Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

A scalable high-porosity wood for sound absorption and thermal insulation

Abstract

The search for more-sustainable materials has motivated research on lightweight, porous structures for thermal insulation and noise reduction, such as for construction and cold-chain transportation. Wood, known as one of the most renewable materials on Earth, has been widely and long used in construction for its high strength/weight ratio, wide abundance, low cost and relative sustainability. However, natural wood is much less effective at reducing noise or preventing heat loss than conventional petroleum- and mineral-based porous structures (for example, expanded polystyrene foam and mineral wool). Here we report the extraordinary noise-reduction and thermal-insulation capabilities of a scalable, high-porosity wood structure, ‘insulwood’, fabricated by removing lignin and hemicelluloses from natural wood using a rapid (~1 h) high-temperature process followed by low-cost ambient drying. Insulwood demonstrates a high porosity of ~0.93, a high noise-reduction coefficient of 0.37 at a frequency range of 250–3,000 Hz (for 10-mm-thick wood), a low radial thermal conductivity of 0.038 W m–1 K–1 and a high compressive strength of ~1.5 MPa at 60% strain. Furthermore, this new wood-based material can be rapidly processed into a vacuum insulation panel (~0.01 W m–1 K–1) for thermal insulation applications with limited space (for example, refrigerators, cold-chain transportation and older buildings). The material is unique in its combination of renewable source materials, high porosity, high sound absorption, low thermal conductivity and high mechanical robustness, as well as in its efficient, cost-effective and scalable manufacturing. These attributes make insulwood promising as a sustainable construction material for improved noise and thermal regulation.

This is a preview of subscription content, access via your institution

Access options

Rent or buy this article

Prices vary by article type

from$1.95

to$39.95

Prices may be subject to local taxes which are calculated during checkout

Fig. 1: The fabrication and thermal performance of insulwood and insulwood-based VIPs.
Fig. 2: Morphology and structure of the natural wood starting material and insulwood.
Fig. 3: Sound absorption of the insulwood.
Fig. 4: Thermal and mechanical properties of insulwood.

Similar content being viewed by others

Data availability

The data that support the findings of this study are available within this article and its Supplementary Information. Source data are provided with this paper.

References

  1. 2020 Global Status Report for Buildings and Construction: Towards a Zero-Emission, Efficient and Resilient Buildings and Construction Sector (UNEP, 2020).

  2. Cao, L., Fu, Q., Si, Y., Ding, B. & Yu, J. Porous materials for sound absorption. Compos. Commun. 10, 25–35 (2018).

    Article  Google Scholar 

  3. Apostolopoulou‐Kalkavoura, V., Munier, P. & Bergström, L. Thermally insulating nanocellulose‐based materials. Adv. Mater. 33, 2001839 (2021).

    Article  Google Scholar 

  4. Zhao, X., Brozena, A. H. & Hu, L. Critical roles of pores and moisture in sustainable nanocellulose-based super-thermal insulators. Matter 4, 769–772 (2021).

    Article  CAS  Google Scholar 

  5. Liu, H. & Zhao, X. Thermal conductivity analysis of high porosity structures with open and closed pores. Int. J. Heat Mass Transf. 183, 122089 (2022).

    Article  CAS  Google Scholar 

  6. Lavoine, N. & Bergström, L. Nanocellulose-based foams and aerogels: processing, properties, and applications. J. Mater. Chem. A 5, 16105–16117 (2017).

    Article  CAS  Google Scholar 

  7. Asdrubali, F., D’Alessandro, F. & Schiavoni, S. A review of unconventional sustainable building insulation materials. Sustain. Mater. Technol. 4, 1–17 (2015).

    CAS  Google Scholar 

  8. Schiavoni, S., Bianchi, F. & Asdrubali, F. Insulation materials for the building sector: a review and comparative analysis. Renew. Sustain. Energy Rev. 62, 988–1011 (2016).

    Article  Google Scholar 

  9. Forouharmajd, F. & Mohammadi, Z. Assessment of normal incidence absorption performance of sound absorbing materials. Int. J. Environ. Health Eng. 5, 10 (2016).

    Article  Google Scholar 

  10. Yang, T. et al. Sound absorption properties of natural fibers: a review. Sustainability 12, 8477 (2020).

    Article  CAS  Google Scholar 

  11. Liu, L. et al. The development history and prospects of biomass-based insulation materials for buildings. Renew. Sustain. Energy Rev. 69, 912–932 (2017).

    Article  CAS  Google Scholar 

  12. Hill, C., Norton, A. & Dibdiakova, J. A comparison of the environmental impacts of different categories of insulation materials. Energy Build. 162, 12–20 (2018).

    Article  Google Scholar 

  13. Papadopoulos, A. M. & Giama, E. Environmental performance evaluation of thermal insulation materials and its impact on the building. Build. Environ. 42, 2178–2187 (2007).

    Article  Google Scholar 

  14. Xia, Q. et al. A strong, biodegradable and recyclable lignocellulosic bioplastic. Nat. Sustain. 4, 627–635 (2021).

    Article  Google Scholar 

  15. Esau, R., Jungclaus, M., Olgyay, V. & Rempher, A. Reducing Embodied Carbon in Buildings (RMI, 2021).

  16. Chen, C. et al. Structure–property–function relationships of natural and engineered wood. Nat. Rev. Mater. 5, 642–666 (2020).

    Article  CAS  Google Scholar 

  17. Koshijima, T. & Watanabe, T. Association Between Lignin and Carbohydrates in Wood and Other Plant Tissues (Springer, 2013).

  18. Suleiman, B., Larfeldt, J., Leckner, B. & Gustavsson, M. Thermal conductivity and diffusivity of wood. Wood Sci. Technol. 33, 465–473 (1999).

    Article  CAS  Google Scholar 

  19. Lin, M.-D., Tsai, K.-T. & Su, B.-S. Estimating the sound absorption coefficients of perforated wooden panels by using artificial neural networks. Appl. Acoust. 70, 31–40 (2009).

    Article  Google Scholar 

  20. Asdrubali, F. et al. A review of structural, thermo-physical, acoustical, and environmental properties of wooden materials for building applications. Build. Environ. 114, 307–332 (2017).

    Article  Google Scholar 

  21. Kang, C., Kang, W., Chung, W., Matsumura, J. & Oda, K. Changes in anatomical features, air permeability and sound absorption capability of wood induced by delignification treatment. 53, 479–483 (Faculty of Agriculture, Kyushu University, 2008).

  22. Kolya, H. & Kang, C. W. High acoustic absorption properties of hackberry compared to nine different hardwood species: a novel finding for acoustical engineers. Appl. Acoust. 169, 107475 (2020).

    Article  Google Scholar 

  23. Li, J., Chen, C., Zhu, J., Ragauskas, A. J. & Hu, L. In situ wood delignification toward sustainable applications. Acc. Mater. Res. 2, 606–620 (2021).

  24. Guan, H., Cheng, Z. & Wang, X. Highly compressible wood sponges with a spring-like lamellar structure as effective and reusable oil absorbents. ACS Nano 12, 10365–10373 (2018).

    Article  CAS  Google Scholar 

  25. Song, J. et al. Highly compressible, anisotropic aerogel with aligned cellulose nanofibers. ACS Nano 12, 140–147 (2018).

    Article  CAS  Google Scholar 

  26. Li, T. et al. Anisotropic, lightweight, strong, and super thermally insulating nanowood with naturally aligned nanocellulose. Sci. Adv. 4, eaar3724 (2018).

    Article  Google Scholar 

  27. Zhu, M. et al. Highly anisotropic, highly transparent wood composites. Adv. Mater. 28, 5181–5187 (2016).

    Article  CAS  Google Scholar 

  28. Wang, J. et al, Carbonate pre-treatment of wood for transformative structural applications through densification. Ind Crops Prod. 183, 188 (2022).

  29. Sun, J. et al. Enhanced mechanical energy conversion with selectively decayed wood. Sci. Adv. 7, eabd9138 (2021).

    Article  CAS  Google Scholar 

  30. Pour, G., Beauger, C., Rigacci, A. & Budtova, T. Xerocellulose: lightweight, porous and hydrophobic cellulose prepared via ambient drying. J. Mater. Sci. 50, 4526–4535 (2015).

    Article  CAS  Google Scholar 

  31. Xiao, S. et al. Lightweight, strong, moldable wood via cell wall engineering as a sustainable structural material. Science 374, 465–471 (2021).

    Article  CAS  Google Scholar 

  32. Ek, M., Gellerstedt, G. & Henriksson, G. Pulping Chemistry and Technology Vol. 2 (Walter de Gruyter, 2009).

  33. Kamali, M. & Khodaparast, Z. Review on recent developments on pulp and paper mill wastewater treatment. Ecotoxicol. Environ. Saf. 114, 326–342 (2015).

    Article  CAS  Google Scholar 

  34. López, F., Pérez, A., Zamudio, M. A., De Alva, H. E. & García, J. C. Paulownia as raw material for solid biofuel and cellulose pulp. Biomass Bioenergy 45, 77–86 (2012).

    Article  Google Scholar 

  35. Yadav, N. K. et al. A review of paulownia biotechnology: a short rotation, fast growing multipurpose bioenergy tree. Am. J. Plant Sci. 4, 2070 (2013).

    Article  Google Scholar 

  36. Borrega, M., Tolonen, L. K., Bardot, F., Testova, L. & Sixta, H. Potential of hot water extraction of birch wood to produce high-purity dissolving pulp after alkaline pulping. Bioresour. Technol. 135, 665–671 (2013).

    Article  CAS  Google Scholar 

  37. Pettersen, R. C. in The Chemistry of Solid Wood (ed. Rowell, R.) 57–126 (ACS, 1984).

  38. Kellogg, R. M. & Wangaard, F. F. Variation in the cell-wall density of wood. Wood Fiber Sci. 1, 180–204 (1969).

    Google Scholar 

  39. Ross, R. J. Wood Handbook: Wood as an Engineering Material General Technical Report FPL-GTR-190 (USDA, 2010).

  40. Acoustics—Determination of Sound Absorption Coefficient and Impedance in Impedance Tubes—Part 2: Transfer-Function Method (ISO, 1998).

  41. Sikora, J. & Turkiewicz, J. Sound absorption coefficients of granular materials. Mech. Control 29, 149–157 (2010).

    Google Scholar 

  42. Putra, A., Abdullah, Y., Efendy, H., Mohamad, W. & Salleh, N. Biomass from paddy waste fibers as sustainable acoustic material. Adv. Acoust. Vib. 2013, 605932 (2013).

  43. Shen, L. et al. Hierarchical pore structure based on cellulose nanofiber/melamine composite foam with enhanced sound absorption performance. Carbohydr. Polym. 255, 117405 (2021).

    Article  CAS  Google Scholar 

  44. Jia, C. et al. Highly compressible and anisotropic lamellar ceramic sponges with superior thermal insulation and acoustic absorption performances. Nat. Commun. 11, 3732 (2020).

    Article  CAS  Google Scholar 

  45. Jelle, B. P. Traditional, state-of-the-art and future thermal building insulation materials and solutions—properties, requirements and possibilities. Energy Build. 43, 2549–2563 (2011).

    Article  Google Scholar 

  46. Eitelberger, J. & Hofstetter, K. Prediction of transport properties of wood below the fiber saturation point—a multiscale homogenization approach and its experimental validation: part I: thermal conductivity. Compos. Sci. Technol. 71, 134–144 (2011).

    Article  Google Scholar 

  47. Zhao, X. et al. Reduced-scale hot box method for thermal characterization of window insulation materials. Appl. Therm. Eng. 160, 114026 (2019).

    Article  Google Scholar 

  48. Beluns, S. et al. From wood and hemp biomass wastes to sustainable nanocellulose foams. Ind. Crops Prod. 170, 113780 (2021).

    Article  CAS  Google Scholar 

  49. Chapelle, L. Characterization and Modelling of the Mechanical Properties of Mineral Wool. PhD thesis, Technical University of Denmark (2016).

  50. Kalnæs, S. E. & Jelle, B. P. Vacuum insulation panel products: a state-of-the-art review and future research pathways. Appl. Energy 116, 355–375 (2014).

    Article  Google Scholar 

  51. Sluiter, A. et al. Determination of Structural Carbohydrates and Lignin in Biomass Technical Report NREL/TP-510-42618 (NREL, 2008).

  52. Standard Test Method for Impedance and Absorption of Acoustical Materials Using a Tube, Two Microphones and a Digital Frequency Analysis System ASTM E1050-19 (ASTM, 2019).

Download references

Acknowledgements

L.H., X.Z., A.G., J.D., D.S. and J.Y.Z. acknowledge the support from the Department of Energy’s Building Technologies Office (BTO) through the Small Business Innovation Research Program under Contract DE-SC0018820. L.H., X.Z., A.P.S., A.G., J.D., J.K. and J.Y.Z. acknowledge the support from the U.S. Department of Energy’s Office of Energy Efficiency and Renewable Energy (EERE) under the Building Technologies Office (BTO), Award Number DE-EE0009702. X.Z. also acknowledges the use and support of the Maryland NanoCenter and its AIMLab.

Author information

Authors and Affiliations

Authors

Contributions

L.H. and X.Z. conceived the idea and designed the experiments. X.Z. and Y.L. contributed to the insulwood fabrication and characterization. Y.M. contributed wide-angle X-ray scattering measurement. A.P.S., S.J., H.X., Z.L., J.L. and B.C.C. contributed to collection of the SEM and digital images. J.D. and J.Y.Z. contributed to the large-scale sample fabrication. L.Z., A.Y. and M.Y. contributed to the sound-absorption measurement and simulation. X.Z. contributed to thermal measurements and simulations. G.S.C. and E.Q.W. contributed to characterization of moisture absorption and flammability. S.H. provided characterization via FTIR. A.O.D. validated the thermal measurements. D.S. and A.G. provided useful suggestions for raw woods selection and insulwood fabrication. J.K. contributed to the design of the VIP fiber core, provided useful suggestions for VIP fabrication, and performed thermal performance analysis. X.Z. and L.H. collaboratively analyzed the data and wrote the manuscript. All authors commented on the final manuscript.

Corresponding author

Correspondence to Liangbing Hu.

Ethics declarations

Competing interests

The authors declare the following competing interests: Dr. Liangbing Hu co-founded a company, InventWood, to commercialize wood-based thermal/acoustic insulation materials. However, all results reported herein were performed under federal sponsorship. The remaining authors declare no competing interests.

Peer review

Peer review information

Nature Sustainability thanks Kai Zhang and the other, anonymous, reviewer(s) for their contribution to the peer review of this work.

Additional information

Publisher’s note Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Disclaimer The identification of any commercial product or trade name does not imply endorsement or recommendation by the National Institute of Standards and Technology.

Supplementary information

Supplementary Information

Supplementary Figs. 1–30, Table 1, Notes 1–6 and references.

Reporting Summary

Source data

Source Data Fig. 2g

FTIR spectra of the natural wood and insulwood.

Source Data Fig. 3b

The sound-absorption coefficient of the natural wood and insulwood as a function of frequency.

Source Data Fig. 4e

Stress–strain curves of the insulwood under compression along the radial direction.

Source Data Fig. 4h

Comparison of the outgassing rate of the insulwood and EPS.

Rights and permissions

Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.

Reprints and Permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Zhao, X., Liu, Y., Zhao, L. et al. A scalable high-porosity wood for sound absorption and thermal insulation. Nat Sustain 6, 306–315 (2023). https://doi.org/10.1038/s41893-022-01035-y

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1038/s41893-022-01035-y

This article is cited by

Search

Quick links

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing