Abstract
Remnant pockets of carriers left over after formation of a charge density wave (CDW) were brought, by virtue of transverse electric and magnetic fields, to a currentcarrying state at quantized Landau Levels. The generated Hall voltage polarizes and puts to sliding the flexible CDW background. The screening from the CDW allows for a so strong redistribution of normal electrons density under the action of the Lorentz force alone, that an integer filling of the lowest Landau level might be reached at one edge at the expense of the full depletion at another edge of the Hall bar. With the Hall field exceeding the sliding threshold, the regime of exactly compensated collective and normal countercurrents develops in the opencircuit direction across the bar. The annihilation of the two currents proceeds via a regular sequence of phase slips which are the spacetime vortices of the CDW phase around the enforced amplitude nodes. The resulting spontaneous generation of coherent high (~GHz) frequency signals was detected by observations of multiple Shapiro steps. This picture results from studies of micronsized Hall bars in crystals of NbSe_{3} prepared by means of focused ion beams. The interpretation is confirmed and illustrated by a numerical solution of the derived equations. The depinning pulse propagates from edges to the bulk and the sliding sets in, accompanied by the generation of periodic phase slips near the Hall bar edge where the CDW phase is advanced in steps of 2π at expense of the CDW amplitude passing through zero.
Introduction
Charge density waves (CDW) are brokensymmetry states ubiquitous in lowdimensional electronic systems. CDWs are directly observed as concomitant periodic modulations of the electronic density and of atomic distortions $\propto \mathrm{cos}\left(\overrightarrow{Q}\overrightarrow{r}+\phi \right)$ characterized by the wave vector $\overrightarrow{Q}$. The CDW is a macroscopic quantum state^{1} described by a complex order parameter $\Psi ~A{e}^{i\phi}$ where A and φ are respectively the amplitude and the phase of the CDW. The approximate degeneracy with respect to displacements of φ gives rise to the most remarkable effects of the CDW sliding. The time dependence of φ determines the collective electric current j_{c} ∝ ∂φ/∂t which can be accompanied by the spontaneous generation of a coherent periodic signal with the same frequency f = ∂φ/∂t/(2π).
In conventional experiments on CDWs (see reviewers^{2,3}), the driving force for the depinning and the sliding is provided by the electric field, E_{ x }, in the direction x of CDW chains. The penetration of E_{ x } originated by the applied voltage V_{ x } is mediated by the normal current density, j_{ nx }; so the sliding and the normal currents flow in the same direction x. The initial motivation of the present studies was to show that the CDW can also be driven by the Hall voltage V_{H} originated from the normal current passing in a transverse direction. That has been proved indeed as we shall see below, but the observed effects went well above the best anticipations.
Here we shall show that, thanks to the highly polarizable CDW background, the remnant normal carriers under the quantized magnetic field and the imposed transverse electric current can be put first into the regime of a selftuned nearly integer quantum Hall (IQH) state. With increasing current, that is followed by the sliding regime of the pulsing collective current which is exactly compensated by the countercurrent of normal electrons. The zerosum loop of these two currents is closed by periodic phaseslip processes^{4} giving rise to spontaneous coherent oscillations observed up to the GHz range.
This complex phenomenon essentially integrates the coherency of the collective ground state and the extreme quantum regime of the “normal” component. In NbSe_{3} the normal current is carried by remnant carriers in small pockets of electron and hole types. Their characterization is still incomplete and even contradictory in some respects, particularly intriguing in high magnetic fields (see latest results and discussion in ref. 5 and the Supplementary Discussion 1). Still, there is enough information certifying that in a magnetic field B ≈ 20T the electrons and holes are fully quantized occupying only fractions $\nu ~1{0}^{1}$ of their lowest Landau levels.
Results
Experimental
With the help of the focused ion beam (FIB) technique we have designed a Hall bar scheme by cutting out a narrow channel transversely to the chains’ “b” (x axes) direction of the NbSe_{3} whisker crystal as shown in Fig. 1. The bias current was passed along the channel in the “c” (y axes) direction, the magnetic field B was applied in another transverse direction “a” (z axes), perpendicular to the highly conducting (b, c)plane, for the purpose to generate the Hall voltage V_{ H } along the chain axis.
Figure 1 shows two different fabricated bridgetype structures. The channels, for which length L and width W varied from 20 to 43 μm and from 1 to 6 μm correspondingly, were oriented across the conducting chains, along the crystal caxis. Totally 8 structures have been prepared and studied. We used two geometrical configurations: the twoprobes structure shown in Fig. 1a (sample Nos. 1, 3–8) and the sixprobes structure (sample No.2) with different distances between potential probes and containing the Hall probes (Fig. 1b).
Temperature dependence of the channel resistance in these structures (see Fig. S1a in Supplementary Methods 2) resembles the R_{ yy }(T) one obtained from bulk measurements.^{6} In Fig. S1b we show the field dependencies of the resistance R_{ yy }(B) and the Hall voltage, V_{ x }(B), at T = 4.2 K for the same sample. The plot of R_{ yy }(B) demonstrates the gigantic magnetoresistance which increases more than 20 times by B = 20T. The Hall field V_{ x }(B)/W is a linear function of B (except for low fields B < 0.5T). For the bias current I = 10 μA it reaches ~1.5 V/cm which is comparable with the bulk value of the threshold electric field E_{ xt } for the onset of the CDW sliding at this temperature.^{7}
Figure 2a shows a set of differential I–V curves for sample No. 4 under various magnetic fields B. They are nearly flat at B < 6T, but at higher fields a threshold feature appears in dI/dV(I) and sharpens with the field increase. Above the threshold, the differential conductivity sharply drops down (by 3–5 times at B = 20T). Each curve was swept from zero to the maximum current +I_{max}, then backwards to −I_{max}, and finally to I = 0 with no hysteresis observed.
Figure 2b shows that the threshold feature for sample No.1 is smeared out with temperature and it nearly disappears above 30 K. The threshold current, however, is nearly temperature independent, at least for B = 20T. From Fig. 2a, b it follows that the nonlinearity in IV characteristics appears only at high magnetic field and at low temperatures.
Figure 2c shows dI/dV(I) dependencies at B = 20T for two channels of different lengths, 20 and 30 μ (samples 4 and 5). This pair of structures was fabricated from the same single crystal, so that the thickness D was kept constant. It follows that the threshold current is independent of the channel length but the magnitude of the conductivity drop is directly proportional to the length.
The value of the Hall voltage was directly measured with the Hall probes of the structure shown in Fig. 1b. We measured the dependence of the differential Hall resistance, R_{ xy } = dV_{ x }/dI, as a function of the applied current simultaneously with the differential IV characteristic R_{ yy } = dV/dI along the caxis. As shown in Fig. 2d, the R_{ xy } does not change through the critical current where 1/R_{ yy } shows a sharp drop.
The nature of the sharp anomaly in the nonlinear transport across the chains becomes elucidated when we find that the state at I > I_{t} is accompanied by the emission of a coherent electromagnetic radiation. That was proved by observing on the I–V characteristics the Shapirosteps type response to an external radiation in the MHz–GHz frequency range. Fig. 3a shows that under the RF radiation the plateau at I < I_{t} sharpens into the zero bias peak which is not surprising since the RF amplitude well exceeds the dc threshold. Most striking is the appearance of a sequence of multiple peaks in dI/dV(V) which are nearly equidistant in voltage, like in superconductors, rather than in current as in CDWs. The peaks might correspond to the matching of the external frequency f_{ex} = f and the intrinsically generated frequency f_{int} in the system when f_{ex} = (p/q)f_{int}, with integers p and q. The condition p/q = 1 determines the fundamental Shapiro step ΔV.
The position of the fundamental Shapiro step is shown to be proportional to the external frequency (Fig. 3a) and also to the length of the channel, but it does not depend either on the thickness or on the width of the bridges. The generic linear dependence ΔV ∝ f on the frequency was observed for 7 structures of different lengths. Note also that the Shapiro step structure is absent in the differential Hall conductivity.
In Fig. 3b the period of voltage peaks is shown for the value ΔV/N_{c} normalized to the number of chains N_{c} which reduces the total voltage to the interchain voltage drop. From these data we can calculate ΔV/f = 12.5 mV/GHz for 1 μm of the structure length. According to the crystalline structure of NbSe_{3}, 1 μm along the caxis corresponds to 641 cells or N_{c}(1 μm) = 641 × 2 chains if we consider that the lowT CDW appears on a group of two chains within the cell. Then we get ΔV/(N_{c}f) = 10 μV/GHz per chain which is 4 times the Josephson relation ΔV/f = 2.5 μV/GHz in superconductors.
Evolution of the Shapiro steps structure with temperature is shown in Fig. 3c. As the temperature increases, the amplitude of steps decreases and ΔV increases (Fig. 3d). The Shapiro steps structure completely disappears above T ≈ 30 K. More details on measuring of Shapiro steps can be found in the Supplementary Discussion 2.
The observed properties are completely different from the standard ones when the common CDW sliding is driven by the electric field in the chains direction.^{2,3} Here, the conductivity across the chains drops down above the threshold current, the Shapiro steps are quantized in voltage rather than in current, and these properties appear only in high magnetic field and at low temperature. The threshold current is independent on the length of the channel and varies as ∝1/B.
Theoretical picture
At the basic level of interpretation, the presented data are convincing that we are dealing with a depinning and subsequent sliding of the CDW under the generated Hall voltage. Indeed, the mutually orthogonal magnetic field and the bias current, both lying in transverse interchain directions, should produce the Hall voltage, V_{ x }, in the chains direction. The Hall electric field is E_{H} = V_{ x }/W = R_{H}IB/(DW) where R_{H} is the Hall constant, D is the sample thickness. The threshold current I_{t} corresponding to the critical Hall electric field, E_{Ht} is I_{t} = E_{Ht}WD/(R_{H}B) ∝ W/B which reproduces the experimental dependencies on W and B (recall the inset in Fig. 2a). The value of V_{ x } was directly measured using Hall probes of the structure shown in Fig. 1b which yields the values like E_{Ht} = 0.3 V/cm at B = 20T and T = 4.2 K which is on the right scale of threshold fields in the bulk. Still, this interpretation invoking the CDW sliding faces a vital challenge: the circuit is open in the x direction, hence the total current across the Hall bar must be zero. The collective CDW current must be compensated by a countercurrent of normal carriers, the picture of which is elaborated theoretically below, with more details given in Supplementary Notes 2–4.
Under the HMF but at no applied current yet, the carriers are distributed homogeneously forming a fractionally (ν < 1) filled quantized state. (The value of ν < 1 is estimated as ν ≈ 0.5–0.1 at B = 20T, see Supplementary Discussion 1.) When the transverse current J_{ y } is applied, the Lorentz force in x direction appears pushing the carriers orbits towards one end (which we choose as x = 0) until the charge redistribution gives rise to the compensating Hall field E_{ x }. The first key peculiarity with respect to conventional Hall setup is the presence of the CDW background with its gigantic polarizability, estimated here as $\u03f5$ ∝ 10^{6} (see Supplementary Note 1). The screening by displacements of the CDW phase φ ∝ $\u03f5$E_{ x } allows for a strong redistribution of the electronic density, see Fig. 4, up to (in the T = 0 limit) the complete charge segregation when all carriers occupy, with the maximum filling 1, a segment l = νL_{ x } of the chain length L_{ x }, thus forming here the IQH state while leaving the segment (1 − ν)L_{ x } unoccupied.
The electric field accompanying such a charge separation easily exceeds the pinning threshold for the CDW sliding. Then, as we demonstrate in Fig. 4 and in Supplementary Note 3, Sec. 4, the depinning propagates into the nominally pinned central region via sharp walls. The resulting picture is that of compensated collective j_{c} and normal j_{ nx } pulsing countercurrents driven by the Hall voltage. The appearance of j_{ nx } gives rise to the secondary Hall voltage, now in the y direction, the persistent part of which is registered as a sharp threshold in the I–V curve while the periodic part gives rise to Shapiro steps. This scenario will be illustrated below by a numerical modeling.
In the regime of the extreme Landau quantization, the kinetic energy is no more involved, then the density is determined locally by the electric potential $\Phi \left(\overrightarrow{r}\right)$. The profile for the density of carriers per chain is ${n}_{1}\left(x\right)={f}_{\mathrm{F}}\left(\Phi \left(x\right)\mathrm{\u2215}T\right){\stackrel{\u0304}{n}}_{1}\mathrm{\u2215}\nu $ where $\nu =\left(hc\u2215eB\right)\left({\stackrel{\u0304}{n}}_{1}\u2215{d}_{y}\right)$, ${\stackrel{\u0304}{n}}_{1}={N}_{1}\mathrm{\u2215}{L}_{x}$ is the mean concentration of carriers per unit length of one chain, d_{ y } is the interchain distance, and f_{F}(z) is the Fermi distribution function. Integration over x of the oneparticle transverse current density ecE_{ x }(x)/B, weighted with n_{1}(x), yields the overall current as a function of values of the potentials only at x boundaries:
where N_{a} is the number of (b, c) planes across the sample height. Above the threshold, the CDW starts sliding, carrying on the collective current J_{c}, which must bring about the compensating normal countercurrent J_{ nx } = −J_{c} since the total x current must be zero. Then the new component of the Lorentz force appears in the y direction giving rise to the reciprocal Hall voltage V_{ y }. Its magnitude is given by the universal law similar to Eq. (1) with interchanged indices x and y (and the opposite sign). For the current per chain we get
where ΔV_{ y }(x) = (Φ(x, 0) − Φ(x, L_{ y }))d_{ y }/L_{ y } is the mean interchain voltage drop. The charge separation was important for this conclusion: in Eq. (2) the integration by y was carried on over the line close to the edge x = 0 where f_{F}(Φ(x, y)) ≈ 1.
The last step is to remind that the CDW countercurrent, per chain, is j_{c1} = −e∂_{ t }φ/π and it requires phase slips^{4} to annihilate with the normal current j_{ x1} near the boundary. Let each phase slip absorb/release M electrons per chain, then the repetition frequency is
We arrive at the Josephson type relation with an additional factor M; according to experiments, with a good accuracy being integer M ≈ 4. The phase slip appears to be a spaciotemporal supervortex, with the Mfold circulation. This value may be related to the number of normal carriers within the chain segment which are available for transformation to/from the condensate within each phase slip.
The sharp strong drop of the transverse normal current J_{ y } with the onset of the loop currents in the chains’ direction can also be illustrated by means of quite general phenomenological considerations which we present in Supplementary Note 2.
The modeling
The numerical work was performed on the bases of the timedependent GinzburgLandau approach the adaptation of which leads to nonlinear partial differential equations described in Supplementary Note 4. Here we shall present the most important results.

1.
At the critical current, the time evolution starts with a depinning pulse propagating from edges to the bulk, after which the regime of the homogeneous sliding sets up. Results of the modeling (described in Supplementary Note 3) are shown in Fig. 4 for the lowest experimental temperature 1 K.
The plots demonstrate two propagating fronts of depinning originated (at different moments) at the boundaries where the electric field is enhanced (plot 4b) because of the charge redistribution (plot 4a). The fronts collide showing a strong brief peak of the phase velocity ∂_{ t }φ/π (plot 4c), and then annihilate giving rise to the overall homogeneously sliding state (plot 4c) while on the background of the very inhomogeneous distributions of the electric field and the particles’ density. Initially, the distribution of occupation numbers is homogeneous f_{F}(x, 0) = ν = 0.5. After passing of the first depinning front, the two plateaus with f ≈ 1 and f ≈ 0 are established giving rise to a nearly IQH region at the expense of the nearly unpopulated one.
The rising of occupation numbers f_{F}(t, x) towards the channel edge x = 0, up to the IQH limit f_{F}(t, 0) = 1, can be understood already from the most general relation (1). Indeed, the value J_{ T }N_{a} ≈ 3 μA (with N_{a} ≈ 1000) corresponds to the lowest experimental currents while in most important regimes J_{ y }/(J_{ T }N_{a}) ∝ 10^{2} is big. Then (1) requires inevitably that f_{F}(t, 0) = 1. To keep the mean value of ${\u27e8{f}_{\mathrm{F}}\u27e9}_{x}=\nu $ over x, the compensating depletion should take place towards x = L_{ x }.

2.
At higher currents the regime of a totally depinned sliding sets in, which is accompanied by the generation of periodic phase slips—the events where the CDW phase is advanced in steps of 2π or 2Mπ with integer M. They allow to detach the fast sliding highfield stripe near x = 0 from the slowly sliding body.
Results of the modeling (described in Supplementary Note 4) are presented in Fig. 5. The phase slip is a vortex of the CDW complex order parameter Ψ in space–time coordinates (x,t); hence the amplitude node A(x, t) = 0 develops in the vortex center. The amplitude does not recover completely inbetween the nodes, so its standing depression is formed from which A(x,t) shoots instantaneously further down to zero. This periodic sequence might have given rise to the experimentally observed Shapiro steps.
Discussion
Studies of density waves under high magnetic fields have already brought a firework of effects. Most known is the cascade of phase transitions among the Hallquantized “field induced density waves” (see the reviews’ collection^{8}). Closer to the present work, the magnetic field could suppress the strong zerobias conductance peak in I–V characteristics of CDW mesastructures which allowed to recover the physics of solitons and of electronic vortices^{9,10} in experiments on the internal tunneling.
Spontaneous superstructures of a 2D electron gas in a quantized magnetic field have already attracted much attention in experiment and theory, see a short review in Sec. 11.6.4. of ref. 3. They have been identified as Wigner crystals (see reviews^{11,12}) and as a richness of bubble, stripe, and nematic states (see reviews^{13,14}). These structures have been registered and explained as ground states of electronic systems in the magnetic field, with the collective sliding showing up as a posteriori effect. The state described in this article is fundamentally non static. It appears, under the effect of the Lorentz force, as a stationary state carrying the Hall current. At higher bias currents above the threshold it develops as an essentially dynamical pulsating state.
In conventional sliding CDWs, the normal current injected at junctions is gradually transformed into the collective one in the bulk, and this process is assisted by distributed phase slips.^{15,16} In the experiments reported here, the exactly compensated partial currents flow oppositely across the opencircuit Hall bar. By analogy, we recall observations^{17} of a CDW driven contactlessly by the thermopower which also assume the exact compensation of the normal and the sliding currents.
The intriguing part of the story are the phase slip processes understood as space–time vortices of the CDW complex order parameter. Their regular sequence is clearly observed via the Shapiro steps. Here the phase slips appear under unique circumstances of segregation of the electronic density among the plateaus of maximally filled and totally depleted quantized Landau levels. The modeling confirms that at the overcharged edge the integer quantum Hall state is selftuned even if integrally, via measurements of the resistivity tensor, we do not observe the required integer characteristics of the quantum Hall state (because of the fractionally filled transient bulk region). Experiments at lower temperatures or higher magnetic fields should reach a truly stepwise boundary among the full and the zero field quantum levels. Such an improbable strong deviation of the electronic density from its mean value under the normally small Lorentz force became possible here because of the charge compensation by the gigantic polarization of the CDW, with the help of the FIB design allowing for high currents along the Hall bar.
In summary, the combination of the FIB fabrication of microscopic devices, application of a high magnetic field, and the modeling has allowed to identify the never seen regime of twofluid quantum magnetohydrodynamics with compensated collective and normal conduction in the frame of the QH regime. The basic ingredient of this highly nonlinear and nonstationary regime is a sequence of periodic phase slip processes providing the annihilation of the normal and the collective currents. Beyond the generation of sliding pulses, the CDW plays the role of a screening medium which allows the Lorentz force to spaceseparate the mean noninteger density of normal electrons from the depleted zone to the one where the IQH state is selftuned. The major role is played by ultralight carriers,^{5} suspected to be Weyl fermions, the emergence of which in NbSe_{3} from the ground state reconstruction by the CDW is a new tool in manipulating a quantum material.
Methods
Measurements of IV characteristics and their derivatives have been performed in conventional 4probe configuration using computer controlled current source and nanovoltmeter. For studying nonstationary effects a RF current was superposed upon the dc current using the current contacts connected to the RF generator via two capacitors. Experiments in magnetic field up to B = 20T have been carried out in a Bitter coil and in the superconducting magnet in National Laboratory of High Magnetic Fields in Grenoble. The structure was prepared by means of the focus ion beam (FIB) machine SMI3050, Seiko Inc., Japan, with the resolution of Gaion beam of 6 nm in the regime of low current of few tens of pA. The electrical contacts to the crystal have been made by pressing indium stabs to the golden contact pads prepared by laser evaporation before the FIB process. More details on the material, methods and samples are described in SI: Supplementary Methods 1 and 2 for the experimental work and Supplementary Notes 3 and 4 for the theory and modeling.
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Acknowledgements
Work at Grenoble was partially performed in the frame of the CNRSRAS Associated International Laboratory between Institute Neél and IRE Physical properties of coherent electronic states in condensed matter. A.P.O. and A.A.S. acknowledge support from Russian State Fund for the Basic Research (No. 170200665a). S.B. acknowledges the financial support of the Ministry of Education and Science of the Russian Federation in the framework of Increase Competitiveness Program of NUST MISiS (N K32017033).
Author information
Affiliations
Kotel’nikov Institute of Radioengineering and Electronics of RAS, Mokhovaya 117, 125009, Moscow, Russia
 Andrey P. Orlov
 , Aleksander A. Sinchenko
 & Yuri I. Latyshev
Université Grenoble Alpes, CNRS, Grenoble INP, Institut Néel, 38000, Grenoble, France
 Pierre Monceau
Université Grenoble Alpes, INSA Toulouse, Université Toulouse Paul Sabatier, CNRS, LNCMI, 38000, Grenoble, France
 Pierre Monceau
LPTMSCNRS, Université Parissud, Université ParisSaclay, 91405, Orsay, France
 Serguei Brazovskii
National University of Science and Technology “MISiS”, Moscow, 119049, Russia
 Serguei Brazovskii
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Contributions
Y.I.L. (deceased) was at the origin of the mesajunctions design and their studies in high magnetic fields. A.P.O. and A.A.S. carried out the experimental work and analysis; S.B. formulated the theoretical concept and performed the modeling; A.A.S. and P.M. coped with the experiment and, with S.B., wrote the paper. All authors contributed to discussions.
Competing interests
The authors declare that they have no competing financial interests.
Corresponding authors
Correspondence to Aleksander A. Sinchenko or Pierre Monceau.
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