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The emerging kesterite Cu2ZnSnS4 solar cell offers a potential low-cost, non-toxic, materially abundant platform for next-generation photovoltaics, yet its efficiency has been mired below 10%. Yan et al. now use post-heat treatment of the heterojunction to show device efficiencies that surpass 10%.
Voltage fade is a major obstacle for the efficient use of lithium-rich layered oxide materials in batteries. Here, the authors reveal the link between voltage fade and nucleation of a mobile dislocation network in the oxide nanoparticles, offering design ideas to restore the voltage.
Despite their high efficiencies, perovskite solar cells still suffer from degradation issues that impede their practical deployment. Saidaminov et al. explore the effect of local lattice strain on vacancy formation and show that careful choice of dopants plays a key role, enhancing the device stability.
Achieving transport decarbonization targets depends on vehicle-purchasing decisions. Non-financial consumer preferences presented in six global energy-economy models reveal that diverse policies targeting vehicle buyers are necessary for the widespread adoption of clean technologies.
Interfacial losses between device layers play a key role in determining characteristics of solar cells. Jeon et al. address this in perovskite solar cells by synthesizing a hole-transporting layer that is better matched to the surrounding layers, and show high-efficiency and high-stability devices.
There is an intensive effort in developing grid-scale energy storage means. Here, the authors present a liquid metal battery with a garnet-type solid electrolyte instead of conventional molten salt electrolytes and report promising electrochemical properties at a modest temperature of 240 °C.
Ether-based electrolytes offer many advantages compared to other electrolyte systems, but they are not stable in Li metal batteries when operating at high voltages. Here, the authors develop a concentrated ether electrolyte that enables long-term cycling stability of high-voltage Li metal batteries.
Non-flammable electrolytes such as phosphates offer safety advantages for batteries, but they are prone to decomposition when coupled with graphite anodes. Here, the authors report a phosphate with a high salt-to-solvent ratio that displays high stability as well as compatibility with graphite in a commercial 18650-type cell.
Photocatalysts use light to drive chemical reactions; the effective spatial separation of photogenerated charges is key to their performance in solar energy conversion. Here, using surface photovoltage microscopy, the authors show that charges can be separated in photocatalytic particles by asymmetric light irradiation.
The development of Ni-rich layered lithium transition metal oxides is plagued by their voltage and capacity fading on battery cycling. Here, the authors demonstrate an effective approach to treat these problems by infusing a solid electrolyte into the grain boundaries of the secondary particles of these layered materials.
The scale and nature of energy investments under diverging technology and policy futures is of great importance to decision makers. Here, a multi-model study projects investment needs under countries’ nationally determined contributions and in pathways consistent with achieving the 2 °C and 1.5 °C targets as well as certain SDGs.
Substitution across fuels is hard to study because traditional transport technologies are typically single-fuel. Using Swedish data, this study shows that fuel demand elasticities differ across fuels, and drivers exhibit high preference for fossil fuels, hindering the take-up of alternative fuels.
Lithium cobalt oxides are used as a cathode material in batteries for mobile devices, but their high theoretical capacity has not yet been realized. Here, the authors present a doping method to enhance diffusion of Li ions as well as to stabilize structures during cycling, leading to impressive electrochemical performance.
Enzymatic fuel cells use enzymes for the redox reactions of fuels, and electron transfer is a key process in generating electricity. Here, the authors develop a redox mediator that is able to both immobilize the enzyme and mediate electron transfer, leading to much-enhanced power densities in fuel cells.
Redox flow batteries (RFBs) based on organic redox-active molecules are attractive, but the solubility of those molecules, and consequently the capacity, is generally low. Here, the authors develop a phenazine derivative with high solubility as an energy-dense anolyte for RFBs.
Car dealership experiences may influence EV purchase decisions of the majority of consumers who do not have pre-existing knowledge of EVs. This study shows that car dealerships present barriers to EV adoption because of dealer sales strategies that reflect government and industry conditions.
Investment and policy decisions about low-carbon technologies have been affected by the promise of a ‘unicorn technology’ that may reduce emissions at low costs. Researchers show that such investment delays can have high implications on cost and emissions whether the unicorn technology materializes or not.
Scaling up perovskite film deposition necessitates controlling the film formation dynamics. Here, Deng et al. use amphoteric choline surfactants to blade-coat well-passivated films, reaching module efficiencies of ~15% for aperture areas up to 57 cm2.
Use of wood and crop residue for cooking and heating in rural China is a significant source of carbon emissions and air pollution. Using a survey of more than 34,000 households, researchers show that between 1992 and 2012 usage of these fuels decreased by much more than previous estimates, due primarily to rising incomes.
Wind turbine technologies evolve, as do social acceptability and policies on wind farm siting. Here, Rinne et al. assess wind energy potential taking these evolutions into account and show an increase in the economic potential of wind energy in Finland using modern technology assumptions.