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Coloured low-emissivity films for building envelopes for year-round energy savings

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Abstract

Buildings are responsible for over 40% of total US energy use, of which about 40% is directly related to the operation of heating, ventilation and air-conditioning (HVAC) systems. Saving energy to heat and cool buildings would contribute substantially to sustainability. Here we propose a category of coloured low-emissivity films for building walls that constitute the main component of the building thermal envelope. We demonstrate high reflectance (~90%) in infrared wavelength range and selective reflectance in the visible light wavelength range for desired colours. These films can help minimize radiative heat exchange between the indoor and outdoor environments, thus saving energy for all-year cooling and heating while satisfying the required aesthetical effect. Simulations show that these films can help reduce heat gain and loss by up to 257.6 MJ per installation wall area annually. In the case of a typical midrise apartment building, the HVAC system can save up to 124.46 GJ (equal to 9.87% of the building’s HVAC energy consumption). By rough estimation, a global CO2 emission reduction of 1.14 billion metric tons annually could be achieved. Our work provides insights for innovative energy-saving building envelope materials that can help achieve global carbon neutrality and sustainability.

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Fig. 1: Concept illustration.
Fig. 2: Fabrication and characterization of coloured low-emissivity films.
Fig. 3: Visualized thermal effect of the coloured low-emissivity film.
Fig. 4: Thermal performance demonstration.
Fig. 5: Modelled annual reduction of heat transmission and evaluation of building energy savings.

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Data availability

The original data that support the findings of this study are available from the corresponding author upon request.

Code availability

The code for the building energy consumption model can be made available upon request.

Change history

  • 01 February 2022

    In the PDF version of this article initially published, the sets of heat-flow arrows in Fig. 4a and Fig. 4c were omitted. The arrows have now been restored to the PDF.

References

  1. Yin, X., Yang, R., Tan, G. & Fan, S. Terrestrial radiative cooling: using the cold universe as a renewable and sustainable energy source. Science 370, 786–791 (2020).

    Article  CAS  Google Scholar 

  2. Quadrennial Technology Review: An Assessment of Energy Technologies and Research Opportunities Ch. 5 (US Department of Energy, 2015); https://www.energy.gov/sites/prod/files/2017/03/f34/qtr-2015-chapter5.pdf

  3. Heating and Cooling (US Department of Energy, accessed 16 April 2021); www.energy.gov/heating-cooling

  4. Li, T. et al. A radiative cooling structural material. Science 364, 760–763 (2019).

    Article  CAS  Google Scholar 

  5. Goetzler, W. Energy Savings Potential and RD&D Opportunities for Commercial Building HVAC Systems (US Department of Energy, 2017).

  6. Jelle, B. P. Traditional, state-of-the-art and future thermal building insulation materials and solutions—properties, requirements and possibilities. Energy Build. 43, 2549–2563 (2011).

    Article  Google Scholar 

  7. Pisello, A. L. State of the art on the development of cool coatings for buildings and cities. Sol. Energy 144, 660–680 (2017).

    Article  CAS  Google Scholar 

  8. Zhai, Y. et al. Scalable-manufactured randomized glass–polymer hybrid metamaterial for daytime radiative cooling. Science 355, 1062–1066 (2017).

    Article  CAS  Google Scholar 

  9. Mandal, J. et al. Hierarchically porous polymer coatings for highly efficient passive daytime radiative cooling. Science 362, 315–319 (2018).

    Article  CAS  Google Scholar 

  10. Chen, Y. et al. Colored and paintable bilayer coatings with high solar-infrared reflectance for efficient cooling. Sci. Adv. 6, eaaz5413 (2020).

    Article  CAS  Google Scholar 

  11. Zhou, L. et al. A polydimethylsiloxane-coated metal structure for all-day radiative cooling. Nat. Sustain. 2, 718–724 (2019).

    Article  Google Scholar 

  12. Raman, A. P., Anoma, M. A., Zhu, L., Rephaeli, E. & Fan, S. Passive radiative cooling below ambient air temperature under direct sunlight. Nature 515, 540–544 (2014).

    Article  CAS  Google Scholar 

  13. Hernández-Pérez, I. et al. Thermal performance of reflective materials applied to exterior building components—a review. Energy Build. 80, 81–105 (2014).

    Article  Google Scholar 

  14. Li, X. et al. Integration of daytime radiative cooling and solar heating for year-round energy saving in buildings. Nat. Commun. 11, 6101 (2020).

    Article  CAS  Google Scholar 

  15. Martilli, A., Clappier, A. & Rotach, M. W. An urban surface exchange parameterisation for mesoscale models. Bound. Layer Meteorol. 104, 261–304 (2002).

    Article  Google Scholar 

  16. Albatici, R., Passerini, F., Tonelli, A. M. & Gialanella, S. Assessment of the thermal emissivity value of building materials using an infrared thermovision technique emissometer. Energy Build. 66, 33–40 (2013).

    Article  Google Scholar 

  17. Avdelidis, N. P. & Moropoulou, A. Emissivity considerations in building thermography. Energy Build. 35, 663–667 (2003).

    Article  Google Scholar 

  18. Aditya, L. et al. A review on insulation materials for energy conservation in buildings. Renew. Sustain. Energy Rev. 73, 1352–1365 (2017).

    Article  CAS  Google Scholar 

  19. Jelle, B. P., Kalnæs, S. E. & Gao, T. Low-emissivity materials for building applications: a state-of-the-art review and future research perspectives. Energy Build. 96, 329–356 (2015).

    Article  Google Scholar 

  20. Guo, W., Qiao, X., Huang, Y., Fang, M. & Han, X. Study on energy saving effect of heat-reflective insulation coating on envelopes in the hot summer and cold winter zone. Energy Build. 50, 196–203 (2012).

    Article  Google Scholar 

  21. Juanicó, L. E. Thermal insulation of roofs by using multiple air gaps separated by insulating layers of low infrared emissivity. Constr. Build. Mater. 230, 116931 (2020).

    Article  Google Scholar 

  22. Tenpierik, M. J. & Hasselaar, E. Reflective multi-foil insulations for buildings: a review. Energy Build. 56, 233–243 (2013).

    Article  Google Scholar 

  23. Medina, M. A. A comprehensive review of radiant barrier research including laboratory and field experiments. ASHRAE Trans. 118, 400–407 (2012).

    Google Scholar 

  24. Principi, P. & Fioretti, R. Thermal analysis of the application of PCM and low emissivity coating in hollow bricks. Energy Build. 51, 131–142 (2012).

    Article  Google Scholar 

  25. Fantucci, S. & Serra, V. Experimental assessment of the effects of low-emissivity paints as interior radiation control coatings. Appl. Sci. 10, 842 (2020).

    Article  CAS  Google Scholar 

  26. Joudi, A., Svedung, H., Cehlin, M. & Rönnelid, M. Reflective coatings for interior and exterior of buildings and improving thermal performance. Appl. Energy 103, 562–570 (2013).

    Article  Google Scholar 

  27. Fantucci, S. & Serra, V. Low-E paints enhanced building components: performance, limits and research perspectives. Energy Procedia 126, 274–281 (2017).

    Article  Google Scholar 

  28. Shen, H., Tan, H. & Tzempelikos, A. The effect of reflective coatings on building surface temperatures, indoor environment and energy consumption—an experimental study. Energy Build. 43, 573–580 (2011).

    Article  Google Scholar 

  29. Cai, L. et al. Temperature regulation in colored infrared-transparent polyethylene textiles. Joule 3, 1478–1486 (2019).

    Article  CAS  Google Scholar 

  30. Peng, Y. & Cui, Y. Advanced textiles for personal thermal management and energy. Joule 4, 724–742 (2020).

    Article  CAS  Google Scholar 

  31. Hsu, P.-C. et al. Radiative human body cooling by nanoporous polyethylene textile. Science 353, 1019–1023 (2016).

    Article  CAS  Google Scholar 

  32. Peng, Y. et al. Nanoporous polyethylene microfibres for large-scale radiative cooling fabric. Nat. Sustain. 1, 105–112 (2018).

    Article  Google Scholar 

  33. Hsu, P.-C. et al. A dual-mode textile for human body radiative heating and cooling. Sci. Adv. 3, e1700895 (2017).

    Article  Google Scholar 

  34. Reale, A. et al. Spray coating for polymer solar cells: an up-to-date overview. Energy Technol. 3, 385–406 (2015).

    Article  CAS  Google Scholar 

  35. Chen, Y. et al. Roll-to-roll production of metal–organic framework coatings for particulate matter removal. Adv. Mater. 29, 4–9 (2017).

    Google Scholar 

  36. Fan, L., Li, W., Jin, W., Orenstein, M. & Fan, S. Maximal nighttime electrical power generation via optimal radiative cooling. Opt. Express 28, 25460–25470 (2020).

    Article  CAS  Google Scholar 

  37. Crawley, D. B., Pedersen, C. O., Lawrie, L. K. & Winkelmann, F. C. EnergyPlus: energy simulation program. ASHRAE J. 42, 49–56 (2000).

    Google Scholar 

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Acknowledgements

We thank Q. Li for helpful discussion and kind help. Part of this work was performed at the Stanford Nano Shared Facilities and the Stanford Nanofabrication Facility. S.F. acknowledges the support of the US Department of Energy (grant no. DE-FG-07ER46426).

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Contributions

Y.C. and Y.P. conceived the idea. Y.P. designed the experiments and performed the material preparation and characterization with the help of Y.Y., Z.H., Y.M., J.T. and J.Z. L.F. and W.J. performed the modelling work. S.Z. and X.L. provided helpful discussion on EnergyPlus. L.C.G. helped with writing the manuscript. Y.C., A.M. and S.F. supervised the project. All the authors provided discussion and comments.

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Correspondence to Yi Cui.

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Nature Sustainability thanks Tao Ma and the other, anonymous, reviewer(s) for their contribution to the peer review of this work.

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Supplementary Notes 1–3, Figs. 1–24, Tables 1 and 2, and References.

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Peng, Y., Fan, L., Jin, W. et al. Coloured low-emissivity films for building envelopes for year-round energy savings. Nat Sustain 5, 339–347 (2022). https://doi.org/10.1038/s41893-021-00836-x

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