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Letters to Nature

Nature 414, 731-735 (13 December 2001) | doi:10.1038/414731a; Received 12 June 2001; Accepted 8 October 2001

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High-temperature ultrafast polariton parametric amplification in semiconductor microcavities

M. Saba1, C. Ciuti1, J. Bloch2, V. Thierry-Mieg2, R. André3, Le Si Dang3, S. Kundermann1, A. Mura4, G. Bongiovanni4, J. L. Staehli1 & B. Deveaud1

  1. Physics Department, Swiss Federal Institute of Technology Lausanne, PH-Ecublens, CH-1015 Lausanne-EPFL, Switzerland
  2. Centre National de la Recherche Scientifique, L2M-CNRS, 92225 Bagneux Cedex, France
  3. Laboratoire de Spectrometrie Physique, Université J. Fourier-Grenoble, F-38402 Saint Martin d'Hères Cedex, France
  4. Dipartimento di Fisica and Istituto Nazionale di Fisica della Materia, Università degli Studi di Cagliari, I-09042 Monserrato, Italy

Correspondence to: M. Saba1 Correspondence and requests for materials should be addressed to M.S. (e-mail: Email: Michele.Saba@epfl.ch).

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Cavity polaritons, the elementary optical excitations of semiconductor microcavities, may be understood as a superposition of excitons and cavity photons1. Owing to their composite nature, these bosonic particles have a distinct optical response, at the same time very fast and highly nonlinear. Very efficient light amplification due to polariton–polariton parametric scattering has recently been reported in semiconductor microcavities at liquid-helium temperatures2, 3, 4, 5, 6, 7, 8, 9, 10, 11. Here we demonstrate polariton parametric amplification up to 120 K in GaAlAs-based microcavities and up to 220 K in CdTe-based microcavities. We show that the cut-off temperature for the amplification is ultimately determined by the binding energy of the exciton. A 5-microm-thick planar microcavity can amplify a weak light pulse more than 5,000 times. The effective gain coefficient of an equivalent homogeneous medium would be 107 cm-1. The subpicosecond duration and high efficiency of the amplification could be exploited for high-repetition all-optical microscopic switches and amplifiers. 105 polaritons occupy the same quantum state during the amplification, realizing a dynamical condensate of strongly interacting bosons which can be studied at high temperature.