Featured
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| Open AccessPen-drawn Marangoni swimmer
Marangoni swimmers have high relative speed, considering the body length and absence of a mechanical system but the fabricating is complex. Song et al. transform simple pen strokes into dynamic, programmable robots that can ‘swim’ with striking versatility.
- Seo Woo Song
- , Sumin Lee
- & Jiyun Kim
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Article
| Open AccessPrediction of sub-pyramid texturing as the next step towards high efficiency silicon heterojunction solar cells
The unexpected crystalline silicon epitaxial growth and interfacial nanotwins formation remain a challenging issue for silicon heterojunction technology. Here, the authors design a hybrid interface by tuning pyramid apex-angle to improve c-Si/a-Si:H interfacial morphology in silicon solar cells.
- Feihong Chu
- , Xianlin Qu
- & Yongzhe Zhang
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Article
| Open AccessAll-ferroelectric implementation of reservoir computing
While reservoir computing can process temporal information efficiently, its hardware implementation remains a challenge due to the lack of robust and energy efficient hardware. Here, the authors develop an all-ferroelectric reservoir computing system, showing high accuracies and low power consumptions in various tasks like the time-series prediction.
- Zhiwei Chen
- , Wenjie Li
- & Jun-Ming Liu
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Article
| Open AccessEnabling liquid crystal elastomers with tunable actuation temperature
Isotropization temperature determines the temperature at which Liquid Crystals Elastomer (LCE) material actuates. Here, the authors give a general strategy based on dynamic covalent bonds for tuning the isotropization temperature for LCEs.
- Yanjin Yao
- , Enjian He
- & Yan Ji
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Article
| Open AccessA chemiresistive-potentiometric multivariate sensor for discriminative gas detection
The application of multivariate gas sensors is limited due to their size and cost. Here the authors developed a compact gas sensor with multiple chemiresistive and potentiometric readouts enabling 3D discriminative response of gases at (sub)ppm levels and used the sensor for early fire detection.
- Hong Zhang
- , Zuobin Zhang
- & Jianxin Yi
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Article
| Open AccessBerry curvature contributions of kagome-lattice fragments in amorphous Fe–Sn thin films
The topological character of solids is usually revealed by considering the Berry curvature of electronic bands in a periodic crystal. Here, authors demonstrate the influence of the Berry curvature on the electronic properties of an amorphous thin film.
- Kohei Fujiwara
- , Yasuyuki Kato
- & Atsushi Tsukazaki
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Article
| Open AccessVertically integrated spiking cone photoreceptor arrays for color perception
Future intelligent vision systems need efficient capacitor-free spiking photoreceptor for color perception. Here, Wang et al. report a metal oxide-based vertically integrated spiking cone photoreceptor array which transduces light into spike trains with a power consumption of less than 400 picowatts.
- Xiangjing Wang
- , Chunsheng Chen
- & Qing Wan
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Article
| Open AccessEnergy conversion and storage via photoinduced polarization change in non-ferroelectric molecular [CoGa] crystals
Energy harvesting by utilizing optical control has emerged as a promising solution to alleviate energy and environmental crisis. However, it is challenging to realise nano-scale energy storage and conversion in the same material. Here the authors report a nonferroelectric molecular [CoGa] crystal that uses light as an external stimulus to exhibit photoenergy conversion and energy storage properties.
- Pritam Sadhukhan
- , Shu-Qi Wu
- & Osamu Sato
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Article
| Open AccessThermally stable threshold selector based on CuAg alloy for energy-efficient memory and neuromorphic computing applications
Designing efficient selector devices remains a challenge. Here, the authors propose a CuAg alloy-based selector with excellent ON/OFF ratio and thermal stability. It can effectively suppress the sneak-path current in 1S1R arrays, making it suitable for storage class memory and neuromorphic computing applications.
- Xi Zhou
- , Liang Zhao
- & Dongdong Li
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Article
| Open AccessNanowire-based smart windows combining electro- and thermochromics for dynamic regulation of solar radiation
Smart windows offer more efficient sunlight modulation and heat management. Here, the authors propose a co-assembly strategy to produce smart windows that combine electrochromic and thermochromic functions with tunable components and ordered structures for dynamic solar radiation regulation.
- Si-Zhe Sheng
- , Jin-Long Wang
- & Shu-Hong Yu
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Article
| Open AccessDischarge domains regulation and dynamic processes of direct-current triboelectric nanogenerator
Arising from contact electrification and electrostatic breakdown, DC triboelectric nanogenerators are a promising solution to the air breakdown bottleneck in conventional TENGs. Here, authors reveal and regulate three discharge domains enhancing the device output power by an order of magnitude.
- Jiayue Zhang
- , Yikui Gao
- & Jie Wang
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Article
| Open AccessIontronic pressure sensor with high sensitivity over ultra-broad linear range enabled by laser-induced gradient micro-pyramids
Developing iontronic pressure sensors with high sensitivity in a wide linear range can be challenging due to a trade-off between sensitivity and linear range. Here, authors bypass this limitation by using laser-assisted gradient micro-pyramids and insights from multiphysics simulations.
- Ruoxi Yang
- , Ankan Dutta
- & Huanyu Cheng
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Article
| Open AccessSemiconducting MOFs on ultraviolet laser-induced graphene with a hierarchical pore architecture for NO2 monitoring
NO2 monitoring is important in urban areas where pollutant levels are typically higher. Here authors present a hybrid structure of laser-induced graphene and Cu3HHTP2, a 2D semiconducting MOF, for highly sensitive and rapid detection of NO2 at the parts-per-billion level.
- Hyeongtae Lim
- , Hyeokjin Kwon
- & Hyuk-Jun Kwon
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Article
| Open AccessLight-driven dandelion-inspired microfliers
Insect-scale untethered micro aerial vehicles such as artificial dandelion devices suffer from high flight randomness and inadequate controllability. Chen et al. design and fabricate an untethered dandelion-inspired microflier, which is spatially and temporally controlled by an ultralight and supersensitive light-driven bimorph soft actuator.
- Yuanhao Chen
- , Cristian Valenzuela
- & Wei Feng
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Article
| Open AccessEnabling metallic behaviour in two-dimensional superlattice of semiconductor colloidal quantum dots
Charge carrier transport in colloidal quantum dot assemblies is slow due to hopping transport nature. Here, the authors report the demonstration of gate-tuned metallic state in epitaxially-connected quantum dot superlattices by minimizing disorders.
- Ricky Dwi Septianto
- , Retno Miranti
- & Satria Zulkarnaen Bisri
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Article
| Open AccessStructure-evolution-designed amorphous oxides for dielectric energy storage
Here, the authors propose a strategy to create amorphous oxides by bridging fluorite HfO2 and perovskite hafnate, which exhibit ultrahigh breakdown strength of 12 MV/cm and energy density of 155 J/cm3.
- Yahui Yu
- , Qing Zhang
- & Zheng Wen
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Article
| Open AccessBimodal ionic photomemristor based on a high-temperature oxide superconductor/semiconductor junction
Designing efficient photonic neuromorphic systems remains a challenge. Here, the authors develop a new class of memristor sensitive to the dual electro-optical history obtained by exploiting electrochemical, photovoltaic and photo-assisted oxygen ion motion effects at a high temperature superconductor / semiconductor interface.
- Ralph El Hage
- , Vincent Humbert
- & Javier E. Villegas
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Article
| Open AccessInsulator-to-metal-like transition in thin films of a biological metal-organic framework
Temperature-induced insulator-to-metal transitions are usually accompanied by structural phase transitions. Here the authors demonstrate an enhancement of the electrical conductance in a thin film of a biologically relevant metal-organic framework, without noticeable change in the structure, assigned to be of mainly electronic origin.
- Pooja Sindhu
- , K. S. Ananthram
- & Nirmalya Ballav
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Article
| Open AccessNon-volatile electric control of spin-orbit torques in an oxide two-dimensional electron gas
A central goal of spintronics is electric control of magnetism. One particularly promising method makes use of spin-orbit torques which arise due to the combination of electric current, and the intrinsic spin-orbit effect in a material. Here, Grezes et al demonstrate non-volatile electrical control of the spin-orbit torque generated at the interface between an oxide and a metal.
- Cécile Grezes
- , Aurélie Kandazoglou
- & Jean-Philippe Attané
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Article
| Open AccessConfining donor conformation distributions for efficient thermally activated delayed fluorescence with fast spin-flipping
The distribution of dihedral angles in film state has significant influence on excited state lifetimes of thermally activated delayed fluorescence emitters. Here authors report conformation distribution confinement strategy to achieve fast spin-flipping for efficient organic light-emitting diodes.
- Weidong Qiu
- , Denghui Liu
- & Shi-Jian Su
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Article
| Open AccessReconfigurable signal modulation in a ferroelectric tunnel field-effect transistor
Increasing functional density is desirable for future scaling of electronics. Here, the authors use a nanowire ferroelectric tunnel field-effect transistor to achieve reconfigurable signal modulations for low-power and high-density analogue circuits.
- Zhongyunshen Zhu
- , Anton E. O. Persson
- & Lars-Erik Wernersson
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Article
| Open AccessTriboelectric-induced ion mobility for artificial intelligence-enhanced mid-infrared gas spectroscopy
Isopropyl alcohol can play a significant role in anti-virus diagnosis but generally yields limited response in conventional detection. Here, authors propose a methodology of AI-enhanced ion mobility and mid-infrared spectroscopy for accurate gas identification despite presence different carbon-based gases.
- Jianxiong Zhu
- , Shanling Ji
- & Chengkuo Lee
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Article
| Open AccessMultimodal dynamic and unclonable anti-counterfeiting using robust diamond microparticles on heterogeneous substrate
Practical anticounterfeiting labels should possess both high-capacity and robustness, and should allow easy fabrication and readout. Here, the authors show how to heterogeneously grow robust and stable chaotic pattern of diamond microparticles - containing SiV defects - on silicon substrates.
- Tongtong Zhang
- , Lingzhi Wang
- & Zhiqin Chu
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Article
| Open AccessTwo-dimensional semiconducting SnP2Se6 with giant second-harmonic-generation for monolithic on-chip electronic-photonic integration
2D semiconductors with nonlinear optical properties hold promise for multifunction integration in electronic-photonic integrated circuits. Here, the authors report the synthesis of 2D SnP2Se6 and its integration with a SiN photonic platform, showing strong odd-even layer-independent second harmonic generation activity at 1550 nm and broadband photoresponse.
- Cheng-Yi Zhu
- , Zimeng Zhang
- & Cheng-Yan Xu
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Article
| Open AccessLayered BiOI single crystals capable of detecting low dose rates of X-rays
The complex coupling between charge-carriers and phonons in bismuth oxyiodide (BiOI) are uncovered, showing how carrier localisation is avoided and long transport lengths achieved. As a result, BiOI is revealed to be highly effective for X-ray detection.
- Robert A. Jagt
- , Ivona Bravić
- & Robert L. Z. Hoye
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Article
| Open Access3D Printing and processing of miniaturized transducers with near-pristine piezoelectric ceramics for localized cavitation
Despite advances in additive manufacturing of piezoceramics, resultant transducers generally suffer from high porosity, weak piezoelectric responses, and limited geometry. Here, authors report the design and printing of fully packaged freeform ultrasonic transducers capable of traveling inside mm-sized channels and deliver localized high ultrasound energy.
- Haotian Lu
- , Huachen Cui
- & Xiaoyu (Rayne) Zheng
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Article
| Open AccessGiant dynamic electromechanical response via field driven pseudo-ergodicity in nonergodic relaxors
High-performance relaxor ferroelectrics have been widely used in industry. Here the authors show that the enhanced electromechanical response is related to the pseudo ergodicity of nonergodic relaxor ferroelectrics under periodic electric field.
- He Qi
- , Tengfei Hu
- & Jun Chen
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Article
| Open AccessDesigning tailored combinations of structural units in polymer dielectrics for high-temperature capacitive energy storage
Polymer dielectrics face huge challenges in the harsh environments of emergent applications. Now, increased energy storage of polymer dielectrics at temperatures up to 250 °C by designing tailored combinations of structural units is reported.
- Rui Wang
- , Yujie Zhu
- & Qi Li
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Article
| Open AccessWafer-scale high-κ dielectrics for two-dimensional circuits via van der Waals integration
The integration of high-κ dielectric layers with 2D semiconductors is essential for electronic applications, but remains challenging. Here the authors report a dry transfer method of wafer-scale Al2O3 and HfO2 thin films for the realization of top-gated monolayer MoS2 transistors and logic gates.
- Zheyi Lu
- , Yang Chen
- & Yuan Liu
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Article
| Open AccessIntegrated opposite charge grafting induced ionic-junction fiber
Ionic-junction devices are difficult to integrate with fiber-shaped tissues like nerves and muscles for applications in implantable bioelectronics due to their large size and bulk structure. Authors realize here easy to implant fiber-shaped iontronics through an integrated opposite charge grafting process, enabling the construction of ionic logic gates and artificial neural pathways.
- Yi Xing
- , Mingjie Zhou
- & Gang Wang
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Comment
| Open AccessEthical considerations for researchers developing and testing minimal-risk devices
This comment explores ethical aspects in developing and testing minimal-risk devices, such as wearables and biomedical sensors. Authors outline the process of independent review, emphasizing the different levels of review depending on the research design and risk level. They also share examples of practical scenarios, highlighting key ethical considerations.
- Anna Wexler
- & Emily Largent
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Article
| Open AccessImproved photovoltaic performance and robustness of all-polymer solar cells enabled by a polyfullerene guest acceptor
Fullerene acceptors typically suffer from undesirable segregation and dimerization. Here, the authors report a poly(fullerene-alt-xylene) acceptor as guest component to facilitate charge transfer and suppress charge recombination, achieving efficiency of 18% for ternary all-polymer solar cells.
- Han Yu
- , Yan Wang
- & Shangshang Chen
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Article
| Open AccessBioinspired soft robots based on organic polymer-crystal hybrid materials with response to temperature and humidity
Response by mechanical deformation to give actuation is essential in the design of soft robots. Here, the authors demonstrate that combining organic molecular crystals with polymers makes it possible to create materials with susceptible properties to changes in temperature and humidity.
- Xuesong Yang
- , Linfeng Lan
- & Hongyu Zhang
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Article
| Open AccessTetrachromatic vision-inspired neuromorphic sensors with ultraweak ultraviolet detection
Sensing and processing UV light is essential for advanced artificial visual perception system. Here, the authors report a controllable UV-ultrasensitive neuromorphic vision sensor using organic phototransistors to integrate sensing, memory and processing functions, and perform the static image and dynamic movie recognition.
- Ting Jiang
- , Yiru Wang
- & Wenping Hu
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Article
| Open AccessUltra-stretchable and biodegradable elastomers for soft, transient electronics
Stretchable and degradable elastomers are crucial for developing transient and bioresorbable electronics. Herein, Han et al. tuned the diverse properties of biodegradable PLCL elastomers and demonstrated their application in soft, perceptive robotic grippers and transient, suture-free cardiac jackets.
- Won Bae Han
- , Gwan-Jin Ko
- & Suk-Won Hwang
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| Open AccessDynamic self-organisation and pattern formation by magnon-polarons
Increasing the speed of magnetization switching is an obvious pathway to improve spintronic device performance. However, very fast magnetization switching is accompanied by instabilities. Here, Gidding et al study these instabilities using optical pumping, and show that instability generated spin-waves can achieve a high enough amplitude to drive switching of the magnetization, with a distinctive coherent pattern.
- M. Gidding
- , T. Janssen
- & A. Kirilyuk
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Article
| Open AccessRandom fractal-enabled physical unclonable functions with dynamic AI authentication
In order to be used on a large scale, unclonable tags for anti-counterfeiting should allow mass production at low cost, as well as fast and easy authentication. Here, the authors show how to use one-step annealing of gold films to quickly realize robust tags with high capacity, allowing fast deep-learning based authentication via smartphone readout.
- Ningfei Sun
- , Ziyu Chen
- & Qian Liu
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Article
| Open AccessDynamic machine vision with retinomorphic photomemristor-reservoir computing
Dynamic machine vision requires recognizing the past and predicting the future of moving objects. Here, the authors demonstrate retinomorphic photomemristor networks with inherent dynamic memory for accurate motion recognition and prediction.
- Hongwei Tan
- & Sebastiaan van Dijken
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Article
| Open AccessHalide Perovskite glues activate two-dimensional covalent organic framework crystallites for selective NO2 sensing
2D COFs are promising for resistance-related applications, but usually form powders where poor contacts at grain boundaries inhibit the conductivity. Here authors show that halide perovskites can act as electric glues to bond 2D COFs to improve their conductivity, activating them to detect NO2 with high selectivity and sensitivity.
- Wen Ye
- , Liangdan Zhao
- & Jian-Mei Lu
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Article
| Open AccessA supramolecular gel-elastomer system for soft iontronic adhesives
Electroadhesion in soft robotics provides controllable interfacial attraction for robotic functionalities but materials selection is limited. Here, Gao et. al. present an iontronic adhesive to design a soft iontronic gripper with self-healability, tunable adhesion at reduced voltages and rapid release.
- Dace Gao
- , Gurunathan Thangavel
- & Pooi See Lee
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Article
| Open AccessA neuromorphic bionic eye with filter-free color vision using hemispherical perovskite nanowire array retina
Designing full-color spherical artificial eyes remains a challenge. Here, Long et al. report a bionic eye where each pixel on the hemispherical retina can recognize different colors based on the unique bidirectional photo response; with optical adaptivity and neuromorphic preprocessing ability
- Zhenghao Long
- , Xiao Qiu
- & Zhiyong Fan
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Article
| Open AccessA two-dimensional mid-infrared optoelectronic retina enabling simultaneous perception and encoding
Designing an infrared machine vision system that can efficiently perceive, convert, and process a massive amount of data remains a challenge. Here, the authors present a retina-inspired 2D optoelectronic device based on van der Waals heterostructure that can perform the data perception and spike-encoding simultaneously for night vision, sensing, spectroscopy, and free-space communications.
- Fakun Wang
- , Fangchen Hu
- & Qi Jie Wang
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Article
| Open AccessSwitchable biomimetic nanochannels for on-demand SO2 detection by light-controlled photochromism
Conventional nanochannel sensors are passively responsive and may be slowly damaged by analytes present in the environment before detection. Here, authors developed a light-controlled inert/active-switchable biomimetic nanochannel sensor to achieve SO2 on-demand detection and long-term preservation.
- Dan Zhang
- , Yongjie Sun
- & Xuanjun Zhang
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Article
| Open AccessLight-driven peristaltic pumping by an actuating splay-bend strip
Small-scale manipulation of liquids is being controlled with bulky pumps or power sources. Dradrach et al. show a light-driven pumping of micro-liter liquid using a centimeter-long liquid crystal elastomer strip.
- Klaudia Dradrach
- , Michał Zmyślony
- & Piotr Wasylczyk
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Article
| Open AccessOrigami-based integration of robots that sense, decide, and respond
Origami-inspired engineering has enabled intelligent materials and structures to react to environments, yet a complete sense-decide-act autonomous loop is still challenging. Yan et al. introduce autonomous origami robots by embedding sensing, computing, and actuating in compliant, conductive materials.
- Wenzhong Yan
- , Shuguang Li
- & Ankur Mehta
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Article
| Open AccessOrganic electrochemical transistors as on-site signal amplifiers for electrochemical aptamer-based sensing
Electrochemical aptamer-based sensors typically exhibit limited sensitivity especially when the area of electrode is reduced for miniaturization. Here, the authors demonstrate electrochemical transistors as universal on-site amplifiers for enhancement in sensitivity of over 3 orders of magnitude.
- Xudong Ji
- , Xuanyi Lin
- & Jonathan Rivnay
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Article
| Open AccessD-O-A based organic phosphors for both aggregation-induced electrophosphorescence and host-free sensitization
Pure organic room-temperature phosphorescencent materials draw much attention but realising electroluminescence under electric excitation is challenging. Here the authors propose a donor-oxygen-acceptor molecular design realizing aggregation-induced organic room-temperature electrophosphorescence with high external quantum efficiency.
- Lulin Xu
- , Yuhang Mo
- & Junqiao Ding
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Article
| Open AccessUnraveling two distinct polymorph transition mechanisms in one n-type single crystal for dynamic electronics
Cooperative transitions have acquired much attention for low transition barriers, ultrafast kinetics, and structural reversibility but cooperative transitions are rare in molecular crystals and their origin is poorly understood. Here the authors show that reorientation of the alkyl side chains in a 2-dimensional quinoidal terthiophene triggers cooperative behavior, and establish alkyl chain engineering to control the polymorphic behavior.
- Daniel William Davies
- , Bumjoon Seo
- & Ying Diao
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Article
| Open AccessPolyvinyl chloride-based dielectric elastomer with high permittivity and low viscoelasticity for actuation and sensing
Dielectric elastomers (DEs) are widely used in soft actuators but existing DE actuators often require high driving electrical fields. Here the authors demonstrate that introducing cyanoethyl cellulose into plasticized PVC gel confers high dielectric permittivity and allows the fabrication of elastomer actuators with high permittivity and low viscoelasticity
- Jianjian Huang
- , Xiaodie Zhang
- & Dongjie Guo