Introduction

According to the well-known Moore’s law, the development of electronic device is undergoing the bottleneck of the power and performance with continuous minimization1,2. Spintronics manipulates the electron spin instead of charge as state variable for electrical information processing, which gives rise to the possibility of many applications such as ultra-low power logic and non-volatile storage3,4,5,6. Spintronics devices have been proposed to perform logic operations, but most of them suffer from the large dynamic power inherent in the magnetic field to be used or in the requirement to frequently transform data between electrical and magnetic states for pipeline computing7,8,9. All-spin logic device (ASLD) is one of the most promising candidates to overcome the above issues since it both stores and computes with spin information and logic-in-memory structure10. The essential physical basis of ASLD is nonlocal spin transfer torque (STT) effect11,12 attributing to pure spin injection and detection in the lateral nonlocal spin valve (LNLSV)13. This phenomenon has been observed experimentally in all-metal LNLSV14,15,16,17, generally copper is considered as typically channel material. Recently, a benchmarking methodology based on copper channel ASLD for computing system has been further introduced and simulated18. Furthermore, ASLD with perpendicular magnetic anisotropy (PMA) nano-magnet is suggested to lower STT switching critical current density18,19. Nonetheless, with shrinking device dramatically, the current density challenges to exceeding the breakdown limit of copper due to electromigration (EM) crisis in 201520. For nanometer size ASLD, the breakdown characteristic of metal channel cannot be ignored and new material is also in great demand.

With the features of high electronic mobility, weak spin orbit coupling and hyperfine interactions, graphene has attracted considerable interests for future spintronics material21,22,23. In addition, the breakdown current density of graphene is at least two orders magnitude larger than that of copper24,25,26,27. Moreover, nonlocal STT effect in graphene-based LNLSV has been experimental demonstrated28,29, subsequently graphene-based all-spin logic gate (G-ASLG) with PMA nano-magnet has been proposed and evaluated19. However, the current-limiting factors of ASLD are lacking in detailed analysis, especially the current conditions, which is very important to assess the feasibility and optimization.

In this paper, we investigate the current-limiting factors of ASLD and develop a physics-based model including nano-magnet switching, spin transport properties and breakdown characteristic of channel. First, we present different structures of ASLD. Second, we introduce the compact model of ASLD based on STT effect in PMA nano-magnet, spin transport properties in LNLSV and breakdown current density of channel, such as graphene and copper. Finally, we address the current-limiting conditions and energy dissipation to assess and optimize ASLD, which contributes to the design and implement of future spintronics devices.

Results and Discussions

All-spin logic device (ASLD)

Firstly, as Fig. 1 shows, main part of ASLD is the structure of LNLSV, which is composed of PMA input and output nano-magnet (F1 and F2) connected by a nonmagnetic channel (such as copper or graphene). It is based on spin transport properties in LNLSV and nonlocal STT switching to perform logic operation. Once a charge current, Iinj, is injected into the device, spin current beneath input nano-magnet can diffuse in both directions, i.e., toward leftside (as a spin and charge current) and toward rightside (as a pure spin current). Then a voltage Vdet can be measured in the output nano-magnet as a result of spin accumulation in parallel (P) or antiparallel (AP) alignments of magnetizations and the spin signal is defined as Rs = (VdetAP – VdetP)/Iinj. The spin current following into the output nano-magnet Idet is used to switch its magnetization based on nonlocal STT effect. Thus ASLD stores information as the magnetizations of input and output and communicates through pure spin current, just as its name implies.

Figure 1
figure 1

Main part of all-spin logic device (ASLD), i.e. structure of lateral nonlocal spin valve (LNLSV).

(a) Structure with tunnel barrier contact in both the input and output F1/T/C/T/F2. (b) Structure with tunnel barrier contact in the input and transparent contact in the output F1/T/C/F2. (c) Structure with transparent contact both in the input and output F1/C/F2. Js and Jc are spin current density and charge current density, respectively.

To alleviate the conductance mismatch problem30,31,32 for graphene channel LNLSV, tunnel barrier has been added, seen in Fig. 1(a), to enhance the spin injection or detection efficiency P1, 2 and contribute to large spin signal Rs. Besides, asymmetric structure is presented as Fig. 1(b), where tunnel barrier is only added in the input. It can ensure high spin injection efficiency and large absorption with low contact resistance. For metal channel LNLSV or all-metal ASLD proposal, the transparent contact is generally used instead of tunnel barrier, as shown in Fig. 1(c). In the following, the performance of current-limiting and energy with these three structures are compared and discussed.

Current-limiting Models of ASLD

Afterwards, in order to study the current-limiting factors of the ASLD, we have developed a physics-based compact model that integrates STT switching of output nano-magnet, spin transport properties of LNLSV and breakdown characteristic of channel. It allows us to analyze parameters such as device dimension, material parameters and contact resistance and their interdependences, as well as to explore how to overcome current-limiting challenges and optimize ASLD performance.

Critical current of switching nano-magnet

Firstly, compared to in-plane magnetic anisotropy, PMA nano-magnet can reduce critical current density Jc0 or current Ic0 due to absence of the easy-plane anisotropy term11. Therefore we consider ASLD with PMA nano-magnet so as to reduce required current essentially. In addition, the perpendicular anisotropy energy density of PMA is high enough to ensure high thermal stability Δ = Eb/kBT, where Eb, kB, T are energy barrier, Boltzmann constant and temperature, respectively. Regarding the nano-magnet size below the domain wall width, we assume single-domain magnetization reversal with STT effect12,13,33. Since size effect of demagnetization factors is considered based on macrospin model33, Jc0 for PMA output nano-magnet can be derived as follows

where MS is saturation magnetization and P is spin polarization factor. Ac is nano-magnet area and tF is free layer thickness of output nano-magnet. e, ħ, μ0 are the elementary charge, reduced Planck constant and vacuum permeability, respectively. The demagnetization factors Nz is calculated to decrease with shrinking the nano-magnet size34, consequently it enhances the effective perpendicular energy density shown in Fig. 2(a). Satisfying that Jc0 is independent of nano-magnet area or only depends on nano-magnet thickness in the macrospin model33, we can obtain effective damping constant αeff shown in Fig. 2(a). Then the time-dependent magnetization dynamic is governed by the Landau-Lifshitz-Gilbert equation including spin torque11,12. As a result, we give static and dynamic properties of switching output nano-magnet with scaling down (nano-magnet width W from 30 nm to 4 nm) in Fig. 2. It shows that thermal stability Δ scales almost linearly with nano-magnet width W, but critical current Ic0 decreases in proportion to nano-magnet area Ac, leading to increasing STT efficiency Δ/Ic0 with shrinking nano-magnet. The above modified macrospin model is able to demonstrate STT behavior with size effect, whose theoretical results agree well with experimental observations33,35. Note that, as shown in Fig. 3(c), the critical current for required switching time 2 ns, Itsw=2ns, which is equal to Idet, tsw=2ns, is utilized to further estimate the performance of ASLD in this paper.

Figure 2
figure 2

Static and dynamic properties for switching the output nano-magnet.

The critical current density Jc0 is calculated as 4.68 MA/cm2 based on Eq. (1) and all the used parameters are listed in the Table 1. (a) Calculated effective perpendicular magnetic anisotropy energy density Keff and effective damping constant αeff as a function of nano-magnet width W. (b) Thermal stability Δ with respect to nano-magnet width W. (c) Calculation of the critical current Ic0 and current for 2 ns switching time Itsw=2ns as a function of square nano-magnet area AC. (d) The dependence of spin-torque switching efficiency Δ/Ic0 on nano-magnet width W.

Figure 3
figure 3

Calculation of spin transport efficiency Idet/Iinj of ASLD with graphene channel based on Eq. (2).

The default device geometry is (W, L) = (30 nm, 100 nm) and the other parameters of graphene are listed in Table 1. (a) Calculation of Idet/Iinj as a function of contact resistivity R1W and R2W. (b) Calculation of Idet/Iinj as a function of spin injection/detection efficiency P1 and P2. (c) Calculation of Idet/Iinj as a function of device geometry (W, L). (d) Calculation of Idet/Iinj as a function of diffusion length of graphene λG.

Spin transport properties of ASLD

Most importantly, spin transports properties are figured out to diminish input charge current Iinj that generates Idet. Based on spin-dependent and one-dimensional drift-diffusion theory, we define and calculate spin transport efficiency η as13,19

where is nano-magnet spin resistance with spin diffusion length λF, resistivity ρF, thickness tF and contact or nano-magnet area AC. is spin resistance of nonmagnetic channel, where ρN, W, tN and λN are the resistivity, width, thickness and spin diffusion length of channel, respectively. Ri is contact resistance of the injector (i = 1) or the detector (i = 2). P and Pi are the spin polarization of the electrode and the interfaces, respectively. Eq. (2) and Fig. 3 show that spin transport efficiency η depends strongly on the material parameters (Ri, Pi, ) as well as the device geometry (channel width W and length L shown in Fig. 1). Especially, as shown in Fig. 2 (a), higher efficiency can be obtained by increasing input contact resistance R1 and decreasing output contact resistance R2, thus asymmetric structure (as Fig. 1(b)) is expected. Note that, RiW type of contact resistivity is generally utilized for graphene instead of RiA type36. According to nano-magnet switching and spin transport properties of channel, the lower limit of Iinj for workable ASLD is deduced as Ic0/η.

Breakdown current density of ASLD

Furthermore, with the object of finding the upper limit of Iinj of ASLD, we study the breakdown current density of channel JBR. In this work, we focus on typically spin channel materials, graphene and copper. For graphene channel due to Joule heating mechanism, we apply the size-dependent model of Liao et al.37 Taking into account both heat loss to the substrate and to the interface, the breakdown current density of graphene channel JBR, G is calculated as37

In our calculation, TBD is the breakdown temperature (~873 K oxidation in air); T0 is ambient temperature (295 K); is thermal healing length, kG is thermal conductivity of graphene and RT is the thermal resistance at the metal contacts. The thermal contact resistance per unit length from the graphene channel to substrate is calculated as37

Where kox is the thermal conductivity of substrate; tox is the thickness of substrate; RCox is thermal resistance of the graphene-substrate interface. Taking graphene-SiO2 as example based on above model and experimental results27, we require lower resistivity, smaller dimension and thinner substrate for higher JBR, G as illustrated in Fig. 4. Based on Eq. (3) and Eq. (4), higher thermal conductivity (kox) or lower thermal resistance of graphene-substrate interface (RCox) can achieve higher breakdown current density. It is a possible solution to utilizing diamond substrates (higher kox) or graphene-BN substrates (lower RCox due to smoother interface).

Figure 4
figure 4

Breakdown current density JBR of graphene and copper.

(a) The breakdown current density vs resistivity for 32 nm × 80 nm (W × L) graphene channel on 90 nm thickness SiO2. Thermal conductivity of graphene and SiO2 are kG = 100 W·m−1·K−1 and kox = 1.4 W m−1·K−1, respectively. Graphene-oxide interface thermal resistance Rcox = 10−8 m2 K W−1. (b) Calculated dependence of JBR on oxide thickness tox and graphene channel width W based on Eqs. (3 and 4). The inset shows that percentage of contribution to total thermal resistance (g-1) from the graphene-oxide interface and substrate, as a function of graphene channel width at tox = 90 nm. Parameters used are same as above. (c) Calculated dependence of JBR as a function of channel width. L = 100 nm and the other parameters are same as Table 1. The inset shows the resistivity of copper will dramatically increase for sub-100 nm wide based on Eq. (11), resulting in the decrease of JBR, Cu based on Eq. (5). (d) Calculated dependence of JBR as a function of channel length.

Going forward metal channel, electromigration (EM) is one of the key current density limitations with shrinking size of device rapidly. We consider EM-failure mechanism for size-dependent breakdown current density of copper channel JBR, Cu with Blech model and the threshold product is described as38,39

where Ω, Δσ, Z* are the atomic volume of copper, the normal stress difference between channel ends and effective charge of copper. The threshold product can be obtained experimentally, for example, 1500 A/cm for Cu/SiO2, then the length-effect design can be realized. Furthermore, the increasing resistivity of copper ρCu with narrow-width effect is also under consideration40, resulting in decreasing JBR, Cu based on Eq. (5). Therefore calculated JBR, Cuwith size-effect are presented in Fig. 4(c,d). It shows that, JBR, Cu will suffer from the great growing resistivity and benefit from the short-length effect. In contrast, graphene can sustain current density around 1010A/cm2, 2 orders of magnitude higher than that of copper.

Current-limiting conditions and optimization

Finally, the whole current-limiting factors have been investigated as above, namely the current-limiting conditions of ASLD can be written as following,

Given a workable injection current Iinj, we can obtain its switching time tsw by solving LLG equation. Note that the process time of ASLD is determined by the STT switching and the time of spin current propagation is ignored2,41. To demonstrate the entire performance of ASLD, the device energy dissipation per bit can be estimated as

where Rin (~R1) is input resistance related to the input charge current path. Based on Eq. (2), as contact resistance R1 increases, spin transport efficiency η is higher, which can reduce injection current Iinj so as to help lower energy. However, the increase of R1 leads to the augmentation of energy. Thus contact resistance R1 has optimal value for the minimum energy of ASLD. As mentioned, the LLG solution value of Idet, tsw=2ns for nano-magnet W = 10 nm, tF = 2 nm is taken into account. Figure 5 shows the injection current and energy as a function of contact resistance for both graphene and copper channel in different lengths L, the breakdown current is also illustrated as the upper limitation. In Fig. 5(a) and Fig. 5(c), the injection current Iinj exhibits a minimum, since increasing R1 will reduce η and boost Iinj after the saturation of spin signal Rs with R1RN. The advantage of the breakdown current density of graphene makes a broad workable current range for ASLD, that is to say, we can enhance injection current Iinj for fast speed 1/tsw. But it is true that the spin resistance of graphene RG is larger than that of copper, the optimal contact resistance of graphene channel corresponds to be larger. As shown in Fig. 5(b) and Fig. 5(d), the optimized energy of graphene channel ASLD is almost ten times larger than that of copper channel ASLD. In addition, it is found that the optimal value of contact resistance increases as the channel length.

Figure 5
figure 5

Analysis and optimization of injection current and energy based on contact resistance.

(a) Calculated injection current Iinj for switching time tsw = 2 ns, Iinj, tsw=2ns and input resistance Rin as a function of contact resistance R1 at different values of channel length for structure F1/T/G/F2. The dash line stands for the corresponding breakdown current density JBR, G. (b) Calculated energy for switching time tsw = 2 ns, Etsw=2ns as a function of contact resistance R1 at different values of channel length for structure F1/T/G/F2. (c) Calculated Iinj, tsw=2ns and Rin as a function of contact resistance R1 at different values of channel length for structure F1/T/Cu/F2. JBR, Cu is illustrated as dash line. (d) Calculated Etsw=2ns as a function of contact resistance R1 at different values of channel length for structure F1/T/Cu/F2.

At last, we have demonstrated and analyzed all the performances of ASLD in different materials (graphene and copper) and structures as shown in Fig. 6. The dependence of each parameter is analyzed. Thanks to spin transport efficiency, asymmetric structure is the optimal structure for lower injection current Iinj to overcome current-limiting issue. To reduce injection current and energy dissipation in the same structure, smaller device with larger aspect ratio W/L, higher spin injection efficiency P1 and longer diffusion length λN are expected. For the copper channel, the device geometry and material parameters are strictly satisfied due to the breakdown current. For example, if we take 10 nm wide copper channel with both transparent contacts, F1/Cu/F2, breakdown will always occur unless the channel length L is within 20 nm as shown in Fig. 6(a). Even so, the required spin injection efficiency must reach up to 0.5 at least and the minimal spin diffusion length is 200 nm. Compared with copper, graphene can sustain higher breakdown current so that it can easily obtain an achievable ASLD. However, the energy performance of graphene channel ASLD is restricted by its large contact resistance. It is a possible solution to finding new tunnel material that realizes lower contact resistance as well as high efficiency.

Figure 6
figure 6

Calculated injection current Iinj and energy for switching time tsw = 2 ns in different materials and structures considering the breakdown current density JBR. The transparent contact resistivity of copper channel is used as RiA = 0 and the other default parameters are listed in Table 1. (a,b) give the calculated dependence Iinj, tsw=2ns and Etsw=2ns on channel length L. (c,d) give the calculated dependence Iinj, tsw=2ns and Etsw=2ns on channel width W. (e,f) give the calculated dependence Iinj, tsw=2ns and Etsw=2ns on spin injection efficiency P1. (g,h) give the calculated dependence Iinj, tsw=2ns and Etsw=2ns on spin diffusion length λN.

Conclusions

In summary, we have developed a physic-based model for ASLD including PMA nano-magnet switching, spin transport properties and breakdown characteristic of channel. Its current-limiting factors, i.e., critical current of nano-magnet, spin transport efficiency and breakdown current of channel, have been investigated. In order to estimate the feasibility and performance of ASLD, the current-limiting conditions and energy dissipation have been addressed. Moreover, it has been shown that the contact resistance can be optimized for minimum energy. Regardless of the spin channel materials, the asymmetric structure is the most effective for ASLD in terms of current limitation. Copper channel outperforms graphene in term of energy but seriously suffers from the breakdown current limit. By exploring the current limit and performance tradeoffs, we can expect larger aspect ratio W/L, higher spin injection efficiency P1 and longer diffusion length λN. Our work is significant in the design and implementation of reduced ASLD facing current-limiting challenges, which gives a promising prototype for future spintronics applications.

Methods

Statistic and dynamic model of switching nano-magnet

Spin transfer torque (STT) effect is simulated based on the model deriving from Slonczewski and Berger11,12. The critical current density (Jc0) and switching time (tsw) for PMA nano-magnet vector () have been calculated by following macrospin model based on Landau-Lifshitz-Gilbert (LLG) equation with STT term. The main parameters are described and listed in Table 1. Jc0 is given as Eq. (1) and the LLG equation reads

Table 1 Main parameters for Calculation.

where aJ is the strength of spin transfer torque, , J is the current density and p is a unit vector representing the direction of the magnetization of the input nano-magnet. As the size of device shrinks, we consider the nano-magnet width W smaller than the domain wall width (e.g.30 nm35) and assume that single-domain magnetization reversal takes place. Providing that interfacial and bulk magnetic anisotropies are intact, the effective perpendicular anisotropy field is expressed as

where Nx, Ny, Nz are demagnetization factors, which depend on the nano-magnet dimensions and satisfy that 34. As a result, the effective perpendicular anisotropy energy density increases with decreasing W owing to decrease of Nz34. Supposing that critical current density only relies on the material parameters and thickness of nano-magnet, we can obtain the calculated effective damping constant that reduces with W below 30 nm.

In addition, the disturbance caused by thermal agitation during the magnetization switching is supposed to be negligible, but the initial position of the nano-magnet vector is thermally distributed at a finite temperature. Here we use root square average value calculated by Eq. (10) as an initial angel θ

In this work, we simulated time-dependent magnetization dynamics of 2-nm-thick nano-magnet width of 4 nm~30 nm by solving LLG equation and obtained the different critical current density or current for required switching time, e.g. Itsw=2ns.

Spin transport model of LNLSV

The lateral non-local spin valve (LNLSV) is the key element of the ASLD. Aimed at the spin transport efficiency , we analyzed the interface effects and spin accumulation based on the spin transport model of Takahashi13, taking into account the spin dependent and the one-dimensional drift-diffusion theory.

Physical model of copper resistivity

Regarding surface scattering of the conduction electrons and scattering due to grain boundaries, the resistivity is calculated as follows41

where p, Q, λm, Cu, d is the specularity parameter, the reflectivity coefficient at grain boundaries, the mean free path and the average distance between grain boundaries, respectively. C is a constant with value 1.2 for rectangular cross section channel. The parameters are set as p = 0.49, Q = 0.27, λm, Cu = 45, d = 80 nm and the others are listed in Table 1.

Additional Information

How to cite this article: Su, L. et al. Current-limiting challenges for all-spin logic devices. Sci. Rep. 5, 14905; doi: 10.1038/srep14905 (2015).