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| Open AccessThe role of interfacial donor–acceptor percolation in efficient and stable all-polymer solar cells
The underlying charge generation dynamics and structure-property relationships in organic solar cells are not fully understood. Here, the authors demonstrate that interfacial donor-acceptor percolation plays a key role in enabling both high charge generation efficiency and device stability.
- Zhen Wang
- , Yu Guo
- & Philip C. Y. Chow
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Article
| Open AccessMemristor-based storage system with convolutional autoencoder-based image compression network
Dealing with the explosive growth of diverse image data in the era of big data poses challenges for storage. Feng et al. propose a memristor-based near-storage in-memory processing system to boost the energy and storage efficiency.
- Yulin Feng
- , Yizhou Zhang
- & Jinfeng Kang
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| Open AccessSteep-slope vertical-transport transistors built from sub-5 nm Thin van der Waals heterostructures
2D vertical transport transistors (VTFETs) may promote the downscaling of electronic devices, but their performance is usually restricted by the thermionic limit. Here, the authors report the realization of short-channel steep-slope VTFETs based on MoS2/MoTe2 heterojunctions integrated with resistance threshold switching cells.
- Qiyu Yang
- , Zheng-Dong Luo
- & Genquan Han
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Article
| Open AccessInterfacial magnetic spin Hall effect in van der Waals Fe3GeTe2/MoTe2 heterostructure
Charge-to-spin conversion allows for the generation and control of spin polarization via a charge current. Typically, this is done with non-magnetic materials with large spin-orbit interactions such as Platinum. Herein, Dai et al demonstrate an intriguing charge-to-spin mechanism, a magnetic spin Hall effect, in a van der Waals heterostructure.
- Yudi Dai
- , Junlin Xiong
- & Feng Miao
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Article
| Open AccessStrong coupling between a microwave photon and a singlet-triplet qubit
By coupling a spin-qubit to a superconducting resonator, remote spin-entanglement becomes feasible. Here, Ungerer et al achieve strong coupling between a superconducting resonator and a singlet-triplet spin qubit, in an InAs nanowire.
- J. H. Ungerer
- , A. Pally
- & C. Schönenberger
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Article
| Open AccessApproaching a fully-polarized state of nuclear spins in a solid
Highly polarized nuclear spins can supress decoherence of electron spin qubits, but this requires near-unity polarization. Here the authors implement a protocol combining optical excitation and fast carrier tunnelling to achieve nuclear spin polarizations above 95% in GaAs quantum dots on a timescale of 1 minute.
- Peter Millington-Hotze
- , Harry E. Dyte
- & Evgeny A. Chekhovich
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Article
| Open AccessNon-hermiticity in spintronics: oscillation death in coupled spintronic nano-oscillators through emerging exceptional points
Exceptional points emerge in systems with loss and gain when loss and gain in the system are balanced. Due to the careful balancing involved, they are highly sensitive to perturbations, making them exceptionally useful for sensors and other devices. Here, Wittrock et al observe a variety of complex dynamics associated with exceptional points in coupled spintronic nano-oscillators.
- Steffen Wittrock
- , Salvatore Perna
- & Vincent Cros
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| Open AccessClocked dynamics in artificial spin ice
Artificial spin ices are nanomagnetic metamaterials, whose collective magnetization self-organizes into extended domains. However, controlling when, where and how domains change has proven difficult, yet is crucial for technological applications. Here, Jensen and Strømberg et al. introduce astroid clocking, which enables controlled, stepwise growth and reversal of magnetic domains, using only global fields.
- Johannes H. Jensen
- , Anders Strømberg
- & Erik Folven
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Article
| Open AccessSwitchable unidirectional emissions from hydrogel gratings with integrated carbon quantum dots
Directional emission of photoluminescence is an emerging technique for light-emitting fields and nanophotonics. Here, the authors demonstrate a hydrogel grating with integrated quantum dots for switchable unidirectional emission tuning.
- Chenjie Dai
- , Shuai Wan
- & Zhongyang Li
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Article
| Open AccessA genetic circuit on a single DNA molecule as an autonomous dissipative nanodevice
Achieving genetic circuits on single DNA molecules could have varied applications. Here, authors observed proteins emerging from single DNA molecules through coupled transcription-translation complexes, and show that nascent proteins lingered on DNA, regulating cascaded reactions on the same DNA and allowing the design of a pulsatile genetic circuit.
- Ferdinand Greiss
- , Nicolas Lardon
- & Roy Bar-Ziv
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| Open AccessPulse irradiation synthesis of metal chalcogenides on flexible substrates for enhanced photothermoelectric performance
Here, the authors report a low-temperature pulse irradiation synthesis method to prepare thermoelectric metal chalcogenide (Bi2Se3, SnSe2 and Bi2Te3) thin films on various flexible substrates, showing their application for the realization of broadband photothermoelectric detectors.
- Yuxuan Zhang
- , You Meng
- & Johnny C. Ho
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Article
| Open AccessToward grouped-reservoir computing: organic neuromorphic vertical transistor with distributed reservoir states for efficient recognition and prediction
Existing neuromorphic hardware, focusing mainly on shallow-reservoir computing, is challenged in providing adequate spatial and temporal scales characteristic for effective computing. Here, Gao et al. report an ultra-short channel organic neuromorphic vertical transistor with distributed reservoir states.
- Changsong Gao
- , Di Liu
- & Huipeng Chen
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| Open AccessPowering AI at the edge: A robust, memristor-based binarized neural network with near-memory computing and miniaturized solar cell
The authors present an AI engine with 32,768 memristors powered by a miniature solar cell. This circuit exploits near-memory computing, naturally adjusting its accuracy depending on the illumination level, and paves the way for self-powered AI.
- Fadi Jebali
- , Atreya Majumdar
- & Jean-Michel Portal
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Article
| Open AccessMagnetoresistive-coupled transistor using the Weyl semimetal NbP
L. Rocchino et al. experimentally demonstrate a magnetic field effect transistor based on the Weyl semimetal NbP as the active channel material. A gate magnetic field is generated by current flowing in an integrated superconductor NbN. The device operation relies on the extreme magnetoresistance of the NbP.
- Lorenzo Rocchino
- , Federico Balduini
- & Cezar B. Zota
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| Open AccessGiant tunnelling electroresistance in atomic-scale ferroelectric tunnel junctions
The authors report ferroelectric tunnel junctions based on samarium-substituted layered bismuth oxide, which show tunnelling electroresistance of 7 × 105 and high endurance over 5 billion cycles, even when the film is down to one nanometer.
- Yueyang Jia
- , Qianqian Yang
- & Rui Yang
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Article
| Open AccessMicrowave quantum diode
Quantum devices exhibiting non-reciprocal behaviour have been attracting attention for fundamental studies and applications. Here the authors report a microwave quantum diode based on a superconducting flux qubit coupled to two resonators, which has the advantage of compactness and scalability.
- Rishabh Upadhyay
- , Dmitry S. Golubev
- & Jukka P. Pekola
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Article
| Open AccessFlexible switch matrix addressable electrode arrays with organic electrochemical transistor and pn diode technology
Organic neural implants hold considerable promise for biocompatible neural interfaces. Here, the authors employ polymer-based organic electrochemical diodes and transistors to develop neuron-sized complex circuits, enabling multiplexing without crosstalk and demonstrate that, when integrated onto ultra-thin plastic, these circuits achieve high performance while maintaining minimal invasiveness.
- Ilke Uguz
- , David Ohayon
- & Kenneth L. Shepard
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Article
| Open AccessCompact and wideband nanoacoustic pass-band filters for future 5G and 6G cellular radios
This work addresses the fundamental challenge of the frequency up-scaling of microacoustic devices. The manuscript presents the first bank of on-chip multi-frequency, low-loss, wideband, and compact passband filters for mobile 5G and 6G applications.
- Gabriel Giribaldi
- , Luca Colombo
- & Matteo Rinaldi
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| Open AccessUltrashort vertical-channel MoS2 transistor using a self-aligned contact
The simultaneous scaling down of the channel length and gate length of 2D transistors remains challenging. Here, the authors report a self-alignment process to fabricate vertical MoS2 transistors with sub-1 nm gate length and sub−50 nm channel length, exhibiting on-off ratios over 105 and on-state currents of 250 μA/μm at 4 V bias.
- Liting Liu
- , Yang Chen
- & Yuan Liu
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| Open AccessParity-conserving Cooper-pair transport and ideal superconducting diode in planar germanium
M. Valentini et al. study superconducting quantum interference devices (SQUIDs) where the weak link of the Josephson junctions is a germanium 2D hole gas. They report signatures of the tunneling of pairs of Cooper pairs. For a particular microwave drive power, they observe a 100% efficient superconducting diode effect.
- Marco Valentini
- , Oliver Sagi
- & Georgios Katsaros
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Article
| Open AccessInjectable hydrogel electrodes as conduction highways to restore native pacing
No preventive treatment addresses the underlying condition that leads to cardiac arrest. Here, researchers developed an injectable hydrogel electrode that achieves pacing that mimics physiological conduction with the potential to eliminate lethal arrhythmias and provide painless defibrillation.
- Gabriel J. Rodriguez-Rivera
- , Allison Post
- & Elizabeth Cosgriff-Hernandez
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| Open AccessElastocapillarity-driven 2D nano-switches enable zeptoliter-scale liquid encapsulation
In this work, authors demonstrate programmable nanostructures using two-dimensional materials for nanoscale liquid manipulation. The nanoswitches and capsules can hold zeptoliter liquid volumes, enabling active nanofluidics circuits and confined reactors.
- Nathan Ronceray
- , Massimo Spina
- & Slaven Garaj
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Article
| Open AccessPurely self-rectifying memristor-based passive crossbar array for artificial neural network accelerators
Designing memristor-integrated passive crossbar arrays to accelerate artificial neural networks with high reliability remains a challenge. Here, the authors propose a self-rectifying resistive switching device incorporated into a crossbar array with a density of 1 kb whose operational performance is assessed in terms of defected-cell proportion, reading margin, and selection functionality.
- Kanghyeok Jeon
- , Jin Joo Ryu
- & Gun Hwan Kim
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Article
| Open AccessExtendable piezo/ferroelectricity in nonstoichiometric 2D transition metal dichalcogenides
Nonstoichiometric transition metal dichalcogenides break symmetry, enabling piezo/ferroelectric effects. Here, the authors propose an approach to integrate these properties with diverse 2D materials, advancing multifunctional materials and devices.
- Yi Hu
- , Lukas Rogée
- & Shu Ping Lau
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Article
| Open AccessHigh quality factor metasurfaces for two-dimensional wavefront manipulation
Wavefront manipulation with metasurfaces is typically limited to low quality factors. Here, the authors show how higher-order Mie modes can be leveraged to design high quality factor optical metasurfaces for wavefront manipulation in two dimensions.
- Claudio U. Hail
- , Morgan Foley
- & Harry A. Atwater
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Article
| Open AccessA hard molecular nanomagnet from confined paramagnetic 3d-4f spins inside a fullerene cage
Shortening the inter-spin distance is an effective way to enhance magnetic coupling. However, it is typically challenging to change the inter-ion distance in most magnetic systems. Here, Huang et al present a strategy for enhancing magnetic interactions, by confining a molecular magnetic system inside a carbon fullerene cage, leading to enhanced magnetic properties.
- Chenli Huang
- , Rong Sun
- & Song Gao
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Article
| Open AccessHydrophobically gated memristive nanopores for neuromorphic applications
Designing efficient nanoscale and adaptable bioinspired memristors remains a challenge. Here, the authors develop a bioinspired hydrophobically gated memristive nanopore capable of learning, forgetting, and retaining memory through an electrowetting mechanism.
- Gonçalo Paulo
- , Ke Sun
- & Alberto Giacomello
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Article
| Open AccessEmbedding security into ferroelectric FET array via in situ memory operation
Existing solutions based Advanced Encryption Standard to address the security issues of nonvolatile memories incurs significant performance and power overhead. Here, the authors propose a lightweight XOR-gate based encryption/decryption technique by exploiting in-situ array operations, which achieves significant area/latency/power reduction compared to conventional designs.
- Yixin Xu
- , Yi Xiao
- & Kai Ni
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Article
| Open AccessPhase-dependent Andreev molecules and superconducting gap closing in coherently-coupled Josephson junctions
S. Matsuo et al. report tunneling spectroscopy measurements on a device consisting of two Josephson junctions (JJ) sharing a single superconducting electrode. In isolation, each JJ would host an Andreev bound state (ABS). In their coherently-coupled JJs, the authors report the formation of an Andreev molecule due to hybridization of the two ABSs.
- Sadashige Matsuo
- , Takaya Imoto
- & Seigo Tarucha
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Article
| Open AccessRecord high room temperature resistance switching in ferroelectric-gated Mott transistors unlocked by interfacial charge engineering
Ferroelectric transistors are promising building blocks for developing energy-efficient memory and logic applications. Here, the authors report a record high 300 K resistance on-off ratio achieved in ferroelectric-gated Mott transistors by exploiting a charge transfer layer to tailor the channel carrier density and mitigate the ferroelectric depolarization effect.
- Yifei Hao
- , Xuegang Chen
- & Xia Hong
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Article
| Open AccessHot luminescence from single-molecule chromophores electrically and mechanically self-decoupled by tripodal scaffolds
A fundamental challenge for molecular electronics is the change in photophysical properties of molecules upon direct electrical contact. Here, the authors observe hot luminescence emitted by single-molecule chromophores that are electrically and mechanically self-decoupled by a tripodal scaffold.
- Vibhuti Rai
- , Nico Balzer
- & Michal Valášek
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Article
| Open AccessIn operando cryo-STEM of pulse-induced charge density wave switching in TaS2
Resistive switching of 1T-TaS2 is promising for next-generation electronics. Here, using in operando electron microscopy, the authors determine that Joule heating drives the switching process, which will aid the engineering of future devices.
- James L. Hart
- , Saif Siddique
- & Judy J. Cha
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Article
| Open AccessHigh-performance van der Waals antiferroelectric CuCrP2S6-based memristors
Layered thio- and seleno-phosphate ferroelectrics show promise for next-generation memory but have thermal stability issues. Using the electric field-driven phase transition in antiferroelectric CuCrP2S6, the authors introduce a robust memristor, emphasizing the potential of van der Waals antiferroelectrics in advanced neuromorphic computing.
- Yinchang Ma
- , Yuan Yan
- & Xixiang Zhang
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Article
| Open AccessCryogenic multiplexing using selective area grown nanowires
The authors demonstrate a large ensemble of quantum dots which is characterized using a cryogenic multiplexer-demultiplexer circuit based on selective area growth nanowires, establishing the feasibility of scaling future quantum circuits.
- Dāgs Olšteins
- , Gunjan Nagda
- & Thomas S. Jespersen
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Article
| Open AccessThe role of halogens in Au–S bond cleavage for energy-differentiated catalysis at the single-bond limit
Investigation of the reaction process at the single-bond interface is key to understanding the catalytic reaction mechanism. Here, the authors develop a STM-BJ method to monitor the catalytic process from the perspective of single-bond energy.
- Peihui Li
- , Songjun Hou
- & Xuefeng Guo
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Article
| Open AccessThermal and electrostatic tuning of surface phonon-polaritons in LaAlO3/SrTiO3 heterostructures
Phonon polaritons are promising for infrared applications while it is difficult to tune the phonon polariton properties. Here, authors report a thermal and electrostatic tuning of surface phonon polaritons in heterostructures of LaAlO3/SrTiO3.
- Yixi Zhou
- , Adrien Waelchli
- & Alexey B. Kuzmenko
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Article
| Open AccessPosition error-free control of magnetic domain-wall devices via spin-orbit torque modulation
For magnetic domain-wall devices, key issue to be addressed is nonstochastic displacement of magnetic domain wall. Here, authors report domain-wall control with a position error-free scheme via spin-orbit torque modulation along nanotrack devices.
- Seong-Hyub Lee
- , Myeonghoe Kim
- & Sug-Bong Choe
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Article
| Open AccessMicroscopic theory, analysis, and interpretation of conductance histograms in molecular junctions
Conductance histograms are common setups to study molecular junctions, but the dispersion of the signals makes it difficult to interpret at microscopic level. Here the authors develop a physical model of molecular junctions that connects this observable with molecular properties.
- Leopoldo Mejía
- , Pilar Cossio
- & Ignacio Franco
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Article
| Open AccessBringing uncertainty quantification to the extreme-edge with memristor-based Bayesian neural networks
Bayesian networks gain importance in safety-critical applications. Authors conducted experiments with a memristor-based Bayesian network trained with variational inference with technological loss, achieving accurate heartbeats classification and prediction certainty.
- Djohan Bonnet
- , Tifenn Hirtzlin
- & Elisa Vianello
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Article
| Open AccessSingle PbS colloidal quantum dot transistors
Colloidal quantum dots remain unexplored for applications in single-electron devices. Here, the authors demonstrate single-electron transistors using single PbS colloidal quantum dot, highlighting their room-temperature operation.
- Kenji Shibata
- , Masaki Yoshida
- & Yoshihiro Iwasa
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Article
| Open AccessAmphibious epidermal area networks for uninterrupted wireless data and power transfer
Body area networks represent a wearable technology suitable for applications like virtual reality and health monitoring. Here, the study presents a wireless battery-free channel that works reliably in harsh environments, including underwater. It utilizes stretchable magneto-inductive metamaterials to enable uninterrupted communication.
- Amirhossein Hajiaghajani
- , Patrick Rwei
- & Peter Tseng
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Article
| Open AccessPhase biasing of a Josephson junction using Rashba–Edelstein effect
The authors study transport in Nb-(Pt/Cu)-Nb Josephson junctions (JJ), where Pt/Cu is a Rashba interface. Due to the Rashba–Edelstein effect, a charge current leads to a non-equilibrium spin moment at the Pt/Cu interface, which can be measured from a shift of the Fraunhofer pattern of the JJ.
- Tapas Senapati
- , Ashwin Kumar Karnad
- & Kartik Senapati
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Article
| Open AccessMultiplexed detection of viral antigen and RNA using nanopore sensing and encoded molecular probes
Fast discrimination of SARS-CoV-2 variants in clinical samples remains a challenge. Here, authors report on single molecule nanopore sensing combined with DNA molecular probes to simultaneously detect various antigens and RNA mutations of SARS-CoV-2 variants in patient samples.
- Ren Ren
- , Shenglin Cai
- & Joshua B. Edel
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Article
| Open AccessA robotic sensory system with high spatiotemporal resolution for texture recognition
Artificial sensory systems are typically limited by their performance and response to static and dynamic stimuli. Here, Bai et al. propose an iontronic slip-sensor, which responds to both static pressure and high-frequency vibrations up to 400 Hz, achieving high spatiotemporal resolution for texture recognition.
- Ningning Bai
- , Yiheng Xue
- & Chuan Fei Guo
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Article
| Open AccessDynamic construction of refractive index-dependent vibrations using surface plasmon-phonon polaritons
Molecular vibrations serve as valuable signatures for the constituent elements and bonding in compounds. Here, using Surface-Enhanced Infrared Absorption spectroscopy, the authors study refractive index dependent vibrations of surface phonon polaritons and surface plasmon platform, targeting dynamic biomonitoring.
- Hong Zhou
- , Zhihao Ren
- & Chengkuo Lee
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Article
| Open AccessLocal control of superconductivity in a NbSe2/CrSBr van der Waals heterostructure
Two-dimensional magnets and superconductors are emerging as tunable building blocks for quantum computing and superconducting spintronic devices. Here, Jo et al. demonstrate NbSe2/CrSBr van der Waals superconducting spin valves that exhibit infinite magnetoresistance and nonreciprocal charge transport, arising from a unique metamagnetic transition in CrSBr.
- Junhyeon Jo
- , Yuan Peisen
- & Luis E. Hueso
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Article
| Open AccessProbabilistic computing with NbOx metal-insulator transition-based self-oscillatory pbit
Probabilistic computing has recently emerged as a promising energy-based computing system for solving non-deterministic polynomial-time-hard (NP-hard) problems. Here the authors develop a novel pbit unit, using NbOx volatile memristor, in which a self-clocking oscillator harnesses noise-induced metal-insulator transition, enabling high-performance probabilistic computing.
- Hakseung Rhee
- , Gwangmin Kim
- & Kyung Min Kim
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Article
| Open AccessMonolithic three-dimensional integration of RRAM-based hybrid memory architecture for one-shot learning
Designing efficient 3D artificial neural networks chip remains a challenge. Here, the authors report a M3D-LIME chip with monolithic three-dimensional integration of hybrid memory architecture based on resistive random-access memory, which achieves a high classification accuracy of 96% in one-shot learning task while exhibiting 18.3× higher energy efficiency than GPU.
- Yijun Li
- , Jianshi Tang
- & Huaqiang Wu
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Article
| Open AccessTunable Tamm plasmon cavity as a scalable biosensing platform for surface enhanced resonance Raman spectroscopy
The researchers present a scalable Tamm plasmon cavity using phase change material with large resonance tunability and demonstrated tunable SERS by matching the plasmonic resonance with the molecule absorption for sensitivity enhanced biosensing.
- Kandammathe Valiyaveedu Sreekanth
- , Jayakumar Perumal
- & Jinghua Teng