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Microrheology of a sticking transition

Abstract

The phenomenon of sticking of one object to another, which drastically reduces their relative motion, is ubiquitous in nature. We have studied the sticking process of a colloid, suspended in a fluid medium by an optical tweezer, to a rigid substrate. The evolution of the frictional coupling between the two as a function of their separation is detected by the diffusivity of the particle and also by its phase-sensitive response to an in-plane external oscillatory drive applied to the substrate. On contact, the coupling changes abruptly from viscous to elastic for a rigid silica particle, whereas it evolves slowly with time, similar to ageing in glassy systems, for a soft and deformable polystyrene particle. Depending on the relative strengths of the particle–substrate interaction, the tweezer potential and the external drive, three regimes of dynamics—stuck, ageing and non-stuck—are observed in the dynamical phase diagram.

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Figure 1: Variation of MSD for the sticking transition.
Figure 2: Response of the trapped particle to an external oscillatory drive applied to the substrate.
Figure 3: Microrheological quantities in the ageing regime.
Figure 4: Rheological characterization of the stuck and non-stuck regimes.
Figure 5: Dynamical phase diagram of sticking.
Figure 6: Memory effect.

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Acknowledgements

We thank P. Chaikin, D. Dhar, D. Grier, M. W. Kim, S. Nagel, D. Pine and G. V. Shivashankar for helpful discussions.

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Correspondence to Shankar Ghosh.

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Sharma, P., Ghosh, S. & Bhattacharya, S. Microrheology of a sticking transition. Nature Phys 4, 960–966 (2008). https://doi.org/10.1038/nphys1105

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