Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

  • Letter
  • Published:

Superconductivity mediated by spin fluctuations in the heavy-fermion compound UPd2 Al3

Abstract

It is well known that any weak attractive electron–electron interaction in metals can in principle cause the formation of Cooper pairs, which then condense into a superconducting ground state1. In conventional superconductors, this attractive interaction is mediated by lattice vibrations (phonons). But for the heavy-fermion and high-temperature superconductors, alternative pairing interactions are considered to be possible2. For example, the low-temperature properties of heavy-fermion systems are dominated by antiferromagnetic spin fluctuations, which have been considered theoretically3 as a possible cause for Cooper-pair formation. This picture recently received some experimental support: the resistivity behaviour under pressure of two cerium-based heavy-fermion compounds was shown to be consistent with a magnetically mediated pairing mechanism4. Here we use tunnelling spectroscopy to investigate the superconducting order parameter of a uranium-based heavy-fermion superconductor—epitaxial thin films of UPd2 Al3. Our observation of a strong-coupling feature in the tunnelling conductivity, combined with recent inelastic neutron scattering data13,14,15 strongly suggest a pairing interaction mediated by spin fluctuations.

This is a preview of subscription content, access via your institution

Access options

Buy this article

Prices may be subject to local taxes which are calculated during checkout

Figure 1: Diagram of a UPd2 Al3 –AlOx –Pb tunnel junction.
Figure 2: Differential conductivity of a UPd2 Al3 –AlOx –Pb tunnel junction at T = 0.3 K.
Figure 3: Differential conductivity of a UPd2 Al3 –AlOx –Pb tunnel junction at various temperatures.
Figure 4: Normalized differential conductivity of a UPd2 Al3 –AlOx –Pb tunnel junction.

Similar content being viewed by others

References

  1. Tinkham, M. Introduction to Superconductivity (McGraw-Hill, New York, (1996)).

    Google Scholar 

  2. Cox, D. L. & Maple, M. B. Electronic pairing in exotic superconductors. Phys. Today 275, 32–40 (1995).

    Article  Google Scholar 

  3. Miyake, K., Schmitt-Rink, S. & Varma, C. M. Spin-fluctuation-mediated even-parity pairing in heavy-fermion superconductors. Phys. Rev. B 34, 6554–6556 (1986).

    Article  ADS  CAS  Google Scholar 

  4. Mathur, N. D.et al. Magnetically mediated superconductivity in heavy fermion compounds. Nature 394, 39–43 (1998).

    Article  ADS  CAS  Google Scholar 

  5. Grewe, N. & Steglich, F. in Handbook on the Physics and Chemistry of Rare Earth (eds Gscheidner, K. A. & Eyring, L.) Vol. 14, Ch. 97 (Elsevier Science, Amsterdam, (1991)).

    Google Scholar 

  6. Gloos, K.et al. Scaling behaviour of point contacts between a tungsten tip and the heavy-fermion superconductors. J. Low. Temp. Phys. 105, 37–65 (1996).

    Article  ADS  CAS  Google Scholar 

  7. von Loehneysen, H. Probing the energy gap of the heavy-fermion superconductors. Physica B 218, 148–156 (1996).

    Article  Google Scholar 

  8. Geibel, C.et al. Heavy-fermion superconductivity at Tc = 2 K in the antiferromagnet UPd2 Al3. Z. Phys. B 84, 1–2 (1991).

    Article  ADS  CAS  Google Scholar 

  9. Huth, M., Kaldowski, A., Hessert, J., Heske, C. & Adrian, H. UPd2 Al3 heavy fermion superconducting films. Physica B 199 & 200, 116–118 (1994).

    Article  Google Scholar 

  10. Hiess, A.et al. Magnetic properties of UPd2 Al3 thin films investigated by resonant magnetic x-ray scattering. Physica B (in the press).

  11. Dynes, R. C., Narayanamurti, V. & Garno, J. Direct measurement of quasiparticle-lifetime broadening in a strong-coupled superconductor. Phys. Rev. Lett. 41, 1509–1512 (1978).

    Article  ADS  CAS  Google Scholar 

  12. Caspary, R.et al. Unusual ground state properties of UPd2 Al3 : Implications for the co-existence of heavy-fermion-superconductivity and local-moment antiferromagnetism. Phys. Rev. Lett. 71, 2146–2149 (1993).

    Article  ADS  CAS  Google Scholar 

  13. Sato, N.et al. Spin fluctuations in the heavy fermion superconductor UPd2 Al3 studied by neutron inelastic scattering. J. Phys. Soc. Jpn 66, 1884–1887 (1997).

    Article  ADS  CAS  Google Scholar 

  14. Metoki, N., Haga, Y., Koike, Y. & Onuki, Y. Superconducting energy gap observed in the magnetic excitation spectra of a heavy fermion superconductor UPd2 Al3. Phys. Rev. Lett. 80, 5417–5420 (1998).

    Article  ADS  CAS  Google Scholar 

  15. Bernhoeft, N.et al. Magnetic fluctuations above and below Tc in the heavy fermion superconductor UPd2 Al3. Physica B (in the press).

  16. Parks, R. D. in SuperconductivityCh. 10 (Marcel Dekker, New York, (1969)).

    Google Scholar 

  17. Millis, A. J., Sachdev, S. & Varma, C. M. Inelastic scattering and pair breaking in anisotropic and isotropic superconductors. Phys. Rev. B 37, 4975–4986 (1988).

    Article  ADS  CAS  Google Scholar 

  18. Tou, H.et al. D-wave superconductivity in antiferromagnetic heavy-fermion compound UPd2 Al3 —evidence from 27A1 NMR/NQR studies. J. Phys. Soc. Jpn 64, 725–729 (1995).

    Article  ADS  CAS  Google Scholar 

  19. Matsuda, K., Kohori, Y. & Kohara, T. Observation of 105Pd NMR and NQR signals in the heavy-fermion superconductor UPd2 Al3. Phys. Rev. B 55, 15223–15227 (1997).

    Article  ADS  CAS  Google Scholar 

  20. Hiroi, M.et al. Thermal conductivity of a heavy fermion superconductor UPd2 Al3 single crystal. J. Phys. Soc. Jpn 66, 1595–1598 (1997).

    Article  ADS  CAS  Google Scholar 

  21. Yip, S. & Garg, A. Superconducting states of reduced symmetry: General order parameters and physical implications. Phys. Rev. B 48, 3304–3308 (1993).

    Article  ADS  CAS  Google Scholar 

  22. Hessert, J.et al. Temperature and angular dependence of the upper critical field of UPd2 Al3 thin films. Physica B 230–232, 373–376 (1997).

    Article  ADS  Google Scholar 

Download references

Acknowledgements

We thank P. Haibach for experimental support. This work was supported by the Deutsche Forschungsgemeinschaft.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to M. Huth.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Jourdan, M., Huth, M. & Adrian, H. Superconductivity mediated by spin fluctuations in the heavy-fermion compound UPd2 Al3. Nature 398, 47–49 (1999). https://doi.org/10.1038/17977

Download citation

  • Received:

  • Accepted:

  • Issue Date:

  • DOI: https://doi.org/10.1038/17977

This article is cited by

Comments

By submitting a comment you agree to abide by our Terms and Community Guidelines. If you find something abusive or that does not comply with our terms or guidelines please flag it as inappropriate.

Search

Quick links

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing