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| Open AccessAmber rainbow ribbon effect in broadband optical metamaterials
The researchers showcased a negative Goos-Hänchen effect in film samples across the entire visible spectrum and discovered an amber rainbow ribbon and an optical black hole where little light leaks out due to perfect back reflection.
- Jing Zhao
- , Xianfeng Wu
- & Xiaopeng Zhao
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Article
| Open AccessLarge exchange-driven intrinsic circular dichroism of a chiral 2D hybrid perovskite
Li et al. report large circular dichroism in 2D chiral perovskite single crystals, arises from the inorganic sublattice, instead of chiral ligands, driven by electron-hole exchange interactions. This is evidenced by both reflective circular dichroism spectroscopy and ab initio theory.
- Shunran Li
- , Xian Xu
- & Peijun Guo
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| Open AccessAn optofluidic antenna for enhancing the sensitivity of single-emitter measurements
Single molecule investigations are often performed in fluidic environments, but molecular diffusion and limited photon counts can compromise studies of processes with fast or slow dynamics. The authors introduce a planar optofluidic antenna which enhances the fluorescence signal from molecules, applicable to a diverse range of studies.
- Luis Morales-Inostroza
- , Julian Folz
- & Vahid Sandoghdar
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| Open AccessUltrafast all-optical second harmonic wavefront shaping
Enhancing the data encoding into the orbital angular momentum of light beams could enable faster and more efficient optical communications. This work demonstrates complex control of the second harmonic wavefront with dynamics solely limited by the pulse duration.
- Artem Sinelnik
- , Shiu Hei Lam
- & Isabelle Staude
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Article
| Open AccessHigh performance artificial visual perception and recognition with a plasmon-enhanced 2D material neural network
Here, the authors demonstrate a low-power neuromorphic visual architecture based on a plasmon-enhanced 2D semiconductor phototransistor array, showing high-speed sensing, preprocessing and image recognition functionalities.
- Tian Zhang
- , Xin Guo
- & Linjun Li
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| Open AccessDirect space–time manipulation mechanism for spatio-temporal coupling of ultrafast light field
Here the authors propose a mechanism for direct space-time manipulation of ultrafast light field and experimentally demonstrate the generation of a spatiotemporally coupling light spring with a broad topological charge bandwidth.
- Qinggang Lin
- , Fu Feng
- & Xiaocong Yuan
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| Open AccessTwisted photonic Weyl meta-crystals and aperiodic Fermi arc scattering
Fermi arcs show unpredictable diffraction features resulting from their long-range scattering order in aperiodic systems. Here, authors continuously twist a bi-block Weyl meta-crystal and experimentally observe the twisted Fermi arc reconstruction.
- Hanyu Wang
- , Wei Xu
- & Biao Yang
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| Open AccessPoincaré sphere trajectory encoding metasurfaces based on generalized Malus’ law
Polarization serves as an excellent information encoding carrier. Here, authors expand the metasurface encoding dimensionality of polarization information by engineering the Poincaré Sphere trajectory with generalized Malus’ law, unveiling new opportunities for advanced polarization optics.
- Zi-Lan Deng
- , Meng-Xia Hu
- & Andrea Alù
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Article
| Open AccessUltrasound-induced reorientation for multi-angle optical coherence tomography
Accessing multi-angle views of organoids is important for biology and oncology. The authors propose ultrasound-induced reorientation for multi-angle optical coherence tomography, using a 3D-printed acoustic trap to levitate and rotate samples with a model-based algorithm for reconstruction.
- Mia Kvåle Løvmo
- , Shiyu Deng
- & Monika Ritsch-Marte
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| Open AccessAssessing intra- and inter-molecular charge transfer excitations in non-fullerene acceptors using electroabsorption spectroscopy
The performance of Y6-containing donor-acceptor active layers in organic solar cells is highly related to the charge-transfer nature in Y6 aggregates. Here, authors study charge-transfer characteristics of excitations of isolated and aggregated Y6 molecules through electroabsorption spectroscopy.
- Sudhi Mahadevan
- , Taili Liu
- & Sai-Wing Tsang
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Article
| Open AccessCavity-coupled telecom atomic source in silicon
T centers in silicon are promising candidates for quantum applications yet suffer from weak optical transitions. Here, by integrating with a silicon nanocavity, the authors demonstrate an enhancement of the photon emission rate for a single T center.
- Adam Johnston
- , Ulises Felix-Rendon
- & Songtao Chen
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Article
| Open AccessPhotooxidation triggered ultralong afterglow in carbon nanodots
Biocompatible afterglow materials have potential in imaging applications, but are challenging to prepare. Here the authors report the development of carbon nanodots with near-infrared afterglow, and demonstrate their use in imaging for tumour resection.
- Guang-Song Zheng
- , Cheng-Long Shen
- & Chong-Xin Shan
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Article
| Open AccessAnomalous and Chern topological waves in hyperbolic networks
Here the authors experimentally demonstrate the anomalous and Chern topological phases in a hyperbolic non-reciprocal scattering network, establishing unidirectional channels to induce new and exciting wave transport properties in curved spaces.
- Qiaolu Chen
- , Zhe Zhang
- & Romain Fleury
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| Open AccessCompact terahertz harmonic generation in the Reststrahlenband using a graphene-embedded metallic split ring resonator array
Compact sources in the frequency range of 6-12 THz are difficult to obtain due to optical phonon absorption in conventional III-V semiconductors. Here, the authors demonstrate third harmonic generation at 9.63 THz by optically pumping monolayer graphene coupled to a circular split ring resonator by using a semiconductor laser.
- Alessandra Di Gaspare
- , Chao Song
- & Miriam S. Vitiello
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Article
| Open AccessMonolithic thin-film lithium niobate broadband spectrometer with one nanometre resolution
A framework to break the inherent trade-off barrier between spectral resolution and operational bandwidth of integrated optical spectrometers is developed and demonstrated on thin-film lithium niobate without sacrificing the compact footprint.
- Giovanni Finco
- , Gaoyuan Li
- & Rachel Grange
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| Open AccessUltra-compact exciton polariton modulator based on van der Waals semiconductors
Miniaturized and efficient optical modulators are desired for data transmission, processing and communication. Here, the authors report the fabrication of exciton-polariton Mach–Zehnder modulators based on thin WS2 waveguides with a footprint of ~30 μm², modulation ratio up to −6.20 dB and nanosecond response times.
- Seong Won Lee
- , Jong Seok Lee
- & Su-Hyun Gong
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Article
| Open AccessSubwavelength dielectric waveguide for efficient travelling-wave magnetic resonance imaging
Achieving uniform spin excitation, crucial for MRI, is challenging in the electrically large human body at UHF. Here, authors introduce an innovative dielectric waveguide specifically designed for traveling-wave MRI, which enhances homogeneity and efficiency through effective wave manipulation.
- Yang Gao
- , Tong Liu
- & Xiaotong Zhang
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| Open AccessTime-of-flight detection of terahertz phonon-polariton
Polaritons, light-matter hybridized quasiparticles, are the fundamental excitation of strong coupling systems and are widely applicable in information technologies. Here the authors applied the concept of time-of-flight measurement in terahertz induced second harmonic generation experiments in various systems to comprehensively study the dispersion relation of phonon-polaritons and reveal potential spin-lattice couplings.
- Tianchuang Luo
- , Batyr Ilyas
- & Nuh Gedik
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| Open AccessRoom-temperature strong coupling in a single-photon emitter-metasurface system
Interfacing single-photon emitters (SPEs) with high-finesse cavities can prevent decoherence processes, especially at elevated temperature, but its implementation remains challenging. Here, the authors report room-temperature strong coupling of SPEs in hexagonal boron nitride with a dielectric cavity based on bound states in the continuum, showing a Rabi splitting of ~ 4 meV.
- T. Thu Ha Do
- , Milad Nonahal
- & Son Tung Ha
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Article
| Open AccessBroadband angular spectrum differentiation using dielectric metasurfaces
Metasurfaces processing incoming images have been proposed in the context of real space operations. Here, the authors demonstrate mathematical operations, such as differentiation, on the angular spectrum of an image using metasurfaces, which can be used to enhance spectral features of an image.
- Ming Deng
- , Michele Cotrufo
- & Lin Chen
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| Open AccessRetinal photoisomerization versus counterion protonation in light and dark-adapted bacteriorhodopsin and its primary photoproduct
Malakar et al. investigate the photochemical dynamics in the isomerization of bacteriorhodopsin light and dark-adapted forms and in the first photocycle intermediate, K. The results prompt a reevaluation of the counter ion model, revealing that a different protonation then that shown in the classic quadrupole so far considered must be employed to account for the experimental data.
- Partha Malakar
- , Samira Gholami
- & Sanford Ruhman
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Article
| Open AccessFrequency-selective perovskite photodetector for anti-interference optical communications
Signal transmission without the interference from ambient light is prerequisite for optical communications. Min et al. design an asymmetric 2D-3D-2D perovskite photodetector with frequency-selective photoresponse for real-time high fidelity optical communications under strong light interference.
- Liangliang Min
- , Haoxuan Sun
- & Liang Li
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Article
| Open AccessFast topographic optical imaging using encoded search focal scan
Quickly acquiring topographical information from a sample remains a challenge in optics. Here, the authors introduce encoded search focal scan, a technique for sub-micrometric imaging of tens of topographies per second based on collecting a reduced set of images.
- Narcís Vilar
- , Roger Artigas
- & Guillem Carles
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| Open AccessSelenium substitution for dielectric constant improvement and hole-transfer acceleration in non-fullerene organic solar cells
Dielectric constant of non-fullerene acceptors plays a critical role in organic solar cells in terms of exciton dissociation and charge recombination. Here, authors report selenium substitution on central core of acceptors to improve dielectric constant, realizing devices with efficiency of 19.0%.
- Xinjun He
- , Feng Qi
- & Wallace C. H. Choy
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| Open AccessBerkSEL: A scale-invariant laser beyond the Schawlow-Townes two-mirror strategy
I argue that a surface emitting laser that remains single mode irrespective of its size, a scale-invariant laser, should of necessity also waste light at the edge. This is a fundamental departure from the Schawlow-Townes two-mirror strategy that keeps light away from mirrors and edges to preserve gain and minimize loss. The strategy was implemented in the recent discovery of the Berkeley Surface Emitting Laser (BerkSEL).
- Boubacar Kanté
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Article
| Open AccessSpectral-temporal-spatial customization via modulating multimodal nonlinear pulse propagation
The authors introduce a method for modulating the multimodal nonlinear pulse propagation in fibers by controlled bending, achieving a tunable broadband high-peak-power femtosecond light source that could empower nonlinear imaging and spectroscopy.
- Tong Qiu
- , Honghao Cao
- & Sixian You
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Article
| Open AccessWandering principal optical axes in van der Waals triclinic materials
Principal optical axes define light-matter interactions in crystals and they are usually assumed to be stationary. Here, the authors report the observation of wavelength-dependent principal optical axes in ternary van der Waals crystals (ReS2 and ReSe2), leading to wavelength-switchable propagation directions of their waveguide modes.
- Georgy A. Ermolaev
- , Kirill V. Voronin
- & Kostya S. Novoselov
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Article
| Open AccessFully bioresorbable hybrid opto-electronic neural implant system for simultaneous electrophysiological recording and optogenetic stimulation
Bioresorbable neural implants offer a promising solution to the challenges of secondary surgeries required for the removal of implanted devices. Here, the authors introduce a fully bioresorbable flexible hybrid opto-electronic system for simultaneous electrophysiological recording and optogenetic stimulation.
- Myeongki Cho
- , Jeong-Kyu Han
- & Ki Jun Yu
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Article
| Open AccessContact-separation-induced self-recoverable mechanoluminescence of CaF2:Tb3+/PDMS elastomer
A composite CaF2:Tb3+/polydimethylsiloxane elastomer with contact-separation-induced self-recoverable mechanoluminescence is demonstrated, and a contact-separation cycle model is established to understand its mechanoluminescence.
- Wenxiang Wang
- , Shanwen Wang
- & Jiachi Zhang
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Article
| Open AccessOptically addressable spin defects coupled to bound states in the continuum metasurfaces
Previous research reported enhanced emission from spin defects in hBN by coupling to optical resonators; however, this approach has limited scalability. Here the authors use a monolithic metasurface featuring quasi bound states fabricated from hBN to enhance photoemission and optical spin-readout efficiency of defects in the same material.
- Luca Sortino
- , Angus Gale
- & Andreas Tittl
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Article
| Open AccessLight-field flow cytometry for high-resolution, volumetric and multiparametric 3D single-cell analysis
Current imaging flow cytometry approaches remain limited in their ability to reveal subcellular information with high-resolution and instrumental simplicity. Here, the authors present a light-field flow cytometer capable of high-content, multi-color imaging of cells with high-resolution in 3D.
- Xuanwen Hua
- , Keyi Han
- & Shu Jia
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Article
| Open AccessNon-Hermitian non-equipartition theory for trapped particles
The authors propose a generalization of the equipartition theorem of thermal physics to account for non-Hermitian trapping forces, relevant for the problems in non-equilibrium open systems and advanced nanotechnology.
- Xiao Li
- , Yongyin Cao
- & Jack Ng
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Article
| Open AccessHigh-density volumetric super-resolution microscopy
Current approaches for volumetric super-resolution microscopy can yield large and complex PSF spatial footprints. Here, the authors show a super-resolution microscopy approach using a hexagonal microlens array, which offers speed improvements in volumetric imaging compared to other single-molecule methods.
- Sam Daly
- , João Ferreira Fernandes
- & Steven F. Lee
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Article
| Open AccessCross-layer transmission realized by light-emitting memristor for constructing ultra-deep neural network with transfer learning ability
Parallel information transmission components and hardware strategies are still lacking in neural networks. Here, the authors propose a strategy to use light emitting memristors with negative ultraviolet photoconductivity and intrinsic parallelism to construct direct information cross-layer modules.
- Zhenjia Chen
- , Zhenyuan Lin
- & Huipeng Chen
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Article
| Open AccessModulation-free laser stabilization technique using integrated cavity-coupled Mach-Zehnder interferometer
Stable lasers are crucial in many applications like sensing. Here, the authors demonstrate a laser frequency locking method that maintains performance, eliminates modulation, simplifies architecture, and enables miniaturization on a photonic chip.
- Mohamad Hossein Idjadi
- , Kwangwoong Kim
- & Nicolas K. Fontaine
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Article
| Open AccessSpatiotemporal control of photochromic upconversion through interfacial energy transfer
Achieving spatiotemporal control of photochromic upconversion from a single lanthanide emitter remains challenging. Here, the authors present a conceptual model enabling such control of Er3+ photochromic upconversion via interfacial energy transfer in a core-shell nanostructure.
- Long Yan
- , Jinshu Huang
- & Bo Zhou
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| Open AccessProbing molecules in gas cells of subwavelength thickness with high frequency resolution
Using gas cells for spectroscopic studies opens possibility for miniaturized platforms that can be integrated with other optical components. Here the authors demonstrate molecular rovibrational spectroscopy by confining molecules in a cell of subwavelength thickness.
- Guadalupe Garcia Arellano
- , Joao Carlos de Aquino Carvalho
- & Athanasios Laliotis
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Article
| Open AccessCoherent control of enhanced second-harmonic generation in a plasmonic nanocircuit using a transition metal dichalcogenide monolayer
Here, the authors integrate monolayer MoSe2 with a plasmonic nanocircuit and demonstrate the coherent selective routing of the enhanced nonlinear optical signal emitted by the 2D semiconductor, with routing extinction ratios up to 14.86 dB.
- Pei-Yuan Wu
- , Wei-Qing Lee
- & Chen-Bin Huang
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Article
| Open AccessElectron/infrared-phonon coupling in ABC trilayer graphene
Via Raman and infrared spectroscopy measurements, X. Zan et al. find that rhombohedral ABC trilayer graphene has stronger electron/infrared-phonon coupling than Bernal ABA trilayer graphene.
- Xiaozhou Zan
- , Xiangdong Guo
- & Guangyu Zhang
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Article
| Open AccessMode-multiplexing deep-strong light-matter coupling
The authors show an original approach to achieve strong light-matter interaction harnessing the coupling between plasmonic resonators and the Landau resonances of an underlying quantum well, demonstrating remarkably high coupling strengths.
- Joshua Mornhinweg
- , Laura Katharina Diebel
- & Christoph Lange
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Article
| Open AccessWide-field mid-infrared hyperspectral imaging beyond video rate
Mid-infrared hyperspectral imaging is valuable for sample characterisation but suffers limited scanning rates. The authors develop such an imaging system based on parametric upconversion of supercontinuum illumination in the Fourier plane, enabling a 100-Hz acquisition rate of spectral datacubes.
- Jianan Fang
- , Kun Huang
- & Heping Zeng
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Article
| Open AccessSingle-pixel p-graded-n junction spectrometers
The miniaturization of spectrometers to a submillimeter-scale footprint opens opportunities for applications in hyperspectral imaging and lab-on-a-chip systems. Here, the authors report a high-performance single-pixel photodetector spectrometer based on the III-V semiconductor p-graded-n junction, featuring a voltage-tunable optical response.
- Jingyi Wang
- , Beibei Pan
- & Baile Chen
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Article
| Open AccessObservation of continuum Landau modes in non-Hermitian electric circuits
Non-Hermitian systems have many physical properties without Hermitian counterparts. Here, the authors demonstrate a non-Hermitian topolectrical circuit hosting continuous bound states under pseudomagnetic fields with no counterparts in Hermitian systems.
- Xuewei Zhang
- , Chaohua Wu
- & Gang Chen
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Article
| Open AccessReconfigurable perovskite X-ray detector for intelligent imaging
In-sensor computing requires detectors with polarity reconfigurability and linear responsivity. Pang et al. report a CsPbBr3 perovskite single crystal X-ray detector for edge extraction imaging with a data compression ratio of 46.4% and classification task with an accuracy of 100%.
- Jincong Pang
- , Haodi Wu
- & Guangda Niu
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Article
| Open AccessSEMORE: SEgmentation and MORphological fingErprinting by machine learning automates super-resolution data analysis
There is a lack of universal tools to analyse protein assemblies and quantify underlying structures in single-molecule localization microscopy. Here, the authors present SEMORE, a semi-automatic machine learning framework for system- and input-dependent analysis of super-resolution data.
- Steen W. B. Bender
- , Marcus W. Dreisler
- & Nikos S. Hatzakis
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Article
| Open AccessAll-in-one, all-optical logic gates using liquid metal plasmon nonlinearity
Multifunctional all-optical logic gate (AOLG) with broadband-based massively parallel processing is desirable for high-speed optical processor. Here, authors propose a reconfigurable all-in-one ultra-broadband AOLG with experimentally achieving 9 fundamental Boolean logics in a single configuration.
- Jinlong Xu
- , Chi Zhang
- & Lin Zhou
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Article
| Open AccessEnergy transfer driven brightening of MoS2 by ultrafast polariton relaxation in microcavity MoS2/hBN/WS2 heterostructures
Here, the authors design a microcavity-confined 2D heterojunction to realize the strong coupling among donor exciton, acceptor exciton, and cavity photon mode, leading to an unconventional energy transfer via polariton relaxation with an enhancement factor of ~440.
- Zehua Hu
- , Tanjung Krisnanda
- & Qihua Xiong
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Article
| Open AccessBroadband thermal imaging using meta-optics
Exploring the miniaturization of imaging systems, researchers use inverse-design for broadband meta-optics in the LWIR spectrum. Here, authors achieve a six-fold Strehl ratio improvement in image quality over conventional metalenses using a novel design and computational techniques.
- Luocheng Huang
- , Zheyi Han
- & Arka Majumdar
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Article
| Open AccessStrong interactions between solitons and background light in Brillouin-Kerr microcombs
Here the authors demonstrate a strong interaction between the generated solitons and background light in a Brillouin-Kerr microcomb system. Based on this unique physical mechanism, they achieve a monostable single soliton microcomb and a turnkey single-soliton microcomb without employing any optical/electrical control or feedback.
- Menghua Zhang
- , Shulin Ding
- & Xiaoshun Jiang