Featured
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Article |
Equilibrium climate sensitivity above 5 °C plausible due to state-dependent cloud feedback
Simulations suggest a shift to a high sensitivity of Earth’s climate to increasing CO2 can be attributed to the decline in the ice content in clouds as the climate warms.
- Jenny Bjordal
- , Trude Storelvmo
- & Tim Carlsen
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Editorial |
Up in smoke
Where there is smoke, there are radiative feedbacks. With wildfires becoming a growing problem in the Anthropocene, we need to better understand the influence of fire on the climate system.
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Article |
Longwave radiative effect of the cloud twilight zone
The transitional state between cloudy and clear skies, known as the twilight zone, has a substantial effect on the atmospheric energy budget, according to an analysis of cloud fields using global satellite observations.
- Eshkol Eytan
- , Ilan Koren
- & Ayala Ronen
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Article |
Widespread biomass burning smoke throughout the remote troposphere
Aerosol particles produced by biomass burning are ubiquitous in the remote troposphere, according to global airborne measurements over remote ocean regions.
- G. P. Schill
- , K. D. Froyd
- & D. M. Murphy
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Article |
Amplified transboundary transport of haze by aerosol–boundary layer interaction in China
Secondary air pollution events are enhanced in the Yangtze River delta, China, due to the interaction of long-range transport and aerosol–boundary layer feedback, according to a combination of observations and simulations of haze events from 2013 to 2018.
- Xin Huang
- , Aijun Ding
- & Congbin Fu
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News & Views |
Clues to late accretion from Venus’s atmosphere
Whether Earth’s water was delivered early or late in its formation is debated. The composition of Venus’s atmosphere may indicate that late accretion, the final stage of planet formation, delivered little water to the terrestrial planets.
- Ramon Brasser
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Article |
Dry late accretion inferred from Venus’s coupled atmosphere and internal evolution
Venus’s atmospheric composition suggests limited water delivery to the terrestrial planets by late accretion, according to numerical simulations of the interior and atmospheric evolution of Venus under various late accretion scenarios.
- C. Gillmann
- , G. J. Golabek
- & V. Debaille
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Article |
The influence of the stratospheric Quasi-Biennial Oscillation on trace gas levels at the Earth’s surface
Interannual variations of long-lived trace gas mole fractions at the Earth’s surface are primarily driven by the stratospheric Quasi-Biennial Oscillation, according to surface measurements and model simulations. Ignoring this variability may induce errors in estimating emissions of trace gases.
- Eric A. Ray
- , Robert W. Portmann
- & Karen H. Rosenlof
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Article |
Efficient control of atmospheric sulfate production based on three formation regimes
Distinct dependence of atmospheric SO42– formation on NOx levels in haze-fog events is revealed by SO42– production isopleths that are obtained through simulations of atmospheric chemistry with a box model.
- Jian Xue
- , Xin Yu
- & Jian Zhen Yu
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Article |
A two-pollutant strategy for improving ozone and particulate air quality in China
Observations confirm that cleaning up fine particulate matter in the North China Plain has exacerbated ozone pollution, suggesting that both NOx and VOC emissions need to be reduced to improve air quality.
- Ke Li
- , Daniel J. Jacob
- & Shixian Zhai
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Matters Arising |
Reply to: Complexities between plants and the atmosphere
- A. Rap
- , C. E. Scott
- & D. V. Spracklen
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Perspective |
Challenges for the recovery of the ozone layer
Recovery of the stratospheric ozone layer above Antarctica has not been straightforward, as a result of human activities and climate change. The recovery process might be delayed by up to decades if further mitigation actions are not taken.
- Xuekun Fang
- , John A. Pyle
- & Ronald G. Prinn
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Article |
Ammonium nitrate particles formed in upper troposphere from ground ammonia sources during Asian monsoons
Solid ammonium nitrate particles are formed in the upper troposphere during the Asian monsoons, which bring large amounts of ground ammonia to this altitude, according to integrated analyses of measurements on ammoniated aerosol, together with model simulations.
- Michael Höpfner
- , Jörn Ungermann
- & Ingo Wohltmann
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Editorial |
Cleaner air for China
China’s rigorous air-pollution control has greatly reduced the levels of fine particles in the atmosphere. Further progress for air quality more broadly will rely on fully accounting for complex chemical reactions between pollutants.
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News & Views |
China’s nitrogen management
Nitrogen deposition in China has stabilized over the past decade, thanks to efficient regulation of fertilizer use, suggests an analysis of wet and dry deposition.
- Maria Kanakidou
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News & Views |
To sink or swim in Titan’s lakes
Flotation of aerosols as a film on the hydrocarbon lakes of Saturn’s moon Titan may explain the lakes’ stillness, and could influence the atmospheric hydrocarbon cycle.
- Isabelle Couturier-Tamburelli
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Article |
The floatability of aerosols and wave damping on Titan’s seas
Organic aerosols that sediment from Titan’s atmosphere may float, form a film and damp waves on Titan’s seas, according to computations. This damping effect could explain the observed smoothness of Titan’s seas.
- Daniel Cordier
- & Nathalie Carrasco
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Article |
Stabilization of atmospheric nitrogen deposition in China over the past decade
Nitrogen deposition in China has been almost constant over the past decade, as decreasing wet deposition has balanced increasing dry deposition, according to analyses of extensive datasets on wet and dry nitrogen depositions in China.
- Guirui Yu
- , Yanlong Jia
- & Keith Goulding
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Article |
Atmospheric transport and deposition of microplastics in a remote mountain catchment
Microplastics can reach and affect regions far from where they are released because of atmospheric transport, suggest analyses of atmospheric deposition in a remote, pristine mountain catchment in France.
- Steve Allen
- , Deonie Allen
- & Didier Galop
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Article |
Independent confirmation of a methane spike on Mars and a source region east of Gale Crater
A methane spike 15.5 ± 2.5 parts per billion by volume was detected in the Martian atmosphere above Gale Crater on 16 June 2013 by Mars Express, independently confirming the debated in situ observation by the Curiosity rover a day earlier.
- Marco Giuranna
- , Sébastien Viscardy
- & Marilena Amoroso
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Article |
Methane seasonal cycle at Gale Crater on Mars consistent with regolith adsorption and diffusion
The seasonal cycle in the methane mixing ratio observed at Gale Crater on Mars can be explained by adsorption onto and diffusion through the regolith, suggests a one-dimensional numerical model with geological constraints.
- John E. Moores
- , Raina V. Gough
- & Christopher R. Webster
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Article |
Insignificant influence of the 11-year solar cycle on the North Atlantic Oscillation
Any influence of the 11-year solar cycle on the North Atlantic Oscillation is insignificant, and could have been a chance occurrence, suggest analyses of the instrumental record and of chemistry–climate model simulations.
- Gabriel Chiodo
- , Jessica Oehrlein
- & Anne K. Smith
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Article |
Rapid increase in ozone-depleting chloroform emissions from China
Atmospheric levels of chloroform increased after 2010, as a result of emissions in eastern China, according to analyses of measurements and inverse modelling.
- Xuekun Fang
- , Sunyoung Park
- & Ronald G. Prinn
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Article |
O2 solubility in Martian near-surface environments and implications for aerobic life
Despite little O2 in the Martian atmosphere, concentrations of dissolved O2 in near-surface brines on Mars may be sufficient to support aerobic life, according to solubility calculations.
- Vlada Stamenković
- , Lewis M. Ward
- & Woodward W. Fischer
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Article |
Enhanced global primary production by biogenic aerosol via diffuse radiation fertilization
Biogenic aerosols produced by terrestrial vegetation substantially enhance global primary productivity of plants, according to integrated model analyses.
- A. Rap
- , C. E. Scott
- & D. V. Spracklen
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Article |
Magnetite authigenesis and the warming of early Mars
Experiments suggest that magnetite precipitation on early Mars was accompanied by the release of H2 that may have helped to warm the planet and stabilize liquid water at the Martian surface.
- Nicholas J. Tosca
- , Imad A. M. Ahmed
- & Joel A. Hurowitz
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Article |
Major secondary aerosol formation in southern African open biomass burning plumes
A substantial amount of secondary aerosols form within hours of biomass burning in southern African savannah and grassland fires, according to analyses of 5.5 years of continuous field measurements.
- Ville Vakkari
- , Johan P. Beukes
- & Pieter G. van Zyl
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Review Article |
A post-Cassini view of Titan’s methane-based hydrologic cycle
The Cassini mission revealed the complex workings of Titan’s methane-based hydrologic cycle over a range of timescales, providing a potential window into the future of Earth and its water cycle.
- Alexander G. Hayes
- , Ralph D. Lorenz
- & Jonathan I. Lunine
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Editorial |
Mars at war
Whether the climate of early Mars was warm and wet or cold and dry remains unclear, but the debate is overheated. With a growing toolbox and increasing data to tackle the open questions, progress is possible if there is openness to bridging the divide.
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Perspective |
The geological and climatological case for a warmer and wetter early Mars
A warm and semi-arid climate may be most consistent with geological evidence for flowing water on the surface of early Mars, despite the challenges of warming Mars under a faint young Sun.
- Ramses M. Ramirez
- & Robert A. Craddock
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Article |
A vegetation control on seasonal variations in global atmospheric mercury concentrations
Terrestrial vegetation contributes to the seasonal variation of atmospheric mercury concentrations, according to analyses of atmospheric trace gas dynamics and satellite data. The data show that the photosynthetic activity of vegetation correlates with atmospheric mercury.
- Martin Jiskra
- , Jeroen E. Sonke
- & Aurélien Dommergue
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Article |
Observationally derived rise in methane surface forcing mediated by water vapour trends
Observations of the radiative forcing from methane at the Earth’s surface are influenced by absorption effects from water vapour, according to spectroscopic measurements and line-by-line calculations.
- D. R. Feldman
- , W. D. Collins
- & M. S. Torn
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Article |
Discrepancy between simulated and observed ethane and propane levels explained by underestimated fossil emissions
Observations of ethane and propane distributions in the atmosphere are reproduced in simulations with an atmospheric chemistry transport model, if fossil emissions are a factor of two to three higher than previously assumed.
- Stig B. Dalsøren
- , Gunnar Myhre
- & Markus Wallasch
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Article |
Effects of primitive photosynthesis on Earth’s early climate system
Amplification of the methane cycle by anyoxygenic photosynthesis could have warmed early Earth and countered the faint young Sun, geochemical modelling suggests. A combination of H2-based and Fe2+-based photosynthesis acts to enhance methane fluxes.
- Kazumi Ozaki
- , Eiichi Tajika
- & Christopher T. Reinhard
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News & Views |
Tracking pollutant emissions
Progress in the post-combustion treatment of diesel vehicle exhaust has led to shifting proportions of the constituents of nitrogen oxides. Observations from 61 European cities suggest that the outlook on attaining NO2 standards is more optimistic than expected.
- Drew R. Gentner
- & Fulizi Xiong
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Article |
Lower vehicular primary emissions of NO2 in Europe than assumed in policy projections
The fraction of NO2 in NO x emitted from European road transport is up to a factor of two smaller than used in policy projections, suggests an analysis of 130 million roadside observations. Roadside air quality standards may thus be obtained faster.
- Stuart K. Grange
- , Alastair C. Lewis
- & David C. Carslaw
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News & Views |
Icy Mars lakes warmed by methane
The release of methane trapped in Martian subsurface reservoirs following planetary obliquity shifts may have contributed to episodic climate warming between 3.6 and 3 billion years ago, explaining evidence for ancient ice-covered lakes.
- Alberto G. Fairén
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Article |
Methane bursts as a trigger for intermittent lake-forming climates on post-Noachian Mars
Bursts of methane stored in the Martian subsurface may explain intermittent warm climates on ancient Mars, according to numerical simulations. Sedimentary evidence for palaeolakes requires infrequent, yet sustained, lake-forming climates.
- Edwin S. Kite
- , Peter Gao
- & Yuk L. Yung
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Article |
Comprehensive characterization of atmospheric organic carbon at a forested site
Atmospheric organic compounds are central to key chemical processes that influence air quality. Concurrent measurements of a wide range of these compounds, including previously unmeasured ones, provide closure on OH reactivity.
- James F. Hunter
- , Douglas A. Day
- & Jesse H. Kroll
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Article |
The strength of the meridional overturning circulation of the stratosphere
The strength of the global meridional overturning circulation in the stratosphere is uncertain. An analysis of satellite data, reanalyses and model simulations reveals a strength of 6.3–7.6 × 109 kg s−1, but no convergence at higher altitudes.
- Marianna Linz
- , R. Alan Plumb
- & Jessica L. Neu
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Article |
Small fraction of marine cloud condensation nuclei made up of sea spray aerosol
Sea spray aerosols are thought to alter cloud properties in remote ocean regions. Aerosol analyses over four ocean regions reveal that these aerosols represent less than 30% of cloud condensation nuclei in typical marine boundary layer clouds.
- P. K. Quinn
- , D. J. Coffman
- & T. S. Bates
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Large sulfur isotope fractionations in Martian sediments at Gale crater
Ancient Mars may have had an active sulfur cycle. In situ analyses by the Curiosity rover reveal large variations in the current sulfur isotopic composition of Martian sediments that can be explained by geologic and atmospheric processes.
- H. B. Franz
- , A. C. McAdam
- & B. Sutter
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Editorial |
For people and planet
The emerging field of geohealth links human well-being and ecosystem health. A deeper understanding of these linkages can help society mitigate the health costs of economic growth before they become crises.
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Article |
Transition from high- to low-NOx control of night-time oxidation in the southeastern US
The influence of NOx levels at night on atmospheric oxidation is unclear. Analyses of aircraft observations suggest that night-time oxidation is transitioning from a high- to low-NOx regime in the southeast US due to declines in NOx levels.
- P. M. Edwards
- , K. C. Aikin
- & S. S. Brown
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Perspective |
The deep atmosphere of Venus and the possible role of density-driven separation of CO2 and N2
The only temperature profile of the lowermost Venusian atmosphere appears unstable. Compositional heterogeneity due to density-driven separation of N2 from CO2 gas in the lower atmosphere of Venus may be a viable explanation.
- Sebastien Lebonnois
- & Gerald Schubert
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Article |
Large anomalies in lower stratospheric water vapour and ice during the 2015–2016 El Niño
The El Niño of 2015–2016 was unusual and exceptionally strong. Satellite observations and modelling suggest that convective lofting and sublimation of ice particles during this event contributed to moistening of the lower stratosphere.
- Melody A. Avery
- , Sean M. Davis
- & Andrew E. Dessler
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Article |
Detection of a persistent meteoric metal layer in the Martian atmosphere
Collisions of dust particles with a planet’s atmosphere lead to the accumulation of metallic atoms at high altitudes. MAVEN spacecraft observations reveal a persistent—but temporally variable—metal layer of Mg+ ions in the Martian atmosphere.
- M. M. J. Crismani
- , N. M. Schneider
- & B. M. Jakosky
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Article |
Top-of-atmosphere radiative forcing affected by brown carbon in the upper troposphere
Brown carbon absorbs light, but its climate impacts in the upper troposphere are not well known. A series of aircraft observations in the US reveals that convection lofts brown carbon to high altitudes, causing greater warming than at lower altitudes.
- Yuzhong Zhang
- , Haviland Forrister
- & Rodney J. Weber
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News & Views |
Warming or cooling dust?
Mineral dust particles interact with solar and terrestrial radiation. Statistical analyses of observational data and global simulations reveal that atmospheric dust is coarser than previously thought, and could cause warming of the atmosphere.
- Paul Ginoux