Abstract
Harvesting energy from the ambient is a promising approach to fulfil decentralized energy demands and facilitate the transition to low-carbon economy. Moisture-sorption-based energy harvesting (MSEH) is a promising strategy for obtaining heat, cold and electricity from ubiquitous moisture anywhere and anytime. Advances in water-sorption materials have promoted the development of sustainable moisture energy. However, MSEH technology faces the challenges of low-energy productivity and limited recognition of its working mechanisms and thermodynamic analysis. We centre this Perspective article around an in-depth understanding of the underlying mechanisms and thermodynamic limitations of sustainable moisture energy. We first introduce the working principles of MSEH for heat, cold and electricity generation, and summarize recent progress in water sorbents. We then discuss thermodynamic limitations and evaluate global potential for sustainable moisture energy. We outline future challenges of water-sorption kinetics and propose technical directions for accelerating water sorption-desorption with ordered cross-scale energy transfer and mass transport. Finally, we offer an overview of future research areas for water sorbents with higher water uptake, tunable water affinity and faster water sorption for next-generation high-performance MSEH.
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Acknowledgements
The authors acknowledge the support of the National Natural Science Foundation of China for Young Scientists (Grant No. 52206266), the National Natural Science Funds for Distinguished Young Scholar of China (Grant No. 52325601), the Major Program of National Natural Science Foundation of China (Grant No. 52293412), and National Natural Science Foundation of China (Grant No. 22035005 and No. 52022051).
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J.X. contributed to writing, reviewing and editing the manuscript and creating the figures. P.W. and Z.B. contributed to reviewing and editing the manuscript. H.C., R.W. and L.Q. contributed to reviewing, editing and discussing the manuscript. T.L. contributed to writing, reviewing and editing the manuscript and supervised the project.
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Xu, J., Wang, P., Bai, Z. et al. Sustainable moisture energy. Nat Rev Mater (2024). https://doi.org/10.1038/s41578-023-00643-0
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DOI: https://doi.org/10.1038/s41578-023-00643-0