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| Open AccessUltrastrong exciton-plasmon couplings in WS2 multilayers synthesized with a random multi-singular metasurface at room temperature
Here, the authors fabricate a metasurface with nanometre-sized plasmonic hotspots that interact coherently with WS2 excitons, achieving ultrastrong exciton-plasmon coupling.
- Tingting Wu
- , Chongwu Wang
- & Yu Luo
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Article
| Open AccessUltrafast photoluminescence and multiscale light amplification in nanoplasmonic cavity glass
This article presents a unique nanocomposite plasmonic-excitonic glass with extraordinary amplified optical properties: ultra-narrow photoluminescence (FWHM = 13 nm) and ultrashort photoluminescence lifetime (90 ps) at room temperature
- Piotr Piotrowski
- , Marta Buza
- & Dorota A. Pawlak
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Article
| Open AccessA terahertz meta-sensor array for 2D strain mapping
The researchers showcase a flexible meta-sensor array based on classical Mie resonance, enabling precise detection of in-plane strain direction and magnitude using dynamically transmitted terahertz (THz) signals. The sensor array holds immense promise for the real-life applications as it possesses high sensor density and has a very large size up to (110 ×130 mm2).
- Xueguang Lu
- , Feilong Zhang
- & Qiang Cheng
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Article
| Open AccessObservation of spatiotemporal optical vortices enabled by symmetry-breaking slanted nanograting
A microscale platform composed of a slanted nanograting is experimentally demonstrated to efficiently generate spatiotemporal optical vortex. This approach paves the way towards an integrated system for ultrafast pulse shaping.
- Pengcheng Huo
- , Wei Chen
- & Ting Xu
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Article
| Open AccessA 2D chiral microcavity based on apparent circular dichroism
Here the authors induce asymmetric transmission in planar Fabry–Pérot microcavities by embedding organic thin films exhibiting apparent circular dichroism (ACD), an optical phenomenon based on 2D chirality.
- Tzu-Ling Chen
- , Andrew Salij
- & Randall H. Goldsmith
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Article
| Open AccessWide field-of-hearing metalens for aberration-free sound capture
Achieving a wide angular response in single layer acoustic metalenses is challenging. By leveraging perfect acoustic symmetry conversion, the authors realize an aberration free metalens with a wide field-of-hearing, up to 140 degrees.
- Dongwoo Lee
- , Beomseok Oh
- & Junsuk Rho
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Article
| Open AccessNonlinear optical diode effect in a magnetic Weyl semimetal
Here the authors demonstrate a broadband nonlinear optical diode effect and its electric control in the magnetic Weyl semimetal CeAlSi. Their findings advance ongoing research to identify novel optical phenomena in topological materials.
- Christian Tzschaschel
- , Jian-Xiang Qiu
- & Su-Yang Xu
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Article
| Open AccessLaMg6Ga6S16: a chemical stable divalent lanthanide chalcogenide
Synthesising chemically stable divalent lanthanide compounds is still faced by great challenges. Here, by using octahedra coupling tetrahedra single/double chains to construct an octahedral crystal field, authors synthesised a stable crystalline La(II)-chalcogenide, LaMg6Ga6S16.
- Yujie Zhang
- , Jiale Chen
- & Hongwei Yu
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Article
| Open AccessCompact meta-differentiator for achieving isotropically high-contrast ultrasonic imaging
High-contrast ultrasonic imaging holds significant importance in biomedical and engineering applications. Here, the authors present a compact spatial differentiator tailored for underwater isotropic edge-enhanced imaging, facilitating the realization of high-contrast ultrasonic imaging.
- Yurou Jia
- , Suying Zhang
- & Xiaojun Liu
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Article
| Open AccessIntelligent wireless power transfer via a 2-bit compact reconfigurable transmissive-metasurface-based router
The rapid emergence of the Internet of Things has led to new power supply challenges. Here, authors propose a compact wireless power transfer framework that can intelligently deliver wireless power to devices in dynamic environments and simultaneously transfer information.
- Wenzhi Li
- , Qiyue Yu
- & Jiaran Qi
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Article
| Open AccessObservation of naturally canalized phonon polaritons in LiV2O5 thin layers
Canalized polaritons are light-matter excitations characterized by intrinsic collimation of electromagnetic energy along a specific crystal axis. Here, the authors report the observation of intrinsically canalized phonon polaritons in a single thin layer of a van der Waals crystal, LiV2O5.
- Ana I. F. Tresguerres-Mata
- , Christian Lanza
- & Pablo Alonso-González
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Article
| Open AccessQuantifying the interfacial triboelectricity in inorganic-organic composite mechanoluminescent materials
Mechanoluminescence enables sensing applications of mechanical stimuli. Here, the authors reveal the importance of interfacial triboelectricity to this phenomenon in inorganic-organic composite materials.
- Xin Pan
- , Yixi Zhuang
- & Rong-Jun Xie
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Article
| Open AccessHigh-security learning-based optical encryption assisted by disordered metasurface
In this work, the employment of disordered metasurface as an ultra-stable and actively polarized speckle generator in a passive manner, coupled with a double-secure treatment to the plaintext, enables a highly secure speckle-based cryptosystem.
- Zhipeng Yu
- , Huanhao Li
- & Puxiang Lai
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Article
| Open AccessDefect-induced helicity dependent terahertz emission in Dirac semimetal PtTe2 thin films
Defect engineering of topological materials provides an avenue for the controllable manipulation of optoelectronic properties. Here, the authors introduce a defect gradient into a Dirac semimetal to control the Berry curvature dipole-driven THz emission in the material.
- Zhongqiang Chen
- , Hongsong Qiu
- & Xuefeng Wang
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Article
| Open AccessTunable anisotropic van der Waals films of 2M-WS2 for plasmon canalization
Anisotropic light-matter excitations in van der Waals materials are expected to have an impact on nanophotonics applications. Here, the authors report the observation of canalized in-plane mid-infrared plasmons in the semimetallic phase of WS2 and demonstrate their electrical tunability via ion intercalation.
- Qiaoxia Xing
- , Jiasheng Zhang
- & Hugen Yan
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Article
| Open AccessAmber rainbow ribbon effect in broadband optical metamaterials
The researchers showcased a negative Goos-Hänchen effect in film samples across the entire visible spectrum and discovered an amber rainbow ribbon and an optical black hole where little light leaks out due to perfect back reflection.
- Jing Zhao
- , Xianfeng Wu
- & Xiaopeng Zhao
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Article
| Open AccessLarge exchange-driven intrinsic circular dichroism of a chiral 2D hybrid perovskite
Li et al. report large circular dichroism in 2D chiral perovskite single crystals, arises from the inorganic sublattice, instead of chiral ligands, driven by electron-hole exchange interactions. This is evidenced by both reflective circular dichroism spectroscopy and ab initio theory.
- Shunran Li
- , Xian Xu
- & Peijun Guo
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Article
| Open AccessCapturing ion trapping and detrapping dynamics in electrochromic thin films
Ion trapping has been found to be responsible for the performance degradation in electrochromic oxide thin films. This paper visualizes ion trapping and detrapping dynamics, and provides a general picture of electrochromism in amorphous WO3.
- Renfu Zhang
- , Qinqi Zhou
- & Rui-Tao Wen
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Article
| Open AccessUltra-compact exciton polariton modulator based on van der Waals semiconductors
Miniaturized and efficient optical modulators are desired for data transmission, processing and communication. Here, the authors report the fabrication of exciton-polariton Mach–Zehnder modulators based on thin WS2 waveguides with a footprint of ~30 μm², modulation ratio up to −6.20 dB and nanosecond response times.
- Seong Won Lee
- , Jong Seok Lee
- & Su-Hyun Gong
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Article
| Open AccessTwisted moiré conductive thermal metasurface
Authors control heat transfer through twisting moiré conductive thermal metasurface, showcasing the potential for manipulating thermal conductivity and temperature gradients with imitated magic angles, thereby realizing multifunctional thermal metadevices.
- Huagen Li
- , Dong Wang
- & Cheng-Wei Qiu
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| Open AccessWandering principal optical axes in van der Waals triclinic materials
Principal optical axes define light-matter interactions in crystals and they are usually assumed to be stationary. Here, the authors report the observation of wavelength-dependent principal optical axes in ternary van der Waals crystals (ReS2 and ReSe2), leading to wavelength-switchable propagation directions of their waveguide modes.
- Georgy A. Ermolaev
- , Kirill V. Voronin
- & Kostya S. Novoselov
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Article
| Open AccessOrbitronics: light-induced orbital currents in Ni studied by terahertz emission experiments
Several recent works have highlighted the importance of the orbital currents in transferring angular momentum within materials. In combination with spin-orbit coupling, such orbital currents can be used to alter the magnetization of a material. Herein, the authors demonstrate the inverse effect, showing orbital current driven terahertz emission in Nickel based heterostructures.
- Yong Xu
- , Fan Zhang
- & Weisheng Zhao
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Article
| Open AccessColor construction of multi-colored carbon fibers using glucose
Color construction of black carbon fibers is a challenge due to their stable physicochemical properties. Here, the authors demonstrate the tunable structural color of carbon fibers endowed by the dynamic growth of carbon spheres using glucose.
- Sijie Zhou
- , Chunhua Zhang
- & Weilin Xu
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Article
| Open AccessBoosting exciton mobility approaching Mott-Ioffe-Regel limit in Ruddlesden−Popper perovskites by anchoring the organic cation
Exciton transport in 2D Ruddlesden−Popper perovskite plays a key role for their optoelectronic performance. Here, authors significantly enhance free exciton mobilities in exfoliated thin flakes by anchoring butyl ammonium cation with polymethyl methacrylate, which also improves lattice rigidity.
- Yiyang Gong
- , Shuai Yue
- & Xinfeng Liu
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Article
| Open AccessAll-in-one, all-optical logic gates using liquid metal plasmon nonlinearity
Multifunctional all-optical logic gate (AOLG) with broadband-based massively parallel processing is desirable for high-speed optical processor. Here, authors propose a reconfigurable all-in-one ultra-broadband AOLG with experimentally achieving 9 fundamental Boolean logics in a single configuration.
- Jinlong Xu
- , Chi Zhang
- & Lin Zhou
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Article
| Open AccessAnomalously bright single-molecule upconversion electroluminescence
The efficiency of upconversion electroluminescence remains very low for single-molecule emitters. Here, the authors report over one order of magnitude improvement in the emission efficiency via engineering energy-level alignments for triplet relayed upconversion involving only carrier injection.
- Yang Luo
- , Fan-Fang Kong
- & Zhen-Chao Dong
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Article
| Open AccessVision-driven metasurfaces for perception enhancement
Authors showcase a framework for visual perception enhancement system based on vision-driven metasurfaces. It can help humans obtain information in multiple frequency bands and allows the metasurface platform with more interesting functions.
- Tianshuo Qiu
- , Qiang An
- & Shaobo Qu
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Article
| Open AccessMeasuring entanglement entropy and its topological signature for phononic systems
Entanglement entropy exhibits rich phenomenology connected to different kinds of phases in condensed matter. Here, the authors confirm some of these predictions by experimentally probing nonlocal correlations in 1D and 2D phononic crystal based on interconnected resonating acoustic cavities.
- Zhi-Kang Lin
- , Yao Zhou
- & Jian-Hua Jiang
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Article
| Open AccessDynamic light manipulation via silicon-organic slot metasurfaces
In this work, the authors present an active optical metasurface based on a silicon-organic platform. The metasurface can modulate the amplitude of a reflected beam via electric voltage actuation lower than ± 17V.
- Tianzhe Zheng
- , Yiran Gu
- & Andrei Faraon
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Article
| Open AccessTunable templating of photonic microparticles via liquid crystal order-guided adsorption of amphiphilic polymers in emulsions
The role of polymers in stabilizing liquid crystal (LC)-water interfaces is well studied but how the LC affects stabilizers is not fully explored yet. Here, Ma et al. show that amphiphilic polymers change their behavior when the LC is heated towards its transition to the isotropic state, and propose that this is due to an entropic repulsion active at low temperatures where the orientationally ordered LC restricts the mobility of the flexible polymer chains.
- Xu Ma
- , Yucen Han
- & Jan P. F. Lagerwall
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Article
| Open AccessGiant electric field-induced second harmonic generation in polar skyrmions
Electric modulation of second harmonic generation finds applications in integrated photonics. Here, authors introduce electric field-induced second harmonic generation by polar skyrmions in PbTiO3/SrTiO3 superlattices with giant modulation depth.
- Sixu Wang
- , Wei Li
- & Qian Li
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Article
| Open AccessDual-color emissive OLED with orthogonal polarization modes
The authors present a switchable dual colour orthogonal linear polarized OLED by internally integrating a nanograting for selective diffraction of optical modes, which is appealing for applications including polarisation-encrypted colourful optical images and autostereoscopic naked-eye 3D displays.
- Ruixiang Chen
- , Ningning Liang
- & Tianrui Zhai
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Article
| Open AccessVisualizing the interfacial-layer-based epitaxial growth process toward organic core-shell architectures
Organic heterostructures with controlled geometry on the micro and nanoscale are important in nanotechnology, but epitaxial growth processes with high lattice mismatching are challenging to achieve. Here, the authors report a visualisation process for morphology evolution on epitaxial growth.
- Ming-Peng Zhuo
- , Xiao Wei
- & Liang-Sheng Liao
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Article
| Open AccessRapid synthesis of phosphor-glass composites in seconds based on particle self-stabilization
Phosphor-glass composites can serve as efficient and stable photonic converters, but their synthesis generally requires harsh and time-consuming procedures. Here, the authors report an alternative synthesis route that requires only a few seconds and is based on particle self-stabilization.
- Yongsheng Sun
- , Yuzhen Wang
- & Zhiguo Xia
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Article
| Open AccessSlow light topological photonics with counter-propagating waves and its active control on a chip
Topological slow light is of fundamental importance for science and technology. Here the authors reveal that the presence of magnetic phase vortices along with glide symmetric interfaces is crucial for the existence of slow light modes in topological valley photonic crystal waveguide.
- Abhishek Kumar
- , Yi Ji Tan
- & Ranjan Singh
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Article
| Open AccessAnisotropic carrier dynamics and laser-fabricated luminescent patterns on oriented single-crystal perovskite wafers
Based on differently-oriented MAPbBr3 single-crystal wafers, the authors revealed anisotropic carrier dynamics by using angle-resolved pump-probe technique, and the microstructural mechanism of the femtosecond laser-induced emission enhancement
- Chao Ge
- , Yachao Li
- & Yang Liu
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Article
| Open AccessSwitchable unidirectional emissions from hydrogel gratings with integrated carbon quantum dots
Directional emission of photoluminescence is an emerging technique for light-emitting fields and nanophotonics. Here, the authors demonstrate a hydrogel grating with integrated quantum dots for switchable unidirectional emission tuning.
- Chenjie Dai
- , Shuai Wan
- & Zhongyang Li
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Article
| Open AccessA dual-selective thermal emitter with enhanced subambient radiative cooling performance
Radiative cooling is a sustainable subambient cooling technology. Here, authors show a scalable and practical design of a dual-selective thermal emitter that is shown to have enhanced radiative cooling potential over existing typical designs.
- Xueke Wu
- , Jinlei Li
- & Rufan Zhang
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Article
| Open AccessEfficient, narrow-band, and stable electroluminescence from organoboron-nitrogen-carbonyl emitter
Multi-resonance thermally activated delayed fluorescent emitters composed of only period-2 elements are important for achieving comprehensive performances. Here, authors report hybridization of organoboron-nitrogen and carbonyl groups in the emitter to achieve a long device operational stability.
- Ying-Chun Cheng
- , Xun Tang
- & Xiao-Hong Zhang
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Article
| Open AccessHelical-caging enables single-emitted large asymmetric full-color circularly polarized luminescence
Circularly polarised luminescence (CPL) is essential for asymmetric synthetic photochemistry. Here, the authors integrate white quantum dots with chiral nematic liquid crystal or liquid crystal polymer to achieve single-emitted tuneable full-colour or white CPL for enantioselective polymerization.
- Yajie Zhou
- , Yaxin Wang
- & Taotao Zhuang
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Perspective
| Open AccessPlanar hyperbolic polaritons in 2D van der Waals materials
In this Perspective, the authors illustrate the physics of hyperbolic polaritons in anisotropic 2D and 1D materials, proposing new potential material candidates, forward looking opportunities and technological applications.
- Hongwei Wang
- , Anshuman Kumar
- & Tony Low
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Article
| Open AccessMid-infrared supermirrors with finesse exceeding 400 000
The researchers showcase all-crystalline and hybrid mid-infrared supermirrors with the lowest optical losses ever demonstrated in this wavelength range, representing an unprecedented improvement over any existing mirrors made with any production technology.
- Gar-Wing Truong
- , Lukas W. Perner
- & Garrett D. Cole
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Article
| Open AccessReal-data-driven real-time reconfigurable microwave reflective surface
The authors demonstrate how flexible metasurfaces powered by artificial neural network can dynamically manipulate the EM scattering behavior from an arbitrary surface - an ultimate ambition for many EM stealth and communication problems.
- Erda Wen
- , Xiaozhen Yang
- & Daniel F. Sievenpiper
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Article
| Open Access3.5 × 3.5 μm2 GaN blue micro-light-emitting diodes with negligible sidewall surface nonradiative recombination
Here Wang et al. demonstrate the fabrication of GaN micro-light emitting diodes with a low rate of efficiency decrease in low current density regions, these features are strongly desired for augmented-reality glass applications.
- Xuelun Wang
- , Xixi Zhao
- & Seiji Samukawa
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Article
| Open AccessEngineering chirality at wafer scale with ordered carbon nanotube architectures
Methods for generating macroscopic chiral matter struggle with limited scalability. Here, the authors show two vacuum filtration methods - twist stacking and mechanical rotation - to align carbon nanotubes into chiral structures at wafer scale with tunable circular dichroism.
- Jacques Doumani
- , Minhan Lou
- & Weilu Gao
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Article
| Open AccessHierarchically manufactured chiral plasmonic nanostructures with gigantic chirality for polarized emission and information encryption
The application of chiral metamaterials is limited by the fabrication of large-area chiral plasmonic structures with high dissymmetry factors. Here, the authors overcome this limitation imparting extrinsic chirality to hierarchical nanostructured polymer substrates with application in quantum and security enhanced optical communications.
- Yoon Ho Lee
- , Yousang Won
- & Joon Hak Oh
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Article
| Open AccessLarge area inkjet-printed OLED fabrication with solution-processed TADF ink
Low-cost manufacturing of large-scale thermally activated delayed fluorescence organic light-emitting diodes has been restricted due to their incompatibility with solution processing techniques. Here, authors develop inkjet printing ink formulation to fabricate patterns without use of lithography.
- Chandra Kant
- , Atul Shukla
- & Monica Katiyar
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Article
| Open AccessDisordered metasurface enabled single-shot full-Stokes polarization imaging leveraging weak dichroism
Polarization imaging can capture information from the scene that cannot directly be recorded by traditional intensity cameras. Here, authors demonstrate a single-shot full Stokes polarization camera incorporating a disordered metasurface array with weak dichroism.
- Qingbin Fan
- , Weizhu Xu
- & Ting Xu
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Article
| Open AccessDouble boron–oxygen-fused polycyclic aromatic hydrocarbons: skeletal editing and applications as organic optoelectronic materials
The development of chemically diverse boron-oxygen-fused polycyclic aromatic hydrocarbons has been limited by their synthetic complexity. Here, authors report a one-pot strategy for their facile synthesis and demonstrate their potential as ultralong afterglow and host materials for deep-blue OLEDs.
- Guijie Li
- , Kewei Xu
- & Yuan-Bin She