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| Open AccessWide field-of-hearing metalens for aberration-free sound capture
Achieving a wide angular response in single layer acoustic metalenses is challenging. By leveraging perfect acoustic symmetry conversion, the authors realize an aberration free metalens with a wide field-of-hearing, up to 140 degrees.
- Dongwoo Lee
- , Beomseok Oh
- & Junsuk Rho
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| Open AccessUltrastiff metamaterials generated through a multilayer strategy and topology optimization
High-performance mechanical metamaterials have been designed through a multilayer strategy and topology optimization, showing capability in approaching the theoretical stiffness limit, as well as prospects in treating multiphysics problems
- Yang Liu
- , Yongzhen Wang
- & Jianbin Du
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| Open AccessProgramming mechanics in knitted materials, stitch by stitch
Knitted fabrics are prized for their stretchability, breathability, and long-wearability in everyday life. This study combines experiments and simulations to present a micromechanical approach to understanding the origin of the anisotropic elasticity of four canonical patterns of knitted fabrics.
- Krishma Singal
- , Michael S. Dimitriyev
- & Elisabetta A. Matsumoto
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| Open AccessLarge-scale modular and uniformly thick origami-inspired adaptable and load-carrying structures
In this work, authors establish general conditions for flat foldability, developability, and uniform thickness in origami-inspired structures and introduce a large-scale modular design capable of deploying into meter-scale configurations, adapting to various shapes, and supporting significant loads.
- Yi Zhu
- & Evgueni T. Filipov
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| Open AccessElectrothermally controlled origami fabricated by 4D printing of continuous fiber-reinforced composites
Effective active origami capable of on-demand modulation are limited by challenges such as limited load-bearing capacity and transformable states. Here, authors report fiber-reinforced composites for controlled electrothermal origami with excellent mechanical performance and spatiotemporal controllability.
- Yaohui Wang
- , Haitao Ye
- & Yi Xiong
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| Open AccessWood-inspired metamaterial catalyst for robust and high-throughput water purification
Continuous industrialization and human activities have led to severe water quality deterioration. Here, a structure-function integrated system is developed by Douglas fir wood inspired metamaterial catalysts with robust and high throughput water purification performances.
- Lei Zhang
- , Hanwen Liu
- & Jian Lu
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| Open AccessSimultaneous enhancement of strength and conductivity via self-assembled lamellar architecture
Simultaneous increase of mechanical and physical properties is highly desirable, but challenging for bimetallic materials. Here, the authors use W-Cu as an example to achieve both high strength and conductivity of the bimetal with a large plasticity by a self-assembled lamellar architecture.
- Tielong Han
- , Chao Hou
- & Xiaoyan Song
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| Open AccessIntrinsic factors responsible for brittle versus ductile nature of refractory high-entropy alloys
Poor ductility is a major drawback of otherwise promising refractory high-entropy alloys (RHEAs) for ultrahigh temperature applications. Here, the authors show how ductility can be enhanced by adding HCP elements to BCC RHEAs, which is a relatively simple way to optimize mechanical properties.
- Tomohito Tsuru
- , Shu Han
- & Haruyuki Inui
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| Open AccessTunable afterglow for mechanical self-monitoring 3D printing structures
Organic afterglow materials have potential in self-monitoring applications but it is challenging to design materials with desired properties. Here, the authors report the development of a lifetime tunable organic afterglow system for use in mechanical self-monitoring 3D printed structures.
- Rongjuan Huang
- , Yunfei He
- & Wei Huang
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Article
| Open AccessRejuvenation as the origin of planar defects in the CrCoNi medium entropy alloy
High and medium-entropy alloys have shown excellent mechanical performance, yet the role of short-range order (SRO) on these properties has been unclear. Here, the authors demonstrate that the reduction of SRO by deformation leads to rejuvenation, explaining their remarkable damage tolerance.
- Yang Yang
- , Sheng Yin
- & Andrew M. Minor
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| Open AccessTough double network hydrogels with rapid self-reinforcement and low hysteresis based on highly entangled networks
Tough hydrogels commonly utilise energy dissipation mechanisms, but this can lead to challenges in achieving low hysteresis. Here, the authors report a hydrogel with a highly entangled double network that allows reversibility following stretching.
- Ruixin Zhu
- , Dandan Zhu
- & Xinling Wang
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Article
| Open AccessUltrastrong and ductile steel welds achieved by fine interlocking microstructures with film-like retained austenite
Weld integrity and performance determine lifetime and safety of structures. Here, the authors report advances in weld quality of ultrahigh strength steels resulting from fine interlocking weld microstructures with film-like retained austenite by utilizing Nb and Cr instead of Ni.
- Joonoh Moon
- , Gyuyeol Bae
- & Dirk Ponge
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Article
| Open AccessDiffusive kinks turn kirigami into machines
Kinks define boundaries between distinct configurations of a material. Here, the authors reveal the emergence of propagating kinks in purely dissipative kirigami and show that such structures can shape-change into different textures depending on how fast they are stretched enabling basic mechanical tasks.
- Shahram Janbaz
- & Corentin Coulais
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Article
| Open AccessElemental partitioning-mediated crystalline-to-amorphous phase transformation under quasi-static deformation
The transformation induced plasticity phenomenon is usually diffusionless. Here, the authors introduce elemental partitioning mediated crystalline-to-amorphous phase transformation in a crystal-glass nanolaminated composite, realizing ultrahigh strength and large plasticity.
- Ge Wu
- , Chang Liu
- & Zhi-Wei Shan
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Article
| Open AccessAccurate additive manufacturing of lightweight and elastic carbons using plastic precursors
This work reports a simple method to produce 3D printed complex carbon materials with low dimensional shrinkage (<4%) from printed to carbonized state, using commercially available carbon fiber-reinforced polypropylene precursors and a fused filament fabrication-based process.
- Paul Smith
- , Jiayue Hu
- & Zhe Qiang
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| Open AccessSub-micro porous thin polymer membranes for discriminating H2 and CO2
The fabrication of polymeric membranes with high permeance and remarkable selectivity for simultaneous H2 purification and CO2 capture is challenging. Here, the authors design a polymer membrane with sub-micro pores via controlled transformation of amine-linked polymer films into benzimidazole- and amine-linked polymer layers.
- Xueru Yan
- , Tianqi Song
- & Xinlei Liu
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| Open AccessAtomic-scale observation of nucleation- and growth-controlled deformation twinning in body-centered cubic nanocrystals
Deformation twinning in body-centered cubic (BCC) metals is generally believed to be controlled by twin nucleation, but facilitated by rapid twin growth once the nucleation energy barrier is overcome. Here, the authors demonstrate both nucleation- and growth-controlled twinning modes in BCC Ta nanocrystals depending on the crystal size.
- Li Zhong
- , Yin Zhang
- & Scott X. Mao
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| Open AccessUnusual flexibility of transparent poly(methylsilsesquioxane) aerogels by surfactant-induced mesoscopic fiber-like assembly
Aerogels are mechanically friable despite their attractive properties such as visible-light transparency and low thermal conductivity. Here the authors show mechanically flexible, highly transparent aerogels based on fiber-like pore skeletons.
- Ryota Ueoka
- , Yosuke Hara
- & Kazuyoshi Kanamori
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| Open AccessStretchable and negative-Poisson-ratio porous metamaterials
In this work, authors demonstrate highly stretchable conductive porous elastomers that can achieve up to 1200% strain with low or negative Poisson’s ratios by uniaxial, biaxial, and triaxial hot-pressing strategies.
- Xiaoyu Zhang
- , Qi Sun
- & Guoqing Zu
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Article
| Open AccessA micro-architectured material as a pressure vessel for green mobility
A shellular is a micro-architectured material, composed of a continuous smooth-curved thin shell in the form of a triply periodic minimal surface. Here, authors propose schellular designs applied to pressure vessels and demonstrate its competitive practical features against spherical and cylindrical vessels.
- Yoon Chang Jeong
- , Seung Chul Han
- & Kiju Kang
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| Open Access3D printing of self-healing personalized liver models for surgical training and preoperative planning
High-fidelity personalized anatomical models can offer invaluable support for precision medicine. Here, the authors show the 3D printing of self-healing liver models, which can be resected in a trial and-error manner for surgical training to enhance the safety of hepatic surgery.
- Yahui Lu
- , Xing Chen
- & Yuhua Zhang
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| Open AccessLarge mechanical properties enhancement in ceramics through vacancy-mediated unit cell disturbance
Ceramics are very brittle and hard to be plastically deformed. Here, the authors report a unit-cell scale disturbance mechanism to improve the deformation ability of ceramics and ultimately achieve large mechanical property enhancement.
- Zhuo Chen
- , Yong Huang
- & Zaoli Zhang
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| Open AccessHighly stretchable polymer semiconductor thin films with multi-modal energy dissipation and high relative stretchability
Stretchable polymer semiconductors with high mechanical and electrical properties are challenging to develop. Wu et al. show that reversible molecular ordering under strain important for performance optimization and relative stretchability can be used to compare the relative strain tolerance of materials.
- Hung-Chin Wu
- , Shayla Nikzad
- & Zhenan Bao
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| Open AccessRevealing the room temperature superplasticity in bulk recrystallized molybdenum
Body-centered cubic refractory metals are known to exhibit excellent high-temperature strength, but often suffer from brittle fracture. Here, the authors produce a bulk pure Mo with stable fine-grain structure after powder metallurgy, Y-type hot rolling and ultra-high temperature annealing (1000~1700 °C) that exhibits room temperature superplasticity.
- Wenshuai Chen
- , Xiyao Li
- & Zenglin Zhou
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| Open AccessOrigamic metal-organic framework toward mechanical metamaterial
This work introduces a 2D porphyrinic metal-organic framework based on DCS origami tessellation, displaying unique folding behavior inspired by origami mechanics. This breakthrough paves the way for MOFs toward mechanical metamaterials.
- Eunji Jin
- , In Seong Lee
- & Wonyoung Choe
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| Open AccessPreferential ice growth on grooved surface for crisscross-aligned graphene aerogel with large negative Poisson’s ratio
Ice formation on grooved surfaces is ubiquitous, but controlling orientation is difficult due to lack of mechanistic insight. Here, the authors observed oriented growth using graphene oxide nanosheets as probes, revealing the effect of groove size, and programmed ice growth to fabricate freeze-cast metamaterials.
- Meng Li
- , Nifang Zhao
- & Hao Bai
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| Open AccessExploration of truss metamaterials with graph based generative modeling
Optimisation tasks in the inverse design of metamaterials with machine learning were limited due to the representations of generative models. Here the author comments a recent publication in Nature Communications which generates a latent space representation that unlocks non-linear optimisations.
- Angkur Jyoti Dipanka Shaikeea
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| Open AccessUnifying the design space and optimizing linear and nonlinear truss metamaterials by generative modeling
Truss metamaterials are ubiquitous but their vast design space is far from fully explored. Here, authors use machine learning to present a unified, continuous latent space description, enabling the rapid generation of trusses with tunable or exceptional linear and nonlinear mechanical properties.
- Li Zheng
- , Konstantinos Karapiperis
- & Dennis M. Kochmann
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| Open AccessWoven organic crystals
The entanglement of fibrous elements produces flexible structures with enhanced strength and resilience to abrasion. Here, the authors report the weaving of organic crystals into flexible and robust patches with plain, twill, and satin topologies of arbitrary porosity, expanding one-dimensional crystals into flexible, two-dimensional planar structures with potential for future applications in flexible electronics.
- Linfeng Lan
- , Liang Li
- & Hongyu Zhang
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| Open AccessRoom-temperature super-elongation in high-entropy alloy nanopillars
Small-scale metallic materials often suffer from a lack of tensile ductility. Here, the authors report an unusual room-temperature super-elongation in CoCrFeNi nanopillars from spatial and synergistic coordination of deformation twinning and dislocation slips due to chemical heterogeneities.
- Qian Zhang
- , Ranming Niu
- & Xiaoyan Li
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| Open AccessLead-free Zr-doped ceria ceramics with low permittivity displaying giant electrostriction
Electrostrictors are materials that develop mechanical strain proportional to the square of the applied electric field. Here authors report. Zr-doped-Ceria as a new lead-free electrostrictive material with a similar electrostriction coefficient to the best electrostrictor material currently in use.
- Maxim Varenik
- , Boyuan Xu
- & Igor Lubomirsky
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| Open AccessStrong yet flexible ceramic aerogel
Mechanically robust, flexible and thermally insulating ceramic aerogels are challenging to obtain due to the conflicting nature of these properties. Here the authors resolved these contradictions and developed a strong yet flexible aerogel, for application in extreme conditions, by laminated structure design.
- Lei Su
- , Shuhai Jia
- & Hongjie Wang
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| Open AccessAdditive manufacturing of alloys with programmable microstructure and properties
The traditional way of beating metals to improve their properties is not practical to 3D printed parts with intricate geometry. Here, the authors demonstrate how to program microstructural modifications of metals site-specifically during 3D printing to tune their properties.
- Shubo Gao
- , Zhi Li
- & Matteo Seita
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| Open AccessA reprogrammable mechanical metamaterial with origami functional-group transformation and ring reconfiguration
Programmability is a key property for multifunctional metamaterials, but it is limited by homo-element. Here, the authors show a mechanical metamaterials with heterogeneous elements, achieving various mechanical behaviours by functional group transformation and ring configuration.
- Xinyu Hu
- , Ting Tan
- & Zhimiao Yan
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Article
| Open AccessAutonomous self-healing organic crystals for nonlinear optics
There are many potential applications for non-centrosymmetric molecular crystals, but due to their typical brittle nature, efficiency of applications declines on prolonged use. Here, the authors report an autonomous self-healing ability of dibenzoate derivative single crystals that can retain its non-linear optical response.
- Saikat Mondal
- , Pratap Tanari
- & C. Malla Reddy
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| Open AccessLight-oriented 3D printing of liquid crystal/photocurable resins and in-situ enhancement of mechanical performance
Complex computerized geometries can be obtained by additive manufacturing. However, the printing of purely three-dimensional polymer shapes possesses inherent poor mechanical stability. Here, the authors overcome this drawback by the light-driven orientation of liquid crystals to guide the alignment of acrylate prepolymers along the direction parallel to UV light vibrations.
- Xiaolu Sun
- , Shaoyun Chen
- & Dongxian Zhuo
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| Open AccessGrowing recyclable and healable piezoelectric composites in 3D printed bioinspired structure for protective wearable sensor
Smart monitoring devices with integrated mechanical protection and piezoelectric induction are limited. Here, the authors report a strategy to grow piezoelectric Rochelle salt crystals in 3D-printed cuttlebone-inspired structures to produce smart monitoring devices with integrated mechanical protection and electrical sensing capability.
- Qingqing He
- , Yushun Zeng
- & Yang Yang
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| Open AccessThin lamellar films with enhanced mechanical properties for durable radiative cooling
Practical application of radiative cooling technology in harsh outdoor conditions remains challenging. Here, the authors develop a lamellar ANFs/Mica@TiO2 composite via a “solvent exchange-reprotonation” process enabling durable outdoor cooling.
- Lianhu Xiong
- , Yun Wei
- & Hua Deng
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| Open AccessTensorial stress-plastic strain fields in α - ω Zr mixture, transformation kinetics, and friction in diamond-anvil cell
Fields of stress and plastic strain tensors in a sample under high pressures in diamond-anvil cells are important, but measuring them is difficult. Here, the authors suggest a coupled experimental-analytical-computational approach to measure them before, during, and after α−ω transformation in Zr.
- Valery I. Levitas
- , Achyut Dhar
- & K. K. Pandey
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Article
| Open AccessSmart dynamic hybrid membranes with self-cleaning capability
The performance of membrane desalination of seawater is hampered by fouling. Here the authors develop smart gating hybrid membranes by surface coating with polymer-embedded thermosalient crystals. These membranes enhance pure water flux by over 40% in saltwater desalination by osmotic distillation.
- Elvira Pantuso
- , Ejaz Ahmed
- & Gianluca Di Profio
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| Open AccessSuperhard bulk high-entropy carbides with enhanced toughness via metastable in-situ particles
High-entropy carbides (HECs) with high hardness usually suffer from low fracture toughness. Here, the authors demonstrate a metastability engineering strategy for toughening superhard HECs by introducing in situ metastable ceramic particles, which are transformable under mechanical loading.
- Jiaojiao Hu
- , Qiankun Yang
- & Zhiming Li
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Article
| Open AccessChemical inhomogeneity–induced profuse nanotwinning and phase transformation in AuCu nanowires
How the random solid solution (RSS) alloys accommodate plasticity and overcome strength-ductility trade-off remain unresolved. Here, the authors reveal atomic-scale plastic deformation of AuCu alloy, which shed light on the effect of chemical inhomogeneity on plastic deformation of RSS alloys.
- Chengpeng Yang
- , Bozhao Zhang
- & Xiaodong Han
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Article
| Open AccessUnexpected doping effects on phonon transport in quasi-one-dimensional van der Waals crystal TiS3 nanoribbons
Doping generally hinders phonon transport. Here, authors significantly increase the thermal conductivity of TiS3 nanoribbons through doping, originating from the intensified bonding strength along the molecular chain direction without distorting the one-dimensional structure induced by doped atoms.
- Chenhan Liu
- , Chao Wu
- & Yunfei Chen
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Article
| Open AccessJanus particle-engineered structural lipiodol droplets for arterial embolization
Embolization is one of the most promising strategies for clinical disease treatments, however, the existing embolic materials normally have poor embolization effectiveness. Here, the authors report Janus particle-engineered structural lipiodol droplets by programming the self-assembly of Janus particles at the lipiodol-water interface to achieve highly efficient renal embolization.
- Sijian Tao
- , Bingquan Lin
- & Jun-Bing Fan
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Article
| Open AccessHighly sensitive and broadband meta-mechanoreceptor via mechanical frequency-division multiplexing
There’s a trade-off between the sensitivity and bandwidth for mechanics guided sensor designs. Here, authors report a mechanical sensor comprised of piezoelectric resonators with near infinite effective piezoelectric coefficients, leading to highly sensitive and broadband micromotion sensing.
- Chong Li
- , Xinxin Liao
- & Qingbo He
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Article
| Open AccessLarge-scale assembly of isotropic nanofiber aerogels based on columnar-equiaxed crystal transition
In this work, the authors present an ice-templating strategy to produce large-scale isotropic nanofiber aerogels using a unique process of freezing the material on a rotating cryogenic drum surface, crushing it, and then re-casting the nanofiber slurry enabling high-throughput and design flexibility.
- Lei Li
- , Yiqian Zhou
- & Hui Wu
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Article
| Open AccessElectrically insulating PBO/MXene film with superior thermal conductivity, mechanical properties, thermal stability, and flame retardancy
Constructing thermally conductive but electrically insulating composites remains a challenge. Here, Ti3C2 MXene is combined in a nacre-like structure with the polymer PBO to form such materials, also exhibiting high thermal stability and flame retardancy.
- Yong Liu
- , Weizhi Zou
- & Jian Xu
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Article
| Open AccessProtein fibers with self-recoverable mechanical properties via dynamic imine chemistry
Manipulating the internal interactions within biological fibers to tune macroscopic properties is important but challenging, and can limit applications. Here, the authors report the use of dynamic imine chemistry for engineering molecular interactions and forming strong and tough protein fibers.
- Jing Sun
- , Haonan He
- & Kai Liu
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| Open AccessIn-memory mechanical computing
Here, Mei and Chen propose an in-memory mechanical computing architecture with simplified and reduced data exchange, where computing occurs within mechanical memory units, to facilitate the design of intelligent mechanical systems.
- Tie Mei
- & Chang Qing Chen