Time-reversal invariant topological insulator is widely recognized as one of the fundamental discoveries in condensed matter physics, for which the most fascinating hallmark is perhaps a spin-based topological protection, the absence of scattering of conduction electrons with certain spins on matter surface. Recently, it has created a paradigm shift for topological insulators, from electronics to photonics, phononics and mechanics as well, bringing about not only involved new physics but also potential applications in robust wave transport. Despite the growing interests in topologically protected acoustic wave transport, T-invariant acoustic topological insulator has not yet been achieved. Here we report experimental demonstration of anomalous Floquet topological insulator for sound: a strongly coupled metamaterial ring lattice that supports one-way propagation of pseudo-spin-dependent edge states under T-symmetry. We also demonstrate the formation of pseudo-spin-dependent interface states due to lattice dislocations and investigate the properties of pass band and band gap states.
The study of topological properties or invariants in periodic physical systems has become one of the most active fields in many branches of physics1,2,3,4,5,6,7,8,9,10,11,12,13,14,15,16,17,18,19,20. As basic elements of topological band theory, these topological invariants are very interesting, because they imply the presence of non-trivial bulk topologies, giving rise to the presence of gapless edge or surface states featured with the absence of scatterings. Probably the most well-known example should be the integer quantum Hall effect discovered by Klitzing et al.21 under strong magnetic fields and low temperatures, where the quantized Hall conductivity is insensitive to local perturbations and the quantization (TKNN integer) was afterwards discovered to have an expression of the first Chern number of the bands below the chemical potential22. Another seminal work is the Kane and Mele model, dealing with time-reversal (T) invariant systems of strong spin–orbit couplings23. In that work, Kane and Mele23 introduce a distinctive Z2 index to describe the T-invariant quantum spin Hall phase that has a spin-dependent topological protection and robustness against non-magnetic disorder and interactions under T-symmetry. The new topological phase in the presence of T-symmetry was later termed topological insulators, now widely recognized as a fundamental discovery in condensed matter physics1,2,3,4,5.
In the past decade, exploration for new types of topological insulators is substantively followed up in different subfields of physics, making a paradigm shift for topological states, from electronics to photonics6,7,8,9,10,11,12,24,25, phononics13,14 as well as mechanics15,16,17. In photonics, the field of topological insulators is rapidly developing in the past few years, where one of most representative example should be the Floquet topological insulator, proposed in periodically driven systems. There are basically two types of Floquet topological insulator. One is based on temporal modulation26. As the time reversal symmetry is broken, such topological insulator can support non-trivial one-way edge states that are immune to disorder-induced backscattering. The other relies on the three-dimensional chiral couplings9, where the z direction wave evolution can be mapped into the temporal modulation in the x–y plane. In reality, it is quite challenging to realize very fast temporal modulation or fabricate delicate three-dimensional helical waveguide array on chip. A more attractive solution is proposed by Hafezi et al.7,8 employing a two-dimensional (2D) coupled resonator optical waveguide (CROW) lattice to exhibit an optical analoge of quantum spin Hall effect. In stark contrast with aforementioned two types of Floquet topological insulator, the CROW lattice is a 2D time-reversal invariant system, which does not require any type of external driven and can be easily demonstrated in experiments. The CROW lattice, for which the configuration is specifically designed to be periodic, is termed as anomalous Floquet topological insulator (AFI)11,12 and has zero Chern number due to the time-reversal symmetry. In acoustics, unidirectional edge channels have been recently proposed for scalar acoustic waves propagating in a fluid circulation array18,27,28, mimicking the integer quantum Hall effect by breaking T-symmetry via the Doppler effect. However, the missing part corresponding to T-invariant topological phase for sound has still not yet been achieved.
In this study, we have theoretically proposed and experimentally demonstrated the prototype of T-invariant AFI for sound. The proposed AFI is inspired from the Chalker–Coddington network model developed in the 1980s for the study of Anderson transition in quantum Hall systems29. The model of AFI is a 2D coupled metamaterial ring lattice, presented in Fig. 1a, which can support topological edge states at sufficiently large coupling strength between neighbouring lattice rings. Figure 1b schematically shows a unit-cell of the 2D lattice, comprising one lattice ring in the centre surrounded by four coupling rings. Here we define a pseudo-spin for acoustic waves based on wave circulation direction in the lattice rings7,8,11,30, viz. pseudo-spin-up↔clockwise and pseudo-spin-down↔anti-clockwise. By purposely designing the lattice configuration, we have successfully constructed the acoustic AFI, which can support the pseudo-spin-dependent edge states, scattering immune to boundary abrupt variations or lattice dislocations. The edge states with different pseudo-spins can propagate in opposite directions under T-symmetry at the same boundary. We emphasize that the edge states with different pseudo-spins are regarded as decoupled due to nearly unitary coupling between neighbouring rings, closing the time-reversed channels for backscatterings. In this case, the rings no longer act as resonators and the edge state is essentially a conventional waveguide mode31 (see Supplementary Note 1). For one specific pseudo-spin, there exists a pair of edge states propagating along the upper and lower boundaries, respectively, with opposite group velocities7,8,11,24. The observations reveal that when the coupling strength between adjacent lattice rings surpasses a threshold, acoustic waves carrying a pseudo-spin in one lattice ring may tunnel into the neighbouring coupling ring with the pseudo-spin flipped and then go to another lattice ring with the pseudo-spin restored or conserved, rendering an interesting zigzag route. Our work represents an important step in the implementation of a diverse family of topological structures and networks for sound with new properties and functionalities.
Projected band structure for acoustic AFI
As shown in Fig. 1c, our acoustic metamaterial waveguide is constructed by subwavelength air–metal layers (metal: aluminum alloys) periodically stacking along the azimuthal direction of the ring. The effective refractive index of the fundamental guided mode can be expressed as32,33
where t, w are the thickness and width of metal plates, p is the structural period. ω=2πf denotes the angular frequency of acoustic waves. Here, the refractive index of air nair=1 and the speed of sound in air at room temperature cair=343.21 m s−1. For the fabricated sample, the structural parameters are R=77.4 mm, w=17.2 mm, t=1.7 mm and P=4.3 mm. In stark contrast to the natural existing materials with refractive indices always lower than nair34, the extremely anisotropic metamaterial can support tightly guided acoustic waves, as the effective refractive index is much larger than nair. To suppress high-order guided modes, the operation frequency should satisfy the cutoff condition of ω<πcair/w.
For calculating the projected band structure of AFI, we first map the lattice onto the equivalent Chalker–Coddington network model composed of links and nodes28,29. As shown schematically in Fig. 2a, each red arrow refers to a link, viz. a quarter lattice ring, and each blue circle refers to a node, viz. a coupling ring. In the link, the phase delay of acoustic waves is ϕ=(πR/2)ωneff/cair, which is dependent on the operation frequency. Each node can be described by a scattering matrix in a parameterization form refs 11, 30
where θ∈[0, π/2] characterizes the coupling strength between adjacent lattice rings. χ, ϕ and ξ∈[0, 2π] are the phase parameters to be determined. As the coupling ring is symmetric under 180° rotation, the scattering matrix should satisfy S11=S22 and S12=S21, that is, eiχ=ei(ϕ−χ) and eiξ=−ei(ϕ−ξ). Therefore, we obtain χ=ϕ/2 and ξ=(π+ϕ)/2. The scattering matrix can thus be rewritten into
where ϕ denotes the phase shift in the coupling process. As ϕ has no influence on the coupling strength, it can be arbitrarily chosen. For simplicity, we set ϕ=0 and obtain
From equation (4), the scattering matrix S is only determined by θ, which characterizes the coupling strength between adjacent lattice rings. It should be mentioned that the coupling strength θ is highly dispersive in our case, whereas in previous theoretical works11,30, θ has always been considered as non-dispersive for the calculation of ’quasi-energy’ band structures (see Supplementary Fig. 1). In Fig. 2a, we consider a strip coupled ring lattice that is periodic in x direction and finite in y direction. The sites of lattice rings are indicated by (m, n), where m and n are the column and row indices, respectively. Then, we employ |ϕm,n〉=[am,n bm,n cm,n dm,n]T to represent the amplitudes of acoustic waves in the lattice ring at the site (m, n). The scattering matrixes of coupling rings in x and y directions are the same Sx=Sy=S(θ). Coupling relations between the lattice rings at sites (m, n) and (m+1, n) in x direction, as well as those at sites (m, n) and (m, n+1) in y direction are respectively expressed as follows
By applying the Bloch condition in x direction |ϕm+1,n〉=eiKx|ϕm,n〉 and the boundary condition in y direction cm,1=e−2iϕbm,1, am,N=e2iϕdm,N, we can obtain the following governing equation11
where Kx is the Bloch wave vector, |ψ〉=[bm,1 dm,1 bm,2 dm,2 ··· bm,N dm,N]T the wave amplitudes in the mth column, G=G1·G2 with G1 and G2 being
The sub-matrixes G10 and G20 are
Figure 2b has clearly illustrated the coupling strength θ between neighbouring lattice rings as the frequency f varies from 7.1 to 7.7 kHz. The parameter θ=arcsin(|Pout|/|Pin|) is numerically extracted from the U-Ring-U shape configuration by using a finite element solver (COMSOL Multiphysics TM 4.3b), where Pin and Pout are the pressure amplitudes at input and output ports, respectively. The yellow region in Fig. 2b covers the frequency range of strong coupling for θ>π/4 and the coupling strength reaches a maximum θ≈0.43π at 7.46 kHz. The inset has shown the simulated pressure amplitude distribution at 7.46 kHz to validate the nearly unitary coupling.
In Fig. 2c, we map out the projected band structure for pseudo-spin-up Bloch modes in the semi-infinite ring lattice by solving the governing equation (6). Specifically, the number of unit cells in y direction is set as N=20 and the band structure is plotted by sweeping the frequency from 7.1 to 7.7 kHz with the step of Δf=0.1 Hz. Each dot in the bands corresponds to a Bloch mode with an explicit frequency f and a Bloch wave vector k. In Supplementary Fig. 2, we also show the band structures calculated by different frequency steps, viz., Δf=1, 0.1 and 0.025 Hz, which clearly shows that the central blank parts of the band structure in Fig. 2c are shrinking by decreasing the frequency step. In the strong coupling range for θ>π/4, our system may turn into a topological insulator. It should be mentioned that θ>π/4 is a necessary but not sufficient condition to judge whether the coupled ring lattice is a topological insulator. Therefore, the yellow region in Fig. 2b just shows the frequency range where the ring lattice may possibly be a topological insulator. To accurately predict the frequency range of topological phase, we need to refer to the projected band structure plotted in Fig. 2c. We note that the topological insulator studied in refs 11, 12, 30 also has bulk state bands and gapless edge state bands at θ>π/4. In Fig. 2c, the red and blue curves denote the upper and lower edge states spanning the band gaps with positive and negative group velocities, respectively. Obviously, the non-trivial edge states exist in the frequency range of 7.4∼7.6 kHz, showing a good agreement with the shaded region in Fig. 2b. However, in the weak coupling range for θ<π/4, the lattice turns into a trivial insulator supporting two-way edge states. To be specific, at the frequency around 7.2 kHz, there are actually two pseudo-spin-up edge states with different group velocities for either boundary. In Fig. 2c, we have neglected the pseudo-spin-flipping processes at each coupling connection. If we consider both pseudo-spins, the projected band structure will have a time-reversal counterpart11. For a certain pseudo-spin, the Berry curvature F(k) is an odd function in momentum space (or k-space). Therefore, the Chern number C is calculated to be zero according to the definition of , where the surface integral is operated for a specific bulk band in the Brillouin zone. According to refs 11, 30, we can use the none-zero ν1 invariant to describe the non-trivial topological properties of time-reversal invariant systems, for example, AFI, even though the Chern number is zero. The non-zero ν1 is defined by
Coupling in the U-Ring-U shape waveguide complex
To demonstrate the coupling properties between neighbouring lattice rings in the strong coupling regime, we experimentally study a U-Ring-U shape waveguide complex displayed in Fig. 3a, which serves as the fundamental element of AFI. In the waveguide complex, the lattice rings are replaced by U-shape waveguides, thus forming a four-port system described by a scattering matrix S(θ). The coupling between two U-shape waveguides is realized via two connections, as marked by the red elliptic circles. The experimental setup is shown in Fig. 3b, where the fabricated U-Ring-U shape waveguide is sealed in rigid rectangular pipes to prevent unwanted radiation losses during propagation and isolate ambient noises. In the experiment, we launch acoustic waves from Port 1 and measure pressure amplitude distributions in the coupling ring by inserting a condenser microphone into holes perforated on the pipes. Meanwhile, we plug the unmeasured holes with screws.
Figure 3c has shown pressure amplitude distribution in the coupling ring along the azimuthal direction from 0° to 360°. The frequency range is taken from 7.4 to 7.6 kHz, which corresponds to the non-trivial band gap in Fig. 2c. It is observed that the sound energy is mainly distributed along the lower half ring, leaving the upper half part almost soundless within the frequencies of our interest. For a more intuitive presentation, we extract the data on the vertical dashed line at 7.46 kHz in Fig. 3c and replot the pressure amplitude distribution on a ring in Fig. 3d. The measured field distribution in Fig. 3d agrees well with the simulated result in Fig. 2b, thus validating the nearly unitary coupling efficiency. In Fig. 3d, the pressure amplitude field in the lower half ring manifests inevitable attenuation. Such attenuation mainly stems from thermo-viscous loss in the metamaterial waveguide with subwavelength slit arrays. The ratio between the pressure amplitudes at 90° and 270° of the coupling ring is illustrated in Fig. 3e, which is plotted by using the data on horizontal dashed lines in Fig. 3c. It clearly shows that the measured pressure amplitude contrast is above 20 from 7.44 to 7.48 kHz and reaches the maximum value of around 42 at 7.46 kHz. We find out that the measured contrast agrees well with the simulated one, as shown in Fig. 3e. After studying the properties of U-Ring-U shape waveguide complex, we can further design a 2D AFI and investigate the topological edge states in the strong coupling regime.
Topological wave transportation in acoustic AFI
Basically, in the strong coupling regime, the direction of propagation and pseudo-spin of acoustic waves are locked at the boundaries of AFI. For example, the upper edge supports forward propagating waves with pseudo-spin-up and backward propagating waves with pseudo-spin-down, and conversely for the lower edge. In this section, we will numerically and experimentally display varied topological wave transportations, such as one-way edge states and interfacial states, in the acoustic AFI of different lattice configurations. The simulations are operated in lossless systems. It is necessary to emphasize that those phenomena are observable even in the presence of decay processes as revealed in experiments.
The first demonstration is pseudo-spin-dependent topological transportation of edge states in a lattice composed of 3 × 4 unit cells. One ring is purposely removed to form a dented edge as shown in Fig. 4. U-shape waveguides are imposed to selectively excite or extract pseudo-spin-up or pseudo-spin-down acoustic edge states. In Fig. 4a, we launch guided waves from the lower arm of the left U-shape waveguide and the pseudo-spin-up edge state is perfectly excited. The excited edge state is circulating clockwise in each lattice ring and immune to the dented edge. Therefore, it propagates through six sharp corners of the lattice smoothly. Owing to the nearly unitary coupling at each connection, the backward reflection of pseudo-spin-down component is negligible, leading to the fact that the output sound energy is closely equal to the input. However, when we launch guided waves from the upper arm, we will instead excite the pseudo-spin-down edge state, as shown in Fig. 4b. The guided wave in each lattice ring is circulating anti-clockwise and propagates along a different route with only two sharp corners. It should be mentioned that the pseudo-spin-dependent topological transportation of edge states even holds after weak lattice distortion is imposed (see Supplementary Fig. 4). We conduct the proof-of-concept experiment in an anechoic chamber. To prevent unwanted radiation losses during the propagation, the fabricated metamaterial ring lattice is sealed in rigid rectangular pipes and pressure amplitude distribution in the ring lattice is measured by inserting a condenser microphone into perforated holes on the pipe wall (see Supplementary Fig. 5). During the measurement, the lab-made sound source is operating at 7.46 kHz and the unscanned holes are bolted to prevent sound leakage (see Supplementary Figs 6 and 7). The measured pressure amplitude distributions for pseudo-spin-up and pseudo-spin-down acoustic one-way edge states are respectively shown in Fig. 4c,d, which agrees well with the simulated ones despite of obvious field attenuation. The significant dissipation is mainly due to thermo-viscous damping effect in the narrow air channels between metal plates. The details of experimental measurements are referring to the Supplementary Note 3. Owing to the perfect localization of edge states, the number of unit cells in the bulk region has no influence on the property of edge states. In the Supplementary Fig. 8, we have calculated band structures for the lattices with numbers of unit cells N=3, 5, 10, 20, 50 and 100 in the y direction. The result clearly shows that the edge state bands, viz., the red and blue curves, are unchanged as the number of unit cells N in y direction increases. The number N only influence the bulk state bands very much. For example, as N increases, the number of bulk state bands also increases. In this work, we choose the lattice of 3 × 4 due to the limitation of experimental conditions. However, our results still unequivocally show the existence of topological edge states in the confined system.
In the next, we demonstrate the existence of non-trivial interface states in a dislocated lattice, where two sub-lattices (2 × 4 unit cells) are horizontally dislocated by half a lattice constant. Simulation in Fig. 5a unequivocally shows that the interface state launched at the left can propagate along the dislocated interface to the right output with little reflections. As the coupling and lattice rings are chosen to be of the same size, the lower and upper sub-lattices can match well with each other at the interface under the dislocation of half a lattice constant. Basically, the coupling ring of the lower sub-lattice acts as the lattice ring of the upper sub-lattice and vice versa. Thus, the interface state can be regarded as pseudo-spin-down edge state for the upper sub-lattice and pseudo-spin-up edge state for the lower one, respectively. Differing from the edge states that can be excited from either the lower branch or the upper branch of the U-shape waveguide at the left side, the interface state can only be excited from the lower branch of the U-shape waveguide. If we launch acoustic waves from the upper branch, we will excite the bulk state instead of interface state (see Supplementary Fig. 9). It shows that the field distributions of interface state and bulk state are complementary to each other in the dislocated lattice. In Fig. 5b, we provide the measured sound energy distribution of the interface state, where the interface state can propagate from the left to right with little reflection. Owing to the presence of loss, the sound is attenuated exponentially in the propagation.
At last, the properties of pass band and band gap states are investigated by measuring the sound energy spectra and sound energy distributions in AFI. In Fig. 6a,b, the sound energy spectra (I1 and I2) are shown to check the bandwidths of the edge states. In the experiments, I1 and I2 are measured at two different sites, as marked by the circles in the Supplementary Fig. 10. I1 indicates the sound energy at the output, whereas I2 reflects the sound energy penetrated into the bulk. I1 and I2 are normalized with respect to their maxima (arbitrary unit). In principal, we can determine the edge states, pass band states and band gap states from the amplitudes of I1 and I2. Specifically, I1>0, I2→0 for the edge states, I1>0, I2>0 for the pass band states and I1→0 for the band gap states. From the provided criterion, one can easily obtain that the carrying frequencies of edge states span from 7.4 to 7.5 kHz and from 7.55 to 7.6 kHz, as shown in Fig. 6a, which agrees well with the band structure diagram in Fig. 2c. We also obtain that the bulk band and the band gap span from 7.5 to 7.55 kHz and from 7.24 to 7.25 kHz, respectively. From the above, the bandwidths of gapless edge states below and above the bulk band are thus calculated to be around 100 and 50 Hz, respectively. Figure 6c,d provide the measured sound energy distributions in the pass band (7.526 kHz) and the band gap (7.247 kHz). In the pass band, the sound energy is distributed not only at the edge but also in the inside bulk. In the band gap, the sound energy is rapidly decayed in the x direction. Thus, the sound is completely blocked by the lattice array. We find out that the experimental results fairly agree with the numerical simulations, after comparing Fig. 6 with Supplementary Fig. 11. It is also worthy to be pointed out that the gapless edge states below and above the bulk bands share similar topological properties. Although their bandwidths are quite different, the sound energy distributions are nearly the same, as shown by the experimental results in Supplementary Fig. 12.
In summary, we have experimentally demonstrated the prototype of T-invariant AFI for sound, which permits unidirectionally propagating pseudo-spin-dependent edge states. Here we would like to mention the works by Hafezi et al.7,8, where the coupling rings are aperiodic and well designed for purposely constructing an effective magnetic field to mimick the quantum Hall effects. In stark contrast with the work by Hafezi et al.7,8, our proposed AFI is not only periodic but also featured with the same size of lattice rings and coupling rings. This particular size selection is beneficial for the experimental demonstration, as the processing difficulty of the sample is greatly reduced and the required distribution of the coupling strength between neighbouring rings can be well satisfied in practice. In addition, we have discovered a novel topological interface state after introducing the dislocation of half a lattice constant into AFI. It should be emphasized that all the coupled rings need to be identical for the best excitation of such dislocation-induced topological interface state. It is also necessary to be mentioned that the T-symmetry between electrons and acoustic waves have fundamentally different physical natures. For example, eigenvalues of T2 operator for electrons T2=−1 and for acoustic waves T2=1 (ref. 24). As a result, electrons with different spins are completely decoupled under the protection of T-symmetry, whereas acoustic waves with different pseudo-spins can easily scatter into each other through time-reversed channels, such as imperfect couplings. To solve the backscattering issue in acoustic AFI, it is meaningful to push the coupling up to unitary and make acoustic waves with different pseudo-spins nearly decoupled. Another possible way of eliminating backscattering is breaking T, for example, using well-designed time-varying modulations18,27,28, which however is experimentally challenging and beyond the scope of this work.
Our work provides a fertile ground for novel wave manipulations, such as the unidirectional sound transports and robust sound transports against perturbations, and pushes forward the fundamental explorations of topological acoustics. Of interest will be the extension of our work into non-reciprocal acoustics regime by integrating time-varying (for example, rotating the metamaterial rings), shedding lights on the development of chiral acoustic metamaterials and Chern acoustic topological insulators with various intriguing non-reciprocal properties, such as one-way sound isolation.
We fabricated the waveguide metamaterial with aluminum alloys plates. Periodic grooves are perforated on the plate by numerically controlled machine tools (accuracy: 0.1 mm) with period 4.3 mm, width 17.2 mm and thickness 2.6 mm, whereas the height of each groove is constant (10 mm) and much smaller than the wavelength of sound in air (∼46 mm at 7.46 kHz). For the coupled metamaterial ring lattice, the inner and outer radii are 77.4 and 94.6 mm for each ring, respectively, distance of centres of nearest-neighbour rings is 198 mm and the angle between adjacent grooves in each ring is 3°.
Experiments setup and measurements
In the experiment, a lab-made sound source driven by a multifunctional signal generator (SRS MODEL DS345) and a lab-made power amplifier was placed in front of the tapered end of the metamaterial waveguide, to generate stable waveguide modes (see Supplementary Fig. 6). The sound energy is measured through a 1/8-inch diameter Brüel&Kjær Type-LAN-XI-3160 condenser microphone. The data are recorded with Brüel&Kjær PULSE 3160-A-042 4-channel analyser. The frequency response is obtained with fast fourier transform (FFT) analysis of Brüel&Kjær PULSE software LabShop version 184.108.40.206. To efficiently suppress the unwanted back reflections at input (or output) facets, we use gradient metamaterials with acoustic impedance fairly matched to air in broadband (see Supplementary Fig. 13). The fabricated metamaterial waveguides are all sealed in rigid rectangular pipes, to prevent unwanted radiation losses during propagation. Pressure amplitude distribution in the ring lattice is measured by inserting a condenser microphone into perforated holes on the pipe wall, where the perforated holes are azimuthally periodic and segregated by 12°. In each measurement, the unscanned holes are bolted to prevent sound leakage.
We employ COMSOL MultiphysicsTM 4.3b to perform FEM simulations. The geometrical model of the metamaterial waveguide complex is built up in the commercial software Pro/Engineer and then is loaded into the acoustic–solid interaction multi-physics module for the full-wave simulations. The materials applied in simulations were air and Aluminum (6061 T6). Perfectly matched layers are imposed on the outer boundaries of simulation domains to prevent reflections. The largest mesh element size was set lower than 1/10 of the lowest wavelength and finer meshes were applied at the domain with abrupt geometry changes.
The data that support the findings of this study are available from the corresponding author upon request.
How to cite this article: Peng, Y.-G. et al. Experimental demonstration of anomalous Floquet topological insulator for sound. Nat. Commun. 7, 13368 doi: 10.1038/ncomms13368 (2016).
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This work was supported by the National Natural Science Foundation of China under Numbers 11674119, 11404125, 11304351 and 11304105, and the ‘Strategic Priority Research Program’ of the Chinese Academy of Sciences (Grant Number XDA06020201). X.-F.Z. acknowledges the financial support from the Bird Nest Plan of HUST and the 973 Programs under Grant 2014CB921301.
Supplementary Figures 1-14, Supplementary Notes 1-3 and Supplementary References
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Scientific Reports (2017)