Abstract
External driving of passive, nonlinear optical resonators has emerged over the past decade as a novel route for the generation of ultrashort optical pulses and corresponding broadband frequency combs. Although the pulse formation dynamics in such systems dramatically differ from those manifesting themselves in conventional mode-locked lasers, the demarcation between the two traditionally distinct paradigms has recently begun to blur, with demonstrations of hybrid systems incorporating both external driving and active media shown to offer specific advantages. Here we explore a new pathway for ultrashort pulse generation at the interface of externally driven passive resonators and lasers. By leveraging the nonlinear Raman gain inherent in fused silica, we achieve the deterministic generation of low-noise dissipative solitons with durations well below 100 fs via the phase-coherent pulsed driving of resonators made of standard, commercially available optical fibre. We explore and explain the physics of the new dissipative Raman soliton states, identifying scaling laws that govern the pulses’ characteristics and that allow output repetition rates to be scaled at will without influencing the soliton duration. The scheme explored in our work enables the shortest-ever pulses generated in resonators (active or passive) made from a single commercially available optical fibre, to the best of our knowledge, and it has the potential to be transferred into a chip-scale format by using existing dispersion-engineered silica microresonators.
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Data availability
The data that support the plots within this paper and the other findings of this study are available from the corresponding author upon reasonable request.
References
Wabnitz, S. Suppression of interactions in a phase-locked soliton optical memory. Opt. Lett. 18, 601–603 (1993).
Leo, F. et al. Temporal cavity solitons in one-dimensional Kerr media as bits in an all-optical buffer. Nat. Photon. 4, 471–476 (2010).
K. Jang, J., Erkintalo, M., G. Murdoch, S. & Coen, S. Ultraweak long-range interactions of solitons observed over astronomical distances. Nat. Photon. 7, 657–663 (2013).
Herr, T. et al. Temporal solitons in optical microresonators. Nat. Photon. 8, 145–152 (2014).
Obrzud, E., Lecomte, S. & Herr, T. Temporal solitons in microresonators driven by optical pulses. Nat. Photon. 11, 600–607 (2017).
J. Kippenberg, T., L. Gaeta, A., Lipson, M. & L. Gorodetsky, M. Dissipative Kerr solitons in optical microresonators. Science 361, eaan8083 (2018).
Lilienfein, N. et al. Temporal solitons in free-space femtosecond enhancement cavities. Nat. Photon. 13, 214–218 (2019).
Yi, X., Yang, Q.-F., Y. Yang, K., Suh, M.-G. & Vahala, K. Soliton frequency comb at microwave rates in a high-Q silica microresonator. Optica 2, 1078–1085 (2015).
Joshi, C. et al. Thermally controlled comb generation and soliton modelocking in microresonators. Opt. Lett. 41, 2565–2568 (2016).
Brasch, V. et al. Photonic chip–based optical frequency comb using soliton Cherenkov radiation. Science 351, 357–360 (2016).
Marin-Palomo, P. et al. Microresonator-based solitons for massively parallel coherent optical communications. Nature 546, 274–279 (2017).
Corcoran, B. et al. Ultra-dense optical data transmission over standard fibre with a single chip source. Nat. Commun. 11, 2568 (2020).
Xu, X. et al. 11 TOPS photonic convolutional accelerator for optical neural networks. Nature 589, 44–51 (2021).
Feldmann, J. et al. Parallel convolutional processing using an integrated photonic tensor core. Nature 589, 52–58 (2021).
Yi, M.-G. Suh,X. et al. Searching for exoplanets using a microresonator astrocomb. Nat. Photon. 13, 25–30 (2019).
Obrzud, E. et al. A microphotonic astrocomb. Nat. Photon. 13, 31–35 (2019).
Suh, M.-G. & Vahala, K. J. Soliton microcomb range measurement. Science 359, 884–887 (2018).
Riemensberger, J. et al. Massively parallel coherent laser ranging using a soliton microcomb. Nature 581, 164–170 (2020).
Gaeta, A. L., Lipson, M. & Kippenberg, T. J. Photonic-chip-based frequency combs. Nat. Photon. 13, 158–169 (2019).
Coen, S. & Erkintalo, M. Universal scaling laws of Kerr frequency combs. Opt. Lett. 38, 1790–1792 (2013).
Nielsen, A. U., Garbin, B., Coen, S., Murdoch, S. G. & Erkintalo, M. Invited article: emission of intense resonant radiation by dispersion-managed Kerr cavity solitons. APL Photon. 3, 120804 (2018).
Spiess, C., Yang, Q., Dong, X., G. Bucklew, V. & Renninger, W. H. Chirped dissipative solitons in driven optical resonators. Optica 8, 861–869 (2021).
Dong, X., Wang, Z. & Renninger, W. H. 120-fs single-pulse generation from stretched-pulse fiber Kerr resonators. Opt. Lett. 47, 4443–4446 (2022).
Xiao, Z. et al. Near-zero-dispersion soliton and broadband modulational instability Kerr microcombs in anomalous dispersion. Light Sci. Appl. 12, 33 (2023).
Moille, G. et al. Ultra-broadband Kerr microcomb through soliton spectral translation. Nat. Commun. 12, 7275 (2021).
Firth, W. Buffering optical data. Nat. Photon. 4, 415–417 (2010).
Bao, H. et al. Laser cavity-soliton microcombs. Nat. Photon. 13, 384–389 (2019).
Englebert, N., Mas Arabí, C., Parra-Rivas, P., Gorza, S.-P. & Leo, F. Temporal solitons in a coherently driven active resonator. Nat. Photon. 15, 536–541 (2021).
Columbo, L. et al. Unifying frequency combs in active and passive cavities: temporal solitons in externally driven ring lasers. Phys. Rev. Lett. 126, 173903 (2021).
Rowley, M. et al. Self-emergence of robust solitons in a microcavity. Nature 608, 303–309 (2022).
Spillane, S. M., Kippenberg, T. J. & Vahala, K. J. Ultralow-threshold Raman laser using a spherical dielectric microcavity. Nature 415, 621–623 (2002).
Lee, H. et al. Chemically etched ultrahigh-Q wedge-resonator on a silicon chip. Nat. Photon. 6, 369–373 (2012).
Chembo, Y. K., Grudinin, I. S. & Yu, N. Spatiotemporal dynamics of Kerr-Raman optical frequency combs. Phys. Rev. A 92, 043818 (2015).
Lin, G., Diallo, S., Dudley, J. M. & Chembo, Y. K. Universal nonlinear scattering in ultra-high Q whispering gallery-mode resonators. Opt. Express 24, 14880–14894 (2016).
Ivars, S. B., Kartashov, Y. V., Torner, L., Conejero, J. A. & Milián, C. Reversible self-replication of spatiotemporal Kerr cavity patterns. Phys. Rev. Lett. 126, 063903 (2021).
Lin, G. & Song, Q. Kerr frequency comb interaction with Raman, Brillouin, and second order nonlinear effects. Laser Photon. Rev. 16, 2100184 (2022).
Milián, C., Gorbach, A. V., Taki, M., Yulin, A. V. & Skryabin, D. V. Solitons and frequency combs in silica microring resonators: interplay of the Raman and higher-order dispersion effects. Phys. Rev. A 92, 033851 (2015).
Webb, K. E., Erkintalo, M., Coen, S. & Murdoch, S. G. Experimental observation of coherent cavity soliton frequency combs in silica microspheres. Opt. Lett. 41, 4613–4616 (2016).
Wang, Y., Anderson, M., Coen, S., Murdoch, S. G. & Erkintalo, M. Stimulated Raman scattering imposes fundamental limits to the duration and bandwidth of temporal cavity solitons. Phys. Rev. Lett. 120, 053902 (2018).
Yang, Q.-F., Yi, X., Yang, K. Y. & Vahala, K. Stokes solitons in optical microcavities. Nat. Phys. 13, 53–57 (2017).
Babin, S. A. et al. Multicolour nonlinearly bound chirped dissipative solitons. Nat. Commun. 5, 4653 (2014).
Völkel, A., Nimmesgern, L., Mielnik-Pyszczorski, A., Wirth, T. & Herink, G. Intracavity Raman scattering couples soliton molecules with terahertz phonons. Nat. Commun. 13, 2066 (2022).
Xu, Y. et al. Frequency comb generation in a pulse-pumped normal dispersion Kerr mini-resonator. Opt. Lett. 46, 512–515 (2021).
Kafka, J. D. & Baer, T. Fiber Raman soliton laser pumped by a Nd:YAG laser. Opt. Lett. 12, 181–183 (1987).
Gouveia-Neto, A. S., Gomes, A. S. L. & Taylor, J. R. Soliton Raman fibre-ring oscillators. Opt. Quant. Electron. 20, 165–174 (1988).
Keller, U., Li, K., Rodwell, M. & Bloom, D. Noise characterization of femtosecond fiber Raman soliton lasers. IEEE J. Quant. Electron. 25, 280–288 (1989).
Harvey, J. D. & Leonhardt, R. Argon pumped fiber Raman laser. In Conference on Lasers and Electro-Optics (1990) JTUA6 (Optica Publishing Group, 1990).
Yang, K. Y. et al. Broadband dispersion-engineered microresonator on a chip. Nat. Photon. 10, 316–320 (2016).
Fujii, L. et al. Dispersion tailoring in wedge microcavities for Kerr comb generation. Opt. Lett. 45, 3232–3235 (2020).
Li, Z., Xu, Y., Coen, S., Murdoch, S. G. & Erkintalo, M. Experimental observations of bright dissipative cavity solitons and their collapsed snaking in a Kerr resonator with normal dispersion driving. Optica 7, 1195–1203 (2020).
Agrawal, G.P. Nonlinear Fiber Optics 6th edn (Academic Press, 2019).
Rishøj, L., Tai, B., Kristensen, P. & Ramachandran, S. Soliton self-mode conversion: revisiting Raman scattering of ultrashort pulses. Optica 6, 304–308 (2019).
Antikainen, A., Rishøj, L., Tai, B., Ramachandran, S. & Agrawal, G. P. Fate of a soliton in a high order spatial mode of a multimode fiber. Phys. Rev. Lett. 122, 023901 (2019).
Skryabin, D. V. & Gorbach, A. V. Colloquium: looking at a soliton through the prism of optical supercontinuum. Rev. Mod. Phys. 82, 1287–1299 (2010).
Margalit, M., Orenstein, M. & Haus, H. Injection locking of a passively mode-locked laser. IEEE J. Quantum Electron. 32, 155–160 (1996).
Komarov, A., Komarov, K., Niang, A. & Sanchez, F. Nature of soliton interaction in fiber lasers with continuous external optical injection. Phys. Rev. A 89, 013833 (2014).
Ribenek, V. A., Korobko, D. A., Fotiadi, A. A. & Taylor, J. R. Supermode noise mitigation and repetition rate control in a harmonic mode-locked fiber laser implemented through the pulse train interaction with co-lased CW radiation. Optics Letters 47, 5236–5239 (2022).
Moille, G., Stone, J., Chojnacky, M., Menyuk, C. & Srinivasan, K. Kerr-induced synchronization of a cavity soliton to an optical reference for integrated frequency comb clockworks. Preprint at https://arxiv.org/abs/2305.02825 (2023).
Xu, Y. et al. Harmonic and rational harmonic driving of microresonator soliton frequency combs. Optica 7, 940–946 (2020).
Tong, Y. C., Chan, L. Y. & Tsang, H. K. Fibre dispersion or pulse spectrum measurement using a sampling oscilloscope. Electron. Lett. 33, 983–985 (1997).
Goda, K. Dispersive Fourier transformation for fast continuous single-shot measurements. Nat. Photon. 7, 102–112 (2013).
Runge, A. F. J., Broderick, N. G. R. & Erkintalo, M. Observation of soliton explosions in a passively mode-locked fiber laser. Optica 2, 36–39 (2015).
Herink, G., Kurtz, F., Jalali, B., Solli, D. R. & Ropers, C. Real-time spectral interferometry probes the internal dynamics of femtosecond soliton molecules. Science 356, 50–54 (2017).
Krupa, K., Nithyanandan, K., Andral, U., Tchofo-Dinda, P. & Grelu, P. Real-time observation of internal motion within ultrafast dissipative optical soliton molecules. Phys. Rev. Lett. 118, 243901 (2017).
Cole, D. C., Gatti, A., Papp, S. B., Prati, F. & Lugiato, L. Theory of Kerr frequency combs in Fabry-Perot resonators. Phys. Rev. A 98, 013831 (2018).
Hollenbeck, D. & Cantrell, C. D. Multiple-vibrational-mode model for fiber-optic Raman gain spectrum and response function. J. Opt. Soc. Am. B 19, 2886–2892 (2002).
Acknowledgements
We acknowledge financial support from the Marsden Fund of the Royal Society Te Apārangi of New Zealand, the Development of National Major Scientific Research Instrument from National Natural Science Foundation of China (61927816), the Introduced Innovative Team Project of Guangdong Pearl River Talents Program (2021ZT09Z109) and the Natural Science Foundation of Guangdong Province (2021B1515020074).
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Z.L. performed all of the experiments and most of the simulations with the help of Y.X. and M.E. S.S. performed numerical simulations of soliton characteristics. X. Wen, W.W., X. Wei and Z.Y. fabricated the dielectric mirrors used in the resonators. S.C. assisted with the analysis of results. S.G.M. helped to supervise the experiments and interpret the results. M.E. supervised the overall project and wrote the paper with Z.L.
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Li, Z., Xu, Y., Shamailov, S. et al. Ultrashort dissipative Raman solitons in Kerr resonators driven with phase-coherent optical pulses. Nat. Photon. 18, 46–53 (2024). https://doi.org/10.1038/s41566-023-01303-z
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DOI: https://doi.org/10.1038/s41566-023-01303-z