Abstract
We investigate, experimentally and theoretically, polarization rotation effects in dilute photonic crystals with transverse permittivity inhomogeneity perpendicular to the traveling direction of waves. A capsize, namely a drastic change of polarization to the perpendicular direction is observed in a one-dimensional photonic crystal in the frequency range 10 ÷ 140 GHz. To gain more insights into the rotational mechanism, we have developed a theoretical model of dilute photonic crystal, based on Maxwell’s equations with a spatially dependent two dimensional inhomogeneous dielectric permittivity. We show that the polarization’s rotation can be explained by an optical splitting parameter appearing naturally in Maxwell’s equations for magnetic or electric fields components. This parameter is an optical analogous of Rashba like spin-orbit interaction parameter present in quantum waves, introduces a correction to the band structure of the two-dimensional Bloch states, creates the dynamical phase shift between the waves propagating in the orthogonal directions and finally leads to capsizing of the initial polarization. Excellent agreement between theory and experiment is found.
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Introduction
The problem of the polarization rotation (PR) of an incident electromagnetic wave is one of the most interesting in photonic crystals (PC)1. The investigations in this field are stimulated by the possibility of creation of polarization controlling devices, where the polarization of the propagating light could be precisely manipulated and controlled2,3,4. One of the mechanism that can account for this PR can be associated with the geometrical anisotropy of photonic crystal (PC)5. The anisotropy, imposing asymmetry into a periodic two dimensional (2d) structure in xy–plane, leads to a different speed in the x–and y–axes resulting in a phase delay between H x (E x ) and H y (E y ) components. Another mechanism that can lead to the PR of propagating light is due to dielectric permittivity inhomogeneity of medium. This phenomenon known long ago6,7,8,9,10 and accepted view of the physics behind the effect is that the rotation is controlled by the parameter λ/Λ0 (λ is the wave length and Λ0 is the typical length scale of the system’s inhomogeneity). In the geometrical optics approximation when wavelength is much smaller than inhomogeneity characteristic scale, rotation angle is negligible11. However, in the opposite limit, the rotation of polarization due to dielectric permittivity inhomogeneity, is quite significant. Particularly, such effects are observed both in dielectric (see ref.12 and references therein) and metallic13 PCs.
In this paper we investigate, experimentally and theoretically, the PR effects in a dilute photonic crystals (DPC) with transverse permittivity inhomogeneity perpendicular to the z–traveling direction of waves. Interest to DPC is largely motivated by a peculiar behavior of the transmission coefficient, recently studied in ref.14. Using parabolic (forward) scattering approximation to investigate electromagnetic wave propagation in inhomogeneous media15,16,17, in ref.14 was found an independence of the transmission coefficient of the central diffracted wave from the incident wavelength in a dilute perforated metal system. As we will see below, it turns out that the DPC along with the interesting transport properties lead to unusual polarization effects as well.
Our direct measurements indicate that under certain conditions the initial polarization changes its direction by π/4 in 1d DPCs in the frequency range of 10 ÷ 140 GHz (see below). The main experimental finding consists of not typical shift of distribution’s minimum and maximum regions in the spectra of the transmitted intensity (see below). To understand and explain the rotating mechanism of the DPC, we have developed a theoretical model, based on Maxwell’s equations with a spatially dependent two dimensional dielectric permittivity ε(x, y). Using the same parabolic approximation, mentioned above, we show that the polarization’s rotation in 1d and 2d DPCs can be explained by an optical splitting parameter appearing naturally in Maxwell’s equations for magnetic or electric fields components. This term is an optical analogous of Rashba type spin-orbit interaction parameter, introduces a correction to the band structure of the two-dimensional Bloch states, creates the dynamical phase shift between the waves propagating in the orthogonal directions and finally leads to capsizing of the initial polarization. A photonic analog of Rashba type term in homogeneous chiral medium was considered in18.
Note that one should differ polarization rotation due to inhomogeneity and chirality or magnetoactivity of the medium. In the last two cases the dielectric permittivity tensor has non-diagonal terms in contrary to the former case. Non-diagonal terms lead to different velocities of left hand and right hand circular polarized waves in a chiral or magnetoactive medium. In PC situation is different. Here two waves polarized in orthogonal directions have different velocities. This difference leads to polarization rotation because every linearly polarized wave can be presented as a superposition of waves in two orthogonal directions. The possibility of large polarization rotation by PC was noticed in19.
Experiment
To study capsize effect in 1d PC system, we have performed an experiment where electromagnetic waves propagate through the dilute structure. The schematic setup of the experiment is shown in Fig. 1. It consists of transmitter and receiver antennas, an anechoic chamber with photonic crystal, scalar network analyzer and recorder. One-dimensional photonic crystal is formed from 7 alumina ceramic plates with permittivity ε = 10, thickness b = 0.5 mm and sizes 60 × 96 mm2. They are parallel substituted along the x–axis at the distance a = 10 mm from each other. The structure is supported by the low loss and low dielectric permittivity ε = 1.07 foam layers, see Fig. 2.
The measurements were carried out in the frequency range 10 ÷ 140 GHz (wavenumber k 0 = 0.21 ÷ 2.93 mm−1) using set of scalar network analyzers. Open end rectangular waveguides of corresponding frequency range are used as a transmitting and receiving antennas. Such a choice of antennas allow high level cross-polarization isolation smaller than 10−3 in their mutual orthogonal location. The PC and the receiving antenna can be rotated in the xy–plane, where the electric field vector E(H) is located. We remind that the wave incidence direction is z–axis and plates are located in the yz-plane. The PC and the antennas were placed in an anechoic chamber to avoid the influence of unwanted external signals. The distances between them were chosen large enough that far field approximation is applicable. The frequency dependence of transmission coefficient was displayed on the recorder. The results of experiment with one dimensional photonic crystal are presented in Fig. 3. In the upper panel (black line) the frequency dependence of transmission coefficient I (normalized intensity) is shown provided that wave’s incidence direction (x–axis) is perpendicular to the plates. Due to the periodicity in x–direction we expect to have frequency bands over which the propagation of the waves is forbidden, that is the transmission coefficient becomes zero. The panel indicates that at wave numbers above 0.48 mm−1 the forbidden band begins to form. In the middle and lower panels (red and blue lines, respectively) the wave incidence direction is z–axis, as discussed below. However, the plots differ from each other by the direction of receiving antenna: in the middle panel it is orthogonal to transmitter antenna (y–axis) and in the lower panel it is parallel to transmitter, that is directed in x–axis. The maxima in the middle panel corresponds to the resonance wavelengths v 1d L = π/2 + πn (see theory below) for which polarization change the direction from π/4 (initial linear polarization angle) to π/2. In the lower panel (blue line) for the same wavelengths one has minimums instead of maximums. This shift of the intensity distribution is due to the change of receiver’s direction: the latter now is pointed out on x–direction, that is parallel to the transmitter polarization. To verify the preceding discussion on the PR in 1d PC around resonance wavelengths v 1d L = π/2 + πn, one needs to evaluate v 1d . Using equation (22) we have calculated v 1d (k 0) for the resonant wavelength k 0 = 0.49 mm−1 and for cos v 1d (k 0 = 0.49)L we get −0.008 (L = 96 mm) which is very close to 0, as was predicted. Note the logarithmic scale used in the experimental plot Fig. 3. This means that the capsize phenomena takes place with very high accuracy 10−3.
As we mentioned above, at θ 0 = π/4 and for resonant frequencies v 1d L = π/2 + πn, the transmitted wave is linearly polarized but directed on y–axis. This means that the theoretical imaginary part of rotation angle that describes the ellipticity (ratio of ellipse axes) should become infinite. However, in general, for arbitrary θ 0 there is a finite ellipticity and the imaginary portion Imθ(L) is also finite. In Fig. 4 we compare experimentally measured ellipticity at resonance wavenumber k 0 = 0.49 mm−1 (red line) with the theoretical ellipticity (blue line) (see below, equation (24)).
Theory
In achieving a better understanding of the experimentally observed capsize effect, discussed in the previous section, we develop an analytical approach that predicts the capsize of polarization in 1d and 2d DPCs.
Let us consider a dielectric medium with periodic array of two dimensional holes. The inhomogeneity of the medium in xy–plain will be taken into account through a spatially dependent two dimensional dielectric permittivity ε(x, y). Suppose a plane wave enters the medium from the z < 0 half-space at normal incidence. Using Maxwell equations one can obtain a wave equation for H in the form
where k 0 = ω/c is the wave number corresponding to the angular frequency ω of the incident wave. The last term in l.h.s. of equation (1) accounts for the contribution of the dielectric permittivity inhomogeneity and, as we will see below, introduces a correction to the band structure of the two-dimensional Bloch states. This correction creates the dynamical phase shift between the waves propagating in the orthogonal directions in the xy–plain and finally leads to capsizing of the initial polarization of H.
Before proceeding further, we would like to mention that similarly to equation (1) for H, one can write a wave equation for the electric field E. However, the wave equation for E will contain en extra term \({\bf{E}}\nabla (\nabla \varepsilon /\varepsilon )\) that does not affect the initial polarization. For this reason and for simplicity in what follows, we study only the peculiar rotation of the H in xy–plain caused for the dielectric permittivity inhomogeneity.
Following refs14,15,16,17, we seek the solution for the propagation in the system wave as a product of a fast and a slowly varying, \(\tilde{{\bf{H}}}({\bf{x}},{\bf{y}},{\bf{z}})\), function on a wave incident z–direction
Substituting equation (2) into equation (1) and neglecting the second derivative of \(\tilde{H}\) with respect to z one gets in the parabolic equation approximation
where \(\tilde{{\bf{H}}}\equiv (\begin{array}{c}{\tilde{H}}_{x}\\ {\tilde{H}}_{y}\end{array})\) is a spinor and \(\hat{H}={\hat{H}}_{0}+\hat{V}\) is a 2 × 2 matrix.
The explicit form of \({\hat{H}}_{0}\) is
where \({\nabla }_{\perp }^{2}\equiv {\partial }^{2}/\partial {x}^{2}+{\partial }^{2}/\partial {y}^{2}\) and the inhomogeneity term is given by
Let us stress that ignoring the second derivative of \(\tilde{H}\) with respect to z in equation (3) is justified by the fact that in a dilute system with a small fraction of dielectric (or metal) the light propagates in z–direction mostly forwardly, without back scattering.
So the problem of propagation of electromagnetic waves in a dilute dielectric medium with periodic array of two dimensional holes is reduced to a quantum motion of a particle with mass k 0 in a 2d periodic potential \(V(x,y)=\frac{{k}_{0}}{2}(1-\varepsilon (x,y))\) with inhomogeneity term \(\hat{V}\), where spatial coordinate z plays the role of time in a Schrödinger-like equation. In this approach, if the initial parameters at z = 0 are known (for example the incoming wave front), then one can find them at z > 0. Such a mapping has been performed previously14,17 and made it possible to study the propagation of light through a semi-infinite medium with transverse disorder17 and through a dilute metal with two-dimensional hole arrays14.
It can furthermore be shown that if one associates \({\tilde{H}}_{x,y}\) components with spin components then the term \(\hat{V}\) reminds Rashba spin-orbit interaction (see for a review ref.20, for photon spin-orbit interaction21 and the review22). The remarkable similarity between \(\hat{V}\), equation (5), and a Rashba spin-orbital interaction term allow us to stress that both are closely related phenomena. The term \(\hat{V}\) will introduce a correction to the band structure of the two-dimensional Bloch states, creates the dynamical phase shift between the waves propagating in the x– and y–directions and finally leads to rotation of the initial polarization. Hence, the calculation of the spectrum of Hamiltonian \(\hat{H}(x,y)={\hat{H}}_{0}+\hat{V}\) could provide a sensitive means to analyze polarization effects in dilute photonic crystal and may be used as a starting point to evaluate the wave transmission coefficient at z–direction.
To find the band structure let us represent the solution of equation (3) through the eigenfunctions of the Hamiltonian equations (4) and (5),
and
Finally, substitution of equation (6) into equation (2) yields the solution of Maxwell equation
which can serve as a basis for qualitative understanding of spectral properties of dilute systems. Such an approach allows one to pinpoint the specific details and provide information about the energy band structure.
To close this section let us note that if the dielectric permittivity ε(x, y) is a periodical function, then the spectrum of the Hamiltonian (4) consists of allowed and forbidden energy bands, if the term \(\hat{V}\) is zero. If \(\hat{V}\ne 0\) then the electronic energy bands are split by \(\hat{V}\) and as a consequence the polarization of the propagated light is rotated.
Spectrum of photonic crystal
Before discussing the physics induced by \(\hat{V}\) coupling let us consider \(\hat{V}=0\). For this case the quantum-mechanical problem is reduced to the well-known Kronig-Penney (KP) model due to the fact that the periodic ε(x, y) spectrum of Hamiltonian consists of energy bands separated by gaps and wave functions described by Bloch states. In this section we will investigate band structure for symmetric KP model in one and two dimensional systems for quasimomentum q = 0, that is at the center of Brillouin zone. Note that only these states give contribution to the transmitted light intensity in the normal direction14.
We first discuss a two-dimensional symmetric KP model where the dielectric function has the form
The Bloch state wave function \(u(x,y)\equiv {u}_{q=0}(x,y)\) obeys the Schrödinger equation
and energy E 0 ≡ E (q = 0) (for q = 0 state) is determined from the similar to the one dimensional Kronig-Penney dispersion relation
Putting all of this information together one can, at least numerically, evaluate not only the energy E 0, using equation (11), but also calculate the intensity of central diffracted wave in 2d system in terms of dielectric (metal) fraction.
As for the 1d PC case (dielectric permittivity ε(x) periodically depends only one coordinate) it can be obtained from above formulas by the following substitutions (assuming that \(y\equiv 0\)): \(\beta =\sqrt{2{k}_{0}{E}_{0}}\) and \(\alpha =\sqrt{2{k}_{0}({V}_{d}+{E}_{0})}\). We have presented the photonic band structure of transversal motion for the 1d crystal used in our experiment in Fig. 5.
The border value \({E}_{0}\equiv E(q=\mathrm{0)}=0.401 < {k}_{0}\) is the transversal wavenumber. The incident wavenumber k 0 lies in the forbidden band. After a brief sketch of the steps of calculating of spectrum of periodic PC in 1d and 2d systems we start a detailed discussion of the interaction \(\hat{V}\) role in a PR. We will see below that in some cases the interaction term \(\hat{V}\) plays a central role of the capsizing of initial polarization.
Polarization rotation
Two dimensional photonic crystal
As mentioned above the interaction \(\hat{V}\) splits E 0 into two energy levels. To find energy splitting in the mean field approximation in a 2d case, we substitute the operator \(\hat{V}\) by its expectation value and diagonalize 2 × 2 matrix Hamiltonian
where
Note that for the symmetrical Kronig-Penney model all the integrals in \(\hat{V}\) are equal to v 2d . Direct calculation of the integral (13) yields
where A 2, as was mentioned, is the normalization parameter with dimensionality a −1 (a is the period of the system).
For the magnetic field of central diffracted wave we get
One can interpret this result as an PR due to the interaction term \(\hat{V}\) or Rashba splitting parameter v. The latter, imposing asymmetry into a periodic 2d structure in xy–plane, leads to a different speed in the x and y axes resulting in a phase delay between H x and H y components.
Introducing parameter c = c 1/c 2, the PR angle at z = L can be written in the form
provided that an initial polarization angle θ 0 at L = 0 is given by
By applying equation (17) and calculating the real part of rotation angle θ from equation (16) one obtain (\({E}_{1}-{E}_{2}\equiv 2{v}_{2d}\))
where the principal interval of the arccotangent function is chosen 0 ≤ arccot x < π to avoid discontinuity at x = 0.
The above expression Reθ(L) is a general expression for PR angle and valid for dilute photonic crystal with inhomogeneity in the plane perpendicular to the propagation direction. The value of Reθ(L) strongly depends on the frequency of the electromagnetic wave, traveling distance L and on the initial polarization angle θ 0.
Some obvious results that follow from equation (18) above. It is clear, that for the particular values v 2d L = πn (n = 0, 1, …) the Reθ(L) = θ 0. In the limit \(2{v}_{2d}L\ll 1\) the Re θ(L) ≈ θ 0 and completely independent of a particular value of θ 0. Next, if the initial angle θ 0 → π/4 (\(c\gg 1\)- maximum difference between two orthogonally polarized eigenmodes of polarization) the Reθ(L) → π/4 for all L. This means that the initial wave polarization at π/4 does not change when crossing the medium and becomes independent of the traveling distance.
However, a significant rotation of Reθ(L) from the initial value θ 0 occurs when cos 2vL being positive changes the sign. In fact, if cot 2θ 0 → ∞, then the Reθ(L) asymptotically tends to zero, if cos 2v 2d L > 0 and tends to π/2 if cos 2v 2d L < 0. Hence, for the particular value of θ 0 = 0 (or c = 1), the jump from 0 to π/2 of the Reθ(L) occurs at v 2d L = π/4. This quite drastic change of the initial polarization can be completely controlled having the appropriate parameters L and frequency-dependent v (see Fig. 2). In a special case of cos 2v 2d L = −1 the θ(L) = π/2 − θ(L = 0) and we recover the result of ref.12.
Note that capsize effect takes place for all values of 2vL in the range [π/2, 3π/2] including the value 2vL = π, considered in ref.12. When vL = π/4, as we mentioned, Reθ(L) = π/4 and independent of the initial polarization, beside θ 0 = 0.
As another manifestation of the drastic change of the polarization, one can study the behavior of the imaginary portion of the θ(L = 0) (the ellipticity or the ratio of ellipse axes) at resonant frequencies cos 2v 2d (k 0)L = 0. The latter can be written in the compact form, based on Eqs (16) and (17)
This expression provides useful information about the ratio of ellipse axes (within the sign accuracy) near the particular angle θ 0 ≈ 0. Exactly at θ 0 = 0 the imaginary portion, Imθ(L), tends to infinity. This means that light remains linearly polarized after traveling distance L while the polarization direction rotates by π/2.
One dimensional photonic crystal
Knowing the explicit form of the inhomogeneity term (5) it is not difficult to calculate the splitting interaction \(\hat{V}\) in the 1d case
The splitting parameter v 1d reads
where ε(x) = 1 + (ε − 1) Θ (x − (a − b)) is the 1d periodic dielectric constant in a unit cell [0, a]. Evaluating this integral, we find
where A 1d is the normalization parameter with dimensionality a −1/2. Comparing splitting parameters in 2d, equation (14), and 1d, equation (22), one can see that the 2d splitting parameter consists of an additional \(b/a\ll 1\) multiplier. As a consequence, the small v 2d in dilute photonic crystals leads to a large optical path difference between the two polarizations and make difficult to observe experimentally a capsize in 2d dilute crystals. This statement was supported by our numerical calculations of the splitting parameters v 1d and v 2d versus k 0 using the structural parameters of the photonic crystal, used in experimental purposes. Indeed, as seen from Fig. 6, for b = 0.5 mm, a = 10 mm, and ε = 10 there is a large factor in between v 1d and v 2d parameters. As we will see below, due to the small value of v 2d in the frequencies range of our set up, we were not able clearly see the capsize in 2d case. However, in 1d case the capsize takes place precisely at the resonance frequencies, predicted by theory.
In a similar fashion, demonstrated in the previous section, while calculating the real part of rotation angle Reθ(L) (see equation 18), one can find PR angle for 1d case
The only difference between the two equations (18) and (23) (without taking into account the factor 2) is that the cos v 1d L in 1d case appears in the denominator. A direct consequence of this flip is that the drastic change of the polarization now takes place at v 1d L = π/2 + πn, n = 0, ±1, …. In this case Reθ(L) = 0 if 0 < θ 0 < π/4 and Reθ(L) = π/2 if π/4 < θ 0 < π/2. So for the resonant frequencies cos v 1d (k 0)L = 0, Reθ(L) acquires only two values 0 and π/2 depending on initial polarization angle θ 0. Capsize takes place exactly at θ 0 = π/4.
As for the imaginary part of rotation angle that describes the ellipticity of transmitted wave at resonance frequencies cos v 1d (k 0)L = 0 one can write
The infinity value of imaginary part at θ 0 = π/4 is an clear evidence of a linear polarization and a change of an initial polarization to π/2.
Conclusions
We have carried out an experimental and theoretical investigation on the PR effects in dilute photonic crystals with transverse permittivity inhomogeneity perpendicular to the traveling direction of waves. For 1d DPC the reported experimental data show that at θ 0 = π/4 occurs capsize of an initial direction in the frequency range 10 ÷ 140 GHz. At the resonant frequencies v 1d (k 0)L = π/2 + πn the initial direction rotates by π/4 and coincides with π/2, in full agreement with the theoretical result (see equation (23)). In order to understand the capsize effect in 1d and 2d DPC a theoretical model, based on Maxwell’s equations with a spatially dependent 2d inhomogeneous dielectric permittivity ε(x, y), have been developed.
For one and two dimensional dilute photonic crystals we have calculated the real and imaginary parts of rotation angle. According to our calculations a capsize of initial polarization take place at resonance frequencies v 1d L = π/2 + πn and v 2d L = π/4 + πn, in 1d and 2d, respectively. In the 1d case the jump of real part of rotation angle to π/2 occurs at θ 0 = π/4 (in full agreement to our experimental data, see Fig. 3), while in 2d crystals it happens at θ 0 = 0. In order to give a more complete analysis of the capsize effect in these systems, we have also demonstrated that at the mentioned resonance frequencies and initial angles, the imaginary parts of the rotation angle tends to infinity. This reflect the fact that in both cases waves remains linearly polarized after traveling distance L while the polarization direction rotates by π/2 and π/4 in 2d and 1d cases, respectively. The main contribution to the transmission coefficient of central diffracted wave is connected with 2d extended states that are close to the center q = 0 of the 2d Brillouin zone. This means that in order to observe the above mentioned peculiarities in periodical systems, it is enough that the system exhibits long or quasi-long-range structural order in xy–plain14.
We have considered polarization rotation effects in dielectric DPC. However the same effects take place in metallic DPC. The only difference is the specific form of splitting parameter v which should be calculated using Bloch wave functions for metallic case14. Note that optical activity in the form of circular dichroism was earlier considered in the 2D array of metallic spheres23.
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Acknowledgements
Zh.G. is grateful to A. Hakobian for his technical help and to E. Yuzbashyan and T. Shahbazyan for helpful discussions. E.C. and V.G. thank partial financial support by the Murcia Regional Agency of Science and Technology (project 19907/GERM/15). V.G. acknowledges the kind hospitality extended to him at Murcia University during his sabbatical leave.
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A.H. conducted the experiment, Zh.G. and V.G. develope the theory, E.C. carry out the numerical calculations. All the authors review the manuscript.
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Gevorkian, Z., Hakhoumian, A., Gasparian, V. et al. Capsize of polarization in dilute photonic crystals. Sci Rep 7, 16593 (2017). https://doi.org/10.1038/s41598-017-16847-8
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DOI: https://doi.org/10.1038/s41598-017-16847-8
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