condensate of IXs. This phenomenon is discussed below.
The spatial separation of an electron and a hole in an IX reduces the overlap of the electron and hole wave functions suppressing the spin relaxation mechanism due to electron–hole exchange^{23}. In a classical IX gas, spin transport in the studied structure is limited by 1−2 μm^{24} due to Dyakonov–Perel spin relaxation^{25}. As a result, for uncondensed IXs at r < r_{coh}, the spin relaxation is fast and coherent spin precession is not observed. However, the suppression of scattering in IX condensate results in the suppression of the Dyakonov–Perel and Elliott–Yafet mechanisms of spin relaxation^{25} enabling longrange coherent spin transport in IX condensate. Therefore, IX condensation at r > r_{coh} dramatically enhances the spin relaxation time leading to coherent spin precession and, in turn, precession of the polarization state of IX emission. This precession generates the evolving Pancharatnam–Berry phase of IXs, which is detected as the shift of interference fringes. Figure 4d shows that no decay of the evolving Pancharatnam–Berry phase is observed over macroscopic lengths exceeding 10 μm. This indicates the achievement of macroscopic longrange coherent spin transport in the IX condensate.
Simulation
To demonstrate a concept of the Pancharatnam–Berry phase acquired due to the IX spin precession, we simulate the polarization evolution within the model of IX spin precession^{8} (a brief description is given in Supplementary Note 4). We use the electron and hole spin–orbit interaction constants and splittings between four IX states (with spin projections J_{ z } = ±2, ±1) obtained to fit the IX polarization patterns^{8}. The initial polarization in the simulations is taken as horizontal to follow the experiment (Fig. 1e).
The simulated S1 component of Stokes’ vector corresponding to linear polarization of IX emission is presented in Fig. 5a, b. The polarization shows an oscillatory behaviour. Its longscale component is responsible for the polarization pattern shown in Fig. 1e and studied earlier in ref. ^{8}. The shortscale component has the spatial period ~0.3 μm and is not resolved with 1.5 μm optical resolution in the imaging experiment. However, these fast changes of the polarization state generate the evolving Pancharatnam–Berry phase of IXs. Figure 5c shows the simulated IX polarization state on the Poincaré sphere for one fast polarization oscillation cycle in Fig. 5a. The IX polarization state goes over a nearly closed contour on the Poincaré sphere. The Pancharatnam–Berry phase acquired by IXs over this contour can be estimated by connecting the initial and final points and calculating half the solid angle subtended by the obtained contour at the centre of the sphere, Ω/2 (ref. ^{1}). In turn, a momentum k_{PB} associated with the acquired Pancharatnam–Berry phase can be estimated as ~Ω/(2l) where l is the IX path passed during the polarization cycle. For Ω/2 ~ π/2 (Fig. 5c) and l ~ 0.3 μm (Fig. 5a, b), this gives k_{PB} ~ 5 μm^{−1}, in qualitative agreement with the jump in IX momentum (Fig. 4d), which occurs when the coherent spin precession generating the evolving Pancharatnam–Berry phase starts in IX condensate.
In summary, shiftinterferometry and polarization imaging show that the phase shifts of interference fringes correlate with the polarization pattern of IX emission and onset of IX spontaneous coherence, demonstrating the Pancharatnam–Berry phase in a condensate of IXs. The measured Pancharatnam–Berry phase indicates longrange coherent spin transport.
Methods
The experiments are performed on n − i − n GaAs/AlGaAs CQW structure. The i region consists of a single pair of 8nm GaAs QWs separated by a 4nm Al_{0.33}Ga_{0.67}As barrier and surrounded by 200nm Al_{0.33}Ga_{0.67}As layers. The n layers are Sidoped GaAs with Si concentration 5 × 10^{17} cm^{−3}. The indirect regime where IXs form the ground state is realized by the voltage applied between n layers. The small inplane disorder in the CQW is indicated by the emission linewidth of 1 meV. IXs cool to temperatures within ~50 mK of the lattice temperature^{26}, which was lowered to 100 mK in an optical dilution refrigerator. This cools IXs well below the temperature of quantum degeneracy, which is in the range of a few kelvin for typical IX density 10^{10} cm^{−2}(ref. ^{26}). The laser excitation is performed by a 633 nm HeNe laser. It is more than 400 meV above the energy of IXs and farther than 80 μm away from the studied region. Therefore, IX coherence and polarization are not induced by photoexcitation and form spontaneously. LBS are sources of cold IXs due to their separation from the laser excitation spot.
Data availability
All relevant data are available from the authors.
References
 1.
Pancharatnam, S. Generalized theory of interference and it’s applications. Proc. Indian Acad. Sci. A 44, 247–262 (1956).
 2.
Berry, M. V. Quantal phase factors accompanying adiabatic changes. Proc. R. Soc. Lond. A 392, 45–57 (1984).
 3.
Bhandari, R. & Samuel, J. Observation of topological phase by use of a laser interferometer. Phys. Rev. Lett. 60, 1211–1213 (1988).
 4.
Simon, R., Kimble, H. J. & Sudarshan, E. C. G. Evolving geometric phase and its dynamical manifestation as a frequency shift: an optical experiment. Phys. Rev. Lett. 61, 19–22 (1988).
 5.
Bomzon, Z., Biener, G., Kleiner, V. & Hasman, E. Spacevariant PancharatnamBerry phase optical elements with computergenerated subwavelength gratings. Opt. Lett. 27, 1141 (2002).
 6.
Devlin, R. C. et al. Spintoorbital angular momentum conversion in dielectric metasurfaces. Opt. Express 25, 377–393 (2017).
 7.
High, A. A. et al. Spontaneous coherence in a cold exciton gas. Nature 483, 584–588 (2012).
 8.
High, A. A. et al. Spin currents in a coherent exciton gas. Phys. Rev. Lett. 110, 246403 (2013).
 9.
Wu, C. & MondragonShem, I. Exciton condensation with spontaneous timereversal symmetry breaking. arXiv:0809.3532v1; Wu, CongJun, MondragonShem, Ian, Zhou, XiangFa. Chin. Phys. Lett. 28, 097102 (2011).
 10.
Matuszewski, M., Liew, T. C. H., Rubo, Y. G. & Kavokin, A. V. Spinorbit coupling and the topology of gases of spindegenerate cold excitons in photoexcited GaAsAlGaAs quantum wells. Phys. Rev. B 86, 115321 (2012).
 11.
Kyriienko, O., Magnusson, E. B. & Shelykh, I. A. Spin dynamics of cold exciton condensates. Phys. Rev. B 86, 115324 (2012).
 12.
Vishnevsky, D. V. et al. Skyrmion formation and optical spinHall effect in an expanding coherent cloud of indirect excitons. Phys. Rev. Lett. 110, 246404 (2013).
 13.
Kavokin, A. V. et al. Ballistic spin transport in exciton gases. Phys. Rev. B 88, 195309 (2013).
 14.
Sigurdsson, H., Liew, T. C. H., Kyriienko, O. & Shelykh, I. A. Vortices in spinor cold exciton condensates with spinorbit interaction. Phys. Rev. B 89, 035302 (2014).
 15.
Bardyn, C.E., Karzig, T., Refael, G. & Liew, T. C. H. Topological polaritons and excitons in gardenvariety systems. Phys. Rev. B 91, 161413(R) (2015).
 16.
Li, Yi, Zhou, X. & Wu, C. Threedimensional quaternionic condensations, Hopf invariants, and skyrmion lattices with synthetic spinorbit coupling. Phys. Rev. A 93, 033628 (2016).
 17.
Kavokin, A., Malpuech, G. & Glazov, M. Optical spin Hall effect. Phys. Rev. Lett. 95, 136601 (2005).
 18.
Leyder, C. et al. Observation of the optical spin Hall effect. Nat. Phys. 3, 628–631 (2007).
 19.
Cilibrizzi, P. et al. Polariton spin whirls. Phys. Rev. B 92, 155308 (2015).
 20.
Lozovik, Yu. E. & Yudson, V. I. A new mechanism for superconductivity: pairing between spatially separated electrons and holes. Sov. Phys. JETP 44, 389–397 (1976).
 21.
Yang, S., Butov, L. V., Simons, B. D., Campman, K. L. & Gossard, A. C. Fluctuation and commensurability effect of exciton density wave. Phys. Rev. B 91, 245302 (2015).
 22.
Fogler, M. M., Yang, S., Hammack, A. T., Butov, L. V. & Gossard, A. C. Effect of spatial resolution on the estimates of the coherence length of excitons in quantum wells. Phys. Rev. B 78, 035411 (2008).
 23.
Maialle, M. Z., de Andrada e Silva, E. A. & Sham, L. J. Exciton spin dynamics in quantum wells. Phys. Rev. B 47, 15776–15788 (1993).
 24.
Leonard, J. R. et al. Spin transport of excitons. Nano Lett. 9, 4204–4208 (2009).
 25.
Dyakonov, M. I. Spin Physics in Semiconductors. (Springer, New York, 2008).
 26.
Butov, L. V., Ivanov, A. L., Imamoglu, A., Littlewood, P. B., & Shashkin, A. A. et al. Stimulated scattering of indirect excitons in coupled quantum wells: signature of a degenerate BoseGas of excitons. Phys. Rev. Lett. 86, 5608–5611 (2001).
Acknowledgements
We thank Lu Sham and Congjun Wu for discussions. These studies were supported by DOE Office of Basic Energy Sciences under award DEFG0207ER46449 and coherence studies by NSF Grant No. 1640173 and NERC, a subsidiary of SRC, through the SRCNRI Center for Excitonic Devices.
Author information
Affiliations
Contributions
All authors contributed to the work presented in this paper.
Corresponding author
Correspondence to J. R. Leonard.
Ethics declarations
Competing interests
The authors declare no competing interests.
Additional information
Publisher's note: Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Electronic supplementary material
Rights and permissions
Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
About this article
Cite this article
Leonard, J.R., High, A.A., Hammack, A.T. et al. Pancharatnam–Berry phase in condensate of indirect excitons. Nat Commun 9, 2158 (2018). https://doi.org/10.1038/s4146701804667x
Received:
Accepted:
Published:
Further reading

Indirect Excitons and Trions in MoSe2/WSe2 van der Waals Heterostructures
Nano Letters (2020)

Condensation of indirect excitons
MRS Bulletin (2020)

Emergence of the geometric phase from quantum measurement backaction
Nature Physics (2019)

Dynamical formation of a strongly correlated dark condensate of dipolar excitons
Proceedings of the National Academy of Sciences (2019)

Highmobility indirect excitons in wide single quantum well
Applied Physics Letters (2018)
Comments
By submitting a comment you agree to abide by our Terms and Community Guidelines. If you find something abusive or that does not comply with our terms or guidelines please flag it as inappropriate.