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| Open AccessA neuromorphic bionic eye with filter-free color vision using hemispherical perovskite nanowire array retina
Designing full-color spherical artificial eyes remains a challenge. Here, Long et al. report a bionic eye where each pixel on the hemispherical retina can recognize different colors based on the unique bidirectional photo response; with optical adaptivity and neuromorphic preprocessing ability
- Zhenghao Long
- , Xiao Qiu
- & Zhiyong Fan
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Article
| Open AccessA two-dimensional mid-infrared optoelectronic retina enabling simultaneous perception and encoding
Designing an infrared machine vision system that can efficiently perceive, convert, and process a massive amount of data remains a challenge. Here, the authors present a retina-inspired 2D optoelectronic device based on van der Waals heterostructure that can perform the data perception and spike-encoding simultaneously for night vision, sensing, spectroscopy, and free-space communications.
- Fakun Wang
- , Fangchen Hu
- & Qi Jie Wang
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Article
| Open AccessSwitchable biomimetic nanochannels for on-demand SO2 detection by light-controlled photochromism
Conventional nanochannel sensors are passively responsive and may be slowly damaged by analytes present in the environment before detection. Here, authors developed a light-controlled inert/active-switchable biomimetic nanochannel sensor to achieve SO2 on-demand detection and long-term preservation.
- Dan Zhang
- , Yongjie Sun
- & Xuanjun Zhang
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Article
| Open AccessLight-driven peristaltic pumping by an actuating splay-bend strip
Small-scale manipulation of liquids is being controlled with bulky pumps or power sources. Dradrach et al. show a light-driven pumping of micro-liter liquid using a centimeter-long liquid crystal elastomer strip.
- Klaudia Dradrach
- , Michał Zmyślony
- & Piotr Wasylczyk
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Article
| Open AccessOrigami-based integration of robots that sense, decide, and respond
Origami-inspired engineering has enabled intelligent materials and structures to react to environments, yet a complete sense-decide-act autonomous loop is still challenging. Yan et al. introduce autonomous origami robots by embedding sensing, computing, and actuating in compliant, conductive materials.
- Wenzhong Yan
- , Shuguang Li
- & Ankur Mehta
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Article
| Open AccessOrganic electrochemical transistors as on-site signal amplifiers for electrochemical aptamer-based sensing
Electrochemical aptamer-based sensors typically exhibit limited sensitivity especially when the area of electrode is reduced for miniaturization. Here, the authors demonstrate electrochemical transistors as universal on-site amplifiers for enhancement in sensitivity of over 3 orders of magnitude.
- Xudong Ji
- , Xuanyi Lin
- & Jonathan Rivnay
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Article
| Open AccessD-O-A based organic phosphors for both aggregation-induced electrophosphorescence and host-free sensitization
Pure organic room-temperature phosphorescencent materials draw much attention but realising electroluminescence under electric excitation is challenging. Here the authors propose a donor-oxygen-acceptor molecular design realizing aggregation-induced organic room-temperature electrophosphorescence with high external quantum efficiency.
- Lulin Xu
- , Yuhang Mo
- & Junqiao Ding
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Article
| Open AccessUnraveling two distinct polymorph transition mechanisms in one n-type single crystal for dynamic electronics
Cooperative transitions have acquired much attention for low transition barriers, ultrafast kinetics, and structural reversibility but cooperative transitions are rare in molecular crystals and their origin is poorly understood. Here the authors show that reorientation of the alkyl side chains in a 2-dimensional quinoidal terthiophene triggers cooperative behavior, and establish alkyl chain engineering to control the polymorphic behavior.
- Daniel William Davies
- , Bumjoon Seo
- & Ying Diao
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Article
| Open AccessPolyvinyl chloride-based dielectric elastomer with high permittivity and low viscoelasticity for actuation and sensing
Dielectric elastomers (DEs) are widely used in soft actuators but existing DE actuators often require high driving electrical fields. Here the authors demonstrate that introducing cyanoethyl cellulose into plasticized PVC gel confers high dielectric permittivity and allows the fabrication of elastomer actuators with high permittivity and low viscoelasticity
- Jianjian Huang
- , Xiaodie Zhang
- & Dongjie Guo
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Article
| Open AccessSignatures of hot carriers and hot phonons in the re-entrant metallic and semiconducting states of Moiré-gapped graphene
Significant attention has been devoted to understanding the low-electric-field properties of carriers in moiré graphene, but high-electric-field transport has not been as well explored. Here, the authors find non-monotonic transport behavior at moiré minigaps due to competition between inter-band tunneling and coupling to out-of-equilibrium phonons.
- Jubin Nathawat
- , Ishiaka Mansaray
- & Jonathan P. Bird
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Article
| Open AccessHybrid spin Hall nano-oscillators based on ferromagnetic metal/ferrimagnetic insulator heterostructures
Spin-hall nano-oscillators have potential for use in neuromorphic computing applications. Normally they are based around combination platinum and permalloy. Here, the authors combine a permalloy ferromagnet with a low magnetic damping ferrimagnet, leading to significantly improved performance.
- Haowen Ren
- , Xin Yu Zheng
- & Andrew D. Kent
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Article
| Open AccessControlling doping efficiency in organic semiconductors by tuning short-range overscreening
Doping is widely adopted to make organic semiconductors more conductive, yet the impact of molecular electronic properties on doping performance is still not fully understood. Armleder et al. compute host-dopant interactions and show that a short-range overscreening effect strongly affects conductivity.
- Jonas Armleder
- , Tobias Neumann
- & Artem Fediai
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Article
| Open AccessLaser-induced topological spin switching in a 2D van der Waals magnet
Van der Waals magnetic materials, which maintain their magnetic ordering down to a monolayer have been found to host a variety of spin textures, including topological spin textures such as skyrmions. Here, Khela et al. demonstrate laser induced topological switching, between skyrmions, anti-skyrmions and stripe domains in CrGeTe3.
- Maya Khela
- , Maciej Da̧browski
- & Elton J. G. Santos
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Review Article
| Open AccessSmartphone-based platforms implementing microfluidic detection with image-based artificial intelligence
Smartphone-based mobile health platforms have drawn increasing attention from researchers developing point-of-care testing devices. Here the authors summarize recent progress and future directions of approaches combining microfluidics and artificial intelligence.
- Bangfeng Wang
- , Yiwei Li
- & Bi-Feng Liu
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Article
| Open AccessMammalian-brain-inspired neuromorphic motion-cognition nerve achieves cross-modal perceptual enhancement
Inspired by the multisensory cue integration in macaque’s brain for spatial perception, the authors develop a neuromorphic motion-cognition nerve that achieves cross-modal perceptual enhancement for robotics and wearable applications.
- Chengpeng Jiang
- , Jiaqi Liu
- & Wentao Xu
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Article
| Open AccessPolymerizable rotaxane hydrogels for three-dimensional printing fabrication of wearable sensors
While hydrogels find applications in wearable sensors and electronic skins, they are prone to fatigue fractures upon deformation cycling. Xiong et al. report the synthesis of conductive polymerizable rotaxane hydrogels, exhibiting large fatigue resistance, for 3D printable flexible sensors.
- Xueru Xiong
- , Yunhua Chen
- & Yanli Zhao
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Article
| Open AccessLocalizing strain via micro-cage structure for stretchable pressure sensor arrays with ultralow spatial crosstalk
Designing tactile sensors with high spatial resolution are crucial to manufacture large scale flexible electronics. Here, the authors develop a micro-cage structure by exploiting photo-reticulated strain localization films (prslPDMS), which shows the strain local confinement effect and could be used to prepare ultralow crosstalk sensor arrays.
- Yufei Zhang
- , Qiuchun Lu
- & Junyi Zhai
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Article
| Open AccessLifetime over 10000 hours for organic solar cells with Ir/IrOx electron-transporting layer
Long-term stability of organic solar cells is critical to promote practical applications. Here, the authors utilize iridium/iridium oxide nanoparticles as the electron-transporting material and realize enhanced device stabilities under thermal aging with T70 of over 10000 h.
- Yanxun Li
- , Bo Huang
- & Huiqiong Zhou
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Article
| Open AccessVisualizing electroluminescence process in light-emitting electrochemical cells
The recombination between electrons and holes in electroluminescence processes has never been directly evaluated. Here, Yasuji et al. directly visualize, with spectroscopic techniques, operation dynamics in light-emitting electrochemical cells during device operation, leading to a rapid device evaluation.
- Kosuke Yasuji
- , Tomo Sakanoue
- & Katsuichi Kanemoto
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Article
| Open AccessLaser printed microelectronics
Printed organic and inorganic electronics continue to be of large interest for several applications. Here, the authors propose laser printing as a facile process for fabricating printed electronics with minimum feature sizes below 1 µm and demonstrate functional diodes, memristors, and physically unclonable functions.
- Liang Yang
- , Hongrong Hu
- & Martin Wegener
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Article
| Open AccessPhonon-driven intra-exciton Rabi oscillations in CsPbBr3 halide perovskites
Coupling electromagnetic radiation with matter is promising to tailor optoelectronics properties of functional materials. Here, the authors demonstrate that internal fields induced by coherent lattice motions can be used to control transient excitonic optical response in halide perovskite crystals.
- Xuan Trung Nguyen
- , Katrin Winte
- & Antonietta De Sio
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Article
| Open AccessMetallic glass-based triboelectric nanogenerators
Surface wear is a major hindrance in the solid/solid interface of triboelectric nanogenerators, severely affecting output performance and stability. Here, authors show metallic glass as one triboelectric interface can enhance the triboelectrification efficiency and endow the device with humidity- and wear-resistance.
- Xin Xia
- , Ziqing Zhou
- & Yunlong Zi
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Article
| Open AccessWafer-scale and universal van der Waals metal semiconductor contact
Laminated van der Waals (vdW) metallic electrodes can improve the contact of 2D electronic devices, but their scalability is usually limited by the transfer process. Here, the authors report a strategy to deposit vdW contacts onto various 2D and 3D semiconductors at the wafer scale.
- Lingan Kong
- , Ruixia Wu
- & Yuan Liu
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Article
| Open AccessEmergence of high piezoelectricity from competing local polar order-disorder in relaxor ferroelectrics
Understanding high piezoelectricity in relaxors is challenging due to the heterogeneous structures. Here, the authors demonstrate that the competing local polar order-disorder state with balanced length and direction randomness is the key.
- Hui Liu
- , Xiaoming Shi
- & Jun Chen
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Article
| Open AccessDeformation constraints of graphene oxide nanochannels under reverse osmosis
Nanochannels in laminated graphene oxide nanosheets featuring confined mass transport have attracted interest in multiple research fields. As an important aspect for efficient pressure-driven membrane processes, authors investigate the response and deformation behaviours of such nanochannels to different external conditions.
- Kecheng Guan
- , Yanan Guo
- & Hideto Matsuyama
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Article
| Open AccessResponsive materials and mechanisms as thermal safety systems for skin-interfaced electronic devices
Minimizing patient risk to thermal failure in wearable electronics typically requires complex circuit control, sensors, or passive materials. Here, Yoo et al. present an active materials system with a self-inflating bladder that delaminates upon excessive heat, mitigating the risk of thermal injury.
- Seonggwang Yoo
- , Tianyu Yang
- & John A. Rogers
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Article
| Open AccessFrom nanohole to ultralong straight nanochannel fabrication in graphene oxide with swift heavy ions
While porous graphene oxide with nm-sized pores can be of great interest to biofluidic and energy storage applications, achieving precisely controlled porosity remains a technical challenge. Here, the authors exploit swift heavy ions to create uniform nanoholes and ultralong straight nanochannels in GO films.
- Andrzej Olejniczak
- & Ruslan A. Rymzhanov
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Article
| Open AccessAcoustic metamaterials-driven transdermal drug delivery for rapid and on-demand management of acute disease
Treating acute disease like anaphylaxis is challenging due to the inability to administer therapeutics in a timely manner and regulate pharmacokinetics precisely within a short time window. Here the authors develop active acoustic metamaterials-driven transdermal drug delivery for rapid and on-demand acute disease management.
- Junhua Xu
- , Hongwei Cai
- & Feng Guo
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Article
| Open AccessElectrical and magnetic anisotropies in van der Waals multiferroic CuCrP2S6
Manipulating electrical and magnetic anisotropies will stimulate multi-terminal device applications. Here, the authors discover axis dependence of current rectifications, magnetic properties and magnon modes in van der Waals multiferroic CuCrP2S6.
- Xiaolei Wang
- , Zixuan Shang
- & Jianhua Zhao
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Article
| Open AccessA flexible artificial chemosensory neuronal synapse based on chemoreceptive ionogel-gated electrochemical transistor
Developing an artificial olfactory system that can mimic the biological functions remains a challenge. Here, the authors develop an artificial chemosensory synapse based on a flexible organic electrochemical transistor gated by the potential generated by the interaction of gas molecules with ions in a chemoreceptive ionogel.
- Hamna Haq Chouhdry
- , Dong Hyun Lee
- & Nae-Eung Lee
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Article
| Open AccessUltrarobust subzero healable materials enabled by polyphenol nano-assemblies
Self-healing materials hold great promise for applications in wearable electronics, artificial muscles and soft robots but selfhealing at subzero temperatures remains a great challenge. Here, the authors present a robust subzero healable glassy polymer by incorporating polyphenol nano-assemblies with a large number of end groups into polymerizable deep eutectic solvent elastomers.
- Nan Wang
- , Xin Yang
- & Xinxing Zhang
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Article
| Open AccessPolymer-dispersed liquid crystal elastomers as moldable shape-programmable material
Development of Soft shape-memory materials is often limited to the synthesis of two-dimensional specimens and rely on bending mechanisms and scaffolding topology to perform three-dimensional morphing. Here, the authors demonstrate a shape-memory composite material made from main-chain liquid crystal elastomer microparticles dispersed in a silicone polymer matrix which enables molding into full-volume objects of any shape or size.
- Matej Bobnar
- , Nikita Derets
- & Andraž Rešetič
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Article
| Open AccessPulse-driven self-reconfigurable meta-antennas
Metasurface-based antennas show variable beam-patterns in response to the time width of electromagnetic pulses. This concept advances the design of antennas and wireless communication environments by using the pulse width as a new degree of freedom.
- Daiju Ushikoshi
- , Riku Higashiura
- & Hiroki Wakatsuchi
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Article
| Open AccessConductive and elastic bottlebrush elastomers for ultrasoft electronics
Conductive materials with tissue-matched softness are needed for ultra-soft electronics. Here, the authors report ultra-soft and conductive bottlebrush elastomer composites and fabricate them into electronics with laser cutting and 3D printing methods.
- Pengfei Xu
- , Shaojia Wang
- & Xinyu Liu
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Article
| Open AccessHighly-scaled and fully-integrated 3-dimensional ferroelectric transistor array for hardware implementation of neural networks
Hardware-based neural networks can provide a significant breakthrough in artificial intelligence. Here, the authors demonstrate an integrated 3-dimensional ferroelectric array with a layer-by-layer computation for area-efficient neural networks.
- Ik-Jyae Kim
- , Min-Kyu Kim
- & Jang-Sik Lee
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Article
| Open AccessWearable in-sensor reservoir computing using optoelectronic polymers with through-space charge-transport characteristics for multi-task learning
Designing efficient photonic neuromorphic systems remains a challenge. Here, the authors develop an in-sensor Reservoir Computing system for multi-tasked pattern classification based on a light-responsive semiconducting polymer (p-NDI) with efficient exciton dissociations, charge trapping capability, and through-space charge-transport characteristics.
- Xiaosong Wu
- , Shaocong Wang
- & Weiguo Huang
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Article
| Open AccessEnhanced gain and detectivity of unipolar barrier solar blind avalanche photodetector via lattice and band engineering
The limited breakdown electric field and the high dark current hider the application of solar blind avalanche photodiodes. Here, Zhang et al., by lattice and band engineering, construct a unipolar barrier avalanche photodiode with suppressed dark current and reinforced reverse breakdown.
- Qingyi Zhang
- , Ning Li
- & Jianhua Hao
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Article
| Open AccessEfficient pure blue hyperfluorescence devices utilizing quadrupolar donor-acceptor-donor type of thermally activated delayed fluorescence sensitizers
A suppressed energy loss through Dexter energy transfer is crucial to achieve highly efficient blue organic light-emitting diodes. Here, authors synthesize quadrupolar donor-acceptor-donor type thermally activated delayed fluorescence sensitizers and realize device with maximum efficiency of 43.9%.
- Hyuna Lee
- , Ramanaskanda Braveenth
- & Jang Hyuk Kwon
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Article
| Open AccessExclusive detection of volatile aromatic hydrocarbons using bilayer oxide chemiresistors with catalytic overlayers
Bilayer sensors and sensor arrays with a catalytic CeO2 filter are proposed as a facile platform for high-performance gas sensors and electronic noses. Authors show the bilayer sensors enhance selectivity toward aromatic compounds, and the arrays provide comprehensive information such as gas concentration and composition.
- Seong-Yong Jeong
- , Young Kook Moon
- & Jong-Heun Lee
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Article
| Open AccessA three-terminal magnetic thermal transistor
Thermal analogues to electrical transistors offer the potential for heat flow switching and amplification. Here, the authors demonstrate a macroscopic magnetic thermal transistor with applications in thermal control and thermal logic circuits.
- Lorenzo Castelli
- , Qing Zhu
- & Geoff Wehmeyer
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Article
| Open AccessAcid enhanced zipping effect to densify MWCNT packing for multifunctional MWCNT films with ultra-high electrical conductivity
Exploiting the electrical and mechanical properties of CNT films remain elusive because of the difficult material process. Here, Wang et al. report multifunctional MWCNT films with crystalline structure which exhibited great electromagnetic interference shielding efficiency, high thermoelectric power factor, and large ampacity.
- Hong Wang
- , Xu Sun
- & Junjie Yan
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Article
| Open AccessPhotosensitive ion channels in layered MXene membranes modified with plasmonic gold nanostars and cellulose nanofibers
Artificial ion channels are in demand for ionotronic devices. Here, the authors use layered MXene membranes modified with plasmonic gold nanostars and cellulose nanofibers to convert a thermal gradient into an ion current for photosensitive ion channeling.
- Jeonghee Yeom
- , Ayoung Choe
- & Hyunhyub Ko
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Article
| Open AccessUltralow contact resistance in organic transistors via orbital hybridization
The limitation in metal-semiconductor contact has been a major challenge for high-performance organic field-effect transistors. Here, the authors fabricate the contact by transferring platinum electrode on solution-processed organic films, realizing ultralow total contact resistance down to 14 Ω ∙ cm.
- Junpeng Zeng
- , Daowei He
- & Xinran Wang
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Article
| Open Access2D Titanium carbide printed flexible ultrawideband monopole antenna for wireless communications
Designing ultrathin and flexible antenna is of great interest for efficient wireless data communication and transmission at fast-growing IoT applications. The authors report a flexible ultrawideband Ti3C2 monopole antenna by combining strategies of interfacial modification and advanced extrusion printing technology.
- Weiwei Zhao
- , Hao Ni
- & Qiang Zhao
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Article
| Open AccessBlue light-emitting diodes based on colloidal quantum dots with reduced surface-bulk coupling
The surface localized charges in colloidal quantum dots induce a degradation that limits the electroluminescence performance. Here, Chen et al. propose quantum dots with monmonotonically-graded core/shell/shell structures to boost the device’s performance by reducing the surface-bulk coupling.
- Xingtong Chen
- , Xiongfeng Lin
- & Song Chen
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Article
| Open AccessAn artificial synapse based on molecular junctions
Designing scaled electronic devices for neuromorphic applications remains a challenge. Here, Zhang et al. develop an artificial molecular synapse based on self-assembled peptide molecule monolayer whose conductance can be dynamically modulated and used for waveform recognition.
- Yuchun Zhang
- , Lin Liu
- & Yong Yan
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Article
| Open AccessForce-induced ion generation in zwitterionic hydrogels for a sensitive silent-speech sensor
The development of sensitive hydrogel sensor without additional mobile ionic species is challenging. Here, the authors demonstrate force-induced ion generation in a skin sensor based on zwitterionic hydrogel, and build a throat-worn silent-speech recognition system with high recognition accuracy.
- Sijia Xu
- , Jie-Xiang Yu
- & Lei Zhang
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Article
| Open AccessSolid state ionics enabled ultra-sensitive detection of thermal trace with 0.001K resolution in deep sea
Exploration of deep sea areas relies on sonar and other visual and auditory sensors, but gaining information via temperature sensing in deep sea areas is difficult to realize. Here, the authors design an elastic, self-healable and sensitive thermal sensor which can identify a temperature difference as low as 0.01 K with a resolution of 0.001 K
- Yucheng Zhang
- , Dekai Ye
- & Chao Wang
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Article
| Open AccessBio-inspired magnetic-driven folded diaphragm for biomimetic robot
Soft robotics holds promise for realizing easy control over complex locomotion and deformation. Lin et al. report an earthworm-inspired untethered magnetic robot that consists one-piece-mold folded diaphragm to achieve large three-dimensional deformation with inside-volume change capability.
- Dezhao Lin
- , Fan Yang
- & Ruihong Li