Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

  • Letter
  • Published:

Nano Josephson superconducting tunnel junctions in YBa2Cu3O7–δ directly patterned with a focused helium ion beam

Abstract

Since the discovery of the high-transition-temperature superconductors (HTSs), researchers have explored many methods to fabricate superconducting tunnel junctions from these materials for basic science purposes and applications. HTS circuits operating at liquid-nitrogen temperatures (77 K) would significantly reduce power requirements in comparison with those fabricated from conventional superconductors. The difficulty is that the superconducting coherence length is very short and anisotropic in these materials, typically 2 nm in the a–b plane and 0.2 nm along the c axis. The electrical properties of Josephson junctions are therefore sensitive to chemical variations and structural defects on atomic length scales1. To make multiple uniform HTS junctions, control at the atomic level is required. In this Letter we demonstrate all-HTS Josephson superconducting tunnel junctions created by using a 500-pm-diameter focused beam of helium ions to directly write tunnel barriers into YBa2Cu3O7−δ (YBCO) thin films. We demonstrate the ability to control the barrier properties continuously from conducting to insulating by varying the irradiation dose. This technique could provide a reliable and reproducible pathway for scaling up quantum-mechanical circuits operating at liquid-nitrogen temperatures, as well as an avenue to conduct novel planar superconducting tunnelling studies for basic science.

This is a preview of subscription content, access via your institution

Access options

Buy this article

Prices may be subject to local taxes which are calculated during checkout

Figure 1: Focused helium ion beam Josephson junction fabrication.
Figure 2: Electrical transport measurements for an SNS Josephson junction fabricated using a dose of 2 × 1016 He+ per cm2 and for a SIS Josephson junction fabricated with a dose of 6 × 1016He+ per cm2.
Figure 3: Measurements of the energy gap of the SIS Josephson junction at higher bias currents.

Similar content being viewed by others

References

  1. Koelle, D., Kleiner, R., Ludwig, F., Dantsker, E. & Clarke, J. High-transition-temperature superconducting quantum interference devices. Rev. Mod. Phys. 71, 631–686 (1999).

    Article  CAS  Google Scholar 

  2. Tsai, J. et al. Tunneling study of clean and oriented Y-Ba-Cu-O and Bi-Sr-Ca-Cu-O surfaces. Physica C 157, 537–550 (1989).

    Article  CAS  Google Scholar 

  3. Yi, H. R., Winkler, D. & Claeson, T. Tunneling through grain boundaries of YBa2Cu3O7 step-edge junctions. Appl. Phys. Lett. 68, 2562–2564 (1996).

    Article  CAS  Google Scholar 

  4. Hirata, K. et al. Tunneling measurements on superconductor/insulator/superconductor junctions using single-crystal YBa2Cu3O7−x thin films. Appl. Phys. Lett. 56, 683–685 (1990).

    Article  CAS  Google Scholar 

  5. Kusumori, T. & Iguchi, I. Fabrication of YBCO/CeO2/YBCO multilayer junctions and their characteristics. Jpn J. Appl. Phys. 31, L956–L959 (1992).

    Article  CAS  Google Scholar 

  6. Bari, M. et al. C-axis tunneling in YBa2Cu3O7−δ trilayer junctions with PrBa2Cu3O7−δ barrier. Physica C 256, 227–235 (1996).

    Article  CAS  Google Scholar 

  7. Ward, B. W., Notte, J. A. & Economou, N. P. Helium ion microscope: a new tool for nanoscale microscopy and metrology. J. Vac. Sci. Technol. B 24, 2871–2874 (2006).

    Article  CAS  Google Scholar 

  8. Clark, G. J., Marwick, A. D., Koch, R. H. & Laibowitz, R. B. Effects of radiation damage in ion-implanted thin films of metal-oxide superconductors. Appl. Phys. Lett. 51, 139–141 (1987).

    Article  CAS  Google Scholar 

  9. Pauza, A., Campbell, A., Moore, D., Somekh, R. E. & Broers, A. High-TC Josephson junctions by electron beam irradiation. IEEE Trans. Appl. Supercond. 3, 2405–2408 (1993).

    Article  Google Scholar 

  10. Tolpygo, S. K. et al. High quality YBa2Cu3O7 Josephson junctions made by direct electron beam writing. Appl. Phys. Lett. 63, 1696–1698 (1993).

    Article  CAS  Google Scholar 

  11. Tinchev, S. S. Investigation of RF SQUIDs made from epitaxial YBCO films. Supercond. Sci. Tech. 3, 500–503 (1990).

    Article  CAS  Google Scholar 

  12. Chen, K., Cybart, S. A. & Dynes, R. C. Planar thin film YBa2Cu3O7−δ Josephson junction pairs and arrays via nanolithography and ion damage. Appl. Phys. Lett. 85, 2863–2865 (2004).

    Article  CAS  Google Scholar 

  13. Bergeal, N. et al. High-quality planar high-Tc Josephson junctions. Appl. Phys. Lett. 87, 102502 (2005).

    Article  Google Scholar 

  14. Cybart, S. A., Anton, S. M., Wu, S. M., Clarke, J. & Dynes, R. C. Very large scale integration of nanopatterned YBa2Cu3O7−δ Josephson junctions in a two-dimensional array. Nano Lett. 9, 3581–3585 (2009).

    Article  CAS  Google Scholar 

  15. Chen, K., Cybart, S. A. & Dynes, R. C. Study of closely spaced YBa2Cu3O7−δ Josephson junction pairs. IEEE Trans. Appl. Supercond. 15, 149–152 (2005).

    Article  CAS  Google Scholar 

  16. Blonder, G., Tinkham, M. & Klapwijk, T. Transition from metallic to tunneling regimes in superconducting microconstrictions: excess current, charge imbalance, and supercurrent conversion. Phys. Rev. B 25, 4515–4532 (1982).

    Article  CAS  Google Scholar 

  17. Stewart, W. C. Current–voltage characteristics of Josephson junctions. Appl. Phys. Lett. 12, 277–280 (1968).

    Article  Google Scholar 

  18. McCumber, D. E. Effect of ac impedance on dc voltage–current characteristics of superconductor weak-link junctions. J. Appl. Phys. 39, 3113–3118 (1968).

    Article  Google Scholar 

  19. Cybart, S. A., Chen, K. & Dynes, R. C. Planar YBa2Cu3O7–δ ion damage Josephson junctions and arrays. IEEE Trans. Appl. Supercond. 15, 241–244 (2005).

    Article  CAS  Google Scholar 

  20. Lang, W. et al. Tailoring the transport properties of YBa2Cu3O7–δ thin films by light–ion irradiation. Inst. Phys. Conf. Ser. 181, 1549–1555 (2004).

    Google Scholar 

  21. Rosenthal, P. A., Beasley, M. R., Char, K., Colclough, M. S. & Zaharchuk, G. Flux focusing effects in planar thin-film grain-boundary Josephson junctions. Appl. Phys. Lett. 59, 3482–3484 (1991).

    Article  CAS  Google Scholar 

  22. Humphreys, R. & Edwards, J. YBa2Cu3O7 thin film grain boundary junctions in a perpendicular magnetic field. Physica C 210, 42–54 (1993).

    Article  CAS  Google Scholar 

  23. Clem, J. R. Josephson junctions in thin and narrow rectangular superconducting strips. Phys. Rev. B 81, 144515 (2010).

    Article  Google Scholar 

  24. Clarke, J. & Braginski, A. I. The SQUID Handbook Vol II Applications of SQUIDs and SQUID Systems (Wiley-VCH, 2006).

    Book  Google Scholar 

  25. Kornev, V. K., Soloviev, I. I., Klenov, N. V., Sharafiev, A. & Mukhanov, O. A. Array designs for active electrically small superconductive antennas. Physica C 479, 119–122 (2012).

    Article  CAS  Google Scholar 

  26. Cybart, S. A. et al. Large voltage modulation in magnetic field sensors from two-dimensional arrays of Y-Ba-Cu-O nano Josephson junctions. Appl. Phys. Lett. 104, 062601 (2014).

    Article  Google Scholar 

  27. Cybart, S. A. et al. Large scale two-dimensional arrays of magnesium diboride superconducting quantum interference devices. Appl. Phys. Lett. 104, 182604 (2014).

    Article  Google Scholar 

Download references

Acknowledgements

This work was supported by the Office of Science and Office of Basic Energy Sciences of the US Department of Energy (contract no. DEAC02 05CH11231) and by an AFOSR grant (FA9550-07-1-0493). M.M. and B.W. were supported by the UC scholars programme. The authors thank G. Schlenvogt for help with ion implantation simulations, K. Chen and P. Roediger for experimental discussions, J. Wu for help with the BCS fit, and K.D. Derr, B. Goetze and J. Notte for helping with setting up the experiment.

Author information

Authors and Affiliations

Authors

Contributions

S.A.C. conceived the experiment and wrote the manuscript. S.A.C., E.Y.C. and C.H. fabricated the devices. All authors provided technical and scientific insight that contributed to characterization of the devices and interpretation of the results.

Corresponding author

Correspondence to Shane A. Cybart.

Ethics declarations

Competing interests

The authors declare no competing financial interests.

Supplementary information

Supplementary information

Supplementary information (PDF 1828 kb)

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Cybart, S., Cho, E., Wong, T. et al. Nano Josephson superconducting tunnel junctions in YBa2Cu3O7–δ directly patterned with a focused helium ion beam. Nature Nanotech 10, 598–602 (2015). https://doi.org/10.1038/nnano.2015.76

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1038/nnano.2015.76

This article is cited by

Search

Quick links

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing