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| Open AccessStructural-disorder-driven critical quantum fluctuation and localization in two-dimensional semiconductors
The microscopic mechanism of the metal-insulator transition in 2D disordered semiconductors is not fully understood. Shin et al. propose a universal mechanism due to curvature-induced band gap fluctuations in a structurally disordered system, based on gate-tunable scanning tunneling microscopy on monolayer MoS2.
- Bong Gyu Shin
- , Ji-Hoon Park
- & Soon Jung Jung
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Article
| Open AccessSolution-grown BiI/BiI3 van der Waals heterostructures for sensitive X-ray detection
Many of the most sensitive X-ray detectors are based on toxic elements such as lead, limiting their safe applications. Here, the authors report the realization of sensitive X-ray detectors based on solution-grown thick BiI/BiI3/BiI van der Waals heterostructures, showing a detection limit down to 34 nGy s−1 and high stability.
- Renzhong Zhuang
- , Songhua Cai
- & Shenghuang Lin
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Article
| Open AccessGiant piezoresistivity in a van der Waals material induced by intralayer atomic motions
Lattice shrinkage is a dominating factor for the strain-induced change of the electronic properties in vdW layered materials. Here, the authors discover a piezoresistivity in pressurized β′-In2Se3, which originates from the intralayer atomic motions.
- Lingyun Tang
- , Zhongquan Mao
- & Changxi Zheng
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Article
| Open AccessReducing charge noise in quantum dots by using thin silicon quantum wells
Charge noise degrades the performance of spin qubits hindering scalability. Here the authors engineer the heterogeneous material stack in 28Si/SiGe gate-defined quantum dots, to improve the scattering properties and to reduce charge noise.
- Brian Paquelet Wuetz
- , Davide Degli Esposti
- & Giordano Scappucci
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Article
| Open AccessThe phonon thermal Hall angle in black phosphorus
The origin of phonon thermal Hall Effect in a variety of insulators is elusive. Here, the authors find that black phosphorus hosts the largest thermal Hall conductivity ever reported and the Hall angle does not correlate with the phonon mean-free path.
- Xiaokang Li
- , Yo Machida
- & Kamran Behnia
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Article
| Open AccessNegative-mass exciton polaritons induced by dissipative light-matter coupling in an atomically thin semiconductor
Dissipation and losses are normally perceived as detrimental to the performance of electronic and photonic devices. Here, the authors demonstrate dissipative coupling between excitons and photons in optical microcavities which they then use to create polaritons with a negative effective mass.
- M. Wurdack
- , T. Yun
- & E. Estrecho
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Article
| Open AccessQuasiparticle Andreev scattering in the ν = 1/3 fractional quantum Hall regime
Quantum transport of fractional quasiparticles can drastically differ from conventional charge transport. Here the authors demonstrate Andreev-like reflection of a fractional quasiparticle incident on a barrier in the fractional quantum Hall regime.
- P. Glidic
- , O. Maillet
- & F. Pierre
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Article
| Open AccessCoherence protection of spin qubits in hexagonal boron nitride
Spin defects in 2D hBN are promising for magnetic field sensing but suffer from short spin coherence times. Here the authors extend the coherence time for an ensemble of spins in hBN to 4 microseconds by using a continuous microwave drive and demonstrate qubit control in a protected spin space.
- Andrew J. Ramsay
- , Reza Hekmati
- & Isaac J. Luxmoore
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Article
| Open AccessEnhanced gain and detectivity of unipolar barrier solar blind avalanche photodetector via lattice and band engineering
The limited breakdown electric field and the high dark current hider the application of solar blind avalanche photodiodes. Here, Zhang et al., by lattice and band engineering, construct a unipolar barrier avalanche photodiode with suppressed dark current and reinforced reverse breakdown.
- Qingyi Zhang
- , Ning Li
- & Jianhua Hao
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Article
| Open AccessObservation of electronic modes in open cavity resonator
Electron optics draws upon the resemblance between electron and optical waves. Here, the authors report on the observation of electron mode formation in open cavity resonators realized in a GaAs/AlGaAs two-dimensional electronic gas.
- Hwanchul Jung
- , Dongsung T. Park
- & Hyung Kook Choi
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Article
| Open AccessQuantum interference between dark-excitons and zone-edged acoustic phonons in few-layer WS2
Here, the authors investigate the Raman spectra of few-layered WS2 when the excitation energy is in resonance with the dark exciton, and observe a Fano resonance between dark excitonsand zone-edge acoustic phonons.
- Qing-Hai Tan
- , Yun-Mei Li
- & Jun Zhang
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Article
| Open AccessSiGe quantum wells with oscillating Ge concentrations for quantum dot qubits
Quantum-dot spin qubits in Si/SiGe quantum wells require a large and uniform valley splitting for robust operation and scalability. Here the authors introduce and characterize a new heterostructure with periodic oscillations of Ge atoms in the quantum well, which could enhance the valley splitting.
- Thomas McJunkin
- , Benjamin Harpt
- & M. A. Eriksson
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Article
| Open AccessAtomic fluctuations lifting the energy degeneracy in Si/SiGe quantum dots
Spin qubits in Si/SiGe quantum dots suffer from variability in the valley splitting which will hinder device scalability. Here, by using 3D atomic characterization, the authors explain this variability by random Si and Ge atomic fluctuations and propose a strategy to statistically enhance the valley splitting
- Brian Paquelet Wuetz
- , Merritt P. Losert
- & Giordano Scappucci
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Article
| Open AccessWafer-scale nanofabrication of telecom single-photon emitters in silicon
The recently demonstrated approaches to fabrication of quantum emitters in silicon result in their random positioning, hindering applications in quantum photonic integrated circuits. Here the authors demonstrate controlled fabrication of telecom-wavelength quantum emitters in silicon wafers by focused ion beams.
- Michael Hollenbach
- , Nico Klingner
- & Georgy V. Astakhov
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Article
| Open AccessHigh-throughput screening of 2D van der Waals crystals with plastic deformability
It is still challenging to discover plastically deformable inorganic semiconductors. Here, the authors report a high-throughput screening of tens of potential 2D van der Waals crystals that can deform plastically accompanied with experimental verification.
- Zhiqiang Gao
- , Tian-Ran Wei
- & Xun Shi
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Article
| Open AccessHigh thermal conductivity in wafer-scale cubic silicon carbide crystals
High thermal conductivity electronic materials are critical for next-generation electronics and photonics. Here, the authors report isotropic high thermal conductivity of 3C-SiC wafers exceeding 500 W m−1K−1.
- Zhe Cheng
- , Jianbo Liang
- & David G. Cahill
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Article
| Open AccessMelting of generalized Wigner crystals in transition metal dichalcogenide heterobilayer Moiré systems
Recent experiments on a WSe2/WS2 hetero-bilayer detected incompressible charge ordered states considered to be generalized Wigner crystals. Here, by performing Monte Carlo simulations of a triangular moiré lattice, the authors study the phases which emerge on melting such charge-ordered states in partially filled moiré bands, finding two distinct nematic states and a hexagonal domain wall state.
- Michael Matty
- & Eun-Ah Kim
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Article
| Open AccessProgrammable ferroelectric bionic vision hardware with selective attention for high-precision image classification
Selective attention is an efficient processing strategy to allocate computational resources for pivotal optical information. Here, the authors propose a bionic vision hardware to emulate the behavior, showing a potential in image classification.
- Rengjian Yu
- , Lihua He
- & Huipeng Chen
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Article
| Open AccessGiant gate-controlled odd-parity magnetoresistance in one-dimensional channels with a magnetic proximity effect
Magnetoresistance, where the electric resistance of a material changes under an applied magnetic field, is typically an even function of the applied magnetic field, due to the combination of time reversal and spatial inversion symmetries. Here, Takiguchi et al show an odd-parity magnetoresistance of remarkable size in edge channels of a semiconductor quantum well.
- Kosuke Takiguchi
- , Le Duc Anh
- & Masaaki Tanaka
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| Open AccessDefect free strain relaxation of microcrystals on mesoporous patterned silicon
Many complex devices rely on epitaxial growth with high crystallinity and accurate composition. Here authors report epitaxial growth of Ge on deep etched porous Si pillars to provide a fully compliant substrate enabling elastic relaxation of defect free Ge microcrystals.
- Alexandre Heintz
- , Bouraoui Ilahi
- & Abderraouf Boucherif
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Article
| Open AccessGenerating intense electric fields in 2D materials by dual ionic gating
The application of electric fields >1 V/nm in solid state devices could provide access to unexplored phenomena, but it is currently difficult to implement. Here, the authors develop a double-sided ionic liquid gating technique to generate electric fields as large as 4 V/nm across few-layer WSe2, leading to field-induced semiconductor-to-metal transitions.
- Benjamin I. Weintrub
- , Yu-Ling Hsieh
- & Kirill I. Bolotin
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Article
| Open AccessObservation of room temperature excitons in an atomically thin topological insulator
Here, the authors report the observation of room temperature excitons in a single layer of bismuth atoms epitaxially grown on a SiC substrate - a material of non-trivial global topology - with excitonic and topological physics deriving from the very same electronic structure.
- Marcin Syperek
- , Raul Stühler
- & Christian Schneider
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Article
| Open AccessProbing the ultrafast dynamics of excitons in single semiconducting carbon nanotubes
Excitonic states govern the optical response of low-dimensional nanomaterials and are key for a wide range of applications. Here, the authors investigate the exciton decay dynamics in single carbon nanotubes with few-exciton detection sensitivity.
- Konrad Birkmeier
- , Tobias Hertel
- & Achim Hartschuh
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Article
| Open AccessSlow light in a 2D semiconductor plasmonic structure
Slow light effects are interesting for telecommunications and quantum photonics applications. Here, the authors use coupled exciton-surface plasmon polaritons (SPPs) in a hybrid monolayer WSe2-metallic waveguide structure to demonstrate a 1300-fold reduction of the SPP group velocity.
- Matthew Klein
- , Rolf Binder
- & John R. Schaibley
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Article
| Open AccessInteractions between Fermi polarons in monolayer WS2
Here, the authors investigate the interactions between Fermi polarons in monolayer WS2 by multi-dimensional coherent spectroscopy, and find that, at low electron doping densities, the dominant interactions are between polaron states that are dressed by the same Fermi sea. They also observe a bipolaron bound state with large binding energy, involving excitons in different valleys cooperatively bound to the same electron.
- Jack B. Muir
- , Jesper Levinsen
- & Jeffrey A. Davis
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Article
| Open AccessDirect observation of ultrafast singlet exciton fission in three dimensions
Here, the authors use quantitative ultrafast interferometric pump-probe microscopy to track photoexcitations with sub-10 nm spatial precision in three dimensions and 15 fs temporal resolution to study the spatiotemporal dynamics of singlet exciton fission in polycrystalline pentacene films.
- Arjun Ashoka
- , Nicolas Gauriot
- & Akshay Rao
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Article
| Open AccessA shuttling-based two-qubit logic gate for linking distant silicon quantum processors
A coherent quantum link between distant quantum processors is desirable for scaling up of quantum computation. Noiri et al. demonstrate a strategy to link distant quantum processors in silicon, by implementing a shuttling-based two-qubit gate between spin qubits in a Si/SiGe triple quantum dot.
- Akito Noiri
- , Kenta Takeda
- & Seigo Tarucha
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| Open AccessObservation of Bose-Einstein condensates of excitons in a bulk semiconductor
Bose-Einstein condensate of excitons is expected in photo-excited bulk semiconductors, but a direct experimental evidence has been lacking. Here the authors report the observation of a condensate of 1s paraexcitons in Cu2O using real-space mid-infrared absorption imaging realized in a dilution refrigerator.
- Yusuke Morita
- , Kosuke Yoshioka
- & Makoto Kuwata-Gonokami
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Article
| Open AccessFlying electron spin control gates
Spin qubits are a platform for quantum computing. There are many advantages for quantum information processing if the spin qubit can move. Here, Helgers et al. use a surface acoustic wave to define a moving quantum dot and demonstrate the magneticfield-free control of the spin precession, bringing “flying” spin qubits a step closer.
- Paul L. J. Helgers
- , James A. H. Stotz
- & Paulo V. Santos
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| Open AccessUltrafast pseudospin quantum beats in multilayer WSe2 and MoSe2
Here, the authors investigate excitonic transitions in mono- and multi-layer WSe2 and MoSe2 by time-resolved Faraday ellipticity (TRFE) with in-plane magnetic fields, and attribute the oscillatory TRFE signal in the multilayer samples to pseudospin quantum beats of excitons, a manifestation of spin- and pseudospin layer locking.
- Simon Raiber
- , Paulo E. Faria Junior
- & Christian Schüller
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Article
| Open AccessHigh density integration of stretchable inorganic thin film transistors with excellent performance and reliability
Transistors with inorganic semiconductors have superior performance than organics. However, they are brittle and thus unfavorable for building deformable electronics. Here, authors directly embed such inorganic thin film transistors into serpentine strings to realize highly stretchable and miniaturized electronic circuits.
- Himchan Oh
- , Ji-Young Oh
- & Chi-Sun Hwang
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Article
| Open AccessInelastic phonon transport across atomically sharp metal/semiconductor interfaces
Phonons are thought to transport elastically across most interfaces. Here, the authors show that a substantial portion of phonons transport inelastically, adding another heat conduction channel and enhancing thermal conductance across interfaces.
- Qinshu Li
- , Fang Liu
- & Xinqiang Wang
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Article
| Open AccessAtomic-scale 3D imaging of individual dopant atoms in an oxide semiconductor
Small variations in the density of dopants change the physical properties of complex oxides. Here, the authors resolve doping levels in three dimension, imaging the atomic sites that donors occupy in the small band gap semiconductor Er(Mn,Ti)O3.
- K. A. Hunnestad
- , C. Hatzoglou
- & D. Meier
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Article
| Open AccessParametric longitudinal coupling between a high-impedance superconducting resonator and a semiconductor quantum dot singlet-triplet spin qubit
It has been predicted that longitudinal coupling between a qubit and a superconducting resonator can mediate efficient interactions among distant qubits. Here the authors implement such a coupling between a singlet-triplet qubit in a semiconductor double quantum dot and a high-impedance superconducting resonator.
- C. G. L. Bøttcher
- , S. P. Harvey
- & A. Yacoby
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| Open AccessDielectric catastrophe at the Wigner-Mott transition in a moiré superlattice
The Wigner-Mott insulator is driven by extended Coulomb repulsion, rather than the on-site Coulomb repulsion of the Mott insulator. Here, the authors observe a continuous bandwidth-tuned transition between a metal and a Wigner-Mott insulator in a MoSe2/WS2 moiré superlattice at fractional lattice filling.
- Yanhao Tang
- , Jie Gu
- & Jie Shan
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Article
| Open AccessLong-range charge carrier mobility in metal halide perovskite thin-films and single crystals via transient photo-conductivity
Charge carrier mobility is a fundamental property of semiconductors. The authors of this study demonstrate a novel way to estimate long-range mobilities of perovskite thin-films and single crystals by taking early-time carrier dynamics into account.
- Jongchul Lim
- , Manuel Kober-Czerny
- & Henry J. Snaith
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Article
| Open AccessPinhole-seeded lateral epitaxy and exfoliation of GaSb films on graphene-terminated surfaces
Remote epitaxy represents a promising method for the synthesis of thin films on lattice-mismatched substrates, but its atomic-scale mechanisms are still unclear. Here, the authors demonstrate the growth of exfoliatable GaSb films on graphene-terminated GaSb (001) via seeded lateral epitaxy, showing that pinhole defects in graphene serve as selective nucleation sites.
- Sebastian Manzo
- , Patrick J. Strohbeen
- & Jason K. Kawasaki
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Article
| Open AccessHidden spin-orbital texture at the \(\overline{{{\Gamma }}}\)-located valence band maximum of a transition metal dichalcogenide semiconductor
Materials with time reversal and inversion symmetry have a bulk band structure that is spin degenerate, however, they can still exhibit a hidden spin-polarization when probed in a specific way. Here, using angle and spin resolved photoemission, Clark et al reveal a hidden spin-polarization in 1T-HfSe2 that persists through the time reversal invariant momenta due to effective spin-orbital magnetisations
- Oliver J. Clark
- , Oliver Dowinton
- & Jaime Sánchez-Barriga
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Article
| Open AccessProlonging valley polarization lifetime through gate-controlled exciton-to-trion conversion in monolayer molybdenum ditelluride
Here, the authors devise a strategy for prolonging the valley polarization lifetime in monolayer MoTe2 by converting excitons to trions through gate control, and by taking advantage of the longer valley polarization lifetime of trions.
- Qiyao Zhang
- , Hao Sun
- & Cun-Zheng Ning
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Article
| Open AccessHarnessing many-body spin environment for long coherence storage and high-fidelity single-shot qubit readout
Hybrid quantum devices based on coupled nuclear and electron spins offer promising applications, but require long nuclear spin coherence times. Here the authors demonstrate millisecond coherence times for a nuclear spin ensemble coupled to a single electron spin qubit in a semiconductor quantum dot.
- George Gillard
- , Edmund Clarke
- & Evgeny A. Chekhovich
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Article
| Open AccessLight sources with bias tunable spectrum based on van der Waals interface transistors
Here, the authors report the realization of light-emitting field-effect transistors based on van der Waals heterostructures with conduction and valence band edges at the Γ-point of the Brillouin zone, showing electrically tunable and material-dependent electroluminescence spectra at room temperature.
- Hugo Henck
- , Diego Mauro
- & Alberto F. Morpurgo
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Article
| Open AccessAnderson transition in stoichiometric Fe2VAl: high thermoelectric performance from impurity bands
The mathematical conditions for the best thermoelectric is well known but never realised in real materials. Here, the authors propose the Anderson transition in a narrow impurity band as a physical realisation of this seemingly unrealisable scenario.
- Fabian Garmroudi
- , Michael Parzer
- & Ernst Bauer
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Article
| Open AccessBeam steering at the nanosecond time scale with an atomically thin reflector
Andersen et al. have demonstrated a new type of beam steering device based on the excitonic response of an atomically thin semiconductor. Using electrostatic gates, the authors achieved tunable steering with switching times on the nanosecond scale.
- Trond I. Andersen
- , Ryan J. Gelly
- & Mikhail D. Lukin
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Article
| Open AccessOptical control of exciton spin dynamics in layered metal halide perovskites via polaronic state formation
Spintronic devices will require long spin lifetimes, but the effect of exciton-lattice coupling on spin lifetime in metal-halide perovskites is not well understood. Here, the authors find a 100-fold increase in the lifetime of exciton spins in a 2D perovskite by exciting with excess energy, resulting from strong coupling between excitons and optically excited phonons.
- Sean A. Bourelle
- , Franco V. A. Camargo
- & Felix Deschler
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Article
| Open AccessThe Landé factors of electrons and holes in lead halide perovskites: universal dependence on the band gap
The Landé factors govern all the spin-related basic phenomena and are the key parameters which guide spintronics applications. Here, Kirstein et al. demonstrate a universal dependence of the Landé factors on the bandgap energy of several perovskite materials.
- E. Kirstein
- , D. R. Yakovlev
- & M. Bayer
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Article
| Open AccessBrightening of a dark monolayer semiconductor via strong light-matter coupling in a cavity
Here, the authors show brightening of dark excitons by strong coupling between cavity photons and high energy, spin-allowed, bright excitons in monolayer WSe2. In this regime, the commonly observed photoluminescence quenching stemming from the fast relaxation to the dark ground state is prevented.
- Hangyong Shan
- , Ivan Iorsh
- & Christian Schneider
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Article
| Open AccessWafer-scale epitaxial modulation of quantum dot density
Nucleation control of self-assembled quantum dots is challenging. Here, the authors employ conventional molecular beam epitaxy to achieve wafer-scale density modulation of high-quality quantum dots with tunable periodicity on unpatterned substrates.
- N. Bart
- , C. Dangel
- & A. Ludwig
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| Open Access2D materials for future heterogeneous electronics
Graphene and related two-dimensional (2D) materials have remained an active field of research in science and engineering for over fifteen years. Here, the authors investigate why the transition from laboratories to fabrication plants appears to lag behind expectations, and summarize the main challenges and opportunities that have thus far prevented the commercialisation of these materials.
- Max C. Lemme
- , Deji Akinwande
- & Christoph Stampfer
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Article
| Open AccessLong-range transport of 2D excitons with acoustic waves
Excitons in 2D semiconductors suffer from a weak response to in-plane electric fields, inhibiting their transport beyond the diffusion length. Here, the authors demonstrate the directional, long-range transport of interlayer excitons in bilayer WSe2 driven by the propagating potential traps induced by surface acoustic waves.
- Ruoming Peng
- , Adina Ripin
- & Mo Li