Featured
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| Open AccessLayer-dependent quantum cooperation of electron and hole states in the anomalous semimetal WTe2
Tungsten ditelluride is a semi-metallic two-dimensional material that has exhibited large magnetoresistance. Here, the authors use angle- and spin-resolved photoemission spectroscopy to investigate the band structure of this transition metal dichalcogenide and identify layer-dependent electronic behaviour.
- Pranab Kumar Das
- , D. Di Sante
- & R. J. Cava
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Article
| Open AccessNear-field photocurrent nanoscopy on bare and encapsulated graphene
Graphene grain boundaries and charge inhomogeneities limit its electronic properties. Here the authors combine scanning near-field optical microscopy with electrical read-out to image these defects at the nanoscale under an encapsulation layer, and show that charges build up along the edges of the flake.
- Achim Woessner
- , Pablo Alonso-González
- & Frank H. L. Koppens
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Article
| Open AccessEnhanced spin–orbit torques by oxygen incorporation in tungsten films
When interfaced with a current-carrying heavy metal, spin orbit effects can generate a torque on the magnetization of a ferromagnet, understood as a bulk effect. Here, the authors show evidence of an interfacial contribution to such spin orbit torque in O-doped W/CoFeB thin film systems.
- Kai-Uwe Demasius
- , Timothy Phung
- & Stuart S. P. Parkin
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Article
| Open AccessMagnon spectrum of the helimagnetic insulator Cu2OSeO3
Cu2OSeO3 possesses a helical spin structure which supports a rich phase diagram of magnetic states, including a lattice of particle-like skyrmions. Here, the authors use inelastic neutron scattering to elucidate the three-dimensional magnon spectrum and underlying spin Hamiltonian of Cu2OSeO3.
- P. Y. Portnichenko
- , J. Romhányi
- & D. S. Inosov
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Article
| Open AccessDirectional charge separation in isolated organic semiconductor crystalline nanowires
Photo-induced charge separation in organic semiconductors usually occurs at interfaces between electron donors and acceptors. Here, the authors show using photoluminescence measurements that charge separation is intrinsic and directional in organic crystalline nanowires made of stacked monomers.
- J. A. Labastide
- , H. B. Thompson
- & M. D. Barnes
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Article
| Open AccessPossible observation of highly itinerant quantum magnetic monopoles in the frustrated pyrochlore Yb2Ti2O7
Spin excitations above the ground state of spin ices, geometrically frustrated pyrochlore magnets, are equivalent to pairs of oppositely charged deconfined magnetic monopoles which may propagate through the system. Here, the authors evidence highly itinerant quantum magnetic monopole excitations in Yb2Ti2O7.
- Y. Tokiwa
- , T. Yamashita
- & Y. Matsuda
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Article
| Open Access1s-intraexcitonic dynamics in monolayer MoS2 probed by ultrafast mid-infrared spectroscopy
Excitons—bound electron-hole pairs—in two-dimensional transition-metal dichalcogenides can exhibit a rich spectrum of excited states. Here, the authors use ultrafast mid-infrared spectroscopy to explore the dynamics of these so-called 1s-intraexcitonic transitions in monolayer molybdenum disulphide.
- Soonyoung Cha
- , Ji Ho Sung
- & Hyunyong Choi
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Article
| Open AccessPhotoresponse of supramolecular self-assembled networks on graphene–diamond interfaces
Two-dimensional, self-assembled heteromolecular networks often lack functionality. Here the authors study the photoresponse of self-assembled heteromolecular networks, while controlling their positions and interfaces at an atomic level, suggesting bottom-up assembly of optoelectronics devices.
- Sarah Wieghold
- , Juan Li
- & Carlos-Andres Palma
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Article
| Open AccessSignatures of the Adler–Bell–Jackiw chiral anomaly in a Weyl fermion semimetal
Anomalous conducting behavior of solids may reflect the presence of novel quantum states. Here, Zhang et al. report an increased conductivity in TaAs with a magnetic field applied along the direction of the current, which reveals an inherent property of the Weyl Fermion.
- Cheng-Long Zhang
- , Su-Yang Xu
- & Shuang Jia
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Article
| Open AccessControl of antiferromagnetic domain distribution via polarization-dependent optical annealing
The control of magnetic domains in antiferromagnets is limited by the lack of a net magnetic moment which may be manipulated by external stimuli. Here, the authors present an optical method for switching such domain states in MnF2based on azimuth-dependent absorption of linearly polarized light.
- Takuya Higuchi
- & Makoto Kuwata-Gonokami
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Article
| Open AccessIn situ stress observation in oxide films and how tensile stress influences oxygen ion conduction
Strain engineering is used to tune physiochemical material properties, but detailed insights of how the crystal growth affects the stress are yet lacking. Here, the authors analyse in situ simultaneously the induced stress and growth mode during the epitaxial growth of an oxygen ion conductor.
- Aline Fluri
- , Daniele Pergolesi
- & Thomas Lippert
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Article
| Open AccessOrbital two-channel Kondo effect in epitaxial ferromagnetic L10-MnAl films
In metals, electronic scattering from defects by the two-channel Kondo effect is expected to cause deviation from standard low temperature behaviour, however this effect has not been unambiguously shown. Here, the authors present evidence consistent with all transport signatures of the effect in ferromagnetic L10-MnAl films.
- L. J. Zhu
- , S. H. Nie
- & J. H. Zhao
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Article
| Open AccessSuper-crystals in composite ferroelectrics
Crystalline materials are formed by the periodic order of atomic unit cells. Here, Pierangeli et al. report the formation of a ferrelectric super-crystal with micrometric unit cell from modulated nanoscale disorder in potassium-lithium-tantalate-niobate, which is potentially useful for engineering ordered states out of disorder.
- D. Pierangeli
- , M. Ferraro
- & E. DelRe
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Article
| Open AccessFerroelasticity and domain physics in two-dimensional transition metal dichalcogenide monolayers
The atoms in two-dimensional transition-metal dichalcogenides can arrange into a number of different structures, or polymorphs. Here, the authors use first-principles calculations to show that one such polymorph, 1T', can exhibit a large mechanical response to external applied strain.
- Wenbin Li
- & Ju Li
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Article
| Open AccessAharonov–Bohm oscillations in Dirac semimetal Cd3As2 nanowires
Dirac semimetals are a three-dimensional analogue of graphene that can support massless Dirac fermions in their bulk and Fermi-arc surface states. Here, the authors observe Aharonov–Bohm oscillations in transport measurements on Cd3As2nanowires, revealing these exotic surface states.
- Li-Xian Wang
- , Cai-Zhen Li
- & Zhi-Min Liao
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Article
| Open AccessStimulated Raman adiabatic passage in a three-level superconducting circuit
The precise control and manipulation of the states of a multi-level quantum system are fundamental for quantum information processing. Here, the authors demonstrate the robust adiabatic manipulation of the quantum states of a superconducting circuit via stimulated Raman adiabatic passage.
- K. S. Kumar
- , A. Vepsäläinen
- & G. S. Paraoanu
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Article
| Open AccessTailoring the chiral magnetic interaction between two individual atoms
The Dzyaloshinskii-Moriya exchange interaction arises in magnetic systems with broken inversion symmetry and promotes chiral magnetic order which may be exploited in spintronic devices. Here, the authors demonstrate how such an interaction between magnetic atoms on a metallic surface may be tuned by their separation.
- A. A. Khajetoorians
- , M. Steinbrecher
- & R. Wiesendanger
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Article
| Open AccessReducing dynamic disorder in small-molecule organic semiconductors by suppressing large-amplitude thermal motions
Thermal vibration is harmful to charge transport in molecular semiconductors, which hinders the use of these materials in flexible electronics. Here, Illig et al.show that the vibration is suppressed when molecular side chains are attached to the long axis of conjugated cores.
- Steffen Illig
- , Alexander S. Eggeman
- & Henning Sirringhaus
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Article
| Open AccessNonmagnetic band gap at the Dirac point of the magnetic topological insulator (Bi1−xMnx)2Se3
Doping a topological insulator with magnetic impurities is expected to induce ferromagnetism and open a band gap in its surface states. Here, the authors study Mn-doped Bi2Se3, finding a mechanism for band gap opening in topologically-protected surface states which is not of magnetic origin.
- J. Sánchez-Barriga
- , A. Varykhalov
- & O. Rader
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Article
| Open AccessUnfolding the physics of URu2Si2 through silicon to phosphorus substitution
The heavy fermion compound URu2Si2displays a hidden order phase and superconductivity at low temperatures. Here, the authors perform substitution studies—partially replacing silicon with phosphorus—and study the effects on hidden order and superconductivity.
- A. Gallagher
- , K.-W. Chen
- & R. E. Baumbach
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Article
| Open AccessThermodynamics of deposition flux-dependent intrinsic film stress
Vapour deposition on polycrystalline films can lead to unexpectedly high and reversible compressive stress, the origin of which remains unclear. Here, the authors show, using thermodynamic arguments, that entropic effects in the extremely dilute adatom gas on the surface play a major role.
- Amirmehdi Saedi
- & Marcel J. Rost
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Article
| Open AccessVoltage collapse in complex power grids
A power grid is constrained by both its nonlinear physics and network structure, and violations of these constraints may lead to voltage collapse blackouts, which have been studied mostly numerically. Here the authors derive a closed-form condition to provide an analytic test for voltage collapse.
- John W. Simpson-Porco
- , Florian Dörfler
- & Francesco Bullo
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Article
| Open AccessManipulating the interfacial structure of nanomaterials to achieve a unique combination of strength and ductility
Nanocrystalline metals often exhibit high strength yet suffer from poor ductility. Here, the authors employ grain boundary engineering to overcome this problem by introducing amorphous intergranular films, which enables superior mechanical properties in copper-zirconium alloys.
- Amirhossein Khalajhedayati
- , Zhiliang Pan
- & Timothy J. Rupert
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Article
| Open AccessElectron-lattice interactions strongly renormalize the charge-transfer energy in the spin-chain cuprate Li2CuO2
In transition metal oxides, an insulating band gap is found when the energy scales related to ionic charge excitations dominate over electronic itinerancy. Here, the authors demonstrate strong electron-phonon interactions in Li2CuO2and their effect on the insulating band gap.
- Steve Johnston
- , Claude Monney
- & Jeroen van den Brink
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Article
| Open AccessA four-coordinate cobalt(II) single-ion magnet with coercivity and a very high energy barrier
Bistable single-molecule magnets potentially allow information storage at extremely high densities. Here, the authors study an air- and moisture-stable mononuclear tetrahedral cobalt(II) complex, elucidating the origin of its pronounced magnetic bistability.
- Yvonne Rechkemmer
- , Frauke D. Breitgoff
- & Joris van Slageren
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Article
| Open AccessAthermal domain-wall creep near a ferroelectric quantum critical point
At very low temperature, particle-like objects such as atoms and material phase boundaries become less able to move due to thermally inactivity. Here, Kagawa et al. show that ferroelectric domain walls gain energy for creep motion due to quantum fluctuations at low temperature.
- Fumitaka Kagawa
- , Nao Minami
- & Yoshinori Tokura
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Article
| Open AccessVisualizing the orientational dependence of an intermolecular potential
Intermolecular interactions underpin an array of physical and chemical phenomena. Here, the authors probe the three dimensional potential between fullerene molecules in different orientations showing that the positional variation in the intermolecular binding energy is dominated repulsive interactions.
- Adam Sweetman
- , Mohammad A. Rashid
- & Philip Moriarty
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Article
| Open AccessThermal and quantum depletion of superconductivity in narrow junctions created by controlled electromigration
Nanostructured superconductors allow dissipationless electrical transport to be exploited in technologically relevant devices. Here, the authors follow how detrimental fluctuations of the superconducting order parameter evolve in Al atomic contacts as their width is controlled by electromigration.
- Xavier D. A. Baumans
- , Dorin Cerbu
- & Joris Van de Vondel
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Article
| Open AccessArbitrary cross-section SEM-cathodoluminescence imaging of growth sectors and local carrier concentrations within micro-sampled semiconductor nanorods
Semiconductor nanocrystals are potential nanoelectronic materials but often display nonuniform electric properties due to their anisotropic growths. Here, the authors report cross-sectional cathodoluminescence imaging of a single-crystalline ZnO nanowire to resolve its growth sectors with different carrier concentrations.
- Kentaro Watanabe
- , Takahiro Nagata
- & Yoshiaki Nakamura
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Article
| Open AccessPrediction of an arc-tunable Weyl Fermion metallic state in MoxW1−xTe2
Two-dimensional materials provide possible platforms to map exotic phenomena from particle physics to condensed matter physics. Here, the authors predict doping dependent electronic behaviour in MoxW1−xTe2, in resemblance of a phenomenon which is believed to exist only in particle physics.
- Tay-Rong Chang
- , Su-Yang Xu
- & M. Zahid Hasan
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Article
| Open AccessDirected block copolymer self-assembly implemented via surface-embedded electrets
The controlled orientation of block copolymers promises to deliver high resolution patterning for implementation in future nanoscale technologies. Here, the authors use the electric field from charged electrets to induce extremely localised perpendicularly oriented microdomains in polymer thin films.
- Mei-Ling Wu
- , Dong Wang
- & Li-Jun Wan
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Article
| Open AccessStructural semiconductor-to-semimetal phase transition in two-dimensional materials induced by electrostatic gating
Control of conductivity and optical properties via atomic structure changes is of technological importance in information storage. Here, Li et al.show that electrostatic gating has the potential to drive structural semiconductor-to-semimetal phase transitions in some monolayer transition metal dichalcogenides.
- Yao Li
- , Karel-Alexander N. Duerloo
- & Evan J. Reed
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Article
| Open AccessA dilation-driven vortex flow in sheared granular materials explains a rheometric anomaly
Flowing granular materials exhibit fluid-like features, but not all of them can be described by extending fluid mechanics. Here, the authors show vortex flow in a granular layer sheared between coaxial cylinders, and attribute it to the effect that the material moves away from the sheared region.
- K. P. Krishnaraj
- & Prabhu R. Nott
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Article
| Open AccessHexadecapolar colloids
Colloidal systems can form bulk phases such as liquid and crystals, but they also exhibit interesting behaviours that have no atomic analogues. Here, by dispersing solid polymer microspheres in a nematic liquid crystal, Senyuk et al. demonstrate spontaneous formation of hexadecapolar nematic colloids.
- Bohdan Senyuk
- , Owen Puls
- & Ivan I. Smalyukh
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Article
| Open AccessGiant conductivity switching of LaAlO3/SrTiO3 heterointerfaces governed by surface protonation
The interface between two oxide materials can play host to numerous exotic phenomenon. Here, the authors observe a four order of magnitude change in the conductance at a lanthanum-aluminate–strontium-titanate interface controlled by surface protonation, which can be reversed by exposure to light.
- Keith A. Brown
- , Shu He
- & Jeremy Levy
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Article
| Open AccessExciton diamagnetic shifts and valley Zeeman effects in monolayer WS2 and MoS2 to 65 Tesla
The spin and valley degrees of freedom are coupled in two-dimensional transition-metal dichalcogenides. Here, the authors use high magnetic fields to optically measure the valley Zeeman effect and diamagnetic exciton shift in tungsten disulphide and molybdenum disulphide, and determine the exciton binding energies.
- Andreas V. Stier
- , Kathleen M. McCreary
- & Scott A. Crooker
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Article
| Open AccessTopographical pathways guide chemical microswimmers
Self-propelled colloids can be used as cargo carriers, but it is challenging to control their motion without external fields. Here, Simmchen et al. use submicron patterns on a solid substrate to effectively confine the motion of the chemically active Janus microswimmers along the edges of the patterns.
- Juliane Simmchen
- , Jaideep Katuri
- & Samuel Sánchez
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Article
| Open AccessCommon electronic origin of superconductivity in (Li,Fe)OHFeSe bulk superconductor and single-layer FeSe/SrTiO3 films
The mechanism of high-temperature superconductivity in the iron-based materials remains not fully understood. Here, the authors report on ARPES measurements on an FeSe-based bulk superconductor, whose electronic properties are found to be similar to those of single-layer FeSe/STO films.
- Lin Zhao
- , Aiji Liang
- & X. J. Zhou
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Article
| Open AccessShaping metallic glasses by electromagnetic pulsing
Metallic glasses can be softened to different shapes whilst maintaining mechanical properties, and the related thermoplastic processing requires a heating source and an applied force. Here, the authors show an effective thermoplastic approach by a coupling between electric pulses and a magnetic field.
- Georg Kaltenboeck
- , Marios D. Demetriou
- & William L. Johnson
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Article
| Open AccessSingle crystal functional oxides on silicon
Synthesis of single-crystal complex-oxide films directly on silicon is difficult due to differing interfacial chemistry. Here, the authors demonstrate room-temperature integration of single-crystal lead zirconate titanate on to silicon to act as a gate insulator in a field-effect transistor.
- Saidur Rahman Bakaul
- , Claudy Rayan Serrao
- & Sayeef Salahuddin
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Article
| Open AccessMacrospin dynamics in antiferromagnets triggered by sub-20 femtosecond injection of nanomagnons
Magnetic order in nature is defined by the exchange interaction, however its understanding on the ultrafast- and nanometer-scales is limited. Here, the authors follow the femtosecond sub-nanometer dynamics of the antiferromagnetic order parameter in KNiF3triggered by photo-generated exchange magnons.
- D. Bossini
- , S. Dal Conte
- & A. V. Kimel
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Article
| Open AccessOrigin of the spin Seebeck effect in compensated ferrimagnets
Ferrimagnets possess multiple spin sub-lattices resulting in a complex magnon band structure and subtle spin transport across interfaces. Here, the authors show how the spin Seebeck effect, the thermal generation of pure spin current, may be an effective tool to study these magnetic excitations.
- Stephan Geprägs
- , Andreas Kehlberger
- & Mathias Kläui
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Article
| Open AccessSustained hole inversion layer in a wide-bandgap metal-oxide semiconductor with enhanced tunnel current
Wide-bandgap, metal-oxide thin-film transistors are limited in their application by the lack of available p-type material. Here, the authors demonstrate a wide-bandgap metal-oxide n-type semiconductor that sustains a strong p-type inversion layer using a barrier dielectric with a high-dielectric constant.
- Gem Shoute
- , Amir Afshar
- & Douglas Barlage
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Article
| Open AccessSuppression of the antiferromagnetic pseudogap in the electron-doped high-temperature superconductor by protect annealing
In cuprates, superconductivity exists in a narrow window at high electron doping concentration with strong antiferromagnetic correlations. Here, the authors demonstrate superconductivity with no effect of antiferromagnetic order in a cuprate for a wide electron doping range following a protect anneal process.
- M. Horio
- , T. Adachi
- & A. Fujimori
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Article
| Open AccessQuantum electric-dipole liquid on a triangular lattice
In magnetic materials, geometry-defined competing interactions between spins combined with quantum fluctuations can present the possibility of quantum liquid states which do not order even as 0K is approached. Here, the authors present an analogue built from electric dipoles on a triangular lattice.
- Shi-Peng Shen
- , Jia-Chuan Wu
- & Young Sun
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Article
| Open AccessDesign of crystal-like aperiodic solids with selective disorder–phonon coupling
Conventional crystallography focuses on structurally-ordered systems, where interesting physics or novel material functions emerge. Here, Overy et al. propose an approach of designing functional materials with strongly correlated disorder, which can couple with phonons to affect lattice dynamics.
- Alistair R. Overy
- , Andrew B. Cairns
- & Andrew L. Goodwin
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Article
| Open AccessAbsence of a spin-signature from a single Ho adatom as probed by spin-sensitive tunneling
Magnetic stability of holmium atoms on a platinum(111) surface has recently been reported, raising prospects for atomic-scale spintronics, however contradictory results have since emerged. Here, Steinbrecher et al.find evidence for an invisibility of the holmium spin to scanning tunnelling spectroscopy techniques which challenges recent results.
- M. Steinbrecher
- , A. Sonntag
- & A. A. Khajetoorians
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Article
| Open AccessSeamless growth of a supramolecular carpet
The potential of organic molecular devices are limited by our inability to uniformly arrange them as thin films on metals, especially over imperfect surfaces. Here, the authors demonstrate the growth of a self-organized molecular carpet, which can extend over steps and terraces while retaining regularity.
- Ju-Hyung Kim
- , Jean-Charles Ribierre
- & Yousoo Kim
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Article
| Open AccessFerroelastic switching in a layered-perovskite thin film
Ferroelastic switching in thin films is typically restricted by constraints from the substrate or occurs around twin-like domains. Here, the authors show reversible and non-volatile ferroelastic switching avoiding substrate constraints in layered-perovskite Bi_2WO_6 epitaxial films.
- Chuanshou Wang
- , Xiaoxing Ke
- & Jinxing Zhang
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