Abstract
The precision of matter-wave sensors benefits from interrogating large-particle-number atomic ensembles at high cycle rates. Quantum-degenerate gases with their low effective temperatures allow for constraining systematic errors towards highest accuracy, but their production by evaporative cooling is costly with regard to both atom number and cycle rate. In this work, we report on the creation of cold matter-waves using a crossed optical dipole trap and shaping them by means of an all-optical matter-wave lens. We demonstrate the trade off between lowering the residual kinetic energy and increasing the atom number by reducing the duration of evaporative cooling and estimate the corresponding performance gain in matter-wave sensors. Our method is implemented using time-averaged optical potentials and hence easily applicable in optical dipole trapping setups.
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Introduction
Ever since their first realization, atom interferometers1,2,3,4 have become indispensable tools in fundamental physics5,6,7,8,9,10,11,12,13,14,15,16,17 and inertial sensing18,19,20,21,22,23,24,25,26,27,28,29,30. The sensitivity of such matter-wave sensors scales with the enclosed space-time area which depends on the momentum transferred by the beam splitters as well as the time the atoms spend in the interferometer.
The expansion of the atomic clouds, used in interferometers, needs to be minimized and well controlled to reach long pulse separation times, control systematic shifts, and create ensembles dense enough to detect them after long time-of-flights. Nevertheless, colder ensembles with lower expansion rates typically need longer preparation times. Therefore, matter-wave sensors require sources with a high flux of large cold atomic ensembles to obtain fast repetition rates.
Bose-Einstein condensates (BECs) are well suited to perform interferometric measurements. They are investigated to control systematic effects related to residual motion at a level lower than a few parts in 109 of Earth’s gravitational acceleration20,31,32,33,34. In addition, due to their narrower velocity distribution35, BECs offer higher beam splitting efficiencies and thus enhanced contrast23,36,37, especially for large momentum transfer36,38,39,40,41,42,43. Finally, the inherent atomic collisions present in BECs can enhance matter-wave interferometry by enabling (i) ultra-low expansion rates through collective mode dynamics with a recent demonstration of a 3D expansion energy of \({k}_{B}\cdot 3{8}_{-7}^{+6}\) pK44, and (ii) ultimately the generation of mode entanglement through spin-squeezing dynamics to significantly surpass the standard-quantum limit45,46,47,48.
Today’s fastest BEC sources rely on atom-chip technology, where near-surface magnetic traps allow for rapid evaporation using radio frequency or microwave transitions. This approach benefits from constant high trapping frequencies during the evaporative cooling process, thus leading to repetition rates on the order of 1 Hz with BECs comprising 105 atoms49.
Anyway, since magnetic traps are not suitable in certain situations optical dipole traps become the tool of choice50. Examples are trapping of atomic species with low magnetic susceptibility51,52, or molecules53,54 and composite particles55,56. In optical dipole traps external magnetic field allow tuning parameters, e.g., when using Feshbach resonances57.
Here, the intrinsic link between trap depth and trap frequencies in dipole traps58 inhibits runaway evaporation. Cold ensembles can be only produced in shallow traps, leading to drastically increased preparation time tP. This long standing problem has been recently overcome through the use of time-averaged potentials, where trap depth and trap frequencies can be controlled independently, thus allowing for more efficient and faster evaporation while maintaining high atom numbers52,59.
In this work, we use dynamic time-averaged potentials for efficient BEC generation and demonstrate an all-optical matter-wave lens capable of further reducing the ensemble’s residual kinetic energy. Contrary to pulsed schemes of matter-wave lensing44,60,61,62,63,64,65, we keep the atoms trapped over the entire duration of the matter-wave lens37, which eases implementation in ground-based sensors. Moreover, we show that with this technique one can short-cut the evaporation sequence prior to the matter-wave lens, which increases the atomic flux by enhancing atom number and reducing cycle time while simultaneously reducing the effective temperature. Our method can largely improve the matter-wave sensor’s stability in various application scenarios.
Results
Evaporative cooling
We operate a crossed optical dipole trap at a wavelength of 1960 nm loaded from a 87Rb magneto-optical trap (details in the “Methods” section). The time-averaged potentials are generated by simultaneuos center-position modulation of the crossed laser beams in the horizontal plane. Controlling the amplitude of this modulation and the intensity of the trapping beams enables the dynamic control and decoupling of the trapping frequencies and depth. We chose the waveform of the center-position modulation to generate a parabolic potential52.
Up to 2 × 107 rubidium atoms are loaded into the trap with trapping frequencies ω/2π ≈ {140; 200; 780} Hz in \(\{{x}^{\prime};\,{y}^{\prime};\,z\}\) direction (definition of coordinate systems in the “Methods” section) with a trap depth of 170 μK. For this we operate the trap at the maximum achievable laser intensity of 12 W and the center-position modulation at an amplitude of h0 = 140 μm.
We perform evaporative cooling by reducing the trap depth exponentially in time while keeping the trapping frequencies at a high level by reducing the amplitude of the center-position modulation. This method allows us to generate BECs with up to 4 × 105 atoms within 5 s of evaporative cooling. By shortening the time constant of the exponential reduction we generate BECs with 5 × 104 (2 × 105) particles within 2 s (3 s) of evaporative cooling. At the end of the evaporation sequence the trap has frequencies of ω/2π ≈ {105; 140; 160} Hz and a depth of about 200 nK. The expansion velocity of the condensate released from the final evaporation trap is 2 mm s−1, which corresponds to an effective temperature of 40 nK.
All-optical matter-wave lens
Our matter-wave lens can be applied in any temperature regime explorable in our optical trap. We investigate the creation of collimated atomic ensembles for different initial temperatures of the matter-waves. To this aim, the evaporation sequence is stopped prematurely at different times to generate input atomic ensembles at rest with initial trap frequency ω0 and initial temperature T0. We then initiate the matter-wave lens by a rapid decompression66 of the trap frequency in the horizontal directions from ω0 to ωl. Here we denote by ωl the lensing potential in analogy with the Delta-kick collimation technique. The reduction of the trapping frequencies from the initial ω0 to ωl depends on experimental feasibility, such as the maximum achievable amplitude of the center-position modulation and the modulation amplitude right before the rapid decompression. With ongoing evaporative cooling this amplitude is reduced and thus the trap can be relaxed much further for more continued sequences. However, we need to maintain the confinement in the vertical direction by adjusting the dipole trap’s intensity to suppress heating or loss of atoms.
Subsequent oscillations in the trap result in a manipulation in phase space (Fig. 1a, b) for focusing, diffusion, and, importantly collimation of the matter-wave (Fig. 1c). Figure 1c depicts the expansion of a thermal ensemble in 1D for three different holding times (thold) to highlight the importance of a well chosen timing for the lens. Figure 2 shows exemplary expansion velocities (colored circles) depending on the holding time thold. The colored curves in this graph display the simulated behavior following the scaling ansatz (details in the “Methods” section) with an error estimation displayed by shaded areas. Only for the final measurement (also shown in the inset in Fig. 2) we create a BEC with a condensed fraction of 92.5% of the total atom number and apply the matter-wave lens to it.
With the presented method we observe oscillations of the expansion rate, which are in good agreement with the simulations for different ensemble temperatures. For all investigated temperatures an optimal holding time exists for which the final expansion rate is minimized (Fig. 3a). The ratios of σv,l/σv,0 and ωl/ω0 for each measurement is shown in Fig. 3b.
The change in atom number from the initial to the lensing trap (Fig. 3a) lies within the error bars and arises mainly due to pointing instabilities of the crossed optical dipole trap beams. The lowest expansion rate is achieved with 553(49) μm s−1 with a related effective temperature of 3.2(0.6) nK and an atom number of 4.24(0.02) × 105. With this method we achieve a more than one order of magnitude lower effective temperature while maintaining a comparable atom number compared to evaporative cooling.
Discussion
In this paper, we demonstrate a technique to reduce the expansion velocity of an atomic ensemble by rapid decompression and subsequent release from an dipole trap at a well-controlled time. The efficiency of the matter-wave lens for higher temperatures is mainly limited experimentally by the limited ratio between the initial and the lensing trap frequency ωl/ω0 (Fig. 3b) which is constrained by the maximum possible spatial modulation amplitude of the trapping beams. In general, according to the Liouville theorem, the expansion speed reduction of the matter-wave is proportional to \({({\omega }_{0}/{\omega }_{l})}^{2}\) where a large aspect ratio enables a better collimated ensemble. The atoms are loaded into the time-average potential with an optimized center-position modulation amplitude of 140 μm, while the maximum is 200 μm. During the evaporation sequence this amplitude is decreased. Consequently, the relaxation of the trap is less efficient at the beginning of the evaporative sequence or directly after the loading of the trap.
Another constraint is that the trap’s confinement in the unpainted vertical direction is required to remain constant. If the vertical trap frequency is increased we observe heating effects and suffer from atom loss when it is decreased. To compensate for the trap depth reduction during the switch from the initial to the lensing trap we increase the dipole trap laser’s intensity accordingly.
An additional modulation in the vertical direction, e.g., by means of a two-dimensional acousto-optical deflector, as well as an intersection angle of 90° would enable the generation of isotropic traps. In such a configuration, the determination of the optimal holding time will benefit from the in-phase oscillations of the atomic ensemble’s size67. When applying our matter-wave lens in a dual-species experiment, isotropy of the trap will also improve the miscibility of the two ensembles68.
To illustrate the relevance for atom interferometers, we discuss the impact of our source in different regimes (details in the “Methods” section) operated at the standard quantum limit for an acceleration measurement. In a Mach-Zehnder-like atom interferometer1,18, the instability reads
after an averaging time τ, neglecting the impact of finite pulse durations on the scale factor69,70,71. Eq. (1) scales with the interferometer contrast C, the atom number per cycle N, the effective wave number nℏkeff indicating a momentum transfer during the atom-light interaction corresponding to 2n photons, and the separation time between the interferometer light pulses TI. The cycle time of the experiment tcycle = tP + 2TI + tD includes the time for preparing the ensemble tP, the interferometer 2TI, and the detection tD. In Eq. (1), the contrast depends on the beam splitting efficiency. This, in turn, is affected by the velocity acceptance and intensity profile of the beam splitting light, both implying inhomogeneous Rabi frequencies, and consequently a reduced mean excitation efficiency35,72,73. Due to expansion of the atomic ensemble and inhomogeneous excitation, a constrained beam diameter implicitly leads to a dependency of the contrast C on the pulse separation time TI, which we chose as a boundary for our discussion. We keep the effective wave-number fixed and evaluate σa(1 s) for different source parameters when varying TI.
Figure 4 shows the result for collimated (solid lines) and uncollimated (dotted lines) ensembles in our model (details in the “Methods” section) and compares them to the instability under use of a molasses-cooled ensemble (dash-dotted line). Up to TI = 100 ms and σa(1 s) = 10−8 m s−2, the molasses outperforms evaporatively cooled atoms or BECs due the duration of the evaporation adding to the cycle time and associated losses. In this time regime, the latter can still be beneficial for implementing large momentum transfer beam splitters36,38,39,40,42,43 reducing σa(τ) or suppressing systematic errors20,31,32,33,34,74 which is not represented in our model and beyond the scope of this paper. According to the curves, exploiting higher TI for increased performance requires evaporatively cooled atoms or BECs. This shows the relevance for experiments on large baselines23,37,74,75,76,77 or in microgravity78,79. We highlight the extrapolation for the Very Long Baseline Atom Interferometer (VLBAI)76,80, targeting a pulse separation time of TI = 1.2 s81. Here, the model describing our source gives the perspective of reaching picokelvin expansion temperatures of matter-wave lensed large atomic ensembles.
Methods
Experimental realization
The experimental apparatus is designed to operate simultaneous atom interferometers using rubidium and potassium and is described in detail in references9,10,82.
For the experiments presented in this article only rubidium atoms were loaded from a two dimensional to a three dimensional magneto-optical trap (2D/3D-MOT) situated in our main chamber. After 2 s we turn off the 2D-MOT and compress the atomic ensemble by ramping up the magnetic field gradient as well as the detuning of the cooling laser in the 3D-MOT. Subsequent to compression, the atoms are loaded into the crossed dipole trap by switching off the magnetic fields and increasing the detuning of the cooling laser to about − 30Γ, with Γ being the natural linewidth of the D2 transition.
Figure 5 depicts the setup of our crossed optical dipole trap. The center-position modulation of the trapping beams is achieved by modulating the frequency driving the acousto-optical modulator (AOM) (Polytec, ATM-1002FA53.24). A voltage-controlled oscillator (Mini-Circuits, ZOS-150+) generates the signal for this, which is driven by a programmable arbitrary-waveform generator (Rigol, DG1022Z). We chose the waveform to generate a large-volume parabolic potential based on the derivation shown by Roy et al.52. The amplitude of the displacement of the center-position of the dipole trap beam, h0, is controlled by regulating the amplitude of the AOM’s frequency modulation. This yields a maximum beam displacement of h0 = 200 μm (300 μm) at the position of the atoms for the initial (recycled) beam.
Data acquisition and analysis
We apply our matter-wave lens subsequent to loading the dipole trap and evaporative cooling. The duration of the complete evaporative sequence is 5 s for the measurements presented here we interrupt this sequence after 0 s, 0.2 s, 1 s, 2 s, 3.5 s, 4.3 s and 5 s. Before the step-wise change of the trap frequency (ω0 → ωl) we hold the ensemble in the trap given by the respective evaporation step configuration for 50 ms.
During the matter-wave lens, the rapid decompression of the trap causes oscillations of the ensemble’s radius in the lensing trap. Depending on the release time we observe oscillations by performing absorption imaging with iterating thold for different times after the release from the trap. For each holding time the expansion velocity is extracted by fitting a ballistic expansion. This expansion can be transformed into an effective temperature using:
along each direction. The measurement is performed for different starting temperatures in the thermal regime as well as the BEC.
The simulations shown in Fig. 2 use the scaling ansatz as described in the “Scaling Ansatz” section. Here, the trapping frequencies of the lens potential in x- and y-direction have been extracted by fitting two damped oscillations to the measured data. The starting expansion velocity was set by choosing a reasonable initial radius of the ensemble (Table 1). The other parameters arise from the measurements or simulations of the trapping potentials. The shaded areas in fig. 2 depict an error estimation of the expansion velocity oscillations obtained from performing the simulation by randomly choosing input parameters from within the error bars for 1000 simulation runs and calculating the mean value as well as the standard deviation for each thold.
Scaling Ansatz
In the case of a thermal ensemble in the collision-less regime, the dynamics of a classical gas can be described using the scaling ansatz83,84, which we briefly recall here for sake of simplicity. Here, the size of the ensemble scales with the time dependent dimensionless factor bi(t).
where θi acts as an effective temperature in the directions i ∈ x, y, z. Here ω0,i denotes the initial angular trap frequency and ωi(t) denotes the time-dependent angular trap frequency defined such as: ωi(t) = ωl,i for 0 < t < thold, with ωl,i being the lensing potential, and ωi(t) = 0 after the release (see Fig. 1). This system of coupled differential equations contains the mean field interaction, given by the factor:
with
where as is the s-wave scattering length, n0 the peak density and m the mass of a single particle. Collision effects are also taken into account through
with the relaxation time
and84
In the special case of a BEC, the mean field energy is large compared to the thermal ensemble’s energy (ξ ≈ 1) and the time scale on which collisions appear goes to zero (τ ≈ 0). In this case the time dependent evolution of the matter-wave can be described following Castin & Dum85. Here, the evolution of the BEC’s Thomas-Fermi radius, Ri(t) = bi(t)Ri(0), is described by the time-dependent evolution of the scaling parameter:
and Ri(0) is the initial Thomas-Fermi radius of the BEC along the i-th direction. It is worth to notice that recent studies86,87 extend the analysis of Guéry-Odelin83 and Pedri et al.84 to the BEC regime described by Castin & Dum85.
With this set of equations the time evolution of the ensemble’s size (\({\sigma }_{{r}_{i}}\)) and velocity distribution (\({\sigma }_{{v}_{i}}\)) is determined during the entire sequence of our matter-wave lensing sequence by
and
The scaling parameter bi can be applied either on the radius of a gaussian distributed thermal ensemble or the Thomas-Fermi radius of a BEC.
Estimation of instability in matter-wave sensors
The instability of a matter-wave sensor operating at the standard quantum limit can be estimated using Eq. (1). Here we assume Raman beam splitters (n = 1) with a 1/e2-radius of 1.2 cm and a pulse duration of tπ = 15 μs. The contrast (C) is taken into account as the product of the excitation probabilities of the atom-light interactions during the Mach-Zehnder type interferometer following Loriani et al.72. Table 1 shows the source parameters used for the estimation of the instability. We chose three parameter sets from the here presented measurements of two thermal ensembles released from the optical dipole trap with starting temperatures of T0 = 41μK and 4 μK and the BEC. Besides that we simulated the performance of the interferometer operated with a molasses cooled ensemble combined with a velocity selective Raman pulse of 30 μs73, based on typical parameters in our experiment, and an advanced scenario. For this we assume a BEC with 1 × 106 atoms after a preparation time tP = 1 s with a starting expansion velocity of 2 mm s−1, as anticipated for the VLBAI setup76,80. We extrapolate the performance of our matter-wave lens for this experiment, resulting in expansion velocities of 0.135 mm s−1 corresponding to an equivalent 3D temperature of 200 pK.
Data availability
The data used in this manuscript are available from the corresponding author upon reasonable request.
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Acknowledgements
This work is funded by the German Space Agency (DLR) with funds provided by the Federal Ministry of Economic Affairs and Energy (BMWi) due to an enactment of the German Bundestag under Grant Nos. DLR 50WM1641 (PRIMUS-III), DLR 50WM2041 (PRIMUS-IV), DLR 50WM2245A (CAL-II), DLR 50WM2060 (CARIOQA), and DLR 50RK1957 (QGYRO). We acknowledge financial support from the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation)-Project-ID 274200144-SFB 1227 DQ-mat within the projects A05, B07, and B09, and -Project-ID 434617780-SFB 1464 TerraQ within the projects A02 and A03 and Germany’s Excellence Strategy—EXC-2123 QuantumFrontiers—Project-ID 390837967 and from “Niedersächsisches Vorab” through the “Quantum- and Nano-Metrology (QUANOMET)” initiative within the Project QT3. A.H. and D.S. acknowledge support by the Federal Ministry of Education and Research (BMBF) through the funding program Photonics Research Germany under contract number 13N14875.
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W.E., E.M.R., and D.S. designed the experimental setup and the dipole trapping laser system. H.A., A.H., A.R., and D.S. contributed to the design, operation, and maintenance of the laser system and the overall setup. R.C., E.C. and N.G. set the theoretical framework of this work. H.A., R.C., C.S., and D.S. drafted the initial manuscript. H.A., and R.C. performed the analysis of the data presented in this manuscript. H.A., and R.C. under lead of N.G. and C.S. performed the instability study. C.V., M.W., C.L., S.H. together with the other authors discussed and evaluated the results and contributed to, reviewed, and approved of the manuscript.
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Albers, H., Corgier, R., Herbst, A. et al. All-optical matter-wave lens using time-averaged potentials. Commun Phys 5, 60 (2022). https://doi.org/10.1038/s42005-022-00825-2
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DOI: https://doi.org/10.1038/s42005-022-00825-2
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