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| Open AccessDirect observation of multistep energy transfer in LHCII with fifth-order 3D electronic spectroscopy
Photosynthesis is a complex process, involving the transfer of sunlight driven excitation energy to a reaction centre. Here, the authors directly observe the multistep excitation energy transitions in a light-harvesting complex using ultrafast fifth-order three-dimensional electronic spectroscopy.
- Zhengyang Zhang
- , Petar H. Lambrev
- & Howe-Siang Tan
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Article
| Open AccessMicromotors with asymmetric shape that efficiently convert light into work by thermocapillary effects
The direct conversion of light into work allows the control of micromotors, but typically with low efficiencies and high power density requirements. Here, Maggiet al. demonstrate efficient thermocapillary propulsion of microgears on a liquid–air interface with wide-field, incoherent illumination.
- Claudio Maggi
- , Filippo Saglimbeni
- & Roberto Di Leonardo
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| Open AccessDeep and high-resolution three-dimensional tracking of single particles using nonlinear and multiplexed illumination
Existing single-particle tracking techniques are limited in terms of penetration depth, tracking range or temporal resolution. Here, Perilloet al. demonstrate three-dimensional particle tracking up to 200-μm depth, with 35-nm spatial localization and 50-μs resolution using multiplexed two-photon excitation.
- Evan P. Perillo
- , Yen-Liang Liu
- & Andrew K. Dunn
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| Open AccessNanoscale optical positioning of single quantum dots for bright and pure single-photon emission
Self-assembled quantum dots are good emitters, but lack emission control prior to device fabrication. Here a photoluminescence imaging technique to characterize position and emission properties of such quantum dots is demonstrated, enabling the realization of high-performance single-photon sources.
- Luca Sapienza
- , Marcelo Davanço
- & Kartik Srinivasan
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| Open AccessThree-dimensional nanometre localization of nanoparticles to enhance super-resolution microscopy
Tracking and stabilizing sample drifts is crucial towards realizing nanometer resolution in superresolution microscopy; metal nanoparticles can provide drift information but diffraction remains a challenge. Here, Bonet al. combine intensity and phase information to reach three-dimensional subnanometre accuracies.
- Pierre Bon
- , Nicolas Bourg
- & Sandrine Lévêque-Fort
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| Open AccessUltrafast spontaneous emission source using plasmonic nanoantennas
Typical emitters such as molecules and quantum dots have slow spontaneous emission with lifetimes of 1–10 ns. Here, Hoang et al. have fabricated a hybrid structure of plasmonic nanopatch antennas coupled to quantum dots, achieving ultrafast spontaneous emission with a lifetime of 11 ps.
- Thang B. Hoang
- , Gleb M. Akselrod
- & Maiken H. Mikkelsen
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High-resolution optical spectroscopy using multimode interference in a compact tapered fibre
While desirable for compact solutions, the miniaturization of spectrometers comes at the cost of spectral resolution and operating range. Here, Wanet al. propose a tapered fibre multimode interference spectrometer exhibiting high spectral resolution from the visible to the near infrared in a compact configuration.
- Noel H. Wan
- , Fan Meng
- & Dirk Englund
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Article
| Open AccessHigh density terahertz frequency comb produced by coherent synchrotron radiation
There is considerable interest in generating broadband frequency combs at terahertz frequencies. Here, Tammaro et al.achieve this using coherent synchrotron radiation where the electron bunches emit quasi-synchronous terahertz pulses with high power, broad frequency, zero frequency offset, and high density.
- S. Tammaro
- , O. Pirali
- & G. Mouret
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Article
| Open AccessQuantitative X-ray phase-contrast microtomography from a compact laser-driven betatron source
With excellent resolving power and tissue contrast, X-ray phase-contrast imaging holds great promise but the source requirements have limited its use. Here, Wenz et al. show a phase-contrast microtomogram of a biological sample using X-ray radiation driven by a high-power laser.
- J. Wenz
- , S. Schleede
- & S. Karsch
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Article
| Open AccessCreating semiconductor metafilms with designer absorption spectra
Ultrathin semiconductor metafilms can be designed to achieve near-unity absorption in specific spectral regions. Here, Kim et al. engineer nanoscale optical resonances in sub-50-nm-thick germanium nanobeams metafilms to demonstrate near-unity absorption in one or more desired wavelength regions.
- Soo Jin Kim
- , Pengyu Fan
- & Mark L. Brongersma
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Article
| Open AccessHighly indistinguishable photons from deterministic quantum-dot microlenses utilizing three-dimensional in situ electron-beam lithography
Single indistinguishable photon sources with high flux rates and purity are needed in quantum communications. Here, Gschreyet al. use three-dimensional electron-beam lithography to pattern deterministic quantum-dot microlenses and demonstrate enhanced photon-extraction efficiency and photon indistinguishability.
- M. Gschrey
- , A. Thoma
- & S. Reitzenstein
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Article
| Open AccessA generic concept to overcome bandgap limitations for designing highly efficient multi-junction photovoltaic cells
The efficiency of a single-junction photovoltaic cell is constrained by the Shockley-Queisser limit. Here, the authors adopt a triple-junction configuration which relaxes material and current-matching constraints, providing a generic strategy for advancing the efficiency roadmap of photovoltaic technologies.
- Fei Guo
- , Ning Li
- & Christoph J. Brabec
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Article
| Open AccessLaser chimeras as a paradigm for multistable patterns in complex systems
Chimera states are a class of self-organized solutions of high-dimensional networks with non-local and symmetry breaking coupling. Here the authors study the chimera patterns generated in a non-linear optical setup and uncover the transition between chimera orders as a pattern across clusters of chaoticity.
- Laurent Larger
- , Bogdan Penkovsky
- & Yuri Maistrenko
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Article
| Open AccessDistinguishing between plasmon-induced and photoexcited carriers in a device geometry
Plasmonic excitations of electrons in metallic nanostructures are promising for the enhanced conversion of light in semiconductor solar cells. Here, the authors are able to experimentally distinguish the absorption phenomena of plasmonic carrier generation and excitation of carriers by light absorption.
- Bob Y. Zheng
- , Hangqi Zhao
- & Naomi J. Halas
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Article
| Open AccessVibronic origin of long-lived coherence in an artificial molecular light harvester
Two-dimensional spectroscopy revealed oscillatory signals in photosynthesis’ exciton dynamics, but crowded spectra impede the identification of what sustains the oscillations. Here the authors probe an J-aggregate, whose uncongested response shows that vibronic coupling is responsible for the sustained coherence.
- James Lim
- , David Paleček
- & Jürgen Hauer
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Article
| Open AccessPhased-array sources based on nonlinear metamaterial nanocavities
Controlling light at scales smaller than its wavelength is attractive to manipulate light using small device footprints. Here, the authors propose a scheme to modify light on such small scales using a combination of metamaterial nanocavities coupled to nonlinear semiconductor heterostructures.
- Omri Wolf
- , Salvatore Campione
- & Igal Brener
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Article
| Open AccessElectric-field-induced strong enhancement of electroluminescence in multilayer molybdenum disulfide
The layer-number-dependent optical and electronic properties of transition metal dichalcogenides are promising in optoelectronics. Here, Li et al. demonstrate greatly enhanced electroluminescence emission in multi-layer MoS2attributed to the electric-field-induced carrier redistribution.
- Dehui Li
- , Rui Cheng
- & Xiangfeng Duan
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Article
| Open AccessHyperbolic phonon-polaritons in boron nitride for near-field optical imaging and focusing
Hyperbolic phonon polariton modes in natural hyperbolic materials could have uses in near-field optical imaging, guiding, and focusing applications. Here Li et al.demonstrate enlarged imaging and super-resolution focusing from a flat slab of hexagonal boron nitride enabled by hyperbolic phonon polariton modes.
- Peining Li
- , Martin Lewin
- & Thomas Taubner
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| Open AccessAdiabatic elimination-based coupling control in densely packed subwavelength waveguides
Optical communications and quantum operations require active coupling control in closely packed integrated photonic circuits. Here, Mrejen et al.exploit adiabatic elimination to demonstrate active coupling control between two closely packed waveguides by tuning the mode index of an in-between decoupled waveguide.
- Michael Mrejen
- , Haim Suchowski
- & Xiang Zhang
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| Open AccessLead iodide perovskite light-emitting field-effect transistor
Hybrid organic–inorganic perovskites have shown great potential for use in optoelectronic applications. Here, the authors create solution-processed lead iodide perovskite light-emitting field-effect transistors and demonstrate both ambipolar behaviour and gate-assisted electroluminescence.
- Xin Yu Chin
- , Daniele Cortecchia
- & Cesare Soci
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Temporal tweezing of light through the trapping and manipulation of temporal cavity solitons
Optical tweezing typically refers to the trapping and manipulation of particles using lasers. Here, Jang et al. demonstrate analogous manipulation of ultrashort cavity soliton-pulses in the time domain, trapped by the phase modulation of a continuous wave laser beam, and moved by modifying the phase profile.
- Jae K. Jang
- , Miro Erkintalo
- & Stuart G. Murdoch
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| Open AccessUltralow noise miniature external cavity semiconductor laser
Optical metrology applications require lasers with high spectral purity but on-chip devices with sub-100 Hz linewidth are yet to be realized. Here, Liang et al.present a heterogeneously integrated, chip-scale semiconductor laser with 30 Hz integral linewidth and sub-Hz instantaneous linewidth.
- W. Liang
- , V. S. Ilchenko
- & L. Maleki
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| Open AccessImaging an aligned polyatomic molecule with laser-induced electron diffraction
Laser-induced electron diffraction can provide structural information on gas-phase molecules with high spatial and temporal resolution. Going beyond previous diatomic cases, Pullen et al.apply this approach to acetylene and show that it can be used to measure bond lengths for polyatomic molecules.
- Michael G. Pullen
- , Benjamin Wolter
- & Jens Biegert
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Aging mechanisms in amorphous phase-change materials
Phase-change materials are a route to high-density data storage, but changes in their properties in time are a limiting factor. Here, the authors combine numerical simulations, photothermal deflection spectroscopy and impedance spectroscopy experiments to investigate the aging process in germanium telluride.
- Jean Yves Raty
- , Wei Zhang
- & Matthias Wuttig
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| Open AccessIonic transport in hybrid lead iodide perovskite solar cells
Understanding the mechanism of ionic transport in organic–inorganic halide perovskites is crucial for the design of future solar cells. Here, Eames et al.undertake a combined experimental and computational study to elucidate the ion conducting species and help rationalize the unusual behaviour observed in these perovskite-based devices.
- Christopher Eames
- , Jarvist M. Frost
- & M. Saiful Islam
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| Open AccessHigh-quality sandwiched black phosphorus heterostructure and its quantum oscillations
Black phosphorus is an atomically thin material that exhibits excellent properties for electronics applications, but these degrade in atmospheric conditions. Here, the authors demonstrate the fabrication of stable, ultra-clean and high-mobility black phosphorus sandwiched between the layers of boron nitride.
- Xiaolong Chen
- , Yingying Wu
- & Ning Wang
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Article
| Open AccessInterlayer orientation-dependent light absorption and emission in monolayer semiconductor stacks
Single atomic layers of transition metal dichalcogenides have outstanding electrical and optical properties. Here, the authors show that light absorption and emission from stacks of different transition metal dichalcogenide monolayers can be tuned by rotating the crystals.
- Hoseok Heo
- , Ji Ho Sung
- & Moon-Ho Jo
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| Open AccessSpatial and temporal imaging of long-range charge transport in perovskite thin films by ultrafast microscopy
Determining the mechanism of charge carrier transport in solar cells is important for their development towards higher efficiencies. Here, the authors elucidate the spatial and temporal diffusion of charge carriers in hybrid perovskite thin films through ultrafast transient absorption microscopy.
- Zhi Guo
- , Joseph S. Manser
- & Libai Huang
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Article
| Open AccessControlling dispersion forces between small particles with artificially created random light fields
Natural dispersion forces acting between molecules and particles arise from electromagnetic fields generated by quantum and thermal fluctuations. Here, Brügger et al.show that isotropic dispersion forces between colloidal particles can be induced, controlled and tuned with artificial, fluctuating laser light fields.
- Georges Brügger
- , Luis S. Froufe-Pérez
- & Juan José Sáenz
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| Open AccessHigh-performance flexible perovskite solar cells exploiting Zn2SnO4 prepared in solution below 100 °C
There has been impressive progress in the development of perovskite solar cells in recent years, but the best performing systems tend to be fabricated on glass surfaces. Here, the authors present a cell built on a polymer substrate, allowing flexibility whilst maintaining high efficiency.
- Seong Sik Shin
- , Woon Seok Yang
- & Sang Il Seok
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Article
| Open AccessOptoelectronic crystal of artificial atoms in strain-textured molybdenum disulphide
Periodically strained monolayer molybdenum disulphide funnels photogenerated electron-hole pairs across an electric field induced by a spatially graded band gap, mimicking a crystal of artificial atoms. Here, the authors experimentally demonstrate the artificial crystal in strain-textured molybdenum disulphide.
- Hong Li
- , Alex W. Contryman
- & Xiaolin Zheng
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Article
| Open AccessDynamical properties induced by state-dependent delays in photonic systems
Time delays in feedback loops and connections in dynamical systems and complex networks can depend on the state of the system, but these state-dependent delays are poorly understood. Here, the authors use a photonic system to characterize the switching between two loops with different delay times.
- Jade Martínez-Llinàs
- , Xavier Porte
- & Ingo Fischer
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| Open AccessPhotonic sensing of organic solvents through geometric study of dynamic reflection spectrum
Photonic sensing is a method for detecting individual chemical species, but can fail when they are sufficiently similar in physical properties. Here, the authors report a method that can distinguish even very closely related species, such as homologues and chemical isomers.
- Yuqi Zhang
- , Qianqian Fu
- & Jianping Ge
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Article
| Open AccessEnabling unassisted solar water splitting by iron oxide and silicon
Water splitting using earth-abundant materials promises a low cost solution to the problem of large scale energy storage. Here, the authors fabricate a haematite and silicon-based high-efficiency water splitting device, which operates without the need for an externally applied bias.
- Ji-Wook Jang
- , Chun Du
- & Dunwei Wang
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| Open AccessReconfigurable photonic crystals enabled by pressure-responsive shape-memory polymers
Smart shape-memory polymers based on pressure stimuli have potential biomedical and aerospace applications but are largely unexplored. Here, Fang et al.present a reconfigurable photonic crystal that is reprogrammed at ambient conditions by a pressure-responsive shape-memory polymer.
- Yin Fang
- , Yongliang Ni
- & Peng Jiang
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| Open AccessThe optoelectronic role of chlorine in CH3NH3PbI3(Cl)-based perovskite solar cells
Chlorine incorporation into CH3NH3PbI3improves solar cell performance, but its optoelectronic role is still unclear. Here the authors present a strategy that decouples the morphological impact, to reveal that chlorine incorporation affects carrier transport across the heterojunction interface rather than within the perovskite crystal.
- Qi Chen
- , Huanping Zhou
- & Yang Yang
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| Open AccessEfficient photosynthesis of carbon monoxide from CO2 using perovskite photovoltaics
Artificial photosynthesis is a means of harnessing solar energy to generate fuels but has traditionally been exploited for the generation of hydrogen. Here, Schreier et al. instead employ a perovskite photovoltaic device to effect the solar conversion of CO2to CO with high efficiency.
- Marcel Schreier
- , Laura Curvat
- & Michael Grätzel
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Spatial modulation of light transmission through a single microcavity by coupling of photosynthetic complex excitations to surface plasmons
The interaction between light and molecules can lead to hybrid quantum-physical states of light and matter. Here, the authors demonstrate one such effect, spatial modulation of light, with the protein photosystem I as a first demonstration of this quantum effect with such a biological molecule.
- Itai Carmeli
- , Moshik Cohen
- & Shachar Richter
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| Open AccessHigh-performance ternary blend polymer solar cells involving both energy transfer and hole relay processes
Ternary blend solar cells offer the potential for high-power conversion efficiencies (PCEs); however their performances can be limited by design complexity. Here, the authors integrate multiple materials into a single junction device with 9.2% PCE and elucidate the mechanisms of enhancement at play.
- Luyao Lu
- , Wei Chen
- & Luping Yu
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Resonance shifts and spill-out effects in self-consistent hydrodynamic nanoplasmonics
Recent experiments with plasmonic nanostructures have found phenomena that cannot be explained classically, necessitating new theoretical models. Toscano et al. present a self-consistent hydrodynamic theory that describes both the nonlocal response and the electronic spill-out for noble and simple metals.
- Giuseppe Toscano
- , Jakob Straubel
- & Martijn Wubs
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Article
| Open AccessSTED nanoscopy with fluorescent quantum dots
STED nanoscopy enables sub-diffraction imaging with a wide range of fluorescent probes. Here, the authors show that a bright and very photostable class of fluorescent quantum dots can be super-resolved with STED as biolabels in cellular contexts.
- Janina Hanne
- , Henning J. Falk
- & Stefan W. Hell
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Theory of Floquet band formation and local pseudospin textures in pump-probe photoemission of graphene
Condensed matter research has seen prominent recent advances in ultrafast optical manipulation and topological materials. Here, Sentef et al. simulate the development of the photoemission-measured band structure of Floquet states in graphene excited by low-frequency circularly-polarized laser pulses.
- M.A. Sentef
- , M. Claassen
- & T.P. Devereaux
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High-density waveguide superlattices with low crosstalk
High-density integration will be vital for silicon photonics, but as we approach sub-wavelength distances between components, the crosstalk becomes intolerable. Here, Song et al. demonstrate waveguide integration at a half-wavelength pitch with low crosstalk using advanced superlattice design concepts.
- Weiwei Song
- , Robert Gatdula
- & Wei Jiang
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Article
| Open AccessActive graphene–silicon hybrid diode for terahertz waves
Graphene has demonstrated the ability to modulate terahertz (THz) waves by optical or electrical excitation, but modulation depths have been low. Here, Li et al. demonstrate enhanced modulation and polarity-dependent THz attenuation using external voltage bias and photoexcitation on a graphene–silicon film.
- Quan Li
- , Zhen Tian
- & Weili Zhang
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Article
| Open AccessQuantification of thickness and wrinkling of exfoliated two-dimensional zeolite nanosheets
Two-dimensional sheets of zeolites can function as molecular sieves for applications such as membranes or as catalysts. Here, the authors demonstrate a method using electron diffraction patterns to accurately measure the thickness and wrinkles of thin zeolite nanosheets.
- Prashant Kumar
- , Kumar Varoon Agrawal
- & K. Andre Mkhoyan
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Article
| Open AccessPerovskite–fullerene hybrid materials suppress hysteresis in planar diodes
Metal halide perovskites are promising for solar energy harvesting, but currently prone to a large hysteresis and current instability. Here, Xu et al. show improvements in a hybrid material in which the fullerene is distributed at perovskite grain boundaries and thus passivates defects effectively.
- Jixian Xu
- , Andrei Buin
- & Edward H. Sargent
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Subwavelength-thick lenses with high numerical apertures and large efficiency based on high-contrast transmitarrays
Replacing conventional components with flat optic devices such as flat lenses is desirable for imaging and on-chip integration, but performance has hindered their use. Here, Arbabi et al. report a wavelength-thin, high-contrast transmitarray micro-lens with a 0.57 λfocal spot and 82% focusing efficiency.
- Amir Arbabi
- , Yu Horie
- & Andrei Faraon
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Electronic modulation of infrared radiation in graphene plasmonic resonators
Graphene’s exotic properties make it suitable for many different optoelectronic devices. Brar et al. show that graphene plasmonic resonators can be exploited to produce narrow spectral emission in the mid-infrared, whose frequency and intensity can be modulated by electrostatic gating.
- Victor W. Brar
- , Michelle C. Sherrott
- & Harry A. Atwater
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| Open AccessFast and bright spontaneous emission of Er3+ ions in metallic nanocavity
The Purcell effect predicts a spontaneous emission rate enhancement of several orders of magnitude, but experimental demonstrations have been much lower. Here, Song et al. show emission enhancement of Er3+ions in a metallic nanocavity with a 170 Purcell factor at room temperature and 55% extraction efficiency.
- Jung-Hwan Song
- , Jisu Kim
- & Yong-Hee Lee