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Letters to Nature

Nature 430, 650-654 (5 August 2004) | doi:10.1038/nature02774; Received 18 March 2004; Accepted 22 June 2004

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Two-dimensional geometry of spin excitations in the high-transition-temperature superconductor YBa2Cu3O6+x

V. Hinkov1, S. Pailhès2, P. Bourges2, Y. Sidis2, A. Ivanov3, A. Kulakov1, C. T. Lin1, D. P. Chen1, C. Bernhard1 & B. Keimer1

  1. Max-Planck-Institut für Festkörperforschung, 70569 Stuttgart, Germany
  2. Laboratoire Léon Brillouin, CEA-CNRS, CE-Saclay, 91191 Gif-sur-Yvette, France
  3. Institut Laue-Langevin, 156X, 38042 Grenoble cedex 9, France

Correspondence to: B. Keimer1 Email: b.keimer@fkf.mpg.de

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The fundamental building block of the copper oxide superconductors is a Cu4O4 square plaquette. The plaquettes in most of these materials are slightly distorted to form a rectangular lattice, for which an influential theory predicts that high-transition-temperature (high-Tc) superconductivity is nucleated in 'stripes' aligned along one of the axes1, 2, 3. This theory received strong support from experiments that indicated a one-dimensional character for the magnetic excitations in the high-Tc material YBa2Cu3O6.6 (ref. 4). Here we report neutron scattering data on 'untwinned' YBa2Cu3O6+x crystals, in which the orientation of the rectangular lattice is maintained throughout the entire volume. Contrary to the earlier claim4, we demonstrate that the geometry of the magnetic fluctuations is two-dimensional. Rigid stripe arrays therefore appear to be ruled out over a wide range of doping levels in YBa2Cu3O6+x, but the data may be consistent with liquid-crystalline stripe order5. The debate about stripes has therefore been reopened.

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