Abstract
It is known that in classical fluids turbulence typically occurs at high Reynolds numbers. But can turbulence occur at low Reynolds numbers? Here we investigate the transition to turbulence in the classic Taylor-Couette system in which the rotating fluids are manufactured ferrofluids with magnetized nanoparticles embedded in liquid carriers. We find that, in the presence of a magnetic field transverse to the symmetry axis of the system, turbulence can occur at Reynolds numbers that are at least one order of magnitude smaller than those in conventional fluids. This is established by extensive computational ferrohydrodynamics through a detailed investigation of transitions in the flow structure and characterization of behaviors of physical quantities such as the energy, the wave number and the angular momentum through the bifurcations. A finding is that, as the magnetic field is increased, onset of turbulence can be determined accurately and reliably. Our results imply that experimental investigation of turbulence may be feasible by using ferrofluids. Our study of transition to and evolution of turbulence in the Taylor-Couette ferrofluidic flow system provides insights into the challenging problem of turbulence control.
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Introduction
In classical Newtonian fluid, it is known that turbulence typically occurs in the high Reynolds number regime1,2. Here, the Reynolds number () is a dimensionless quantity defined as , where and are the characteristic length scale and a typical velocity of the flow in a particular geometry, respectively and is the kinematic viscosity. The quantities l and u may differ essentially from the size of the streamline body and the mean velocity around, respectively. As a result, for different flow systems the critical Re values of transition to turbulence can be quite different and, in some cases (e.g., pipe flows), may even approach infinity3. In the paradigmatic setting of a uniform flow of velocity u past a cylinder of diameter l, when Re is of the order of tens, the flow is regular. For Re in the hundreds, von Kármán vortex street forms behind the cylinder4, breaking certain symmetries of the system. Fully developed turbulence, in which the broken symmetries are restored, occurs at very high Reynolds numbers, typically in the thousands, rendering challenging study of turbulence (both experimentally where flow systems of enormous size and/or high velocity are required and computationally where unconventionally high resolution in the numerical integration of the Navier-Stokes equation is needed). It is thus desirable that fluid turbulence can emerge in physical flows of relatively low Reynolds numbers.
The routes to turbulence in different flow systems can be different. For three-dimensional flows described by the Navier-Stokes equations, there are four main routes5,6: (a) quasi-periodicity (with two frequencies on two tori) and phase locking, (b) subharmonic (period doubling) bifurcations, (c) three frequencies (on two or three tori) and (d) intermittency. An example is that, in the Couette flow system with a rotating inner cylinder, fully developed turbulence can occur after a sequence of bifurcations1. In fact, the emergence of fully developed turbulence depends not only on the Reynolds number, but also on the particular characteristics of the underlying flow. For example, it was observed experimentally7 that the flow of a sufficiently elastic polymer solution in a small volume can become irregular even at low velocity. In combination with the high viscosity, the corresponding Reynolds number can be very low - on the order of unity. The irregular flow has all the key features of fully developed turbulence, i.e., it exhibits a broad range of spatial and temporal scales.
To understand and “control” turbulence8,9 is of great interest. Typically, the energy dissipation associated with a turbulent flow can be much larger than that with laminar flows. This can have economical impacts. For example, in oil pipelines the pressure required to pump a turbulent fluid is typically up to thirty times larger than that which would be necessary for laminar flows. To keep the flow laminar for as high values of the Reynolds number as possible, it is common to add polymers into the flow in oil pipelines. Similarly, one can consider ferrofluids in closed circular systems and use an applied magnetic field to keep the flow laminar. There were pioneering experimental10,11 and computational11,12 works on turbulence in ferrofluidic flows. Studying transition to turbulence in non-Newton fluid systems has thus been a topic of continuous interest.
In this paper, we investigate the Taylor-Couette flow13 in finite systems (e.g., aspect ratio Γ = 20) where a rotating ferrofluid14 is confined by axial end walls, i.e., non-rotating lids, in the presence of an external magnetic field. The classic Taylor-Couette flow of non-magnetic fluid has been a computational15,16 and experimental17,18,19 paradigm to investigate a variety of nonlinear and complex dynamical phenomena, including transition to turbulence at high Reynolds numbers20. The system we study consists of two independently rotating, concentric cylinders with viscous ferrofluid filled in between, which has embedded within itself artificially dispersed magnetized nanoparticles. In the absence of any external magnetic field, the magnetic moments of the nanoparticles are randomly oriented, leading to zero net magnetization for the entire fluid. In this case, the magnetized nanoparticles have little effect on the physical properties of the fluid such as density and viscosity. However, when a transverse magnetic field is applied, the physical properties of the fluid can be significantly modified14,21, leading to drastic changes in the underlying hydrodynamics. For example, for the system of rotating ferrofluid14, an external magnetic field can stabilize regular dynamical states22,23,24,25 and induce dramatic changes in the flow topology22,23,26. (In fact, the effects of magnetic field are particularly important for geophysical flows27,28,29,30). In general, the magnetic field can be used effectively as a control or bifurcation parameter of the system, whose change can lead to characteristically distinct types of hydrodynamical behaviors22,23,24,25. In this regard, transition to turbulence in magnetohydrodynamical (MHD) flows with current-driven instabilities of helical fields has been investigated31. There is also a large body of literature on MHD dynamics in Taylor-Couette flows32,33,34,35. Existing works on rotating ferrofluids22,23,24,36,37,38, however, are mostly concerned with steady time-independent flows. Time-dependent ferrofluid flows have been investigated only recently but in the non-turbulent regime39.
The interaction between ferrofluid and magnetic field leads to additional terms in the Navier-Stokes equation22,25,37. Our extensive computations reveal a sequence of transitions leading to time-dependent flow solutions such as standing waves with periodic or quasiperiodic oscillations and turbulence. Surprisingly, we find that turbulence can occur for Reynolds numbers at least one order of magnitude smaller than those required for turbulence to arise in conventional fluids. The occurrence of turbulence is ascertained by carrying out a detailed investigation of the transitions between flow states and by examining the characteristics of the physical quantities such as the energy, the wave number and the angular momentum. We also find that, for the Taylor-Couette ferrofluidic flow, the onset of turbulence can be determined accurately, in contrast to classical fluid turbulence where such a determination is typically qualitative and involves a high degree of uncertainty2. Our findings have the following implications:
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Revisiting and exploring the field of turbulence in ferrofluids can be rewarding, which has become feasible due to progress in computational fluid dynamics.
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In Taylor-Couette ferrofluidic flow the critical magnetic field strength for the onset of turbulence can be pinned down precisely, potentially leading to deeper insights into the physical and dynamical origins of the transition.
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Turbulence in Taylor-Couette ferrofluidic flows can be controlled via an external magnetic field.
In spite of the appealing features of ferrofluid flows, from the experimental point of view there are disadvantages to investigate turbulence in ferrofluids. For example, these fluids are opaque, rendering inapplicable standard methods of laser Doppler anemometry. It is necessary to employ ultrasonic Doppler velocimetry, but this requires rather bulky probes40. In addition, one needs tracer particles in the micrometer regime, which unavoidably create magnetic holes. The holes carry induced dipole moments that self-assemble to chains in direction of the applied magnetic field. The chains may dramatically change the properties of the flow. Such difficulties must be overcome in order to fully exploit ferrofluid for turbulence research.
Results
Ferrohydrodynamical equation of motion
Consider a Taylor-Couette system consisting of two concentric, independently rotating cylinders with an incompressible, isothermal, homogeneous, mono-dispersed ferrofluid of kinematic viscosity ν and density ρ within the annular gap. The inner and outer cylinders of radii R1 and R2 rotate at the angular speeds ω1 and ω2, respectively. The top and bottom end-walls41 are stationary and are at distance Γ(R2 − R1) apart, where Γ is the non-dimensionalized aspect ratio. The system can be described in the cylindrical coordinate system (r, θ, z) by the velocity field (ur, uθ, uz) and the corresponding vorticity ∇ ×u = (ξ, η, ζ). We set the radius ratio of the cylinders and the parameter Γ to typical values in experiments, e.g., R1/R2 = 0.5 and Γ = 20. A homogeneous magnetic field of strength Hx is applied in the transverse x-direction (x = r cosθ). The gap width d = R2 − R1 can be chosen as the length scale and the diffusion time d2/ν serves as the time scale. The pressure can be normalized by ρν2/d2 and the magnetic field H and the magnetization M by where μ0 is the magnetic permeability of free space. We then obtain the following non-dimensionalized equations governing the flow dynamics25,42:
The boundary conditions on the cylinders are u(r1, θ, z) = (0, Re1, 0) and u(r2, θ, z) = (0, Re2, 0), where the inner and outer Reynolds numbers are Re1 = ω1r1d/ν and Re2 = ω2r2d/ν, respectively and r1 = R1/(R2 − R1) and r2 = R2/(R2 − R1) are the non-dimensionalized inner and outer cylinder radii, respectively. To be concrete, we fix the Reynolds numbers at Re1 = 100 and Re2 = −150 so that the rotation ratio β = Re2/Re1 of the cylinders is −3/2.
We need to solve Eq. (1) together with an equation that describes the magnetization of the ferrofluid. Using the equilibrium magnetization of an unperturbed state where homogeneously magnetized ferrofluid is at rest and the mean magnetic moment is orientated in the direction of the magnetic field, we obtain Meq = χH. The magnetic susceptibility χ of the ferrofluid can be approximated by using the Langevin’s formula43, where we set the initial value of χ to be 0.9 and use a linear magnetization law. The ferrofluid studied corresponds to APG93344. The near equilibrium approximations of Niklas37,45 are small ||M − Meq|| and small magnetic relaxation time τ: Using these approximations, one can obtain25 the following equation:
where
is the Niklas coefficient37, μ is the dynamic viscosity, μ0 is the vacuum permeability, Φ is the volume fraction of the magnetic material, is the symmetric component of the velocity gradient tensor and λ2 is the material-dependent transport coefficient42. We choose λ2 = 2, which corresponds to strong particle-particle interaction and chain formation of the ferrofluid42.
Using Eq. (2), we can eliminate the magnetization from Eq. (1) to obtain the following ferrohydrodynamical equation of motion25,42:
where F = (∇ × u/2) × H and pM is the dynamic pressure incorporating all magnetic terms that can be expressed as gradients. To the leading order, the internal magnetic field in the ferrofluid can be approximated as being equal to the externally imposed field24, which is reasonable for obtaining dynamical solutions of the magnetically driven fluid motion. Equation (4) can then be simplified as
This way, the effect of the magnetic field and the magnetic properties of the ferrofluid on the velocity field can be characterized by a single parameter, the magnetic field or the Niklas parameter37,
Transition to turbulence in ferrofluids
We first present a sequence of transitions with the magnetic parameter sx, eventually leading to turbulence. For , the rotating ferrofluid flow is intrinsically three-dimensional22,23,24,25 with increased complexity as sx is increased from zero. Fig. 1(a–c) show, respectively, three key quantities versus sx: the time-averaged modal kinetic energy defined as
its m = 2 contribution and the spatiotemporally averaged axial flow field at midgap for θ = 0 (along the directions of the magnetic field) and θ = π/2 (perpendicular to the field). We see that, for sx < 0.784, the flow is time-independent. In particular, for , the flow patterns show wavy vortices with a two-fold symmetry22, denoted as WVF(2), which appears in Fig. 2(a) as a “two-belly” structure. As sx is increased through , this symmetry is broken and a somewhat tilting pattern in the wavy-vortex structure emerges [denoted as WVF(2)t], as shown in Fig. 2(b). The intuitive reason is that the magnetic force is downward for fluid flow near the annulus and upward where the flow exits, resulting in a split in for θ = 0 and π/2. As sx is increased through the critical point , the flow becomes time-dependent. For , the flow is time periodic (limit cycle), corresponding to standing waves with axial oscillations of characteristic frequency ω1, which is denoted as SWOp. Near the onset of SWOp, the average kinetic energy values and are unaffected, as can be seen from Fig. 1(a,b), respectively. For , the periodic solution becomes unstable due to the emergence of a second incommensurate frequency ω2 (≈ω1/5) associated with defect propagation through the annulus in the axial direction, leading to transition to quasiperiodic flow (denoted as SWOqp). [See movie files movie1.avi, movie2.avi, movie3.avi and movie4.avi in Supplementary Materials (SMs), where the additional frequency can be identified visually in the defect starting from the top of the oscillating region, propagating downward toward the bottom and vanishing there.] While continues to decrease through this transition, both and reach their respective maxima at the transition point. As sx is increased further, the flow becomes more complex. Onset of turbulence occurs for , where globally the flow starts to rotate in the azimuthal direction, as shown in Fig. 2(d) (see also movies movie5.avi, movie6.avi and movie7.avi in SMs). The observed route to turbulence coincides completely with that established previously1,46 for conventional fluid at high Reynolds numbers.
Wave structure of the flows
We next analyze the wave structure of the flows to probe into the transition to turbulence in the low Reynolds-number regime. To get numerical solutions of the ferrohydrodynamical system, we solve the ferrohydrodynamical system by combining a finite-difference, time-explicit method of second order in (r, z) with Fourier spectral decomposition in θ (See Methods). The variables can be written as
where f denotes any one of {ur, uθ, uz, p}. We then perform an axial Fourier analysis22 of the mode amplitudes of the radial velocity field (ur)m(z,t) at midgap to obtain the behavior of the wave number k, as shown in Fig. 3. Prior to the onset of turbulence, the number of vortices in the bulk fluid is invariant, irrespective of whether the flow is time-independent or time-dependent. However, due to the symmetry breaking induced by the magnetic field, the spatial structures of the flows can differ significantly. The top panel of Fig. 3 shows that the axial wave number k begins to split into two branches at , where k is enhanced and reduced as the field enters into and exits perpendicularly from the annulus, respectively and there are dramatic changes in the flow profiles in which the dynamics tend to focus on the θ ≈ 0 region. As sx is increased further, k in the bulk decreases with nearly constant difference between the cases of θ = 0 and θ = π/2. However, the kinetic energies and the axial wave numbers are nearly unaffected when the flow becomes time-dependent as sx is increased through . As the quasiperiodic regime is reached, the energies and the axial wave numbers begin to change where, as shown in Fig. 3, the wave numbers for θ = 0 and θ = π/2 are minimized at sx about 0.8. For both the periodic and quasiperiodic regimes, there is little variation in k and only the vortex pair surrounding the oscillatory region expands and shrinks periodically. Especially, in the periodic regime the flow profile at θ = π/2 exhibits little dependence on sx except for an increasing amplitude, but in the quasiperiodic regime the flow shows a strong dependence on sx, due to the emergence of the second frequency. As is passed, the flow starts to rotate and the split in the axial wave numbers in the directions parallel and perpendicular to the magnetic field vanishes. In fact, as turbulence sets in no distinct wave numbers can be identified, as shown in Figs. 2 and 3(e) (see also movie file movie7.avi in SMs).
Behavior of the angular momentum
We now examine the angular momentum in relation to transition to turbulence. Figure 4 shows, for flows in the periodic regime, the isosurfaces of differences in the angular momentum ruθ between the full flow and its long-time averaged value, namely, . Onset of the periodic regime can be identified by the occurrence of periodic oscillations (up and down) of a single outward directed jet of angular momentum ruθ (see movie files movie2.avi and movie1.avi in SMs). From Fig. 4, we see that, while the full flow pattern in the periodic regime exhibits little variation (see movie files movie10.avi and movie11.avi in SMs), there is relatively large variation in the behavior of the angular momentum (see movie12.avi in SMs). For example, there is a downward flow from θ = 0 and an upperward flow from θ = π, with opposite angular-momentum values. In the middle of the system where the effects of the Ekman boundary layers are minimal, the difference in the angular momentum reaches maximum. As the system enters into the quasiperiodic regime, the appearance of the incommensurate frequency ω2 signifies a kind of defects in the propagation pattern of the flow. As the flow begins to rotate in the azimuthal direction, turbulence sets in.
Low Reynolds number turbulence
A challenging issue in the study of turbulence is precise determination of its onset as a system parameter, e.g., the Reynolds number, is changed. For the type of low-Reynolds number turbulence in ferrofluid uncovered in this paper, this can actually be achieved. In particular, the transition to turbulence coincides with the onset of the azimuthal rotation from the quasiperiodic flow. To illustrate this, we consider the cross-flow energy Ecf(r, t), a commonly used indicator for onset of turbulence in the Taylor-Couette system47, which is the instantaneous energy associated with the transverse velocity component at radial distance r. Small (large) values of Ecf indicate laminar (turbulent) flows. We find that, the maximum value of Ecf(r, t), denoted by , assumes near zero values for but it increases dramatically as sx is increased through , as shown in Fig. 5(a). In this figure we also plot the scaled maximum cross-flow energy value, , versus sx and we observe that and exhibit essentially the same behavior as the system passes through the onset of turbulence. Examples of the spatiotemporal evolution of Ecf(r,t) are shown in Fig. 5(b–d) for periodic, quasiperiodic and turbulent regimes, respectively. We observe regular patterns in the former two regimes, but no apparent patterns in the turbulent regime.
Conclusions
We investigate the route to turbulence in the Taylor-Couette ferrofluid flow driven by a magnetic field transverse to the symmetric axis of the system. We find that the ferrofluidic flow can exhibit axial oscillations but not rotations in the azimuthal direction in the parameter regime where regular dynamics arise and turbulence can occur generically for low values of Reynolds number. We elucidate the bifurcation sequence prior to onset of turbulence in detail. For this we considered either global and local quantities as exemplary presented in Figs. 6 and 7. For fixed (low) Reynolds number and small values of the magnetic parameter, the system exhibits a stationary fixed point. As the parameter is increased, the fixed point loses stability through a supercritical Hopf bifurcation, giving rise to a periodic limit cycle that becomes unstable through another Hopf bifurcation. At this bifurcation, a second incommensurate frequency emerges, leading to a quasiperiodic solution. As the magnetic parameter is increased further, there is a transition directly from quasiperiodic motion to turbulence. We find that turbulence can generically arise for low values of the Reynolds number. This is substantiated by extensive computations of the underlying ferrohydrodynamical equation through a detailed investigation of transitions in the flow structure by using a number of physical quantities. An implication lies in the perspective of controlled generation of turbulence through variations of the external magnetic field, making it possible to locate the onset of turbulence with high precision.
We expect our findings to have values for experimental as well as theoretical investigation of turbulence. To substantiate this, we discuss the effect of different ferrofluid types and provide an estimate of the critical magnetic field strength required for onset of turbulence. The range of the magnetic parameter considered in this paper, i.e., 0 < sx < 0.9, can in fact be realized in experimental studies of ferrofluids. Our computationally determined value of turbulence onset is , which corresponds to the magnetic field strength of about H = 76.6 [kA/m] [see Fig. 8 in Methods, sx(H) as function of the magnetic field H.] In our simulations we use the typical setting of counter-rotating cylinders with Reynolds number Re1 = 100 and Re2 = −150. The corresponding frequencies depend on the system setup and can be calculated from the given system parameters. In fact, the relation demonstrated in Fig. 8 depends on the ferrofluid type. In our simulations we use APG933, a type of magnetite based ferrofluid. For different ferrofluids, for example Cobalt based ferrofluids23, the effects due to magnetic fields can be “stronger,” meaning that similar dynamical behaviors can occur but for weaker magnetic fields. Indeed, for a Cobalt base ferrofluid, the corresponding curve (to that in Fig. 8) is much steeper. For ferrofluid APG933 studied in this paper, we expect onset of turbulence to occur in Taylor-Couette flow systems for critical magnetic strength less than about 80 kA/m, which can be realized in experiments.
Methods
Numerical scheme for ferrodynamical equation
System (4) can be solved22,24,25 by combining a second-order finite-difference scheme in (r,z) with Fourier spectral decomposition in θ and (explicit) time splitting. The variables can be written as
where f denotes one of {ur, uθ, uz, p}. For the parameter regimes considered in our preliminary study, the choice mmax = 10 provides adequate accuracy. We use uniform grids with spacing δr = δz = 0.05 and time-steps δt < 1/3800. For diagnostic purposes, we also evaluate the complex mode amplitudes fm,n(r, t) obtained from the Fourier decomposition in the axial direction , where k is the axial wavenumber.
Detailed illustration of transitions prior to onset of turbulence
A method to ascertain the occurrence of turbulence is through examination of the sequence of transitions preceding the turbulence onset. The seminal work of Gollub and Swinney established that turbulence can arise directly from a quasiperiodic state1. Typical time series and power spectral densities from a detailed study of the type of flow states preceding turbulence onset are shown in Fig. 6, which is in complete agreement with the results in Ref. 1. The representative phase portraits for the periodic and quasiperiodic states are shown in Fig. 7.
Relation between Niklas parameter sx(H) and the magnetic field strength H
Figure 8 shows, for ferrofluid APG933, the relation between sx(H) and H. From our numerically determined critical sx value for onset of turbulence, we can determine the critical value of H using this relation.
Additional Information
How to cite this article: Altmeyer, S. et al. Transition to turbulence in Taylor-Couette ferrofluidic flow. Sci. Rep. 5, 10781; doi: 10.1038/srep10781 (2015).
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Acknowledgements
Y.D. was supported by Basic Science Research Program of the Ministry of Education, Science and Technology under Grant No. NRF-2013R1A1A2010067. Y.C.L. was supported by AFOSR under Grant No. FA9550-12-1-0095.
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S.A., Y.D. and Y.C.L. devised the research project. S.A. performed numerical simulations. S.A., Y.D. and Y.C.L. analyzed the results. S.A., Y.D. and Y.C.L. wrote the paper.
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Altmeyer, S., Do, Y. & Lai, YC. Transition to turbulence in Taylor-Couette ferrofluidic flow. Sci Rep 5, 10781 (2015). https://doi.org/10.1038/srep10781
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DOI: https://doi.org/10.1038/srep10781
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