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High-density logic-in-memory devices using vertical indium arsenide nanowires on silicon

Abstract

In-memory computing can be used to overcome the von Neumann bottleneck—the need to shuffle data between separate memory and computational units—and help improve computing performance. Co-integrated vertical transistor selectors (1T) and resistive memory elements (1R) in a 1T1R configuration offer advantages of scalability, speed and energy efficiency in current mass storage applications, and such 1T1R cells could also be potentially used for in-memory computation architectures. Here we show that a vertical transistor and resistive memory can be integrated onto a single vertical indium arsenide nanowire on silicon. The approach relies on an interface between the III–V semiconductor nanowire and a high-κ dielectric (hafnium oxide), which provides an oxide layer that can operate either as a vertical transistor selector or a high-performance resistive memory. The resulting 1T1R cells allow Boolean logic operations to be implemented in a single vertical nanowire with a minimal area footprint.

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Fig. 1: Vertical III–V 1T1R structure.
Fig. 2: Electrical performance of vertical III–V 1T1R.
Fig. 3: Vertical III–V 1T1R NAND-gate implementation and device variability.
Fig. 4: XPS characterization of the interlayer oxide.

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Data availability

The datasets analysed in this study are available from the corresponding authors upon reasonable request.

References

  1. Ielmini, D. & Wong, H. In-memory computing with resistive switching devices. Nat. Electron. 1, 333–343 (2018).

    Article  Google Scholar 

  2. Wulf, W. & McKee, S. Hitting the memory wall. ACM Comp. Ar. 23, 20–24 (1995).

    Google Scholar 

  3. Xue, C. et al. A CMOS-integrated compute-in-memory macro based on resistive random-access memory for AI edge devices. Nat. Electron. 4, 81–90 (2021).

  4. Sebastian, A., Le Gallo, M., Khaddam-Aljameh, R. & Eleftheriou, E. Memory devices and applications for in-memory computing. Nat. Nanotechnol. 15, 529–544 (2020).

    Article  Google Scholar 

  5. Shulaker, M. et al. Three-dimensional integration of nanotechnologies for computing and data storage on a single chip. Nature 547, 74–78 (2017).

    Article  Google Scholar 

  6. Burr, G. et al. Access devices for 3D crosspoint memory. J. Vac. Sci. Technol. B 32, 040802 (2014).

    Article  Google Scholar 

  7. International Roadmap for Devices and Systems (IRDS)—More Moore (IEEE, 2020).

  8. Fang, Z. et al. Fully CMOS-compatible 1T1R integration of vertical nanopillar GAA transistor and oxide-based RRAM cell for high-density nonvolatile memory application. IEEE Trans. Electron Devices 60, 1108–1113 (2013).

    Article  Google Scholar 

  9. Chen, B. et al. Highly compact (4F2) and well behaved nano-pillar transistor controlled resistive switching cell for neuromorphic system application. Sci. Rep. 4, 6863 (2014).

  10. Yakimets, D. et al. Vertical GAAFETs for the ultimate CMOS scaling. IEEE Trans. Electron Devices 62, 1433–1439 (2015).

    Article  Google Scholar 

  11. Grossi, A. et al. Resistive RAM endurance: array-level characterization and correction techniques targeting deep learning applications. IEEE Trans. Electron Devices 66, 1281–1288 (2019).

    Article  Google Scholar 

  12. Lee, M. et al. A fast, high-endurance and scalable non-volatile memory device made from asymmetric Ta2O5−x/TaO2−x bilayer structures. Nat. Mater. 10, 625–630 (2011).

    Article  Google Scholar 

  13. Persson, K., Ram, M. S. & Wernersson, L. E. Ultra-scaled AlOx diffusion barriers for multibit HfOx RRAM operation. IEEE J. Electron Devices Soc. 9, 564–569 (2021).

  14. Jansson, K., Lind, E. & Wernersson, L. Performance evaluation of III–V nanowire transistors. IEEE Trans. Electron Devices 59, 2375–2382 (2012).

    Article  Google Scholar 

  15. Kilpi, O., Hellenbrand, M., Svensson, J., Lind, E. & Wernersson, L. Vertical nanowire III–V MOSFETs with improved high‐frequency gain. Electron. Lett. 56, 669–671 (2020).

    Article  Google Scholar 

  16. Kilpi, O., Svensson, J., Lind, E. & Wernersson, L. Electrical properties of vertical InAs/InGaAs heterostructure MOSFETs. IEEE J. Electron Devices Soc. 7, 70–75 (2019).

    Article  Google Scholar 

  17. Kilpi, O. et al. High-performance vertical III-V nanowire MOSFETs on Si with gm > 3 mS/μm. IEEE Electron Device Lett. 41, 1161–1164 (2020).

    Article  Google Scholar 

  18. Ram, M. S., Persson, K., Borg, M. & Wernersson, L. Low-power resistive memory integrated on III–V vertical nanowire MOSFETs on silicon. IEEE Electron Device Lett. 41, 1432–1435 (2020).

    Article  Google Scholar 

  19. Hellenbrand, M., Kilpi, O., Svensson, J., Lind, E. & Wernersson, L. Low-frequency noise in nanowire and planar III-V MOSFETs. Microelectron. Eng. 215, 110986 (2019).

    Article  Google Scholar 

  20. Navarro, C. et al. Capacitor-less dynamic random access memory based on a III–V transistor with a gate length of 14 nm. Nat. Electron. 2, 412–419 (2019).

    Article  Google Scholar 

  21. Convertino, C. et al. A hybrid III–V tunnel FET and MOSFET technology platform integrated on silicon. Nat. Electron. 4, 162–170 (2021).

    Article  Google Scholar 

  22. Wang, Z. et al. Efficient implementation of Boolean and full-adder functions with 1T1R RRAMs for beyond von Neumann in-memory computing. IEEE Trans. Electron Devices 65, 4659–4666 (2018).

    Article  Google Scholar 

  23. Pacheco, P. & Malensek, M. An Introduction to Parallel Programming (Morgan Kaufmann, 2011).

  24. Timm, R. et al. Self-cleaning and surface chemical reactions during hafnium dioxide atomic layer deposition on indium arsenide. Nat. Commun. 9, 1412 (2018).

    Article  Google Scholar 

  25. Svensson, J., Dey, A., Jacobsson, D. & Wernersson, L. III–V nanowire complementary metal–oxide semiconductor transistors monolithically integrated on Si. Nano Lett. 15, 7898–7904 (2015).

    Article  Google Scholar 

  26. Sivan, M. et al. All WSe2 1T1R resistive RAM cell for future monolithic 3D embedded memory integration. Nat. Commun. 10, 5201 (2019).

    Article  Google Scholar 

  27. Berg, M. et al. Electrical characterization and modeling of gate-last vertical InAs nanowire MOSFETs on Si. IEEE Electron Device Lett. 37, 966–969 (2016).

    Article  Google Scholar 

  28. Kilpi, O. et al. Sub-100-nm gate-length scaling of vertical InAs/InGaAs nanowire MOSFETs on Si. In 2017 IEEE International Electron Devices Meeting (IEDM) 17.3.1–17.3.4 (IEEE, 2018).

  29. Zhao, X. et al. Sub-10-nm-diameter InGaAs vertical nanowire MOSFETs: Ni versus Mo contacts. IEEE Trans. Electron Devices 65, 3762–3768 (2018).

    Article  Google Scholar 

  30. Jonsson, A., Svensson, J. & Wernersson, L. A self-aligned gate-last process applied to all-III–V CMOS on Si. IEEE Electron Device Lett. 39, 935–938 (2018).

    Article  Google Scholar 

  31. Persson, K., Ram, M. S., Kilpi, O., Borg, M. & Wernersson, L. Cross-point arrays with low-power ITO-HfO2 resistive memory cells integrated on vertical III-V nanowires. Adv. Electron. Mater. 6, 2000154 (2020).

    Article  Google Scholar 

  32. Yong, Z. et al. Tuning oxygen vacancies and resistive switching properties in ultra-thin HfO2 RRAM via TiN bottom electrode and interface engineering. Appl. Surf. Sci. 551, 149386 (2021).

    Article  Google Scholar 

  33. Li, K. et al. Utilizing sub-5 nm sidewall electrode technology for atomic-scale resistive memory fabrication. In 2014 Symposium on VLSI Technology (VLSI-Technology): Digest of Technical Papers 1–2 (IEEE, 2014).

  34. Borghetti, J. et al. ‘Memristive’ switches enable ‘stateful’ logic operations via material implication. Nature 464, 873–876 (2010).

    Article  Google Scholar 

  35. Wang, Z. et al. Functionally complete Boolean logic in 1T1R resistive random access memory. IEEE Electron Device Lett. 38, 179–182 (2017).

    Article  Google Scholar 

  36. Wei, H., Wang, Z., Tian, X., Käll, M. & Xu, H. Cascaded logic gates in nanophotonic plasmon networks. Nat. Commun. 2, 387 (2011).

  37. He, Z. et al. Atomic layer-deposited HfAlOx-based RRAM with low operating voltage for computing in-memory applications. Nanoscale Res. Lett. 125, 51 (2019).

    Article  Google Scholar 

  38. Yeap, G. Smart mobile SoCs driving the semiconductor industry: technology trend, challenges and opportunities. In 2013 IEEE International Electron Devices Meeting 1.3.1–1.3.8 (IEEE, 2013).

  39. Song, J. et al. Effects of RESET current overshoot and resistance state on reliability of RRAM. IEEE Electron Device Lett. 35, 636–638 (2014).

    Article  Google Scholar 

  40. Timm, R. et al. Reduction of native oxides on InAs by atomic layer deposited Al2O3 and HfO2. Appl. Phys. Lett. 97, 132904 (2010).

    Article  Google Scholar 

  41. Schwartz, G. P., Sunder, W. A., Griffiths, J. E. & Gualtieri, G. J. Condensed phase diagram for the In–As–O system. Thin Solid Films 94, 205 (1982).

    Article  Google Scholar 

  42. Lin, S. et al. Improving performance by inserting an indium oxide layer as an oxygen ion storage layer in HfO2-based resistive random access memory. IEEE Trans. Electron Devices 68, 1037–1040 (2021).

    Article  Google Scholar 

  43. Timm, R. et al. Interface composition of InAs nanowires with Al2O3 and HfO2 thin films. Appl. Phys. Lett. 99, 222907 (2011).

    Article  Google Scholar 

  44. Palumbo, F., Shekhter, P. & Eizenberg, M. Influence of the oxide–semiconductor interface on the resistive switching phenomenon in metal/Al2O3/InGaAs. Solid-State Electron. 93, 56–60 (2014).

    Article  Google Scholar 

  45. Sun, J., Lind, E., Maximov, I. & Xu, H. Memristive and memcapacitive characteristics of a Au/Ti–HfO2-InP/InGaAs diode. IEEE Electron Device Lett. 32, 131–133 (2011).

    Article  Google Scholar 

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Acknowledgements

We would like to thank J. Svensson for growing the nanowires for this work. This work is financed through the Swedish Research Council grant no. 2016-06186 Electronics beyond kT/q (L.-E.W.).

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Authors and Affiliations

Authors

Contributions

M.S.R. fabricated the 1T1R devices. M.S.R. and K.-M.P. performed the electrical characterization of 1T1R devices. K.-M.P. fabricated the planar devices for XPS characterization. A.I. and R.T. performed the XPS characterization and prepared Fig. 4 with the corresponding analysis. K.-M.P. actively contributed to the writing process and performed the array simulations. A.J. helped with the SiO2 process module and prepared Fig. 1a. M.S.R. conceptualized the idea of the metal electrode-less RRAM integration. M.S.R. and L.-E.W. wrote the manuscript. L.-E.W. initialized and supervised the project. All the authors discussed and revised the final manuscript.

Corresponding authors

Correspondence to Mamidala Saketh Ram or Lars-Erik Wernersson.

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Peer review information Nature Electronics thanks Cezhou Zhao and the other, anonymous, reviewer(s) for their contribution to the peer review of this work

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Supplementary Information

Supplementary Figs. 1–7 and Tables 1–4.

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Ram, M.S., Persson, KM., Irish, A. et al. High-density logic-in-memory devices using vertical indium arsenide nanowires on silicon. Nat Electron 4, 914–920 (2021). https://doi.org/10.1038/s41928-021-00688-5

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