Letters to Nature

Nature 397, 673-675 (25 February 1999) | doi:10.1038/17755; Received 25 August 1998; Accepted 8 December 1998

Aharonov–Bohm oscillations in carbon nanotubes

Adrian Bachtold1, Christoph Strunk1, Jean-Paul Salvetat2, Jean-Marc Bonard2, Laszló Forró2, Thomas Nussbaumer1 & Christian Schönenberger1

  1. Institut für Physik, Universität Basel, Klingelbergstrasse 82, CH-4056 Basel, Switzerland
  2. Institut de Génie Atomique, École Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland

Correspondence to: Christian Schönenberger1 Correspondence and requests for materials should be addressed to C.S. (e-mail: Email: Schonenberg@ubaclu.unibas.ch).

When electrons pass through a cylindrical electrical conductor aligned in a magnetic field, their wave-like nature manifests itself as a periodic oscillation in the electrical resistance as a function of the enclosed magnetic flux1. This phenomenon reflects the dependence of the phase of the electron wave on the magnetic field, known as the Aharonov–Bohm effect2, which causes a phase difference, and hence interference, between partial waves encircling the conductor in opposite directions. Such oscillations have been observed in micrometre-sized thin-walled metallic cylinders3, 4, 5 and lithographically fabricated rings6, 7, 8. Carbon nanotubes9, 10 are composed of individual graphene sheets rolled into seamless hollow cylinders with diameters ranging from 1 nm to about 20 nm. They are able to act as conducting molecular wires11, 12, 13, 14, 15, 16, 17, 18, making them ideally suited for the investigation of quantum interference at the single-molecule level caused by the Aharonov–Bohm effect. Here we report magnetoresistance measurements on individual multi-walled nanotubes, which display pronounced resistance oscillations as a function of magnetic flux.We find that the oscillations are in good agreement with theoretical predictions for the Aharonov–Bohm effect in a hollow conductor with a diameter equal to that of the outermost shell of the nanotubes. In some nanotubes we also observe shorter-period oscillations, which might result from anisotropic electron currents caused by defects in the nanotube lattice.

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