Article abstract


Nature Physics 5, 515 - 520 (2009)
Published online: 31 May 2009 | Corrected online: 16 June 2009 | doi:10.1038/nphys1285

Subject Categories: Optical physics | Materials physics

Coherent ultrafast magnetism induced by femtosecond laser pulses

Jean-Yves Bigot, Mircea Vomir & Eric Beaurepaire


The quest for ultrafast magnetic processes has triggered a new field of research—femtomagnetism: using femtosecond laser pulses to demagnetize ferromagnetic metallic thin films. Despite being the subject of intense research for over a decade, the underlying mechanisms that govern the demagnetization remain unclear. Here, we investigate how an ultrashort laser pulse couples to the spin of electrons in ferromagnetic metals. It is shown that a single 50-fs laser pulse couples efficiently to a ferromagnetic film during its own propagation. This result indicates that the material polarization induced by the photon field interacts coherently with the spins. The corresponding mechanism has its origin in relativistic quantum electrodynamics, beyond the spin–orbit interaction involving the ionic potential. In addition, this coherent interaction is clearly distinguished from the incoherent ultrafast demagnetization associated with the thermalization of the spins. We forecast that the corresponding coherent self-induced processes are the dawn of a new era for future research in magnetism.

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  1. Institut de Physique et Chimie des Matériaux de Strasbourg, UMR 7504, CNRS, Université de Strasbourg, BP 43, 23 rue du Loess, 67034 Strasbourg Cedex 02, France

Correspondence to: Jean-Yves Bigot e-mail: bigot@ipcms.u-strasbg.fr

* In the version of this article originally published online, corrections were needed to: Fig. 1, right-hand Gel label should read Gsl; Fig. 2b,c, the 0 label on the x axes should read 1; Fig. 3a,c, the legend for the red line should read 0°. These corrections have now been made in all versions of the article.

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