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SO2, silicate clouds, but no CH4 detected in a warm Neptune
The JWST MIRI transmission spectrum of WASP-107b, a transiting planet with Neptune-like mass and Jupiter-like radius, shows observations of sulfur dioxide and silicate clouds but no methane in its atmosphere, providing evidence of disequilibrium chemistry and active photochemistry.
- Achrène Dyrek
- , Michiel Min
- & Gillian Wright
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Article
| Open AccessNatural short-lived halogens exert an indirect cooling effect on climate
Short-lived halogens have a substantial indirect cooling effect on climate and this cooling effect has increased since pre-industrial times owing to anthropogenic amplification of natural halogen emissions.
- Alfonso Saiz-Lopez
- , Rafael P. Fernandez
- & Jean-François Lamarque
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Article
| Open AccessNo thick carbon dioxide atmosphere on the rocky exoplanet TRAPPIST-1 c
The detection of thermal emission from the rocky exoplanet TRAPPIST-1 c using the Mid-Infrared Instrument on the James Webb Space Telescope reveals a dayside brightness temperature that disfavours a thick, CO2-rich atmosphere.
- Sebastian Zieba
- , Laura Kreidberg
- & Gabrielle Suissa
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Vanadium oxide and a sharp onset of cold-trapping on a giant exoplanet
Analysis of transits of an ultra-hot giant exoplanet reports the precise abundance constraints of 14 major refractory elements, showing distinct deviations from proto-solar, along with a sharp transition temperature at which those elements are depleted.
- Stefan Pelletier
- , Björn Benneke
- & Julian Stürmer
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Article
| Open AccessA broadband thermal emission spectrum of the ultra-hot Jupiter WASP-18b
The dayside thermal emission spectrum and brightness temperature map of the ultra-hot Jupiter WASP-18b obtained from the NIRISS instrument on the JWST showed water emission features, an atmosphere consistent with solar metallicity, as well as a steep and symmetrical decrease in temperature towards the nightside.
- Louis-Philippe Coulombe
- , Björn Benneke
- & Peter J. Wheatley
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Article
| Open AccessPhotochemically produced SO2 in the atmosphere of WASP-39b
Observations from the JWST show the presence of a spectral absorption feature at 4.05 μm arising from SO2 in the atmosphere of the gas giant exoplanet WASP-39b, which is produced by photochemical processes and verified by numerical models.
- Shang-Min Tsai
- , Elspeth K. H. Lee
- & Sergei N. Yurchenko
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Article |
Chlorine activation and enhanced ozone depletion induced by wildfire aerosol
Comparison of model simulations with atmospheric observations from the Southern Hemisphere mid-latitudes following the 2020 Australian wildfires shows that the wildfire aerosol composition promotes stratospheric chlorine and ozone depletion chemistry.
- Susan Solomon
- , Kane Stone
- & Peidong Wang
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Article
| Open AccessEarly Release Science of the exoplanet WASP-39b with JWST NIRSpec PRISM
A broad-wavelength 0.5–5.5 µm atmospheric transmission spectrum of WASP-39b, a 1,200 K, roughly Saturn-mass, Jupiter-radius exoplanet, demonstrates JWST’s sensitivity to a rich diversity of exoplanet compositions and chemical processes.
- Z. Rustamkulov
- , D. K. Sing
- & S. Zieba
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Wetland emission and atmospheric sink changes explain methane growth in 2020
Using both bottom-up and top-down approaches, the record high increase in the methane growth rate in 2020 is attributed mainly to emissions from wetlands, which have been exacerbated by a warmer and wetter climate, and to the reduced atmospheric methane sink, in response to emissions reduction of air pollutants during COVID-19 lockdowns.
- Shushi Peng
- , Xin Lin
- & Philippe Ciais
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Article
| Open AccessChiral monoterpenes reveal forest emission mechanisms and drought responses
Analysis of atmospheric data on two enantiomerically separated forms of monoterpene from a controlled drought and rewetting experiment in an enclosed tropical rainforest ecosystem showed distinct diel emission peaks, regulated by different production pathways.
- Joseph Byron
- , Juergen Kreuzwieser
- & Jonathan Williams
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Article |
Integrated ozone depletion as a metric for ozone recovery
An integrated ozone depletion metric indicates the impact of any new emission and provides a useful complementary metric of the impact of specific emissions of an ozone depleting substance for both the scientific and policy communities.
- John A. Pyle
- , James Keeble
- & Paul T. Griffiths
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Article
| Open AccessSynergistic HNO3–H2SO4–NH3 upper tropospheric particle formation
By performing experiments under upper tropospheric conditions, nitric acid, sulfuric acid and ammonia can form particles synergistically, at rates orders of magnitude faster than any two of the three components.
- Mingyi Wang
- , Mao Xiao
- & Neil M. Donahue
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UV absorption by silicate cloud precursors in ultra-hot Jupiter WASP-178b
Analysis is presented that indicates that there is strong evidence that SiO or Mg, the major constituents of silicate condensates, must be present in gaseous form in the atmosphere of ultra-hot Jupiter WASP-178b.
- Joshua D. Lothringer
- , David K. Sing
- & Autumn T. Winch
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Matters Arising |
Reply to: On the role of atmospheric model transport uncertainty in estimating the Chinese land carbon sink
- Jing Wang
- , Liang Feng
- & ChaoZong Xia
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Article
| Open AccessGlobal fine-scale changes in ambient NO2 during COVID-19 lockdowns
The satellite instrument TROPOMI is used to assess ambient NO2 levels at approximately one-kilometre resolution across 215 cities worldwide during COVID-19 lockdowns, finding about 30% lower NO2 concentrations in countries with strict lockdowns.
- Matthew J. Cooper
- , Randall V. Martin
- & Chris A. McLinden
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Article |
Uncovering global-scale risks from commercial chemicals in air
A new framework is proposed for assessing the risks of the atmospheric transformation products of commercial chemicals, combining laboratory and field experiments, advanced techniques for screening suspect chemicals, and in silico modelling.
- Qifan Liu
- , Li Li
- & John Liggio
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Article |
A solar C/O and sub-solar metallicity in a hot Jupiter atmosphere
The C/O ratio of the transiting hot Jupiter WASP-77Ab is measured here and found to be approximately solar, though the (C+O)/H ratio is subsolar.
- Michael R. Line
- , Matteo Brogi
- & Joost P. Wardenier
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Article |
Vast CO2 release from Australian fires in 2019–2020 constrained by satellite
The amount of carbon dioxide released by the Australian wildfires of 2019–2020 is uncertain, but is estimated here using satellite observations of carbon monoxide to be more than twice the amount suggested by fire inventories.
- Ivar R. van der Velde
- , Guido R. van der Werf
- & Ilse Aben
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Article |
Widespread phytoplankton blooms triggered by 2019–2020 Australian wildfires
Oceanic deposition of wildfire aerosols can enhance marine productivity, as supported here by satellite and in situ profiling floats data showing that emissions from the 2019–2020 Australian wildfires fuelled phytoplankton blooms in the Southern Ocean.
- Weiyi Tang
- , Joan Llort
- & Nicolas Cassar
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Article |
The Montreal Protocol protects the terrestrial carbon sink
Modelling suggests that the Montreal Protocol may be mitigating climate change by protecting the land carbon sink, as well as by protecting the ozone layer and reducing greenhouse gas emissions.
- Paul J. Young
- , Anna B. Harper
- & Rolando R. Garcia
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Article
| Open AccessUbiquitous atmospheric production of organic acids mediated by cloud droplets
The oxidation of hydrated formaldehyde from cloud droplets is the dominant source of atmospheric formic acid, increasing atmospheric acidity by reducing cloud and rainwater pH.
- B. Franco
- , T. Blumenstock
- & D. Taraborrelli
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Article |
Five carbon- and nitrogen-bearing species in a hot giant planet’s atmosphere
The signatures of water, carbon monoxide, hydrogen cyanide, methane, ammonia and acetylene are observed in the transmission spectrum of the hot Jupiter HD 209458b, with abundance ratios suggesting a super-solar carbon-to-oxygen ratio.
- Paolo Giacobbe
- , Matteo Brogi
- & Andrea Tozzi
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Article |
A decline in emissions of CFC-11 and related chemicals from eastern China
Atmospheric data and chemical-transport modelling show that CFC-11 emissions from eastern China have again decreased, after increasing in 2013–2017, and a delay in ozone-layer recovery has probably been avoided.
- Sunyoung Park
- , Luke M. Western
- & Matthew Rigby
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Article |
A decline in global CFC-11 emissions during 2018−2019
Atmospheric concentration measurements at remote sites around the world reveal an accelerated decline in the global mean CFC-11 concentration during 2018 and 2019, reversing recent trends and building confidence in the timely recovery of the stratospheric ozone layer.
- Stephen A. Montzka
- , Geoffrey S. Dutton
- & Christina Theodoridi
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Article |
Sources of particulate-matter air pollution and its oxidative potential in Europe
Observations and air-quality modelling reveal that the sources of particulate matter and oxidative potential in Europe are different, implying that reducing mass concentrations of particulate matter alone may not reduce oxidative potential.
- Kaspar R. Daellenbach
- , Gaëlle Uzu
- & André S. H. Prévôt
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Article |
Satellite isoprene retrievals constrain emissions and atmospheric oxidation
Direct satellite measurements of atmospheric isoprene are compared with model predictions, showing broad agreement but highlighting spatial and temporal biases in modelled isoprene and nitrogen oxide emissions.
- Kelley C. Wells
- , Dylan B. Millet
- & Jose D. Fuentes
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Article |
Small lightning flashes from shallow electrical storms on Jupiter
Small lightning flashes detected on Jupiter by Juno have shallow origins above the 2-bar level of Jupiter’s atmosphere where temperatures are too low for liquid water to exist.
- Heidi N. Becker
- , James W. Alexander
- & Paul G. Steffes
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Article |
Preindustrial 14CH4 indicates greater anthropogenic fossil CH4 emissions
Isotopic evidence from ice cores indicates that preindustrial-era geological methane emissions were lower than previously thought, suggesting that present-day emissions of methane from fossil fuels are underestimated.
- Benjamin Hmiel
- , V. V. Petrenko
- & E. Dlugokencky
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Article |
Premature mortality related to United States cross-state air pollution
This analysis of the exchange of air pollution amongst the contiguous United States finds that, on average, around half of the early deaths caused by a state’s air pollution occurs outside that state, with different contributions by different emission sectors and chemical species.
- Irene C. Dedoussi
- , Sebastian D. Eastham
- & Steven R. H. Barrett
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Letter |
A large source of cloud condensation nuclei from new particle formation in the tropics
Widespread formation of new particles from condensable vapours observed in the tropical upper troposphere is an important source of cloud condensation nuclei in the lower troposphere, affecting cloud properties.
- Christina J. Williamson
- , Agnieszka Kupc
- & Charles A. Brock
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Letter |
Isotopic constraint on the twentieth-century increase in tropospheric ozone
Isotope data from polar firn and ice are used to constrain the increase in tropospheric ozone between 1850 and 2005 ad.
- Laurence Y. Yeung
- , Lee. T. Murray
- & Jérôme Chappellaz
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Letter |
Increase in CFC-11 emissions from eastern China based on atmospheric observations
Emissions from eastern China account for approximately 40 to 60 per cent of the global rise in emissions of trichlorofluoromethane (CFC-11), which may be a result of new production and use.
- M. Rigby
- , S. Park
- & D. Young
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Letter |
Martian dust storm impact on atmospheric H2O and D/H observed by ExoMars Trace Gas Orbiter
High-resolution measurements of Martian atmospheric dust, water and semiheavy water, obtained by the ExoMars Trace Gas Orbiter during a global dust storm on Mars, are reported.
- Ann Carine Vandaele
- , Oleg Korablev
- & Maria Paz Zorzano
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Letter |
No detection of methane on Mars from early ExoMars Trace Gas Orbiter observations
Highly sensitive measurements of the atmosphere of Mars with the ExoMars Trace Gas Orbiter do not detect any methane over a range of latitudes in both hemispheres, in contrast to previous local or remote detections.
- Oleg Korablev
- , Ann Carine Vandaele
- & Maria Paz Zorzano
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Article |
Secondary organic aerosol reduced by mixture of atmospheric vapours
Adding reactive gases such as isoprene to mixtures lowers the production of secondary organic aerosol in the atmosphere, thus reducing the atmospheric particulate burden, with implications for human health and climate.
- Gordon McFiggans
- , Thomas F. Mentel
- & Astrid Kiendler-Scharr
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Letter |
Industrial and agricultural ammonia point sources exposed
Satellite observations reveal over 200 ammonia hotspots associated with agricultural and industrial point sources, which emit much larger quantities of ammonia to the atmosphere than previously thought.
- Martin Van Damme
- , Lieven Clarisse
- & Pierre-François Coheur
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Letter |
Atomic iron and titanium in the atmosphere of the exoplanet KELT-9b
Cross-correlation analysis of high-resolution spectra obtained as the exoplanet KELT-9b transited its host star reveals neutral and singly ionized atomic iron and singly ionized atomic titanium in the exoplanet’s atmosphere.
- H. Jens Hoeijmakers
- , David Ehrenreich
- & Luca Di Fabrizio
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Letter |
Helium in the eroding atmosphere of an exoplanet
A detection of helium absorption at 10,833 Å on the exoplanet WASP-107b reveals that its atmosphere is extended and eroding, and demonstrates a new way to study upper exoplanetary atmospheres.
- J. J. Spake
- , D. K. Sing
- & N. Madhusudhan
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Letter |
Large emissions from floodplain trees close the Amazon methane budget
Methane fluxes from the stems of Amazonian floodplain trees indicate that the escape of soil gas through wetland trees is the dominant source of methane emissions in the Amazon basin.
- Sunitha R. Pangala
- , Alex Enrich-Prast
- & Vincent Gauci
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Letter |
Haze heats Pluto’s atmosphere yet explains its cold temperature
Modelling results find that the temperature of Pluto’s atmosphere is regulated by haze particles rather than gas molecules, suggesting that Pluto should be brighter than previously thought at mid-infrared wavelengths.
- Xi Zhang
- , Darrell F. Strobel
- & Hiroshi Imanaka
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Letter |
Role of stacking disorder in ice nucleation
Stacking-disordered ice crystallites are shown to have an ice nucleation rate much higher than predicted by classical nucleation theory, which needs to be taken into account in cloud modelling.
- Laura Lupi
- , Arpa Hudait
- & Valeria Molinero
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Letter |
Photonuclear reactions triggered by lightning discharge
Ground-based observations during a thunderstorm provide conclusive evidence of positrons being produced after lightning, confirming that lightning can trigger photonuclear reactions.
- Teruaki Enoto
- , Yuuki Wada
- & Harufumi Tsuchiya
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Review Article |
Detecting recovery of the stratospheric ozone layer
An overview of the nature and timescales of stratospheric ozone recovery and the extent to which it can currently be detected.
- Martyn P. Chipperfield
- , Slimane Bekki
- & Mark Weber
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Letter |
Minimal geological methane emissions during the Younger Dryas–Preboreal abrupt warming event
Measurements from Antarctic ice suggest that geological methane emissions are much lower than previously thought, and that methane emissions from hydrates and permafrost in response to climate warming are minimal.
- Vasilii V. Petrenko
- , Andrew M. Smith
- & Jeffrey P. Severinghaus
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Letter |
Tundra uptake of atmospheric elemental mercury drives Arctic mercury pollution
A two-year study of mercury deposition in the Arctic finds that the main source of mercury is gaseous elemental mercury, which is deposited throughout the year and leads to very high soil mercury levels.
- Daniel Obrist
- , Yannick Agnan
- & Detlev Helmig
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Letter |
Surface tension prevails over solute effect in organic-influenced cloud droplet activation
A phase-separation mechanism is proposed for the dominance of the surface tension effect over the solute effect in the observed activation of ultrafine cloud condensation nuclei.
- Jurgita Ovadnevaite
- , Andreas Zuend
- & Colin O’ Dowd
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Letter |
Biofuel blending reduces particle emissions from aircraft engines at cruise conditions
Compared to using conventional jet fuel, the use of a biofuel blend reduces aircraft engine particle emissions at cruising altitude by about 50–70 per cent.
- Richard H. Moore
- , Kenneth L. Thornhill
- & Bruce E. Anderson
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Letter |
Molecular-scale evidence of aerosol particle formation via sequential addition of HIO3
Field data from an iodine-rich, coastal environment point to the molecular steps involved in the formation of new aerosol particles from iodine vapours over coastal regions.
- Mikko Sipilä
- , Nina Sarnela
- & Colin O’Dowd
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Letter |
Heating of Jupiter’s upper atmosphere above the Great Red Spot
The upper atmosphere above Jupiter’s Great Red Spot—the largest storm in the Solar System—is hundreds of degrees hotter than anywhere else on the planet; the heating must come from below, suggesting coupling between Jupiter’s lower and upper atmospheres, probably the result of upwardly propagating acoustic or gravity waves.
- J. O’Donoghue
- , L. Moore
- & H. Melin