Abstract
Cavity quantum electrodynamics provides the setting for quantum control of strong interactions between a single atom and one photon. Many such atom–cavity systems interacting by coherent exchanges of single photons could be the basis for scalable quantum networks. However, moving beyond current proof-of-principle experiments involving just one or two conventional optical cavities requires the localization of individual atoms at distances ≲100 nm from a resonator’s surface. In this regime an atom can be strongly coupled to a single intracavity photon while at the same time experiencing significant radiative interactions with the dielectric boundaries of the resonator. Here, we report using real-time detection and high-bandwidth feedback to select and monitor single caesium atoms located ∼100 nm from the surface of a microtoroidal optical resonator. Strong radiative interactions of atom and cavity field probe atomic motion through the evanescent field of the resonator and reveal both the significant role of Casimir–Polder attraction and the manifestly quantum nature of the atom–cavity dynamics.
This is a preview of subscription content, access via your institution
Access options
Subscribe to this journal
Receive 12 print issues and online access
$209.00 per year
only $17.42 per issue
Buy this article
- Purchase on Springer Link
- Instant access to full article PDF
Prices may be subject to local taxes which are calculated during checkout
Similar content being viewed by others
References
Casimir, H. B. G. & Polder, D. The influence of retardation on the London–van der Waals forces. Phys. Rev. 73, 360–372 (1948).
Purcell, E. M. Spontaneous emission probabilities at radio frequencies. Phys. Rev. 69, 681 (1946).
Drexhage, K. H. in Progress in Optics, Vol. XII (ed. Wolf, E.) 163–232 (Elsevier, 1974).
Gabrielse, G. & Dehmelt, H. Observation of inhibited spontaneous emission. Phys. Rev. Lett. 55, 67–70 (1985).
Hulet, R. G., Hilfer, E. S. & Kleppner, D. Inhibited spontaneous emission by a Rydberg atom. Phys. Rev. Lett. 55, 2137–2140 (1985).
Haroche, S. & Kleppner, D. Cavity quantum electrodynamics. Phys. Today 42, 24–30 (1989).
Sukenik, C. I., Boshier, M. G., Cho, D., Sandoghar, V. & Hinds, E. A. Measurement of the Casimir–Polder force. Phys. Rev. Lett. 70, 560–563 (1993).
Berman, P. Cavity Quantum Electrodynamics (Academic Press, 1994).
Odom, B., Hanneke, D., D’Urso, B. & Gabrielse, G. New measurement of the electron magnetic moment using a one-electron quantum cyclotron. Phys. Rev. Lett. 97, 030801 (2006).
Michler, P. et al. A quantum dot single-photon turnstile device. Science 290, 2282–2285 (2000).
Jaynes, E. T. & Cummings, F. W. Comparison of quantum and semiclassical radiation theories with application to the beam maser. Proc. IEEE 51, 89–109 (1963).
Meschede, D., Walther, H. & Müller, G. One-atom maser. Phys. Rev. Lett. 54, 551–554 (1985).
Thompson, R. J., Rempe, G. & Kimble, H. J. Observation of normal-mode splitting for an atom in an optical cavity. Phys. Rev. Lett. 68, 1132–1135 (1992).
Haroche, S. & Raimond, J-M. Exploring the Quantum: Atoms Cavities, and Photons (Oxford Univ. Press, 2006).
Miller, R. et al. Trapped atoms in cavity QED: Coupling quantized light and matter. J. Phys. B 38, S551–S565 (2005).
Vahala, K. J. Optical microcavities. Nature 424, 839–846 (2004).
Khitrova, G., Gibbs, H. M., Kira, M., Koch, S. W. & Scherer, A. Vacuum Rabi splitting in semiconductors. Nature Phys. 2, 81–90 (2006).
Schoelkopf, R. J. & Girvin, S. M. Wiring up quantum systems. Nature 451, 664–669 (2008).
McKeever, J., Boca, A., Boozer, A. D., Buck, J. R. & Kimble, H. J. Experimental realization of a one-atom laser in the regime of strong coupling. Nature 425, 268–271 (2003).
Weber, B. et al. Photon-photon entanglement with a single trapped atom. Phys. Rev. Lett. 102, 030501 (2009).
DiCarlo, L. et al. Demonstration of two-qubit algorithms with a superconducting quantum processor. Nature 460, 240–244 (2009).
Gehr, R. et al. Cavity-based single atom preparation and high-fidelity hyperfine state readout. Phys. Rev. Lett. 104, 203602 (2010).
Kimble, H. J. The quantum internet. Nature 453, 1023–1030 (2008).
Armani, D. K., Kippenberg, T. J., Spillane, S. M. & Vahala, K. J. Ultra-high-Q toroid microcavity on a chip. Nature 421, 925–928 (2003).
Rosenblit, M., Horak, P., Helsby, S. & Folman, R. Single-atom detection using whispering-gallery modes of microdisk resonators. Phys. Rev. A 70, 053808 (2004).
Lev, B., Srinivasan, K., Barclay, P., Painter, O. & Mabuchi, H. Feasibility of detecting single atoms using photonic bandgap cavities. Nanotechnology 15, S556–S561 (2004).
Spillane, S. M. et al. Ultrahigh-Q toroidal microresonators for cavity quantum electrodynamics. Phys. Rev. A 71, 013817 (2005).
Colombe, Y. et al. Strong atom-field coupling for Bose–Einstein condensates in an optical cavity on a chip. Nature 450, 272–276 (2007).
Eichenfield, M., Camacho, R., Chan, J., Vahala, K. J. & Painter, O. A picogram- and nanometre-scale photonic-crystal optomechanical cavity. Nature 459, 550–556 (2009).
Folman, R., Krüger, P., Schmiedmayer, J., Denschlag, J. & Henkel, C. Microscopic atom optics: from wires to an atom chip. Adv. At. Mol. Opt. Phys. 48, 263–356 (2002).
Reichel, J. Microchip traps and Bose–Einstein condensation. Appl. Phys. B 75, 469–487 (2002).
Aoki, T. et al. Observation of strong coupling between one atom and a monolithic microresonator. Nature 442, 671–674 (2006).
Dayan, B. et al. A photon turnstile dynamically regulated by one atom. Science 319, 1062–1065 (2008).
Aoki, T. et al. Efficient routing of single photons by one atom and a microtoroidal cavity. Phys. Rev. Lett. 102, 083601 (2009).
Vernooy, D. W. & Kimble, H. J. Quantum structure and dynamics for atom galleries. Phys. Rev. A 55, 1239–1261 (1997).
Rosenblit, M., Japha, Y., Horak, P. & Folman, R. Simultaneous optical trapping and detection of atoms by microdisk resonators. Phys. Rev. A 73, 063805 (2006).
Birnbaum, K. M., Parkins, A. S. & Kimble, H. J. Cavity QED with multiple hyperfine levels. Phys. Rev. A 74, 063802 (2006).
Buhmann, S. Y. Casimir–Polder forces on excited atoms in the strong atom-field coupling regime. Phys. Rev. A 77, 012110 (2008).
Balykin, V. I., Hakuta, K., Le Kien, F., Liang, J. Q. & Morinaga, M. Atom trapping and guiding with a subwavelength-diameter optical fiber. Phys. Rev. A 70, 011401(R) (2004).
Vetsch, E. et al. Optical interface created by laser-cooled atoms trapped in the evanescent field surrounding an optical nanofiber. Phys. Rev. Lett. 104, 203603 (2010).
Ye, J., Kimble, H. J. & Katori, H. Quantum state engineering and precision metrology using state-insensitive light traps. Science 320, 1734–1738 (2008).
Mabuchi, H. & Kimble, H. J. Atom galleries for whispering atoms: binding atoms in stable orbits around an optical resonator. Opt. Lett. 19, 749–751 (1994).
Spillane, S. M., Kippenberg, T. J., Painter, O. & Vahala, K. J. Ideality in a fiber-taper-coupled microresonator system for application to cavity quantum electrodynamics. Phys. Rev. Lett. 91, 043902 (2003).
Acknowledgements
We acknowledge financial support from NSF, DoD NSSEFF programme, Northrop Grumman Aerospace Systems, ARO and IARPA. N.P.S. acknowledges support of the Caltech Tolman Postdoctoral Fellowship. H.L. thanks the Center for the Physics of Information. Toroid fabrication was done in the Kavli Nanoscience Institute. The authors thank A. S. Parkins, J. Ye and P. Zoller for illuminating discussions.
Author information
Authors and Affiliations
Contributions
T.A. and H.J.K. conceived the experiment. D.J.A. and N.P.S. carried out the measurements, analysed data and implemented simulation modelling. H.L., E.O. and K.J.V. fabricated microtoroids and provided expertise for tapered fibre coupling. D.J.A., N.P.S. and H.J.K. prepared the manuscript.
Corresponding author
Ethics declarations
Competing interests
The authors declare no competing financial interests.
Supplementary information
Supplementary Information
Supplementary Information (PDF 2182 kb)
Rights and permissions
About this article
Cite this article
Alton, D., Stern, N., Aoki, T. et al. Strong interactions of single atoms and photons near a dielectric boundary. Nature Phys 7, 159–165 (2011). https://doi.org/10.1038/nphys1837
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1038/nphys1837
This article is cited by
-
Strong coupling of hybrid states of light and matter in cavity-coupled quantum dot solids
Scientific Reports (2023)
-
Microscale whispering-gallery-mode light sources with lattice-confined atoms
Scientific Reports (2021)
-
Whispering-gallery-mode sensors for biological and physical sensing
Nature Reviews Methods Primers (2021)
-
Cavity QED based on room temperature atoms interacting with a photonic crystal cavity: a feasibility study
Applied Physics B (2020)
-
Fabrication of high-Q lithium niobate microresonators using femtosecond laser micromachining
Scientific Reports (2015)