Abstract
The Schrödinger–Newton equation has gained attention in the recent past as a nonlinear modification of the Schrödinger equation due to a gravitational self-interaction. Such a modification is expected from a fundamentally semi-classical theory of gravity and can, therefore, be considered a test case for the necessity of the quantisation of the gravitational field. Here we provide a thorough study of the effects of the Schrödinger–Newton equation for a micron-sized sphere trapped in a harmonic oscillator potential. We discuss both the effect on the energy eigenstates and the dynamical behaviour of squeezed states, covering the experimentally relevant parameter regimes.
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Introduction
The interaction of nonrelativistic quantum matter with an external gravitational field has been experimentally established by the famous COW experiment1. However, the question whether gravity is fundamentally a quantum theory resembling the other fields, or something different, is still open. There is no unambiguous answer to the question how quantum matter sources the gravitational field. While the standard approach in regard to the great success of quantum field theory is to quantise the gravitational field along similar lines, there is no experimental evidence, nor a strict theoretical necessity, to date, that the gravitational field must be quantised2,3,4.
Taking the possibility of a fundamentally classical description of space-time into account, the most natural way to describe the interaction of quantum matter with such a classical space-time within the framework of general relativity is provided by the semi-classical Einstein equations,
i.e. Einstein’s field equations where the energy-momentum tensor is replaced by the expectation value of a corresponding quantum operator in some quantum state Ψ; a theory that was already suggested in the 1960s by Møller5 and Rosenfeld2. (Although it is often claimed that a fundamentally semi-classical theory of gravity was ruled out by experiment6, the arguments against such a theory are inconclusive3,4,7. It needs to be stressed that, different than in other situations where semi-classical gravity is considered as an effective limit of some underlying quantum theory of gravity8, in this approach equation (1) is taken as fundamental, at least at the microscopic level of single atoms).
In the nonrelativistic limit, such a fundamentally semi-classical theory of gravity adds a nonlinear potential term to the Schrödinger equation7,9. The resulting equation is known as the Schrödinger–Newton equation. For a multi-particle system, it reads
where Ψ is the N-particle wave-function and Vg is the gravitational interaction. The Schrödinger–Newton equation becomes nonlinear due to the dependence of Vg on the absolute-value squared of the wave-function. An intuitive way of looking at this equation is that the probability density, |Ψ|2, acts like a mass density generating a Newtonian gravitational potential, which then appears in the Schrödinger equation in the usual way. Vext is an external potential, which will be a quadratic, i.e. harmonic oscillator, potential here.
Equation (2) was first considered by Diósi10 as a model for wave-function localisation. Because of its derivability from semi-classical gravity, it was suggested that the Schrödinger–Newton equation can provide evidence for or against the necessity to quantise the gravitational field11. The original subject of such a test were heavy molecules in interferometry experiments12 for which the Schrödinger–Newton equation predicts inhibitions of the dispersion of the centre-of-mass wave-function13,14,15,16,17. Although the parameter regime where this effect shows up is much closer to the scope of current experiments than any quantum gravity effect studied so far, the required masses are still several orders of magnitude above what is currently feasible.
An alternative test of the Schrödinger–Newton equation, using macroscopic quantum systems in a harmonic trap potential, is given by Yang et al.18, who show that that the Schrödinger–Newton dynamics lead to a phase difference between the external and internal oscillations of a squeezed Gaussian state. Here, we complement this proposal by a more general analysis of effects of the Schrödinger–Newton equation on harmonically trapped quantum systems, going beyond the limit of narrow wave-functions and considering also the regime where the width of the wave-function becomes comparable to the localisation length of the atoms in the considered microsphere. In addition to the dynamical effects, we also discuss the gravitational perturbation of the spectrum of the stationary energy eigenstates.
While we will find that the dynamical effect on the internal structure of a squeezed state is indeed strongest in the limit of a narrow wave-function, as it has been studied by Yang et al.18, the intermediate regime is the most suitable to observe effects in the energy spectrum. These turn out to be of comparable order of magnitude as the dynamical effects. However, their observation requires slightly smaller masses and, more importantly, there is no necessity to create a squeezed state, which makes it an interesting alternative for feasible experimental tests. A possible experimental setup, achievable with existing technology, has been proposed elsewhere19.
We present the Hamiltonian for the trapped system with Newtonian self-gravitational interaction in the second section. We derive an approximation for the gravitational interaction inside a crystalline spherical many-particle system and discuss the reduction of the three-dimensional equation to a one-dimensional Schrödinger–Newton equation, which is the basis for the discussion thereafter. In the third section, we study the effects of the Schrödinger–Newton interaction on the energy spectrum. We discuss the limiting cases of a narrow and wide wave-function, as well as the intermediate regime. In the fourth section, the dynamical behaviour of a squeezed Gaussian state is derived, recovering the results by Yang et al.18 Their results are extended to the regime of finite, non-narrow wave-function sizes. Finally, our results and the prospects for experimental tests of the Schrödinger–Newton equation are summarised in the Discussion section.
Hamiltonian of a self-gravitating trapped sphere
Consider a three-dimensional Hamiltonian of a self-gravitating quantum system in an external potential:
The coordinates are written as r = (x, y, z). We will specify the external potential Vext later.
The Hamiltonian (4) is supposed to describe the centre-of-mass of a many-particle system. The gravitational potential, which is a function of all particle coordinates, does, however, not separate into centre-of-mass and relative coordinates exactly. Such a separation can only be achieved within a suitable Born–Oppenheimer-type approximation16. The multi-particle gravitational potential can then be reduced to
where ψ is the centre-of-mass wave-function, r is the centre-of-mass coordinate and ρc is the mass density relative to the centre of mass. For a lump of matter, i.e. a molecule, of N atoms which is described by a stationary relative wave-function χ, ρc is given as the sum of the marginal distributions for all but one atoms (the distribution of the N-th particle is given by the centre-of-mass wave-function and can be neglected if N is sufficiently large):
is simply the gravitational potential energy between the mass distribution described by ρc and the same mass distribution, shifted by d. For a homogeneous, spherical mass distribution with radius R it is given by20
Given a solution ψ(0) of the free Schrödinger equation (without the gravitational potential Vg), switching on the state dependent gravitational potential (5) will distort both the energy expectation value and the shape of the solution. To first order in the gravitational constant G, the correction to the Schrödinger evolution due to the nonlinear Schrödinger–Newton gravitational potential term can be obtained in a perturbation expansion. For this purpose, we make the ansatz
for the wave-function. Now note that the perturbation Vg of the Hamiltonian can be expanded as
where the first term is already . is just a linear correction to the Hamiltonian, which is time-independent for a stationary state ψ(0). The Hamiltonian (4) then takes the linear form
This is a good approximation as long as the gravitational interaction is considered to be weak and therefore the difference in the wave-function between the solutions of the unperturbed Schrödinger equation and those of the full Schrödinger–Newton equation is small.
The potential (5) can be considerably simplified in the limits where the wave-function is very narrow or very wide. Provided that the spatial centre-of-mass wave-function is wide compared to the extent of the considered many-particle system, the mass distribution within the system plays no important role and the gravitational potential is approximately the same as in the one-particle case, namely16
Consider, on the other hand, the case where the spatial centre-of-mass wave-function is narrow compared to the extent of the many-particle system, or—to be more precise—where does not vary too much over the width of the centre-of-mass wave-function. In this case the potential (5) can be expanded in a Taylor series in |r − r′| up to second order, yielding16,18
denoting the Hessian of .
If the mass is assumed to be distributed homogeneously over a sphere of radius R and therefore the function takes the form (8), then the potential is16
However, as pointed out by Yang et al.18, a realistic microsphere has a crystalline substructure, which must be taken into account if the wave-function is narrow enough to probe the atomic regime.
Crystalline substructure
A more realistic mass distribution should account for the fact that most of the mass in a crystalline structure is well-localised around the positions of the nuclei. then represents the gravitational interaction of a grid of N atoms with an identical grid, shifted by distance d. We model the quantum system as a sphere of radius R, within which the atoms are homogeneous spheres of radius σ, as depicted in Fig. 1. There are two contributions to :
1. The self-energy of each atom with its own “copy” which, approximately, can be modelled as the gravitational self-interaction of a sphere of radius σ with mass m/N, hence
2. The mutual interaction of each atom with all N − 1 other atoms, which is the Riemann sum for the integral (6) for the full sphere of radius R, if the sphere is split into N sub-areas of volume a3, hence
Therefore, for large N, the total function for a crystalline sphere is
with
Note that the expansion (13) is still valid in the limit of a narrow wave-function, which now means that the width of the wave-function is small compared to the atomic radius σ. Making use of the fact that γ2 ≈ 1 for , the corresponding gravitational potential is
with
where matom is the mass of a single atom in the crystal. This potential has been used by Yang et al.18 to describe the behaviour of a narrow squeezed coherent state in a harmonic trap. Since it is quadratic in r, a Gaussian state will remain Gaussian17,18, but there will be a gravitational contribution to the coupling constant. We come back to this below, in the section about the dynamics of a squeezed state.
If the atoms are, more realistically, modelled by Gaussian matter distributions18,
one can see with equation (6) that the self-interaction part of the function Icr takes the form20
where erf is the Gauss error function. The total Icr then is
For the Gaussian matter distribution, the gravitational potential of a narrow wave-function is of the same shape (19), but with the frequency ωSN and γ0 replaced by
where we assumed . This result should in principle agree with equation (14) in the work by Yang et al.18, provided that their . However, we find a factor of difference compared to their expression for .
It should be remarked that, while the splitting in cubes of volume a3 in the derivation provided here seems to imply the requirement of a simple cubic crystal structure, the result is actually independent of the type of the present crystal structure. Even a non-crystalline, amorphous substructure will still exhibit the behaviour described here, as long as the localisation length σ of the atoms is small compared to the average distance a between the atoms.
Reduction to one dimension
An approximate one-dimensional version of the Schrödinger–Newton equation can be obtained in the case where the shape of the external potential is such that the wave-function will be narrow in the two remaining dimensions. In this case, where the wave-function satisfies approximately
the gravitational potential (5) takes the form
is an even function by definition for any matter distribution ρc, hence the absolute value in the argument of . The dependence of the argument on y and z can be neglected, because the parts where y or z is substantially different from zero do not contribute in the Schrödinger equation after multiplication with the wave-function. Substituting d = |x − x′| the potential can be rewritten as
The functions (17) and (23) can now be applied to this one-dimensional potential without any changes and the Schrödinger equation separates and yields the one-dimensional equation
Note that we assume now that the external potential is quadratic with trap frequency ω0 in x-direction, while the shape of the external potential in y- and z-direction does not play a role, as long as the wave-function will be narrow.
The one-dimensional potential (27) still has the corresponding limits
for a wide (in x-direction) and narrow wave-function, respectively.
Gravitational effects on the energy spectrum
Without the gravitational potential Vg, the Schrödinger equation (28) has the well known energy eigenstates
where the Hermite polynomials Hn are defined by
and the corresponding energy eigenvalues are
As long as one is only concerned with stationary solutions, one can perform a first-order perturbation calculation to obtain the energy correction coming from the gravitational potential. In the quadratic narrow wave-function approximation (19) we immediately get the energy correction
In this approximation, the first term is just a constant shift of all energy levels, while the second term changes the spectral transition energies proportionally to . The transition energies,
are, however, still degenerate, i.e. they depend only on the difference (n2 − n1) and not on n1 and n2 alone. This degeneracy is removed if the higher order terms in the gravitational potential are taken into account, leading to a fine-structure of the spectral lines. Note that this fine-structure of the harmonic oscillator is of a different nature than the well-known fine-structure of atomic spectra. While in the latter there is a degeneracy of the actual energy eigenvalues, that is removed by additional interaction terms, the one-dimensional harmonic oscillator has an infinite number of non-degenerate energy eigenstates whose energy eigenvalues are shifted due to the Schrödinger–Newton potential. The degeneracy here is in the transition spectrum, where transition energies between eigenstates depend on the difference (n2 − n1) only. This is the degeneracy that is removed by the Schrödinger–Newton term.
To arrive at equation (34) we made use of the approximation (10). As mentioned before, in this case the gravitational potential is just a linear correction and the energy shift can be calculated in ordinary perturbation theory. Maintaining this approximation, but now using the full gravitational potential (26) instead of the quadratic approximation for narrow wave-functions, one obtains:
Introducing the dimensionless variables
we get
with
the even polynomials
and the matter distribution functions
for spherical atoms, and
for a Gaussian distribution of the atomic matter density, respectively. The polynomials Pn can be solved analytically and so can the functions fn, at least in principle. We obtained Pn for small n up to n = 14 using Mathematica. The time needed for the evaluation increases, however, exponentially with n. fn can be integrated analytically as well, in terms of integral functions. For realistic physical parameters it is nevertheless necessary to omit the constant contribution (see text below for definition) in a numerical evaluation of the transition energies, since otherwise the subtraction of two comparable, large numbers from each other would lead to a substantial loss of numerical accuracy. The transition energies can then be calculated as
Narrow wave-functions
In the limit of large values for α, i.e. narrow wave-functions, we can write
for the spherical atomic mass distribution, and
for the Gaussian distribution and hence
where we used that γ2 ≈ 1 and β2 ≈ 0 for R ≫ a ≫ σ. This yields exactly the previous results (35) with the frequencies (20) and (24).
Intermediate wave-functions
Now we want to go beyond the quadratic approximation for the potential, to see how the gravitational interaction removes the degeneracy of the transition energies. For this, we consider the intermediate regime where α is of the order of unity. We are, again, interested in the case where N ≫ 1 and R ≫ a ≫ σ. In this case, we have γ0 ≈ β0, and ρ ≫ 1. We can then write for the spherical atomic mass distribution
with
These functions become ρ-independent by taking only the zeroth order of the expansion around infinity. is an n-independent term, which is large but does not contribute to the transition energies. can be neglected since it goes to zero exponentially as ρ becomes large. The remaining terms, , and , are of comparable size, cf. Fig. 2. however enters into the full function fn with the small pre-factor Nσ3/R3 (which is, e.g., less than 10−4 for silicon and less than 10−5 for osmium at a few Kelvin) and therefore can be neglected as well, allowing for a ρ-independent approximation for fn. Figure 2 shows that for α > 1, is also negligible compared to . We nevertheless use both functions to calculate the transition energies with
For the Gaussian atomic mass distribution one obtains instead
with
were we accounted for the n-independent, -proportional, contribution of in . With the same arguments as before, this results in
In Fig. 3 these functions are plotted for the lowest four transitions with Δn = 1, for both the spherical and Gaussian atomic mass distribution. One can see how the degeneracy is removed and there is a split of for the spherical and for the Gaussian distribution, respectively. In the limit of an infinitesimally narrow wave-function, i.e. , all these functions will converge against the same value, in agreement with equation (35).
The order of magnitude of the split of the spectral lines belonging to the same Δn is given by the pre-factor in equation (43). Taking, e.g., silicon21 at a few Kelvin with matom = 28 u and σ ≈ 7.0 × 10−12 m, we get
The best value can be obtained for osmium22 with matom = 190 u and σ ≈ 2.8 × 10−12 m, where the above pre-factor is two orders of magnitude larger. Figure 4 shows the dependence of this pre-factor on the trap frequency and the corresponding masses for different values of α.
Qualitatively, the same effect can be expected from a three-dimensional harmonic oscillator, in situations where the wave-function has comparable width in all directions, although the situation gets more complicated when transitions are allowed in all three dimensions with different frequencies. We study the simpler case of an axially symmetric state which is excited in only the longitudinal direction in the Supplementary Information A.
Wide wave-functions
In the limit of a wide wave-function, α → 0 and , the dominant contribution comes from the function , yielding
with the n-dependent pre-factors
The first six values for the pre-factors are
The resulting transition energies are
is of the order of unity. The magnitude of the pre-factor for different trap frequencies, as well as the transition energies for a fixed frequency of 1 s−1 are plotted in Fig. 5. Since for the same trap frequencies the mass must be smaller in order to still be in the wide wave-function regime, the transition energies are several orders of magnitude below those for the intermediate regime.
There is also a “semi-wide” regime where the wave-function width is between σ and R. We omit the detailed discussion of this regime here. This has no effect on the qualitative results provided, although this regime could in principle be treated along the same lines. Experimentally, the narrow and intermediate regime are the most relevant for trapped microspheres. We mainly discussed the wide wave-function here for reasons of completeness and because this is the situation at hand in experimental tests based on molecular interferometry.
Gravitational dynamics of squeezed coherent Gaussian states
Inspired by the proposal by Yang et al.18, here we discuss the dynamical properties of a trapped microsphere that has been prepared in a squeezed ground state. A particular property of a harmonic potential is that a Gaussian wave packet remains Gaussian during its time evolution. This is because a Gaussian is fully determined by the first and second moments, 〈x〉, 〈p〉, 〈x2〉, 〈p2〉 and the correlation 〈xp + px〉 and the Schrödinger equation gives a closed system of equations for the same.
This property does not persist if a non-quadratic potential, such as our gravitational potential Vg, is added to the Hamiltonian. However, since the potential Vg is usually weak compared to the harmonic trap potential, we can assume that the dynamics of an initially Gaussian wave packet are still approximately determined by the time evolution of the first and second moments16,17,18.
With the general Schrödinger equation (28) one gets for the first moments16
Since is an even function and hence its derivative is odd, the expectation value of the derivative of Vg vanishes for any wave-function and any mass density function ρc. Therefore, the time evolution of the first moments remains completely unchanged by self-gravitation, as one would intuitively expect and in agreement with the Ehrenfest theorem.
For the second moments, first define the three-dimensional vector with components
Then the Schrödinger equation (28) yields the following system of equations:
with
The function h(t) can be shown to equal (see Supplementary Information B)
Redefining , , , and
the system (69) then takes the form
and is equivalent (given corresponding initial conditions) to the third order equation for u1
Up to this point, no restrictions have been imposed on the shape of the wave-function. Note, however, that g(t) depends on the wave-function. Hence, the right-hand-side is not a mere inhomogeneity but it renders the equation nonlinear and in general the system (74) will not be closed. If now we assume that the wave-function is of Gaussian shape,
then the gravitational potential Vg is completely determined (for a given solution of the system of eqns (64) and (65) for the first moments) by the wave-function width u1(t) and so is the function g(t). We then obtain instead of equation (75) the closed equation
where the prime denotes the derivative by u1. In this case, the gravitational interaction acts like a wave-function width dependent change of the frequency of the internal oscillations of a Gaussian state.
Obviously, such internal oscillations appear only in the case of a squeezed state—for a coherent ground state, u1 would be a constant in time. Without the gravitational interaction, starting initially with a state whose width is κ times the width of the ground state, the solution of equation (77) is
Hence, without gravity the width of the wave-function and 〈x〉 oscillate in phase. The gravitational interaction only affects the oscillation frequency of u1 and not that of 〈x〉 and therefore induces a de-phasing. This can, in principle, be observed experimentally.
In order to obtain quantitative results, we calculate the function g. Inserting the gravitational potential (27) and the wave-function (76) into (73) yields
Introducing dimensionless variables, as in the previous section,
this can be rewritten as
where is defined as in the previous section and denotes the derivative by ζ. Evaluating the ξ-integral and taking the derivative leads to the desired function
As before, we discuss the limits of a narrow and wide wave-function and the intermediate regime.
Narrow wave-functions
First we consider the limit α → ∞, corresponding to a narrow wave-function. We have
and
As before, we use that , and for and . With this, to lowest order one simply obtains
with the respective values (20) and (24) for the spherical and the Gaussian mass distributions.
Hence, we recover the result from Yang et al.18, that for a narrow wave-function the Schrödinger–Newton interaction yields a frequency shift to
for the internal oscillations.
Intermediate wave-functions
If α approaches values of the order of unity, we can split up the integral in a similar way as in the case of the energy spectrum above. Making use of , one obtains
and
with
For ρ ≫ 1 both k(0) and k(3) can be neglected. For ρ → ∞, , but since k(2) is multiplied with the small pre-factor Nσ3/R3 it can be neglected in comparison to k(1), k(1,g) and k(4) as well, just like in the case of the energy spectrum. The resulting according to equation (86), is plotted as a function of the parameter α in Fig. 6, for both the spherical and the Gaussian mass distribution, in the regimes of narrow (α ≫ 1) and intermediate wave-functions (α ≈ 1). One can see from Fig. 6a that the values (20) and (24) are recovered in the limit α → ∞.
The α-dependence of turns equation (77) into a nonlinear differential equation for the wave-function width. However, for finite values of α, only becomes smaller compared to the narrow wave-function case. Therefore, in order to experimentally observe the frequency shift for the internal oscillations, the wave-function should be as narrow as possible, contrary to the energy spectrum, where we found the largest effect in the intermediate regime.
Wide wave-functions
Finally, in the limit α → 0, i.e. for very wide wave-functions, the dominant contribution comes from k(3), yielding
Inserting this result into (77) yields a nonlinear differential equation, whose solution gives the deviation from the behaviour without gravity. The effect is, however, much smaller for the wide wave-function than in the case of narrow wave-functions.
Discussion
In this paper we provided a thorough survey of the effects of the gravitational self-interaction, described by the Schrödinger–Newton equation, on both the stationary states and the dynamics of a micron-sized sphere in a harmonic trap potential. We took the finite size of the system into account, as well as its crystalline substructure and discussed the results for the different regimes of a wave-function that is wide, narrow and comparable in width with the localisation of the nuclei in the crystal.
For the dynamics of a squeezed Gaussian state we recover the previous result18, that for a narrow state there is a frequency shift for the internal oscillations and hence a de-phasing compared to the oscillations of the centre, 〈x〉, of the wave-function. The conclusion by Yang et al.18 was that for a silicon crystal at 10 K and a trap frequency of 2π × 10 s−1 a quality factor of would be required for an experimental test of the Schrödinger–Newton effect.
Here, we could show that this result in the limit of a narrow wave-function is a best case scenario, in the sense that for a wider wave-function the de-phasing between internal and external oscillations only becomes smaller. We conclude from our considerations that for the given values18 a minimum mass of about 1015 atomic mass units is required. Below that mass, i.e. for , the amount of de-phasing drops considerably.
Contrary to this, we found that for the energy spectrum the Schrödinger–Newton effect is most pronounced in the regime of intermediate wave-functions. This is because the degenerate spectral lines at , for a fixed n, are all shifted by the same amount in the narrow wave-function regime, while for wider wave-functions this degeneracy is removed, yielding a characteristic effect. The relative size of this effect is comparable to the dynamical frequency shift, providing a second possible basis for an experimental test of the Schrödinger–Newton equation. We propose a particular experiment based on this gravitational fine-structure elsewhere19.
It is also worth to remark that both effects, the dynamical and the spectral effect, scale proportional to the atomic mass and the inverse cubed localisation of the atoms. For elemental crystals, this scaling factor is maximal for osmium, although experimental requirements might necessitate a trade-off with other desirable material properties.
A situation that has not been considered here, but might be of relevance for experimental tests of the Schrödinger–Newton equation, is self-gravitation of a superposition of (a small number of) energy-eigenstates. A naive perturbative approach fails for times that are large compared to the oscillation period of the trap. Hence, alternative approximation schemes are necessary in order to describe these states, that are neither stationary nor Gaussian.
Additional Information
How to cite this article: Großardt, A. et al. Effects of Newtonian gravitational self-interaction in harmonically trapped quantum systems. Sci. Rep. 6, 30840; doi: 10.1038/srep30840 (2016).
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Acknowledgements
The authors gratefully acknowledge funding and support from the John Templeton foundation (grant 39530). A.G. acknowledges funding from the German Research Foundation (DFG). J.B. and H.U. acknowledge support from the UK funding body EPSRC (EP/J014664/1). H.U. acknowledges financial support from the Foundational Questions Institute (FQXi). A.B. acknowledges financial support from the EU project NANOQUESTFIT, INFN and the University of Trieste (grant FRA 2013).
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A.G. performed the calculations, J.B. analysed the experimental feasibility. All authors discussed conceptional ideas and reviewed the manuscript.
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Großardt, A., Bateman, J., Ulbricht, H. et al. Effects of Newtonian gravitational self-interaction in harmonically trapped quantum systems. Sci Rep 6, 30840 (2016). https://doi.org/10.1038/srep30840
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DOI: https://doi.org/10.1038/srep30840