Graphene articles within Nature Communications

Featured

  • Article |

    Investigation of the initial stages of the interaction of light with carriers in graphene is challenging. Here the authors probe the process with ultrafast pump-probe spectroscopy and microscopic theory, and observe the role of collinear scattering, which gives rise to Auger processes, including carrier multiplication.

    • D. Brida
    • , A. Tomadin
    •  & M. Polini
  • Article |

    Local magnetic properties that can be controlled by an applied electric field are desirable for spintronics applications. Nair et al.show that tuning carrier concentration by molecular doping or electric field can be used to control adatoms magnetism on graphene, enabling magnetic moments to be switched on and off.

    • R.R. Nair
    • , I.-L. Tsai
    •  & I.V. Grigorieva
  • Article |

    By patterning graphene with sub-wavelength features to introduce plasmonic modes, its optical properties can be tailored. Freitag et al. show how tunable plasmons in graphene nanoribbons can be exploited to form polarization-sensitive graphene photodetectors in the mid-infrared spectral region.

    • Marcus Freitag
    • , Tony Low
    •  & Phaedon Avouris
  • Article |

    Vertically assembled graphene devices have received less attention than the typical two dimensional arrangements. Chen et al. show that an Au/graphene/Au assembly exhibits a large magnetoresistance ratio of up to 400%, while a Co/graphene/Co device displays a spin valve effect at room temperature.

    • Jing-Jing Chen
    • , Jie Meng
    •  & Da-Peng Yu
  • Article |

    Graphene exhibits interesting optical and electronic properties, resulting from a Dirac dispersion of electrons. Shimano et al.observe quantum magneto-optical Faraday and Kerr effects in the terahertz regime, where plateaus are observed at the quantum-Hall steps.

    • R. Shimano
    • , G. Yumoto
    •  & H. Aoki
  • Article |

    Graphene holds great potential for use in photodetectors, owing to its ability to absorb light over a wide range of wavelengths. Here Zhang et al. report a large photoresponsivity of 8.6 AW-1 over a broad wavelength range in pure monolayer graphene.

    • By Yongzhe Zhang
    • , Tao Liu
    •  & Qi Jie Wang
  • Article
    | Open Access

    Multilayer stacks of graphene and related two-dimensional crystals can be tailored to create new classes of functional materials. Britnell et al. report resonant tunnelling of Dirac fermions and tunable negative differential conductance in a graphene-boron nitride-graphene transistor.

    • L. Britnell
    • , R. V. Gorbachev
    •  & L. Eaves
  • Article |

    It is difficult to observe the edge-bulk correspondence in two-dimensional electron systems, which display the quantum Hall effect. Here Li et al. follow the spatial evolution of Landau levels towards an edge of graphene by scanning tunnelling studies, revealing that the edge-bulk correspondence can be preserved.

    • Guohong Li
    • , Adina Luican-Mayer
    •  & Eva Y. Andrei
  • Article
    | Open Access

    The experimental investigation of relaxation times in graphene quantum dots has long been hindered by the limited tunability of these devices. Here Volk et. al.employ a device design to study this problem and report charge relaxation times of around 60–100 ns.

    • Christian Volk
    • , Christoph Neumann
    •  & Christoph Stampfer
  • Article |

    Understanding heat flow in two-dimensional nanomaterials has wide-ranging implications. Here, the authors show that the thermal conductance of quarter-micron graphene samples is quasi-ballistic, but patterning the graphene into nanoribbons leads to diffusive heat flow strongly limited by edge scattering.

    • Myung-Ho Bae
    • , Zuanyi Li
    •  & Eric Pop
  • Article |

    The specific capacity of an important commercial cathode material, lithium iron phosphate, is much lower than its theoretical value. Hu et al. report that incorporation of electrochemically exfoliated graphene layers in a carbon coating improves capacity beyond that predicted by theory.

    • By Lung-Hao Hu
    • , Feng-Yu Wu
    •  & Lain-Jong Li
  • Article |

    The chemical reduction of graphene oxide can provide large quantities of reduced graphene oxide for potential application in electronics and composite materials. Feng et al. report a highly efficient low-temperature one-pot reduction of graphene oxide that uses sodium-ammonia solution as the reducing agent.

    • Hongbin Feng
    • , Rui Cheng
    •  & Jinghong Li
  • Article
    | Open Access

    Janus materials have distinct chemical functionalities on opposite faces. Zhang et al.report that a two-step covalent functionalisation and poly(methyl methacrylate)-mediated transfer process facilitates the synthesis of nonsymmetrically modified single-layer graphene.

    • Liming Zhang
    • , Jingwen Yu
    •  & Zhongfan Liu
  • Article |

    Metallic particles are known to etch the surface layers of graphite by catalytic hydrogenation. Here, the authors report the sub-surface etching of graphite by Ni nanoparticles, revealing the formation of networks of tunnels, which are observed microscopically and could be modified for various applications.

    • Maya Lukas
    • , Velimir Meded
    •  & Ralph Krupke
  • Article
    | Open Access

    In metals, plasmon properties are fixed once the structure is built, but in graphene they can be altered by electric or magnetic fields. Using electrical time-of-flight measurements, Kumada et al. show wide plasmon velocity tunability in graphene with a varying magnetic field.

    • N. Kumada
    • , S. Tanabe
    •  & T. Fujisawa
  • Article |

    Graphene oxide has been proposed as an alternative to precious metals for the catalysis of aerobic oxidative reactions; however, high catalyst loadings are needed. Here a simple base and acid treatment is shown to enhance its catalytic activity for the oxidative coupling of amines under ambient conditions.

    • Chenliang Su
    • , Muge Acik
    •  & Kian Ping Loh
  • Article |

    The frictional force required to move a liquid drop on a surface is known to depend upon the drop resting time. N'guessan et al. demonstrate that water drops on graphene surfaces are an exception, which is attributable to the chemical homogeneity and stability of graphene surfaces.

    • Hartmann E. N’guessan
    • , Aisha Leh
    •  & Priyanka Wasnik
  • Article |

    The exploitation of the properties of graphene, such as mechanical strength and electrical conductivity, in deformable macroscopic materials is desirable. Here, a combination of graphene chemistry and ice physics is used to fabricate biomimetic, ultralight and superelastic graphene cellular monoliths.

    • Ling Qiu
    • , Jeffery Z. Liu
    •  & Dan Li
  • Article |

    The potential use of graphene in spintronic devices is limited by its weak spin–orbit coupling. Marchenko et al. report an enhancement of the spin splitting in graphene due to hybridization with gold 5dorbitals, showing a very large Rashba spin–orbit splitting of about 100 meV.

    • D. Marchenko
    • , A. Varykhalov
    •  & O. Rader
  • Article
    | Open Access

    Graphene is a single layer of carbon atoms whose high electron mobility offers potential for cheap, high-speed opto-electronic devices. Docherty et al.show that the terahertz frequency photoconductivity in graphene depends crucially on the type and density of environmental gas adsorbed.

    • Callum J. Docherty
    • , Cheng-Te Lin
    •  & Michael B. Johnston
  • Article |

    Graphene and single-walled carbon nanotubes have high electrical conductivities and large specific surface areas. Here, these properties are extended into three dimensions by producing a seamless carbon nanotube graphene hybrid material.

    • Yu Zhu
    • , Lei Li
    •  & James M. Tour
  • Article |

    Intentional defect creation in graphene is key to engineering its electrical, chemical, magnetic and mechanical properties. Robertsonet al. create defects by electron beam irradiation with sub-knock-on damage threshold, and show control over the defect position at the nanoscale and over the defect complexity.

    • Alex W. Robertson
    • , Christopher S. Allen
    •  & Jamie H. Warner
  • Article
    | Open Access

    Microdisk lasers are useful for compact wavelength-scale photonic devices and circuits, but their operation by electrical injection can hamper their optical properties. Kimet al. show that a graphene-contact electrode provides efficient electrical injection while minimising optical losses.

    • Yoon-Ho Kim
    • , Soon-Hong Kwon
    •  & Hong-Gyu Park
  • Article
    | Open Access

    A signature of the Dirac-like physics of charge carriers in graphene is the occurrence of an anomalous Hall effect, resulting in a quantization of the Landau levels. Guoet al. observe Landau levels of Dirac fermions in potassium-intercalated graphite arising in the absence of an applied magnetic field.

    • Donghui Guo
    • , Takahiro Kondo
    •  & Junji Nakamura
  • Article |

    The spectral position of Raman peaks is a useful diagnostic for determining the degree of strain and excess electronic charges present in graphene. This study demonstrates that these two contributions can be separated from each other and therefore be obtained at the same time.

    • Ji Eun Lee
    • , Gwanghyun Ahn
    •  & Sunmin Ryu
  • Article |

    Signal modulation is a mechanism which embeds an information-carrying signal into a carrier wave to broadcast information and is essential for high-speed communication. Zhonget al. report a flexible, transparent all-graphene modulator circuit performing quaternary modulation schemes with only two transistors.

    • Seunghyun Lee
    • , Kyunghoon Lee
    •  & Zhaohui Zhong
  • Article
    | Open Access

    Along with its electronic characteristics, the spin properties of graphene have recently received increasing attention in the context of spintronic applications. Using microwave radiation, Maniet al. identify resistively detected spin resonance in monolayer and trilayer graphene sheets and extract the value for the Landé g-factor.

    • Ramesh G. Mani
    • , John Hankinson
    •  & Walter A. de Heer
  • Article |

    The ability to manipulate single charges is a key requisite for novel nanoelectronic devices. Allenet al. show how to electrostatically confine electrons in suspended bilayer graphene quantum dots by local control of the graphene band structure.

    • M. T. Allen
    • , J. Martin
    •  & A. Yacoby
  • Article
    | Open Access

    Graphene's remarkable properties make it ideal for optoelectronic devices, and its two-dimensional nature enables its integration with photonic structures. By combining a graphene transistor with a planar microcavity, Engelet al. control the spectrum of the photocurrent and the light emitted by the device.

    • Michael Engel
    • , Mathias Steiner
    •  & Ralph Krupke
  • Article |

    Strain engineering has been proposed as a promising strategy for manipulating the electronic properties of graphene. This scanning tunnelling microscopy study demonstrates the feasibility of controlling strain patterns in graphene down to the nanoscale.

    • Jiong Lu
    • , A.H. Castro Neto
    •  & Kian Ping Loh
  • Article
    | Open Access

    Electronic and optoelectronic devices based on gallium nitride suffer from self-heating arising as a result of their operation. This study presents and demonstrates a strategy for managing this problem that relies on graphene quilts which dissipate the heat away.

    • Zhong Yan
    • , Guanxiong Liu
    •  & Alexander A. Balandin
  • Article |

    The terahertz spectral region is desirable for applications such as imaging or spectroscopy, but progress is hampered by a lack of efficient terahertz devices. By exploiting intraband transitions in graphene, Sensale-Rodriguezet al. demonstrate a broadband intensity modulator working at terahertz frequencies.

    • Berardi Sensale-Rodriguez
    • , Rusen Yan
    •  & Huili Grace Xing
  • Article |

    Graphene is characterized by unique physical properties that offer substantial promise, most notably for electronic applications. Mannooret al. present a wireless graphene-based sensor for detecting bacteria on a range of biological tissues.

    • Manu S. Mannoor
    • , Hu Tao
    •  & Michael C. McAlpine
  • Article
    | Open Access

    Grain boundaries in graphene degrade its properties, and large single-crystal graphene is desirable for electronic applications of graphene. Gaoet al. develop a method to produce millimetre-sized hexagonal single-crystal graphene grains, and films composed of the grains, on platinum by chemical vapour deposition.

    • Libo Gao
    • , Wencai Ren
    •  & Hui-Ming Cheng
  • Article
    | Open Access

    Graphene's broad bandwidth makes it promising as a photodetector, but common electronics cannot analyse the currents at high frequencies. Here, using photocurrent measurements, laser-induced carrier generation effects in freely suspended graphene and at graphene–metal interfaces are clarified up to 1 THz.

    • Leonhard Prechtel
    • , Li Song
    •  & Alexander W. Holleitner
  • Article |

    Current methods for fabricating graphene rely on its transfer from metal surfaces to substrates suitable for device applications. This study demonstrates a transfer-free approach for growing graphene on substrates such as thermally oxidized silicon and plastic that forms the material underneath a nickel film, at the nickel–substrate interface.

    • Jinsung Kwak
    • , Jae Hwan Chu
    •  & Soon-Yong Kwon