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Attosecond core-level absorption spectroscopy reveals the electronic and nuclear dynamics of molecular ring opening
Attosecond core-level spectroscopy is used to probe the ultrafast molecular dynamics of furan at the carbon K-edge, demonstrating its ability to simultaneously probe electronic and vibrational dynamics.
- S. Severino
- , K. M. Ziems
- & J. Biegert
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News & Views |
Sub-cycle photonics in correlated materials
Sub-cycle confinement and control of phase transitions in strongly correlated materials are theoretically demonstrated, potentially providing a way to investigate electron dynamics on timescales previously unattainable with these materials.
- Eleftherios Goulielmakis
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Article
| Open AccessUltrafast atomic-scale scanning tunnelling spectroscopy of a single vacancy in a monolayer crystal
Time-resolved lightwave-driven scanning tunnelling spectroscopy is developed to investigate how the spin–orbit-split energy levels of a selenium vacancy within a WSe2 monolayer shift under phonon displacement. Ultrafast snapshots of the electronic tunnelling spectra reveal transient energy shifts up to 40 meV.
- C. Roelcke
- , L. Z. Kastner
- & Y. A. Gerasimenko
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Article
| Open AccessA high-efficiency programmable modulator for extreme ultraviolet light with nanometre feature size based on an electronic phase transition
A reflective spatial light modulator for extreme ultraviolet (EUV) or soft X-ray light is demonstrated in an electronic Wigner crystal material with a sub-90-nm feature size. The diffraction grating imprinted by sub-picosecond EUV beams is rewritable. The projected efficiency according to the modelling exceeds 1%.
- Igor Vaskivskyi
- , Anze Mraz
- & Dragan Mihailovic
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Article
| Open AccessSub-cycle multidimensional spectroscopy of strongly correlated materials
Nonlinear multidimensional spectroscopy that can image the sub-cycle dynamics of strongly correlated systems on the sub-femtosecond timescale is demonstrated by using the carrier–envelope-phase dependence of the correlated multielectron response to decode the complex interplay between different many-body states.
- V. N. Valmispild
- , E. Gorelov
- & O. Smirnova
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Article |
Attosecond-resolved non-dipole photoionization dynamics
Using a self-referenced attosecond photoelectron interferometry on helium atoms, the electron subcycle motion along the light propagation direction is observed in the 15 pm range. A time delay of 15 ± 10 as between the electric-dipole and electric-quadrupole transitions is also revealed.
- Jintai Liang
- , Meng Han
- & Hans Jakob Wörner
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Article
| Open AccessAcousto-optic modulation of gigawatt-scale laser pulses in ambient air
Air-based acousto-optic modulation is shown to be able to efficiently control gigawatt-scale, ultrashort laser pulses.
- Yannick Schrödel
- , Claas Hartmann
- & Christoph M. Heyl
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News & Views |
Ultrashort coils of light
A diffractive axicon (a device that diffracts the input light pulse radially) enables complex correlations between the topological charges and the frequencies of ultrashort laser pulses, resulting in a variety of ultrashort coiled light structures.
- Spencer W. Jolly
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News & Views |
Fresnel time lens empowers quantum networks
Researchers have developed efficient electro-optic tools for manipulating the time and frequency of single photons by taking inspiration from Fresnel lenses.
- John M. Donohue
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Article |
Field-driven attosecond charge dynamics in germanium
Attosecond transient reflectivity spectroscopy, in combination with extensive time-dependent density functional theory calculations, is used to study field-driven carrier injection in germanium in the time window of few femtoseconds around pulse overlap, paving a route towards achieving full optical control over charge carriers in semiconductors.
- Giacomo Inzani
- , Lyudmyla Adamska
- & Matteo Lucchini
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News & Views |
Attosecond movies of nano-optical fields
A transmission electron microscopy technique enables movies of optical near-fields to be recorded with a temporal resolution faster than the oscillation of optical electric fields.
- Yuya Morimoto
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Article |
Megaelectronvolt electron acceleration driven by terahertz surface waves
When near-infrared femtosecond laser pulses are focused onto a metal wire, relativistic electron acceleration is observed in the attached waveguide. An electron energy gain of 1.1 MeV and an effective acceleration gradient up to 210 MV m−1 are achieved using the laser-induced terahertz surface waves.
- Xie-Qiu Yu
- , Yu-Shan Zeng
- & Ru-Xin Li
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News & Views |
Spatio-temporal control of incoherent light with metasurfaces
Dynamic control of incoherent light sources at ultrafast timescales is tremendously challenging. Now, a technique using a spatially structured optical pump and semiconductor metasurfaces has been developed that dynamically steers sub-picosecond pulses of ultrafast incoherent emission.
- Angela Demetriadou
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Article |
Broadband control of topological–spectral correlations in space–time beams
Introduction of a diffractive axicon in a pulse shaper enables imparting topological–spectral correlation to ultrafast pulses over 200 nm in the visible region and with topological charges up to 80.
- Marco Piccardo
- , Michael de Oliveira
- & Antonio Ambrosio
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Article |
Interface between picosecond and nanosecond quantum light pulses
To bridge the ultrafast and slow classes of quantum-information-processing systems, a Fresnel time lens is developed by using a wideband electro-optic phase modulator combined with a dispersion element. The single-photon spectral bandwidth is compressed from picosecond to nanosecond timescales.
- Filip Sośnicki
- , Michał Mikołajczyk
- & Michał Karpiński
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Sub-picosecond steering of ultrafast incoherent emission from semiconductor metasurfaces
Researchers demonstrate sub-picosecond steering of ultrafast incoherent emission from a light-emitting metasurface. The steering is achieved over a 70° range.
- Prasad P. Iyer
- , Nicholas Karl
- & Igal Brener
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Article
| Open AccessLaser-guided lightning
A terawatt laser filament is shown to be able to guide lightning over a distance of 50 m in field trials on the Säntis mountain in the Swiss Alps.
- Aurélien Houard
- , Pierre Walch
- & Jean-Pierre Wolf
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Article
| Open AccessUltrafast serrodyne optical frequency translator
A nonlinear multi-pass cell is shown to be able to shift the central wavelength of a laser by tens of nanometres, offering a new means for control for high-power laser systems
- Prannay Balla
- , Henrik Tünnermann
- & Christoph M. Heyl
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Article |
Nonlinear helical dichroism in chiral and achiral molecules
Nonlinear absorption of helical light beams offers a new chiroptical detection scheme for both chiral and achiral molecules in liquid phase.
- Jean-Luc Bégin
- , Ashish Jain
- & Ravi Bhardwaj
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Letter |
Synthesis of ultrafast wavepackets with tailored spatiotemporal properties
Ultrafast wavepackets are generated featuring precise correlations between spatial and temporal properties.
- Daniel Cruz-Delgado
- , Stephanos Yerolatsitis
- & Miguel A. Bandres
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Article |
Ultrafast intrinsic optical-to-electrical conversion dynamics in a graphene photodetector
Researchers demonstrated a gate-tunable graphene photodetector with a bandwidth of up to 220 GHz. This was achieved by suppressing the ‘RC’ time constant using a resistive zinc oxide top gate.
- Katsumasa Yoshioka
- , Taro Wakamura
- & Norio Kumada
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Letter |
Femtojoule femtosecond all-optical switching in lithium niobate nanophotonics
Researchers exploit the quadratic nonlinearity of lithium niobate nanowaveguides and demonstrate cavity-free all-optical switching. Switching energies down to 80 fJ, switching times down to ~46 fs and energy–time products of 3.7 × 10−27 J s are shown.
- Qiushi Guo
- , Ryoto Sekine
- & Alireza Marandi
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Observation of toroidal pulses of light
Pulses of light with a toroidal structure are experimentally realized in the terahertz and optical regions.
- Apostolos Zdagkas
- , Cormac McDonnell
- & Nikolay I. Zheludev
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| Open AccessToroidal vortices of light
A new solution to Maxwell’s equations, photonic toroidal vortex, is experimentally realized.
- Chenhao Wan
- , Qian Cao
- & Qiwen Zhan
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Article
| Open AccessSingle-cycle infrared waveform control
Continuously adjustable single-cycle waveform spanning from 0.9 to 12.0 μm is obtained by cascaded intrapulse difference-frequency generation in a ZnGeP2 crystal. The cascade-associated phase response—distinct for different spectral bands—provides a new tuning parameter for waveform adjustment.
- Philipp Steinleitner
- , Nathalie Nagl
- & Ka Fai Mak
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Temporal walk-off induced dissipative quadratic solitons
The formation of ultra-short dissipative quadratic solitons is realized using optical parametric amplification at low pump energies and in the presence of substantial temporal walk-off between the pump and signal.
- Arkadev Roy
- , Rajveer Nehra
- & Alireza Marandi
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News & Views |
Probing attosecond phenomena in solids
A sub-cycle modulation in reflectivity is observed in bulk crystals subjected to intense laser fields. The effect provides a new way to probe attosecond dynamics in materials.
- Shambhu Ghimire
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Article |
Attosecond electron motion control in dielectric
Light-field-induced electron dynamics in a silicon dioxide dielectric system are exploited to directly measure the attosecond relative electronic delay response in the dielectric system, potentially extending the speed of data processing and information encoding into the petahertz realm.
- Dandan Hui
- , Husain Alqattan
- & Mohammed Th. Hassan
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News & Views |
Mid-infrared ultrashort pulse generation
The direct generation of femtosecond pulses from an 8-μm quantum cascade laser could prove transformative for sensing and spectroscopy.
- Sukhdeep Dhillon
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Article |
Femtosecond pulses from a mid-infrared quantum cascade laser
Near-transform-limited 630 fs pulses with 4.5 W of peak power are generated by compensating the dispersion of a quantum cascade laser emitting around 8 μm. Their temporal nature is assessed by a new method called asynchronous upconversion sampling.
- Philipp Täschler
- , Mathieu Bertrand
- & Jérôme Faist
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Article
| Open AccessUltra-fast germanium photodiode with 3-dB bandwidth of 265 GHz
By sandwiching a germanium fin between complementary in situ-doped silicon layers, a waveguide-coupled germanium photodiode with a 3-dB bandwidth of 265 GHz, accompanied by high responsivity and low dark current, is realized.
- S. Lischke
- , A. Peczek
- & L. Zimmermann
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Article |
Complete characterization of sub-Coulomb-barrier tunnelling with phase-of-phase attoclock
Electron non-stationary tunnelling dynamics is probed by the attoclock with the two-colour phase-of-phase photoelectron spectroscopy. Contrary to the case of static tunnelling, angle-to-time mapping in attoclock is found to be not angularly uniform.
- Meng Han
- , Peipei Ge
- & Yunquan Liu
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Article |
Reconfigurable electronic circuits for magnetic fields controlled by structured light
Structured beams of light are used to engineer conduction band populations and pattern currents. Using the approach, dynamic optoelectronic interconnects and other applications are demonstrated.
- K. Jana
- , K. R. Herperger
- & S. Sederberg
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Generation and measurement of intense few-femtosecond superradiant extreme-ultraviolet free-electron laser pulses
By amplifying a soliton in a multistage cascade, few-femtosecond extreme-ultraviolet free-electron laser pulses are achieved.
- Najmeh S. Mirian
- , Michele Di Fraia
- & Luca Giannessi
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Subcycle contact-free nanoscopy of ultrafast interlayer transport in atomically thin heterostructures
Subcycle nano-videography of charge-transfer dynamics in WSe2/WS2 heterostructures is obtained by using a terahertz near-field microscopy. The central idea is to probe the local polarizability of electron–hole pairs with evanescent terahertz fields.
- M. Plankl
- , P. E. Faria Junior
- & R. Huber
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Review Article |
Photonics for artificial intelligence and neuromorphic computing
Photonics offers an attractive platform for implementing neuromorphic computing due to its low latency, multiplexing capabilities and integrated on-chip technology.
- Bhavin J. Shastri
- , Alexander N. Tait
- & Paul R. Prucnal
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Letter |
Seven-octave high-brightness and carrier-envelope-phase-stable light source
Using a gas-filled anti-resonant-reflection photonic-crystal fibre, a high-brightness table-top source of coherent carrier-envelope-phase-stable waveforms is demonstrated across seven octaves (340 nm to 40,000 nm) with ultraviolet peak powers up to 2.5 MW and terahertz peak powers of 1.8 MW, without the need for changing nonlinear crystals.
- Ugaitz Elu
- , Luke Maidment
- & Jens Biegert
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Letter |
Lightwave control of topological properties in 2D materials for sub-cycle and non-resonant valley manipulation
A method to control the topological properties of two-dimensional (2D) materials on few-femtosecond timescales is proposed. By controlling the sub-cycle structure of non-resonant driving fields, it may be possible to coherently write, manipulate and read selective valley excitation.
- Á. Jiménez-Galán
- , R. E. F. Silva
- & M. Ivanov
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Quantitative sampling of atomic-scale electromagnetic waveforms
Ultrafast lightwave sampling based on scanning tunnelling microscopy is developed to resolve near fields with sub-picosecond time resolution and sub-nanometre spatial resolution. Parameter-free quantitative measurement is achieved by using a single-molecule switch.
- D. Peller
- , C. Roelcke
- & J. Repp
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News & Views |
Exotic waves in multimode hollow-core fibres
Unexpected multimode solitary waves can be formed spontaneously in hollow-core fibres, hinting at a vast world of exciting nonlinear optics, with applications for generating few-cycle, ultra-intense pulses.
- Logan G. Wright
- & Frank W. Wise
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Letter |
Photoelectronic mapping of the spin–orbit interaction of intense light fields
Sculpting and focusing femtosecond cylindrical vector vortex pulses by a slit allows the controllable transformation of the photon’s orbital angular momentum into spin angular momentum, which can be characterized in situ by a strong-field ionization experiment.
- Yiqi Fang
- , Meng Han
- & Yunquan Liu
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Article |
High-energy multidimensional solitary states in hollow-core fibres
The formation of multidimensional solitary states through the nonlinear propagation of high-energy pulses in a molecular gas-filled large-core hollow-core fibre is demonstrated, offering new opportunities for studying multimodal spatiotemporal dynamics in the high-energy regime.
- Reza Safaei
- , Guangyu Fan
- & François Légaré
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Letter |
Transient optical symmetry breaking for ultrafast broadband dichroism in plasmonic metasurfaces
Inhomogeneity of the photogenerated carrier spacetime distribution enables transient symmetry breaking in a metasurface. As a result, broadband transient dichroism is demonstrated.
- Andrea Schirato
- , Margherita Maiuri
- & Giuseppe Della Valle
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Article |
Vectorized optoelectronic control and metrology in a semiconductor
Engineering of the spatial distribution of currents in a semiconductor is demonstrated using vectorial arrangement of optical fields, enabling an ultrafast magnetic field source.
- Shawn Sederberg
- , Fanqi Kong
- & Paul B. Corkum
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News & Views |
Nasca patterning in the microworld
Launching electrons to the centre of an optical field with a vortex phase profile via extreme-ultraviolet photoionization makes coherent imprinting of the spatial distribution of the vortex beam onto the electron wave packet possible.
- Olga Smirnova
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Article |
Non-adiabatic stripping of a cavity field from electrons in the deep-strong coupling regime
Deactivation of deep-strong light–matter coupling is achieved by femtosecond switching of terahertz cavities. This disruption leads to pronounced high-frequency polarization oscillations evolving much faster than the oscillation cycle of light.
- M. Halbhuber
- , J. Mornhinweg
- & C. Lange
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News & Views |
Ultrashort electron probe opportunities
Technology borrowed from electron accelerator and beam physics looks set to push the performance of ultrafast-electron-diffraction-based pump–probe studies of matter.
- Pietro Musumeci
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Letter |
Attosecond-fast internal photoemission
Femtosecond laser pulses are sent to a graphene/SiC interface to investigate photoinduced charge transfer from graphene to SiC. A charge transfer time of 300 attoseconds is obtained via laser-pulse-duration-dependent saturation fluence determination.
- Christian Heide
- , Martin Hauck
- & Peter Hommelhoff