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Electrochemical conversion of CO2 into high-value products is attractive for lowering net carbon emissions. Lee et al. present the valorization of chemisorbed CO2 to CO in an aqueous monoethanolamine electrolyte via tailoring of the electrochemical double layer, with 72% Faradaic efficiency at 50 mA cm–2.
Owing to sluggish Mg-ion dissociation and diffusion, Mg-based batteries have low power densities. Here the authors carry out rational designs for both the cathode and the electrolyte to enable ultrafast kinetics of a Mg metal battery.
The complex, multi-component environments found in enzymes induce high catalytic specificity, but are difficult to achieve in synthetic catalysts. Now, researchers report a catalyst comprising a dynamic, ordered layer of ligands above a nanoparticle surface that creates a pocket to facilitate CO2 electroreduction.
There is consensus that using firewood negatively impacts women’s well-being, suggesting that clean alternatives will be preferred. However, this study finds that women have different views on how cooking with firewood and LPG support well-being depending on the fuel they currently use.
Two-dimensional Ruddlesden–Popper layered metal-halide perovskites show better performance over three-dimensional versions, but are typically based on quantum wells with random width distribution. Liang et al. show that introducing molten salt spacers gives phase-pure quantum wells and improved solar cell performance.
As wind turbines age and wind fleets expand, their replacement becomes increasingly complex. Kitzing et al. analyse turbine repowering activity in Denmark holistically, uncovering a range of factors that affect repowering decisions beyond physical space that need to be considered carefully.
Hydrogen is a promising vector in the decarbonization of energy systems, but more efficient and scalable synthesis is required to enable its widespread deployment. Towards that aim, Serra et al. present a microwave-based approach that allows contactless water electrolysis that can be integrated with hydrocarbon production.
Lead leakage from damaged perovskite photovoltaic modules poses health and environmental risks limiting the potential use of the technology. Now Chen et al. show that the encapsulation of perovskite modules with a cation-exchange resins reduces lead leakage to 14.3 ppb in waste water.
Home energy reports convey information about others’ energy use (descriptive norms) and social approval for energy saving behaviour (injunctive norms). This study shows that the combined effect of descriptive and injunctive feedback depends on their consistency and relative strength.
Solid-state caloric cooling is a promising alternative to vapour-compression refrigeration yet practical devices are not sufficiently efficient for applications. Meng et al. combine cascade device design with charge recovery and improve the cooling efficiency and temperature lift of an electrocaloric device.
Metal–organic frameworks (MOFs) are increasingly being explored for electrocatalytic oxygen evolution, which is half of the water splitting reaction. Here the authors show that, under reaction conditions, mixed metal oxyhydroxides form at the nodes of bimetallic MOFs, which are highly catalytically active.
The appropriate descriptors for a catalyst’s hydrogen evolution activity in alkaline electrolyte are debated. Combining simulations and single-crystal studies of metal-decorated Pt surfaces, McCrum and Koper show that activity exhibits a volcano-type relationship with the hydroxide binding strength of the catalyst, providing a target for catalyst design.
Estimating the costs of green home improvements is not possible without accurate estimates of their impact on house prices. Now, Shen et al. use the sales data of more than 400,000 properties in the United States to determine how heat pump installations increase house prices.
Low-bandgap tin–lead perovskites are key to all-perovskite tandem solar cells but simultaneous improvement in efficiency and stability has proven challenging. Now, Li et al. fabricate tin–lead perovskite cells with reduced methylammonium content that are 20.4% efficient and stable under illumination for 450 h.
Batteries need to be energy-dense as well as safe. Yi Cui and team develop an ultralight polyimide-based current collector with embedded fire retardants that enables lithium-ion batteries with much-enhanced safety and energy density.
Ensuring both stability and efficiency in mixed lead–tin perovskite solar cells is crucial to the development of all-perovskite tandems. Xiao et al. use an antioxidant zwitterionic molecule to suppress tin oxidation thus enabling large-area tandem cells with 24.2% efficiency and operational stability over 500 hours.
Nickel-rich layered oxide cathodes are at the forefront of the development of automobile batteries. The authors report an atomic and microstructural engineering design for a Li[Ni0.90Co0.09Ta0.01]O2 cathode that exhibits outstanding long-term cyclability and high energy at full depth of discharge in full cells.
While electricity production has a significant impact on air quality, the opposite effect has been suspected but not empirically demonstrated. Now, using pollution and electricity consumption data, He et al. show the impact of air pollution on domestic electricity consumption.
Understanding the severe voltage hysteresis in the first cycle of Li-rich cathodes is essential to realize their full potential in batteries. P. G. Bruce and colleagues report the formation of molecular O2 on charging rather than other oxidized O species is the cause for the voltage hysteresis.
The impact of energy consumption on air pollution in various forms has been studied extensively though less is known about how ambient air pollution affects energy use. Here, Eom et al. show how ambient air pollution increases domestic energy use in South Korea.