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| Open AccessStability and dynamics of membrane-spanning DNA nanopores
Although DNA nanopores are widely explored as synthetic membrane proteins, it is still unclear how the anionic DNA assemblies stably reside within the hydrophobic core of a lipid bilayer. Here, the authors use molecular dynamics simulations to reveal the key dynamic interactions and energetics stabilizing the nanopore-membrane interaction.
- Vishal Maingi
- , Jonathan R. Burns
- & Mark S. P. Sansom
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Article
| Open AccessProposal for dark exciton based chemical sensors
Two-dimensional materials have shown great promise as efficient chemical sensors. Here, the authors present a sensing mechanism to allow the detection of molecules based on dark excitons in atomically thin transition metal dichalcogenides.
- Maja Feierabend
- , Gunnar Berghäuser
- & Ermin Malic
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| Open AccessAn electrically actuated molecular toggle switch
Robust molecular junctions demand highly reproducible switching between two or more well-defined conductance states upon control. Here, Gerhardet al. show the utility of elastic deformation of tripodal spirobifluorene derivatives in the junction of a scanning tunnelling microscope to achieve this goal.
- Lukas Gerhard
- , Kevin Edelmann
- & Wulf Wulfhekel
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| Open AccessControl of randomly scattered surface plasmon polaritons for multiple-input and multiple-output plasmonic switching devices
Losses of bandwidth are inevitable when interfacing between optical and electronic components. Here the authors present a switching device consisting of a two-dimensional disordered array of nanoholes that can potentially transfer information about 40 times faster than conventional switching devices.
- Wonjun Choi
- , Yonghyeon Jo
- & Wonshik Choi
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Article
| Open AccessObservation of optomechanical buckling transitions
Optomechanical systems could form logic gates, but key requirements are two stable static states and the ability to switch between them. Here, the authors observe radiation-pressure induced buckling transitions in an optomechanical system, and control this transition by varying laser power and detuning.
- H. Xu
- , U. Kemiktarak
- & J. M. Taylor
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| Open AccessDynamic plasmonic colour display
Here Duanet al. demonstrate dynamic plasmonic colour displays using catalytic magnesium metasurfaces. Controlled hydrogenation and dehydrogenation of the constituent nanoparticles, which serve as dynamic pixels, allow plasmonic colour printing, tuning, erasing, restoration of colour and encoding of information.
- Xiaoyang Duan
- , Simon Kamin
- & Na Liu
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Article
| Open AccessMagnetization switching in ferromagnets by adsorbed chiral molecules without current or external magnetic field
Spin manipulation in memory devices typically requires large electrical currents, limiting performance. Here the authors demonstrate magnetization switching in ferromagnetic films by depositing chiral molecules, making use of a proximity effect without needing magnetic or electric fields.
- Oren Ben Dor
- , Shira Yochelis
- & Yossi Paltiel
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| Open AccessGate-controlled conductance switching in DNA
Thanks to its base stacking structure, DNA can behave as an electric wire, but external control of its electronic properties has not been achieved yet. Here, the authors show that DNA conductance can be switched electrochemically when a DNA base is replaced by the redox molecule anthraquinone.
- Limin Xiang
- , Julio L. Palma
- & Nongjian Tao
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Article
| Open AccessOptical gating and streaking of free electrons with sub-optical cycle precision
Pulsed electron beams with ultrafast duration are desirable to study atomic processes occurring over the natural time scales of electronic motion. Here the authors demonstrate the generation of electron pulses down to attosecond time scales by using optical gating and streaking method.
- M. Kozák
- , J. McNeur
- & P. Hommelhoff
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Article
| Open AccessScalable high-precision tuning of photonic resonators by resonant cavity-enhanced photoelectrochemical etching
Aligning the resonances of sets of optical cavities is necessary for advanced photonics and sensing applications. Here, the authors introduce resonant photoelectrochemical etching as a method to collectively and permanently tune the resonant wavelengths of ensembles of resonators on a photonic chip.
- Eduardo Gil-Santos
- , Christopher Baker
- & Ivan Favero
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Article
| Open AccessWafer-scale integration of sacrificial nanofluidic chips for detecting and manipulating single DNA molecules
The wide use of microfluidics for biological analysis demands scalable preparation methods, yet in practice it is very challenging. Here, Wanget al. show a wafer-scale fabrication of nanofluidic chips with single-digit nanometre dimension, which is compatible with standard semiconductor processing.
- Chao Wang
- , Sung-Wook Nam
- & Qinghuang Lin
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Article
| Open AccessImperfect two-dimensional topological insulator field-effect transistors
A challenge of using 2D materials for nanoelectronic devices is the need for defect-free lattice supporting efficient carrier transport. Here, the authors show theoretically that 2D topological insulators enable high-performance, low-power field-effect transistors without requiring defect-free materials.
- William G. Vandenberghe
- & Massimo V. Fischetti
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| Open AccessElectrically tunable organic–inorganic hybrid polaritons with monolayer WS2
Hybrid polariton states originating from the strong coupling of photonic and excitonic states hold promise for control of nonlinear light behaviour. Here, the authors fabricate a microcavity containing organic dye and WS2, featuring hybrid polaritons arising from both Frenkel and Wannier-Mott excitons.
- Lucas C. Flatten
- , David M. Coles
- & Jason M. Smith
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Article
| Open AccessInterfacing broadband photonic qubits to on-chip cavity-protected rare-earth ensembles
Solid-state emitters enable broadband quantum information storage, but they are affected by decoherence resulting from inhomogeneous broadening. Here the authors suppress this effect via cavity protection at the single photon level in an ensemble of rare-earth ions coupled to a nanophotonic resonator.
- Tian Zhong
- , Jonathan M. Kindem
- & Andrei Faraon
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Article
| Open AccessLasing in dark and bright modes of a finite-sized plasmonic lattice
Plasmonic dark modes are promising candidates for lasing applications. Here, Hakalaet al. show lasing at visible wavelengths in dark and bright modes of an array of silver nanoparticles combined with optically pumped dye molecules, opening up a route to utilization of all modes of plasmonic lattices.
- T. K. Hakala
- , H. T. Rekola
- & P. Törmä
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Article
| Open AccessMeasurement of transverse emittance and coherence of double-gate field emitter array cathodes
Field emitter arrays are key components for X-ray sources, microwave generators, RF communication and advanced light sources. Tsujinoet al., report double-gate field emitter arrays with competitive beam qualities to the state of the art UV photoexcited cathodes.
- Soichiro Tsujino
- , Prat Das Kanungo
- & R.J. Dwayne Miller
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Article
| Open AccessSuper-resolution imaging of light–matter interactions near single semiconductor nanowires
Light-matter interactions with single quantum emitters are generally difficult to measure with both high-resolution and a large field of view. Here, Johlin et al. develop far-field super-resolution fluorescence methods to map near-field emitter-nanostructure interactions over several microns.
- Eric Johlin
- , Jacopo Solari
- & Erik C. Garnett
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Article
| Open AccessConformation-driven quantum interference effects mediated by through-space conjugation in self-assembled monolayers
Tunnelling currents through molecular junctions are affected by quantum interference effects, but understanding the factors leading to them remains a challenge. Here the authors show that through-space conjugation in self-assembled monolayers leads to conformation-dependent quantum interference that suppresses conductivity.
- Marco Carlotti
- , Andrii Kovalchuk
- & Ryan C. Chiechi
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Article
| Open AccessSpin doping using transition metal phthalocyanine molecules
Molecular magnets are molecules with an inherent non-zero spin that can exhibit magnetic ordering. Here, the authors show that such molecules can change the many-body ground state of nonmagnetic metals at a functional scale with magnetic phthalocyanines.
- A. Atxabal
- , M. Ribeiro
- & L. E. Hueso
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| Open AccessNanomechanical motion transduction with a scalable localized gap plasmon architecture
Flexible approaches are required for building plasmomechanical devices for tunable optical devices. Here, Roxworthyet al. introduce a plasmonic-nanoelectromechanical systems device where gap plasmon resonators are embedded into arrays of moving silicon nitride nanostructures, yielding thousands of devices per chip.
- Brian J. Roxworthy
- & Vladimir A. Aksyuk
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| Open AccessHolographic free-electron light source
Controlling the generation of light in nano-scale systems is a challenging task and is of growing importance. Here, Li et al. propose a means of controlling the wavefront of light emanating from a single nano scale emitter by holographic principles using a plasmonic metasurface.
- Guanhai Li
- , Brendan P. Clarke
- & Nikolay I. Zheludev
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| Open AccessReconfigurable exciton-plasmon interconversion for nanophotonic circuits
Here the authors demonstrate functionality for on-chip optical communications via reconfigurable exciton-plasmon interconversion in 200 nm-diameter silver nanowires overlapping onto two-dimensional transition metal dichalcogenide transistors.
- Hyun Seok Lee
- , Dinh Hoa Luong
- & Young Hee Lee
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Article
| Open AccessDeterministic phase slips in mesoscopic superconducting rings
Understanding the decay of persistent current in superconducting rings remains obscure. Here, the authors show detailed agreement between measurements of the persistent current in isolated flux-biased rings and Ginzburg-Landau theory over a wide range of parameters, providing a quantitative picture of the free energy landscape.
- I. Petković
- , A. Lollo
- & J. G. E. Harris
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| Open AccessA CMOS silicon spin qubit
Silicon is a promising material for realization of quantum processors, particularly as it could be naturally integrated with classical control hardware based on CMOS technology. Here the authors report a silicon qubit device made with an industry-standard fabrication process on a CMOS platform.
- R. Maurand
- , X. Jehl
- & S. De Franceschi
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Article
| Open AccessSelf-assembly of diphenylalanine peptide with controlled polarization for power generation
Piezoelectricity in diphenylalanine peptide nanotubes (PNTs) suggests an avenue towards green piezoelectric devices. Here the authors show ‘smart’ PNTs whose polarization can be controlled with an electric field, and a resultant power generator which harvests biomechanical energy with high power density.
- Vu Nguyen
- , Ren Zhu
- & Rusen Yang
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| Open AccessUniversal domain wall dynamics under electric field in Ta/CoFeB/MgO devices with perpendicular anisotropy
Domain walls in ferromagnetic–oxide structures can be moved using an electric field, which could be useful for low-power electronic devices. Here, the authors demonstrate the modulation of the velocity of these domain walls between a creep and a flow regime.
- Weiwei Lin
- , Nicolas Vernier
- & Dafiné Ravelosona
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Article
| Open AccessUltrafast all-optical coherent control of single silicon vacancy colour centres in diamond
All-optical coherent control schemes offer well-localized and ultrafast control of individual qubits in many-qubit systems. Here the authors report on all-optical resonant and Raman-based control of single silicon vacancies using picosecond pulses, much faster than the ground state coherence time.
- Jonas Nils Becker
- , Johannes Görlitz
- & Christoph Becher
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Article
| Open AccessMass and stiffness spectrometry of nanoparticles and whole intact bacteria by multimode nanomechanical resonators
Mass spectrometry can accurately identify species by molecular mass, but measuring large species can be difficult. Here the authors show that nanomechanical resonators can identify both the mass and stiffness of larger analytes, demonstrating it for gold nanoparticles and E. Colibacteria.
- O. Malvar
- , J. J. Ruz
- & J. Tamayo
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| Open AccessPhotoemission-based microelectronic devices
Most microelectronic devices today exploit the electronic properties of semiconductors. Here, the authors demonstrate a microelectronic device for free-space electrons by using the enhanced fields in a microstructured metal surface to induce effective photoemission.
- Ebrahim Forati
- , Tyler J. Dill
- & Dan Sievenpiper
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| Open AccessThe flux qubit revisited to enhance coherence and reproducibility
Scalable quantum information processing requires controllable high-coherence qubits. Here, the authors present superconducting flux qubits with broad frequency tunability, strong anharmonicity and high reproducibility, identifying photon shot noise as the main source of dephasing for further improvements.
- Fei Yan
- , Simon Gustavsson
- & William D. Oliver
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| Open AccessEnhancing electric-field control of ferromagnetism through nanoscale engineering of high-Tc MnxGe1−x nanomesh
Voltage control of magnetism in ferromagnetic semiconductor is appealing for spintronic applications, which is yet hindered by compound formation and low Curie temperature. Here, Nie et al. report electric-field control of ferromagnetism in MnxGe1−xnanomeshes with a Curie temperature above 400 K and controllable giant magnetoresistance.
- Tianxiao Nie
- , Jianshi Tang
- & Kang L. Wang
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Article
| Open AccessA quantum spin-probe molecular microscope
Single spin defects can allow high-resolution sensing of molecules under an applied magnetic field. Here, the authors propose a protocol for three-dimensional magnetic resonance imaging with angstrom-level resolution exploiting the dipolar field of a spin qubit, such as a diamond nitrogen-vacancy.
- V. S. Perunicic
- , C. D. Hill
- & L.C.L. Hollenberg
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Article
| Open AccessImaging and controlling plasmonic interference fields at buried interfaces
Visualizing surface plasmon polaritons at buried interfaces has remained elusive. Here, the authors develop a methodology to study the spatiotemporal evolution of buried near-fields within complex heterostructures, enabling the characterization of the next generation of plasmonic devices.
- Tom T. A. Lummen
- , Raymond J. Lamb
- & F. Carbone
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| Open AccessHigh-harmonic generation by field enhanced femtosecond pulses in metal-sapphire nanostructure
It has been suggested that strong field enhancement for high harmonic generation may be achievable with nano-antennas. Here, the authors show relevant field enhancement using a metal-sapphire nanostructure that provides a solid tip as the high harmonic emitter, replacing commonly used gaseous atoms.
- Seunghwoi Han
- , Hyunwoong Kim
- & Seung-Woo Kim
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Article
| Open AccessExperimental creation of quantum Zeno subspaces by repeated multi-spin projections in diamond
Repeated observations of quantum states inhibit coherent evolution through the Zeno effect, providing opportunities for controlling multi-qubit systems. Here the authors demonstrate that projecting joint observables of three spins in diamond creates quantum Zeno subspaces that suppress dephasing.
- N. Kalb
- , J. Cramer
- & T. H. Taminiau
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| Open AccessElectronic control of H+ current in a bioprotonic device with Gramicidin A and Alamethicin
Conventional electronics use electrons as charge carriers whereas biological systems use ions, confounding integration of electronics with biology. Here the authors show voltage-regulated flow of protons across a supported lipid bilayer using the ion channel Gramicidin A and the voltage-gated ion channel Alamethicin.
- Zahra Hemmatian
- , Scott Keene
- & Marco Rolandi
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| Open AccessBoosted output performance of triboelectric nanogenerator via electric double layer effect
The energy harvesting potential of triboelectric nanogenerators is currently limited by their output power. Here, the authors design a triboelectric nanogenerator inspired by lightning generation, featuring an electric double layer that delivers impressive charge separation and electric potential.
- Jinsung Chun
- , Byeong Uk Ye
- & Jeong Min Baik
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| Open AccessContextuality without nonlocality in a superconducting quantum system
Tests of the Bell-Kochen-Specker theorem aim at showing that the measurement statistics of a single qutrit are incompatible with noncontextual realism. Here, the authors use a superconducting qutrit with deterministic readouts to violate a noncontextuality inequality, ruling out several loopholes.
- Markus Jerger
- , Yarema Reshitnyk
- & Arkady Fedorov
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Article
| Open AccessA 17 GHz molecular rectifier
Molecular electronics holds promise to overcome scaling limits of conventional technologies, but is currently limited to low frequency operation. Here, Trasobares et al. show radio frequencies of up to 17.8 GHz in a molecular diode based on ferrocenyl undecanethiol self-assembled monolayers on gold nanodots.
- J. Trasobares
- , D. Vuillaume
- & N. Clément
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Article
| Open AccessUnsupervised vector-based classification of single-molecule charge transport data
The stochastic nature of single-molecule charge transport measurements requires collection of large data sets to capture their full complexity. Here, the authors adopt strategies from machine learning for the unsupervised classification of single-molecule charge transport data without a prioriassumptions.
- Mario Lemmer
- , Michael S. Inkpen
- & Tim Albrecht
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Article
| Open AccessQuantized conductance doubling and hard gap in a two-dimensional semiconductor–superconductor heterostructure
Interface transparency between 2D semiconductors and superconductors is a longstanding problem, seriously hindering potential applications. Here, using a new hybrid system, Kjaergaard et al. report quantized conductance doubling and a hard superconducting gap measured via a quantum point contact, indicating a near pristine interface.
- M. Kjaergaard
- , F. Nichele
- & C. M. Marcus
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Article
| Open AccessUnsupervised learning in probabilistic neural networks with multi-state metal-oxide memristive synapses
Artificial neural networks exhibit learning abilities and can perform tasks which are tricky for conventional computing systems, such as pattern recognition. Here, Serb et al. show experimentally that memristor arrays can learn reversibly from noisy data thanks to sophisticated learning rules.
- Alexander Serb
- , Johannes Bill
- & Themis Prodromakis
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Article
| Open AccessRadiative heat transfer exceeding the blackbody limit between macroscale planar surfaces separated by a nanosize vacuum gap
Evanescent coupling between surfaces separated by a distance smaller than the thermal wavelength can lead to radiative heat transfer greater than the blackbody limit. Here, the authors demonstrate this between two macroscopic-scale surfaces, paving the way to harnessing the effect in thermal devices.
- Michael P. Bernardi
- , Daniel Milovich
- & Mathieu Francoeur
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Article
| Open AccessInitiating and imaging the coherent surface dynamics of charge carriers in real space
The charge injected from the tip of a scanning tunnelling microscope quickly spreads across the surface and can manipulate distant adsorbates. Here, the authors use this nonlocal manipulation to probe the ultrafast ballistic dynamics and coherent evolution of the injected charge carrier.
- K. R. Rusimova
- , N. Bannister
- & P. A. Sloan
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Article
| Open AccessAtomically thin quantum light-emitting diodes
Atomically thin transition metal dichalcogenides hold promise as scalable single-photon sources. Here, the authors demonstrate all-electrical, single-photon generation in tungsten disulphide and diselenide, achieving charge injection into the layers, containing quantum emitters.
- Carmen Palacios-Berraquero
- , Matteo Barbone
- & Mete Atatüre
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Article
| Open AccessReal-time encoding and compression of neuronal spikes by metal-oxide memristors
The need for intelligent compression of big data, for example in neuroscience, has sparked interest in neuromorphic data processing. Here, Gupta et al.use memristors as event integrators to encode and compress neuronal spiking activity recorded by multi-electrode arrays.
- Isha Gupta
- , Alexantrou Serb
- & Themistoklis Prodromakis
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Article
| Open AccessDirect-write nanoscale printing of nanogranular tunnelling strain sensors for sub-micrometre cantilevers
Reducing the size of cantilever-based sensors increases the sensitivity and detection speed of techniques such as atomic force microscopy. Here, the authors demonstrate a nanomechanical readout method that can be easily scaled down in size by using electron co-tunnelling through a nanogranular metal.
- Maja Dukic
- , Marcel Winhold
- & Georg E. Fantner
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Article
| Open AccessMolecular transport through large-diameter DNA nanopores
Artificial DNA membrane channels are promising molecular devices for biotechnology but suffer from low affinity for lipid bilayers. Here, the authors report a large DNA nanopore that spontaneously inserts into a flat lipid membrane, driven by engineered hydrophobic or streptavidin-biotin interactions.
- Swati Krishnan
- , Daniela Ziegler
- & Friedrich C. Simmel
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| Open AccessPrimary thermometry triad at 6 mK in mesoscopic circuits
Mesoscopic electrical circuits are an ideal platform to explore quantum phenomena, but this requires cooling the electrons to very low temperature, which is challenging. Here, the authors employ three different in situthermometers to report electronic quantum transport at 6mK in a micrometer-scale circuit.
- Z. Iftikhar
- , A. Anthore
- & F. Pierre