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A unified state diagram for the yielding transition of soft colloids
The yielding transition in concentrated colloidal suspensions and emulsions lacks a universal description. A unified state diagram is now shown to underlie yielding for these materials, analogous to the van der Waals phase diagram for non-ideal gases.
- Stefano Aime
- , Domenico Truzzolillo
- & Luca Cipelletti
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Hierarchical amorphous ordering in colloidal gelation
Dynamic arrest in amorphous gels has so far been ascribed to glass transition. Now, experiments reveal a hierarchical structural ordering in dilute colloidal gels driven by the local potential energy, making this type of gel distinct from amorphous glasses.
- Hideyo Tsurusawa
- & Hajime Tanaka
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Enhanced singular jet formation in oil-coated bubble bursting
A bursting bubble produces a jet drop previously estimated to be too large to contribute to aerosolization. Oil-coated bubbles produce fast and thin jets, which break up into much smaller drops with potential implications for airborne transmission.
- Zhengyu Yang
- , Bingqiang Ji
- & Jie Feng
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Polymorphic crystalline wetting layers on crystal surfaces
Premelting refers to the formation of a thin liquid film on a crystal’s surface before it properly melts. Now, a similar mechanism is shown to occur before solid–solid transitions in colloidal crystals: the formation of a polymorphic crystalline layer.
- Xipeng Wang
- , Bo Li
- & Yilong Han
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Article
| Open AccessNon-specific adhesive forces between filaments and membraneless organelles
Many organelles in the cell are not encapsulated in a membrane—they are liquid-like domains formed through phase separation. The liquid-like nature of such domains leads to adhesive interactions between the cytoskeleton filaments and organelles.
- Thomas J. Böddeker
- , Kathryn A. Rosowski
- & Eric R. Dufresne
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Relationships between structure, memory and flow in sheared disordered materials
Whether and when a material deforms elastically or plastically depends on its microstructure. Experiments on two-dimensional colloidal systems show that in disordered materials, packing density, stress and a microstructure-related entropy govern deformations.
- K. L. Galloway
- , E. G. Teich
- & P. E. Arratia
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Letter |
Polar state reversal in active fluids
Active matter exhibits a plethora of collective phenomena in both biological and artificial systems. In a model system of colloidal rollers, polar states in active liquids can be controlled.
- Bo Zhang
- , Hang Yuan
- & Alexey Snezhko
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News & Views |
Have tail, will travel
The flagella of microorganisms have provided inspiration for many synthetic devices, but they’re typically not easy to produce. A new class of swimmer makes it look simple by spontaneously growing a tail that it can whip to self-propel.
- Sophie Ramananarivo
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Rechargeable self-assembled droplet microswimmers driven by surface phase transitions
A class of synthetic microswimmers self-assembled from alkane oil drops in a surfactant solution offers a rechargeable platform for studying how microorganisms exploit flagellar elasticity to move around.
- Diana Cholakova
- , Maciej Lisicki
- & Nikolai Denkov
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Morphology selection kinetics of crystallization in a sphere
The authors investigate the role of spherical confinement and curvature-induced topological defects on the crystallization of charged colloids. They conclude that crystallization in spherical confinement is due to a combination of thermodynamics and kinetic pathways.
- Yanshuang Chen
- , Zhenwei Yao
- & Peng Tan
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Binary icosahedral clusters of hard spheres in spherical confinement
The authors investigate out-of-equilibrium crystallization of a binary mixture of sphere-like nanoparticles in small droplets. They observe the spontaneous formation of an icosahedral structure with stable MgCu2 phases, which are promising for photonic applications.
- Da Wang
- , Tonnishtha Dasgupta
- & Alfons van Blaaderen
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News & Views |
A moiré foray
The transport properties of many two-dimensional systems are strongly affected by the proximity of a periodic pattern. Colloidal particles are now shown to have preferred sliding routes due to competing symmetries between two unmatched crystalline surfaces.
- Pietro Tierno
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The microscopic role of deformation in the dynamics of soft colloids
Simulations of a system comprising polymer rings with internal elasticity reveal a key role for deformation in controlling the microscopic dynamics of soft colloids.
- Nicoletta Gnan
- & Emanuela Zaccarelli
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Letter |
Targeted assembly and synchronization of self-spinning microgears
Active colloidal particles are shown to be capable of aggregating into stable spinning clusters that constitute self-powered microgears. The demonstration reveals a new design principle for micromachinery using dissipative building blocks.
- Antoine Aubret
- , Mena Youssef
- & Jérémie Palacci
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News & Views |
Brought to the surface
There is growing evidence for the kinetics of homogeneous nucleation being a multi-step process. Colloid experiments and simulations now suggest that heterogeneous nucleation is no exception.
- Rajesh Ganapathy
- & Ajay K. Sood
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Surface-assisted single-crystal formation of charged colloids
Controlled crystal growth can be achieved by initiating nucleation on a substrate — but the mechanisms at play are still poorly understood. Experiments and simulations now reveal conditions for the growth of defect-free crystals of charged colloids.
- Shunto Arai
- & Hajime Tanaka
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News & Views |
A microscopic army
Ensembles of magnetic colloids can undergo an instability triggering the formation of clusters that move faster than the particles themselves. The many-body process relies on hydrodynamics alone and may prove useful for load delivery in fluidics.
- Pietro Tierno
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Letter |
Unstable fronts and motile structures formed by microrollers
Collections of rolling colloids are shown to pinch off into motile clusters resembling droplets sliding down a windshield. These stable dynamic structures are formed through a fingering instability that relies on hydrodynamic interactions alone.
- Michelle Driscoll
- , Blaise Delmotte
- & Paul Chaikin
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News & Views |
Disorder in the wild
Simple models have given us surprising insight into how animals flock, but most assume they do so through a homogeneous landscape. Colloidal experiments now suggest that a little disorder can have unexpected — and spectacular — effects.
- C. J. Olson Reichhardt
- & C. Reichhardt
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Letter |
Distortion and destruction of colloidal flocks in disordered environments
Our understanding of collective animal behaviour generally assumes that flocks and herds move through homogeneous environments. Colloidal experiments suggest that flocking can be distorted or even suppressed by the introduction of disorder.
- Alexandre Morin
- , Nicolas Desreumaux
- & Denis Bartolo
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Correlation between dynamical and structural heterogeneities in colloidal hard-sphere suspensions
Experiments combining dynamic and static light scattering have probed a colloidal hard-sphere system for the formation of dynamical and structural heterogeneities, which play a role in both forms of solidification: crystallization and vitrification.
- Sebastian Golde
- , Thomas Palberg
- & Hans Joachim Schöpe
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Transmission of torque at the nanoscale
A study of a composite soft-matter nanomechanical system consisting of a rotating ring of optically trapped colloidal particles confining a set of untrapped colloids demonstrates the possibility of gearwheel-like torque transmission on the nanoscale.
- Ian Williams
- , Erdal C. Oğuz
- & C. Patrick Royall
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News & Views |
Getting the drops in
When a bubble bursts at a liquid–gas interface, a portion of gas is released from the liquid. Now, another, counterintuitive process is reported: rapid motion generated by bubble-bursting transports oil droplets from the surface into the interior of a volume of water.
- Jens Eggers
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Nanoemulsions obtained via bubble-bursting at a compound interface
When a bubble bursts on reaching a surface, mass transfer from the liquid to the gas phase can occur—aerosol dispersion. Now, the inverse transport process is reported: submicrometre-sized oil droplets, formed during bubble-bursting, are zipped across the interface to the liquid phase.
- Jie Feng
- , Matthieu Roché
- & Howard A. Stone
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News & Views |
Colloidal suspense
According to classical nucleation theory, a crystal grows from a small nucleus that already bears the symmetry of its end phase — but experiments with colloids now reveal that, from an amorphous precursor, crystallites with different structures can develop.
- László Gránásy
- & Gyula I. Tóth
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Visualizing kinetic pathways of homogeneous nucleation in colloidal crystallization
Assemblies of colloidal particles provide a micrometre-scale analogue of atomic and molecular liquids and solids. Now, real-time visualization of the liquid-solid transition in systems of spherical colloids reveals complex pathways involving precursors of hexagonal close-packed, body-centred cubic and face-centred cubic symmetry.
- Peng Tan
- , Ning Xu
- & Lei Xu
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News & Views |
A cool liquid that does not freeze
A simulation study of a model that mimics certain colloidal particles reveals a surprising low-temperature triumph of entropy, whereby the liquid state persists down to zero temperature.
- Jeppe C. Dyre
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Letter |
Liquids more stable than crystals in particles with limited valence and flexible bonds
Patchy colloidal systems consist of particles with attractive patches on them. If the bonds between particles are allowed to be flexible, a colloidal liquid state may be observed as the system approaches zero temperature.
- Frank Smallenburg
- & Francesco Sciortino
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