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News & Views |
Quantum optics meets attosecond science
Generating high harmonics or attosecond pulses of light is normally thought of as a classical process, but a theoretical study has now shown how the process could be driven by quantum light.
- Dong Hyuk Ko
- & P. B. Corkum
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Article |
High-harmonic generation driven by quantum light
High-harmonic generation is a source of high-frequency radiation and is typically driven by strong, but classical, laser fields. A theoretical study now shows that using quantum light states as the driver extends the spectrum of outgoing radiation in a controllable manner.
- Alexey Gorlach
- , Matan Even Tzur
- & Ido Kaminer
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News & Views |
Quantum correlated atoms in intense laser fields
Strongly laser-driven quantum correlated many-body systems lead to the generation of light with exotic quantum features — the quantumness of a many-body system is imprinted on the state of the emitted light.
- Paraskevas Tzallas
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Article |
Light emission from strongly driven many-body systems
Strongly driven light sources have become useful in many ways but are limited to classical emission. A quantum-optical theory now shows how non-classical states of light can be achieved from strongly-driven many-body systems, for example, non-coherent and correlated high-harmonic generation.
- Andrea Pizzi
- , Alexey Gorlach
- & Ido Kaminer
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Article |
Attosecond circular-dichroism chronoscopy of electron vortices
Attosecond circular-dichroism chronoscopy—a spectroscopy technique that employs two circularly polarized pulses in co-rotating and counter-rotating geometries—can measure the amplitudes and phases of continuum–continuum transitions in electron vortices.
- Meng Han
- , Jia-Bao Ji
- & Hans Jakob Wörner
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News & Views |
Harmonic generation in confinement
Quantum confinement effects offer a more comprehensive understanding of the fundamental processes that drive extreme optical nonlinearities in nano-engineered solids, opening a route to unlocking the potential of high-order harmonic generation.
- Julien Madéo
- & Keshav M. Dani
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Letter |
Size-controlled quantum dots reveal the impact of intraband transitions on high-order harmonic generation in solids
Both inter- and intraband transitions contribute to high-harmonic generation in solids, but their exact roles are not fully understood. Experiments with quantum dots show that enhanced intraband transitions lead to increased carrier injection and thus enhanced harmonic generation.
- Kotaro Nakagawa
- , Hideki Hirori
- & Yoshihiko Kanemitsu
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News & Views |
A light imprint
In a study on high-harmonic generation from a dense atomic xenon gas, the strong-field light–matter interaction is shown to leave a quantum mechanical imprint on the incident light that escapes the semiclassical picture of strong-field physics.
- Thomas Fennel
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Letter |
Generation of optical Schrödinger cat states in intense laser–matter interactions
Schrödinger cat states are observed in intense laser–atom interactions. These are a superposition of the initial state of the laser and the coherent state that results from the interaction between the light and atoms.
- M. Lewenstein
- , M. F. Ciappina
- & P. Tzallas
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News & Views |
Reflections off a relativistic mirror
High-order harmonics of laser pulses yield spectral components with shorter wavelength and duration and tighter focus than the original pulse. Precise spatiotemporal characterization of this radiation from a relativistic plasma mirror is relevant for ultrafast science.
- Laszlo Veisz
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Article |
Spatio-temporal characterization of attosecond pulses from plasma mirrors
Relativistic mirrors are a promising tool to reach laser intensities up to the Schwinger limit. Such a mirror is created in ultra-intense laser–solid interactions, and its temporal and spatial effects on the reflected laser beam are characterized.
- Ludovic Chopineau
- , Adrien Denoeud
- & Fabien Quéré
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Letter |
High-harmonic generation from topological surface states
High-harmonic generation up to the seventh harmonic is observed from the intrinsic three-dimensional topological insulator BiSbTeSe2. The parallel components of the even-order harmonics arise directly from the topological surface states.
- Ya Bai
- , Fucong Fei
- & Peng Liu
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Letter |
Origin of strong-field-induced low-order harmonic generation in amorphous quartz
Strong-field-induced nonlinearities from the injection of electrons into the conduction band contribute to harmonic generation in amorphous quartz. Close to the damage threshold, they dominate over intraband and interband contributions.
- P. Jürgens
- , B. Liewehr
- & A. Mermillod-Blondin
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Letter |
High-harmonic generation from an epsilon-near-zero material
High harmonics are generated from a thin film by leveraging the epsilon-near-zero effect. These kinds of harmonic are found to exhibit a pronounced spectral redshift as well as linewidth broadening caused by the time-dependency of this effect.
- Yuanmu Yang
- , Jian Lu
- & Igal Brener
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Review Article |
High-harmonic generation from solids
This Review surveys recent efforts at understanding and characterizing generation of high harmonics from solid-state materials.
- Shambhu Ghimire
- & David A. Reis
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Letter |
Enhanced high-harmonic generation from an all-dielectric metasurface
The demonstration of substantially enhanced high-harmonic emission from a silicon metasurface suggests a route towards novel photonic devices based on a combination of ultrafast strong-field physics and nanofabrication technology.
- Hanzhe Liu
- , Cheng Guo
- & David A. Reis
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Letter |
Diffraction and microscopy with attosecond electron pulse trains
Attosecond light pulses are used to probe ultrafast processes. The experimental observation of attosecond electron pulses now promises the marriage of these techniques with electron microscopy and diffraction.
- Yuya Morimoto
- & Peter Baum
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Article |
Probing electronic binding potentials with attosecond photoelectron wavepackets
Measurements of the electron wavepackets produced by photoionizing noble gas atoms with an XUV harmonic comb enable the reconstruction of the effective binding potential: a new technique that could be extended to molecules.
- D. Kiesewetter
- , R. R. Jones
- & L. F. DiMauro
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Letter |
Tracing the phase of focused broadband laser pulses
In different applications the Gouy phase is used to describe broadband lasers, but new 3D measurements of the spatial dependence of a focused laser pulse show serious deviations from the Gouy phase.
- Dominik Hoff
- , Michael Krüger
- & Peter Hommelhoff
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News & Views |
A twist in coherent X-rays
Light beams with controllable orbital angular momentum can be generated in the extreme-ultraviolet or soft-X-ray regime, pushing the application of twisted light to the nanoscale.
- Carlos Hernández-García
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Letter |
Plasmon-enhanced high-harmonic generation from silicon
High-harmonic emission from crystalline silicon can be made ten times brighter by exploiting local plasmonic fields in arrays of nano-antennas.
- G. Vampa
- , B. G. Ghamsari
- & P. B. Corkum
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Article |
State-resolved attosecond reversible and irreversible dynamics in strong optical fields
An experimental and theoretical study of the real-time dynamics in strong-field ionization of xenon atoms reveals the previously unknown role of transient ground-state polarization.
- Mazyar Sabbar
- , Henry Timmers
- & Stephen R. Leone
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Letter |
Anisotropic high-harmonic generation in bulk crystals
High-harmonic generation in a solid turns out to be sensitive to the interatomic bonding — a very useful feature that could enable the all-optical imaging of the interatomic potential.
- Yong Sing You
- , David A. Reis
- & Shambhu Ghimire
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Letter |
High-harmonic generation from an atomically thin semiconductor
Observations of high-harmonic generation from a single layer of a transition metal dichalcogenide opens the door to studying strong-field and attosecond phenomena in two-dimensional materials.
- Hanzhe Liu
- , Yilei Li
- & David A. Reis
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Letter |
Rotational Doppler effect in nonlinear optics
The change in pitch of a passing car engine is a classic example of the translational Doppler effect, but rotational Doppler shifts can also arise, as shown for circularly polarized light passing through a spinning nonlinear optical crystal.
- Guixin Li
- , Thomas Zentgraf
- & Shuang Zhang
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Letter |
Ptychographic measurements of ultrahigh-intensity laser–plasma interactions
Experimentally probing the dynamics of laser–plasma interactions is hard, owing to the nature of the relevant temporal and spatial scales at play. Ptychography, a phase-problem solving technique, can help the analysis of such interaction measurements.
- A. Leblanc
- , S. Monchocé
- & F. Quéré
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Letter |
Attosecond tunnelling interferometry
An interferometric measurement based on high-harmonic generation now provides direct access to the electron wavefunction during field-induced tunnelling.
- O. Pedatzur
- , G. Orenstein
- & N. Dudovich
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News & Views |
Drive round the twist
Light has long been used to detect the chirality of molecules but high-order harmonic generation now provides access to these chiral interactions on ultrafast timescales.
- Minhaeng Cho
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Letter |
Probing molecular chirality on a sub-femtosecond timescale
Molecules that are mirror images of each other usually behave identically, unless they are interacting with other chiral objects. High-harmonic generation can provide access to the dynamics of chiral interactions on ultrafast timescales.
- R. Cireasa
- , A. E. Boguslavskiy
- & V. R. Bhardwaj
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News & Views |
To the extreme
High-harmonic spectroscopy is a powerful tool for probing the electronic structure of atoms and molecules in gases. Experiments now show that similar emission from solids has a different origin.
- Giulio Vampa
- & David M. Villeneuve