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| Open AccessE-cardiac patch to sense and repair infarcted myocardium
Infarted myocardium hampers the synchronous electroactivity of the cardiac tissue. Here, the authors showcase a battery-free conductive cardiac patch made of reduced graphene and its therapeutic efficacy for cardiac repair.
- Renjie Qiu
- , Xingying Zhang
- & Leyu Wang
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Article
| Open AccessExperimental demonstration of an on-chip p-bit core based on stochastic magnetic tunnel junctions and 2D MoS2 transistors
Probabilistic bits (p-bits) are the base units of probabilistic computing, a computing scheme offering a more efficient approach than conventional binary logic in various applications. Here, the authors report the realization of a p-bit core device by combining stochastic magnetic tunnel junctions and 2D MoS2 transistors on the same chip.
- John Daniel
- , Zheng Sun
- & Joerg Appenzeller
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Article
| Open AccessMolecular fingerprinting of biological nanoparticles with a label-free optofluidic platform
Biosensing tools to detect multiple analytes in a high-throughput manner are still hindered by many limitations. Here, the authors present a label-free optofluidic platform integrating digital holography and microfluidics for analyte detection, allowing for the fingerprinting of heterogenous biological samples.
- Alexia Stollmann
- , Jose Garcia-Guirado
- & Romain Quidant
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Article
| Open AccessUltrastrong magnon-magnon coupling and chiral spin-texture control in a dipolar 3D multilayered artificial spin-vortex ice
Extending magnetic nanostructures into three dimensions offers a vast increase in potential functionalities, but this typically comes at the expense of ease of fabrication and measurement. Here, Dion et al. demonstrate an approach to creating three dimensional magnetic nanostructures while retaining easy fabrication and readout of established two dimensional approaches.
- Troy Dion
- , Kilian D. Stenning
- & Jack C. Gartside
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Article
| Open AccessSynergistic growth of nickel and platinum nanoparticles via exsolution and surface reaction
Utilizing “Chemistry at a point”, Ni is exsolved from a perovskite lattice under deposited Pt nanoparticles. This yields even smaller Ni Pt alloy nanoparticles on a perovskite nanofiber structure, exhibiting high catalytic activity.
- Min Xu
- , Yukwon Jeon
- & John T. S. Irvine
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Article
| Open AccessTuning instability in suspended monolayer 2D materials
Tuning the instabilities of 2D materials can control their wrinkling behavior for interesting physical properties, but still challenging. Here, the authors report a push-to-shear experimental approach to control the wrinkling patterns of monolayer 2D materials and measure their bending stiffness.
- Yuan Hou
- , Jingzhuo Zhou
- & Yang Lu
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Article
| Open AccessUltra-narrowband and rainbow-free mid-infrared thermal emitters enabled by a flat band design in distorted photonic lattices
Narrowband thermal emitters realized with photonic nanostructures usually suffer from the rainbow effect. Here, the authors demonstrate rainbow-free thermal emissions with high temporal coherence through harnessing flatband high-Q resonances.
- Kaili Sun
- , Yangjian Cai
- & Zhanghua Han
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Article
| Open AccessElectrochemical-repaired porous graphene membranes for precise ion-ion separation
The preparation of atom-thick lattices with Å-scale pores is desirable for achieving ion selectivity and high ion flux. Here authors present a cm-scale membrane made of atom-thick graphene film hosting zero-dimensional pores spanning only a few Å, repaired using an in situ electrochemical strategy, yielding high Li+/Mg2+ separation performance.
- Zongyao Zhou
- , Kangning Zhao
- & Kumar Varoon Agrawal
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Article
| Open AccessCavity-enhanced photon indistinguishability at room temperature and telecom wavelengths
Carbon nanotube-based single photon emitters allow for room-temperature operation, but suffer from vanishing indistinguishability due to strong dephasing. Following a theoretical proposal, the authors tackle the problem experimentally by using a cavity to enhance the photon coherence time and the emission spectral density in the regime of incoherent good cavity-coupling.
- Lukas Husel
- , Julian Trapp
- & Alexander Högele
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Article
| Open AccessFirefly-inspired bipolar information indication system actuated by white light
Inspired by fireflies, a bimodal information indication system using a photochemical afterglow material within a photonic crystal matrix is developed to display both static and changing information, such as sample type and degree of degradation.
- Hanwen Huang
- , Jiamiao Yin
- & Changchun Wang
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Article
| Open AccessHalide Perovskite Inducing Anomalous Nonvolatile Polarization in Poly(vinylidene fluoride)-based Flexible Nanocomposites
Wang et al. report large nonvolatile polarization in stretchable polymer ferroelectrics incorporating perovskite nanocrystals. The built-in electric field from poled ferroelectrics stabilises Frenkel defects via interfacial coupling, which can also enhance the polarization of nonferroelectrics.
- Yao Wang
- , Chen Huang
- & Jiangyu Li
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Article
| Open AccessSingle-photon detection using large-scale high-temperature MgB2 sensors at 20 K
Superconducting nanowire single-photon detectors require operation at T < 4 K, and successful attempts to extend their operation at 20 K and above using high-TC BSCCO flakes come at the cost of lower scalability to large areas. Here, the authors break this trade-off by using high-quality MgB2 films and exploiting a helium-ion beam-based irradiation process.
- Ilya Charaev
- , Emma K. Batson
- & Karl K. Berggren
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Matters Arising
| Open AccessTechnical challenges of studying the impact of plasma components on the efficacy of lipid nanoparticles for vaccine and therapeutic applications
- Jens B. Simonsen
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Article
| Open AccessBicontinuous RuO2 nanoreactors for acidic water oxidation
Developing stable water oxidation catalysts is of great importance for proton-exchange membrane water electrolyzers. Here the authors report a bicontinuous nanoreactor composed of multiscale defected RuO2 nanocrystals for robust acidic water oxidation reactivity.
- Ding Chen
- , Ruohan Yu
- & Shichun Mu
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Article
| Open AccessImplication of thermal signaling in neuronal differentiation revealed by manipulation and measurement of intracellular temperature
The role of subcellular thermogenesis during neuronal differentiation remains poorly understood. Here, the authors employ methods to monitor local intracellular temperature, and they investigate the effects of non-invasive temperature changes on cell differentiation using neuron-like cells.
- Shunsuke Chuma
- , Kazuyuki Kiyosue
- & Yoshie Harada
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Article
| Open AccessCorrelating activities and defects in (photo)electrocatalysts using in-situ multi-modal microscopic imaging
Physicochemical heterogeneity poses a significant constraint in photocatalyst advancement. Here the authors introduce a multimodal optical microscopy platform to assess activity and defects concurrently in photoelectrocatalysts, revealing that disorder can unexpectedly enhance local photoelectrocatalytic performance in certain instances.
- Camilo A. Mesa
- , Michael Sachs
- & Raj Pandya
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Article
| Open AccessSelf-assembly of nanocrystal checkerboard patterns via non-specific interactions
The self-assembly of nanocrystals into checkerboard lattice patterns is difficult to control. Here, the authors investigate the formation of such patterns from hydrophilic/hydrophobic bifunctionalized Ag nanocubes and use multiscale simulations to understand the effects of physical forces.
- Yufei Wang
- , Yilong Zhou
- & Andrea R. Tao
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Article
| Open AccessEffect of crystal facets in plasmonic catalysis
Crystal facets are known to be important in traditional heterogeneous catalysis, yet this effect has not been studied in plasmon-assisted catalysis. Here, the authors investigate the impact facets have on CO2 reduction using plasmonic Au NPs.
- Yicui Kang
- , Simão M. João
- & Emiliano Cortés
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Review Article
| Open AccessCritical learning from industrial catalysis for nanocatalytic medicine
The knowledge gained from industrial catalysis benefits advancements of nanocatalytic medicines. Here the authors review the similarities, differences and connections in catalytic reactions between industrial and medical applications to support deep understanding and rational design of nanocatalytic medicines.
- Zhaokui Jin
- , Lingdong Jiang
- & Qianjun He
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Article
| Open AccessCapture of single Ag atoms through high-temperature-induced crystal plane reconstruction
Terminal hydroxyl groups on γ-Al2O3 surfaces serve as anchoring sites for Ag. Based on the surface energy of different crystal planes of γ-Al2O3 at various temperatures, the authors propose a high-temperature-induced crystal plane transformation method to construct terminal hydroxyl anchoring sites.
- Jiaxin Li
- , Kai Li
- & Hong He
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Article
| Open AccessUniversal Murray’s law for optimised fluid transport in synthetic structures
Improving mass transfer through hierarchically porous synthetic materials is a great challenge. Here the authors address this by expanding the original Murray’s law, a biomimetic principle defining the branching of veins in living structures.
- Binghan Zhou
- , Qian Cheng
- & Tawfique Hasan
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Article
| Open AccessA fast-charging/discharging and long-term stable artificial electrode enabled by space charge storage mechanism
Lithium-ion batteries with fast-charging properties are urgently needed for wide adoption of electric vehicles. Here, the authors show a fast charging/discharging and long-term stable electrode made from a mixed electronic/ionic conductor material enabled by a space charge mechanism.
- Linyi Zhao
- , Tiansheng Wang
- & Guihua Yu
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Article
| Open AccessSynthetic molecular switches driven by DNA-modifying enzymes
Molecular switches are ubiquitous in the biochemistry regulatory network. Here, the authors construct synthetic molecular switches controlled by DNA-modifying enzymes such as DNA polymerase and nicking endonuclease to control and cascade assembly and disassembly.
- Hong Kang
- , Yuexuan Yang
- & Bryan Wei
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Article
| Open AccessMulti-site integrated optical addressing of trapped ions
A promising strategy for scaling trapped-ion-based quantum technologies is to use fully integrated optical waveguides to deliver light to numerous ions at multiple sites. Here, the authors. optically address three ions using on-chip waveguides to deliver three distinct wavelengths per ion, and perform Rabi flopping on each ion simultaneously.
- Joonhyuk Kwon
- , William J. Setzer
- & Hayden J. McGuinness
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Article
| Open AccessTunneling current-controlled spin states in few-layer van der Waals magnets
Magnetic tunnel junctions consist of two magnetic layers, separated by a thin insulator. The simplicity belies the industrial importance: magnetic tunnel junctions have a very wide variety of applications in contemporary society. Here, Fu et al present a magnetic tunnel junction composed of single van der Waals magnetic insulator, CrI3, exhibiting remarkably low power consumption.
- ZhuangEn Fu
- , Piumi I. Samarawickrama
- & Jifa Tian
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Article
| Open AccessAn artificial visual neuron with multiplexed rate and time-to-first-spike coding
Multiplexed spiking data coding schemes could enable artificial visual neurons to emulate the human visual system in a more biologically plausible way. Here, Li et al. present an artificial neuron device capable of encoding visual analog signals into spike trains using multiplexed rate and temporal fusion coding. Reviewer recognition:
- Fanfan Li
- , Dingwei Li
- & Bowen Zhu
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Article
| Open AccessBiocomposite thermoplastic polyurethanes containing evolved bacterial spores as living fillers to facilitate polymer disintegration
Plastic pollution severely threatens the resilience of nature. Here, the authors utilize the spore-forming, polymer-degrading bacteria, Bacillus subtilis, as a living filler to develop biocomposite thermoplastic polyurethane with improved mechanical properties and biodegradation.
- Han Sol Kim
- , Myung Hyun Noh
- & Jonathan K. Pokorski
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Article
| Open AccessIntegrated 2D multi-fin field-effect transistors
Here, the authors report the ledge-guided epitaxial growth of high-density 2D Bi2O2Se fin arrays and their application for the realization of 2D multi-channel fin field-effect transistors, showing improved on-state currents as the number of integrated channels is increased.
- Mengshi Yu
- , Congwei Tan
- & Hailin Peng
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Article
| Open AccessIn situ enzymatic control of colloidal phoresis and catalysis through hydrolysis of ATP
The design of synthetic systems that can sense chemical gradients and respond with directional motility and chemical activity is of interest. Here, the authors realize and control such behaviors in a synthetic system by tailoring multivalent interactions of adenosine nucleotides with catalytic microbeads.
- Ekta Shandilya
- , Bhargav Rallabandi
- & Subhabrata Maiti
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Article
| Open AccessAll-natural 2D nanofluidics as highly-efficient osmotic energy generators
Researchers report a sustainable nanofluidic osmotic energy harvester made from natural montmorillonite clay nanosheets and recycled cellulose. Scaled-up films of 700 cm2 show power output of 8 W m−2 with stability over 30 days
- Jiadong Tang
- , Yun Wang
- & Tieyong Zuo
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Article
| Open AccessRoom-temperature low-threshold avalanche effect in stepwise van-der-Waals homojunction photodiodes
The avalanche or carrier-multiplication effect has the potential to improve the performance of photodetectors and solar cells, but usually requires high threshold energies. Here, the authors report stepwise WSe2 homojunctions exhibiting threshold energies approaching the semiconductor bandgap at room temperature.
- Hailu Wang
- , Hui Xia
- & Wei Lu
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Article
| Open AccessRevealing hidden spin polarization in centrosymmetric van der Waals materials on ultrafast timescales
A major challenge for spin-based information technologies is the generation of spin polarization in otherwise nonmagnetic materials. Here, Arnoldi et al. demonstrate how ultrafast laser excitations can be used to generate spin polarization in a fullerene/tungsten diselenide heterostructure.
- B. Arnoldi
- , S. L. Zachritz
- & B. Stadtmüller
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Article
| Open AccessStaggered structural dynamic-mediated selective adsorption of H2O/D2O on flexible graphene oxide nanosheets
Graphene oxide is a promising material for molecular separation technologies. Here, the authors propose a realistic staggered stacking structure that plays a crucial role in H/D recognition in water adsorption, as well as high mobilities of water.
- Ryusuke Futamura
- , Taku Iiyama
- & Katsumi Kaneko
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Article
| Open AccessImaging 3D chemistry at 1 nm resolution with fused multi-modal electron tomography
The authors demonstrate 3D chemical imaging of organic and inorganic materials near or below one-nanometer resolution using multi-modal electron tomography, by fusing elastic and inelastic scattering signals.
- Jonathan Schwartz
- , Zichao Wendy Di
- & Robert Hovden
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Article
| Open AccessMulti-level, forming and filament free, bulk switching trilayer RRAM for neuromorphic computing at the edge
Filamentary RRAM technologies suffer from variations and noise, leading to computational accuracy loss, and increased energy consumption. Park et al. created a trilayer metal-oxide bulk switching RRAM technology without filament formation and showed edge computing for an autonomous navigation task.
- Jaeseoung Park
- , Ashwani Kumar
- & Duygu Kuzum
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Article
| Open AccessSweat permeable and ultrahigh strength 3D PVDF piezoelectric nanoyarn fabric strain sensor
Electronic packaging causes piezoelectric sensors to be airtight, resulting in poor wearing comfort. To address this issue, the authors develop a 3D all-fiber piezoelectric sensor with sweat permeable using the advanced 3D textile technology.
- Wei Fan
- , Ruixin Lei
- & Shengbo Ge
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Article
| Open AccessEnergy-efficient superparamagnetic Ising machine and its application to traveling salesman problems
Ising machines are promising for solving NP-hard problems, but current implementations have power consumption and scalability challenges. Si et al. implement an Ising machine consisting of 80 superparamagnetic tunnel junctions with all-to-all connections and apply it to a large-scale travelling salesman problem.
- Jia Si
- , Shuhan Yang
- & Hyunsoo Yang
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Article
| Open AccessFunctionalized MXene ink enables environmentally stable printed electronics
Here, authors demonstrate the electrohydrodynamic printing of alkylated 3,4-dihydroxy-L-phenylalanine functionalized MXene (AD-MXene) ink. The AD-MXene outperforms vacuum-deposited Au and Al electrodes, providing thin film transistors with good environmental stability due to its hydrophobicity.
- Tae Yun Ko
- , Heqing Ye
- & Insik In
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Article
| Open AccessCorrelation between two distant quasiparticles in separate superconducting islands mediated by a single spin
The authors experimentally study a chain of superconducting islands (SI) and quantum dots (QD), where a Bogoliubov quasiparticle occupies each SI. They demonstrate correlations between the quasiparticles in each SI mediated by a single spin on the QD, known as an “over-screened" doublet state of the QD.
- Juan Carlos Estrada Saldaña
- , Alexandros Vekris
- & Jesper Nygård
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Article
| Open AccessTransparent integrated pyroelectric-photovoltaic structure for photo-thermo hybrid power generation
The full potential of photoelectric devices can possibly be maximized through pyroelectricity for power generation beyond thermodynamic limit. Here, authors report photovoltaic heterostructure device with pyroelectric absorber, achieving 2.5 times more output power due to long-range electric field.
- Malkeshkumar Patel
- , Hyeong-Ho Park
- & Joondong Kim
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Article
| Open AccessExosome-coated oxygen nanobubble-laden hydrogel augments intracellular delivery of exosomes for enhanced wound healing
Challenges including hypoxia, inflammation, and inadequate exosome intracellular delivery hinder wound healing. Here, the authors show that a multifunctional exosome-coated oxygen nanobubble-laden hydrogel enhances exosome delivery and mitigates hypoxia for enhanced wound healing.
- Xiaoxue Han
- , Chaimongkol Saengow
- & Joseph Irudayaraj
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Article
| Open AccessAutonomous self-healing supramolecular polymer transistors for skin electronics
Integrating self-healing capabilities into skin-like stretchable transistors presents a persistent challenge. Here, by using a supramolecular polymer matrix, the authors develop autonomous self-healing transistors and skin-like logic circuits.
- Ngoc Thanh Phuong Vo
- , Tae Uk Nam
- & Jin Young Oh
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Article
| Open AccessHighly defective ultra-small tetravalent MOF nanocrystals
Crystalline materials’ properties are highly dependent on their size. Here authors report a general synthesis of ultrasmall (4–6 nm) and highly defective Zr/Hf-Metal Organic Frameworks nanoparticles that present enhanced peptide hydrolysis performance.
- Shan Dai
- , Charlotte Simms
- & Christian Serre
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Article
| Open AccessAn ultra energy-efficient hardware platform for neuromorphic computing enabled by 2D-TMD tunnel-FETs
The most successful commercial implementations of neuromorphic computing circuits are limited to digital-CMOS-circuit based approaches to date. Along this line, Pal et al. improve the energy efficiency by two orders of magnitude using two-dimensional layered material-based tunnel-field-effect transistors.
- Arnab Pal
- , Zichun Chai
- & Kaustav Banerjee
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Article
| Open AccessInkjet-printed optical interference filters
Optical interference filters are multilayer structures for controlling the propagation of electromagnetic waves. Jin et al. have developed a method of via inkjet printing to fabricate optical interference filters with commercially relevant quality with remarkable A4 paper size (29.7 × 21.0 cm²) in ambient conditions.
- Qihao Jin
- , Qiaoshuang Zhang
- & Uli Lemmer
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Article
| Open AccessHigh-throughput quantum photonic devices emitting indistinguishable photons in the telecom C-band
An efficient way of realising a large number of telecom single-photon emitters for quantum communication is still missing. Here, the authors use a wide-field imaging technique for fast localization of single InAs/InP quantum dots, which are then integrated into circular Bragg grating cavities featuring high single-photon purity and indistinguishability.
- Paweł Holewa
- , Daniel A. Vajner
- & Elizaveta Semenova
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Article
| Open AccessMechanoelectronic stimulation of autologous extracellular vesicle biosynthesis implant for gut microbiota modulation
Pathogenic gut microbiota is responsible for a few debilitating gastrointestinal Diseases. Here, the authors develop a wireless mechanoelectronic device designed to manufacture of functional vesicles in vivo to regulate microbiome.
- Shuangshuang Wan
- , Kepeng Wang
- & Lianhui Wang
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Article
| Open AccessA CMOS-compatible oscillation-based VO2 Ising machine solver
Oscillating neural networks promise ultralow power consumption and rapid computation for tackling complex optimization problems. Here, the authors demonstrate VO2 oscillators to solve NP-complete problems with projected power consumption of 13 µW/oscillator.
- Olivier Maher
- , Manuel Jiménez
- & Siegfried Karg
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Article
| Open AccessExciton polariton condensation from bound states in the continuum at room temperature
Bound states in continuum have attracted attention in various platforms, and recently condensation of bound states in continuum polariton modes was demonstrated at low temperatures. Here the authors report the observation of such a state in a periodic air-hole perovskite-based photonic crystal at room temperature.
- Xianxin Wu
- , Shuai Zhang
- & Xinfeng Liu