Over the last decade, control of atomic-scale electronic motion by non-perturbative optical fields has broken tremendous new ground with the advent of phase-controlled high-energy few-cycle pulse sources1. The development of close to single-cycle, carrier-envelope phase controlled, high-energy optical pulses has already led to isolated attosecond EUV pulse generation2, expanding ultrafast spectroscopy to attosecond resolution1. However, further investigation and control of these physical processes requires sub-cycle waveform shaping, which has not been achievable to date. Here, we present a light source, using coherent wavelength multiplexing, that enables sub-cycle waveform shaping with a two-octave-spanning spectrum and a pulse energy of 15 µJ. It offers full phase control and allows generation of any optical waveform supported by the amplified spectrum. Both energy and bandwidth scale linearly with the number of sub-modules, so the peak power scales quadratically. The demonstrated system is the prototype of a class of novel optical tools for attosecond control of strong-field physics experiments.
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Krausz, F. & Ivanov, M. Attosecond physics. Rev. Mod. Phys. 81, 163–234 (2009).
Goulielmakis, E. et al. Single-cycle nonlinear optics. Science 320, 1614–1617 (2008).
Udem, T., Holzwarth, R. & Hänsch, T. W. Optical frequency metrology. Nature 416, 233–237 (2002).
Kienberger, R. et al. Atomic transient recorder. Nature 427, 817–821 (2004).
Li, C. H. et al. A laser frequency comb that enables radial velocity measurements with a precision of 1 cm s−1. Nature 452, 610–612 (2008).
Corkum, P. B. Plasma perspective on strong field multiphoton ionization. Phys. Rev. Lett. 71, 1994–1997 (1993).
Keldysh, L. V. Ionization in the field of a strong electromagnetic wave. Sov. Phys. JETP 20, 1307–1314 (1965).
Chipperfield, L. E., Robinson, J. S., Tisch, J. W. G. & Marangos, J. P. Ideal waveform to generate the maximum possible electron recollision energy for any given oscillation period. Phys. Rev. Lett. 102, 063003 (2009).
Hänsch, T. W. A proposed sub-femtosecond pulse synthesizer using separate phase-locked laser oscillators. Opt. Commun. 80, 71–75 (1990).
Wei, Z. Y., Kobayashi, Y., Zhang, Z. G. & Torizuka, K. Generation of two-color femtosecond pulses by self-synchronizing Ti:sapphire and Cr:forsterite lasers. Opt. Lett. 26, 1806–1808 (2001).
Shelton, R. K. et al. Phase-coherent optical pulse synthesis from separate femtosecond lasers. Science 293, 1286–1289 (2001).
Krauss, G. et al. Synthesis of a single cycle of light with compact erbium-doped fibre technology. Nature Photon. 4, 33–36 (2010).
Cerullo, G., Baltuška, A., Mücke, O. D. & Vozzi, C. Few-optical-cycle light pulses with passive carrier-envelope phase stabilization. Laser Photon. Rev. 5, 323–351 (2011).
Dubietis, A., Butkus, R. & Piskarskas, A. P. Trends in chirped pulse optical parametric amplification. IEEE J. Sel. Top. Quantum Electron. 12, 163–172 (2006).
Moses, J. et al. Highly stable ultrabroadband mid-IR optical parametric chirped-pulse amplifier optimized for superfluorescence suppression. Opt. Lett. 34, 1639–1641 (2009).
Moses, J., Manzoni, C., Huang, S. W., Cerullo, G. & Kärtner, F. X. Temporal optimization of ultrabroadband high-energy OPCPA. Opt. Express 17, 5540–5555 (2009).
Baltuška, A., Fuji, T. & Kobayashi, T. Controlling the carrier-envelope phase of ultrashort light pulses with optical parametric amplifiers. Phys. Rev. Lett. 88, 1339011 (2002).
Schibli, T. R. et al. Attosecond active synchronization of passively mode-locked lasers by balanced cross correlation. Opt. Lett. 28, 947–949 (2003).
Birge, J. R., Crespo, H. M. & Kärtner, F. X. Theory and design of two-dimensional spectral shearing interferometry for few-cycle pulse measurement. J. Opt. Soc. Am. B 27, 1165–1173 (2010).
Forget, N., Canova, L., Chen, X., Jullien, A. & Lopez-Martens, R. Closed-loop carrier-envelope phase stabilization with an acousto-optic programmable dispersive filter. Opt. Lett. 34, 3647–3649 (2009).
Wittmann, T. et al. Single-shot carrier-envelope phase measurement of few-cycle laser pulses. Nature Phys. 5, 357–362 (2009).
Mücke, O. D. et al. Scalable Yb-MOPA-driven carrier-envelope phase-stable few-cycle parametric amplifier at 1.5 µm. Opt. Lett. 34, 118–120 (2009).
Popmintchev, T. et al. Phase matching of high harmonic generation in the soft and hard X-ray regions of the spectrum. Proc. Natl Acad. Sci. USA 106, 10516–10521 (2009).
Sansone, G. et al. Isolated single-cycle attosecond pulses. Science 314, 443–446 (2006).
Cerullo, G. & De Silvestri, S. Ultrafast optical parametric amplifiers. Rev. Sci. Instrum. 74, 1–18 (2003).
Hommelhoff, P., Kealhofer, C. & Kasevich, M. A. Ultrafast electron pulses from a tungsten tip triggered by low-power femtosecond laser pulses. Phys. Rev. Lett. 97, 247402 (2006).
Arissian, L. et al. Direct test of laser tunneling with electron momentum imaging. Phys. Rev. Lett. 105, 133002 (2010).
Hochstrasser, R. M. Two-dimensional spectroscopy at infrared and optical frequencies. Proc. Natl Acad. Sci. USA 104, 14190–14196 (2007).
Zou, Q. H. & Lu, B. Propagation properties of ultrashort pulsed beams with constant waist width in free space. Opt. Laser Technol. 39, 619–625 (2007).
This work was supported by the Air Force Office of Scientific Research (grants FA9550-09-1-0212, FA8655-09-1-3101 and FA9550-10-1-0063) and by Progetto Roberto Rocca.
The authors declare no competing financial interests.
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Huang, S., Cirmi, G., Moses, J. et al. High-energy pulse synthesis with sub-cycle waveform control for strong-field physics. Nature Photon 5, 475–479 (2011). https://doi.org/10.1038/nphoton.2011.140
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