Abstract
We present a linearoptical scheme for generating an arbitrary state of three qubits. It requires only three independent particles in the input and postselection of the coincidence type at the output. The success probability of the protocol is equal for any desired state. Furthermore, the optical design remains insensitive to particle statistics (bosons, fermions or anyons). This approach builds upon the notouching paradigm, which demonstrates the utility of particle indistinguishability as a resource of entanglement for practical applications.
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Entanglement remains a central theme in quantum foundations research^{1,2}. It is considered a key resource enabling the advantage in quantum information tasks^{3,4}. There is therefore a vital interest in practical entanglement generation schemes capable of delivering the broadest possible range of states, from which one might choose a state desired for a problem at hand. Ideally, we would like to have a generic and efficient tool for constructing an arbitrary multiparticle state from some simpler initial state (possibly having just a few independent particles to begin with). A paradigmatic example is the construction of the full class of singleparticle states (a qudit). In this case, arbitrary unitary transformation can be experimentally implemented by linearoptical devices^{5} and hence any singleparticle state can be deterministically prepared from any given initial state. However, it is not true for multiparticle states that do not transform one into another by means of linear optics^{6}. Thus for the generation of multipartite entanglement, nonlinear effects or postselection of some sort must be employed. Several techniques have been developed to this effect which produce certain classes of states^{7,8,9,10}. However, there is no systematic linearoptical method for obtaining an arbitrary multiparticle entangled state that would start with a supply of independent particles in the input.
In this work, we focus on entanglement generation for three qubits. Notably, this is the first nontrivial case where the arbitrariness of the desired state becomes challenging. An interesting approach to this problem consists in considering the set of stochastic local operations and classical communication (SLOCC)^{11,12,13}. It has been shown that for three qubits there are two inequivalent classes of genuinely tripartite entangled states^{12}. This means that using SLOCCs for filtering arbitrary tripartite entanglement requires two different types of entangled states to begin with, i.e., states of the GHZ and the W type. However, it should be remarked that the efficiency of such protocols drops to zero when moving away from the initial state. Another important result concerns the full set of linear optical transformations (without postselection)^{6}. Then the situation is further complicated as for three qubits the set of entangled states splits into a continuous number of inequivalent classes. Those results illustrate the difficulties in efficiently generating arbitrary entanglement using linear operations without any entanglement from the outset.
Here we will show that linearoptical transformations augmented with postselection of the coincidence type are enough to generate arbitrary entanglement of three qubits from three independent particles (i.e., without requiring any prior entanglement). Our proposal builds on the socalled notouching paradigm in optical designs which draws from the inherent indistinguishability of particles; see Ref.^{14} for a general scheme and Refs.^{15,16,17,18,19} for some examples. Notably, the protocol is an instance of direct and explicit construction of any given state. A distinctive advantage of the proposal is that it has equal efficiency for generating any desired state and it is insensitive to particle statistics.
Results
Simplification by generalised Schmidt decomposition
A general state of three qubits reads
where \(\mathinner {{ijk}\rangle }\) is a computational basis in \(\mathbb {C}^2\otimes \mathbb {C}^2\otimes \mathbb {C}^2\). It turns out that this can be simplified by local transformations to the combination of the following five states
with five real parameters \(a,b,c,d,e\ge 0\) and one phase \(0\le \varphi \le \pi\), such that
This follows from the generalised Schmidt decomposition for three qubits^{20,21} and no further reduction of the number of nonvanishing terms is possible.
Therefore, to generate the state in Eq. (1), it is enough to provide the state in Eq. (2) and then make a local transformation on each qubit. In the following, we give the explicit protocol for optical construction of an arbitrary state in the reduced form of Eq. (2).
Optical realisation
Consider three identical particles injected into an optical circuit which consists of 10 paths (or modes). The particle statistics (bosons, fermions or anyons) is irrelevant for the purpose at hand. Following the idea presented in Ref.^{14} we will group paths at the input and output into three systems, see Fig. 1:
Furthermore, we will distinguish three pairs of paths \(\bar{B}_1\), \(\bar{B}_2\) and \(\bar{B}_3\) in the respective subsystems at the output, i.e. \(\bar{B}_k\subset B_k\). They will play the role of the socalled dualrail qubits, where the computational basis \(\mathinner {{0}\rangle }\),\(\mathinner {{1}\rangle }\) is encoded by the presence of a single particle in the respective path of a given pair \(\bar{B}_k\). Accordingly, we have the following representation for a general qubit state \(\alpha \mathinner {{0}\rangle }+\beta \mathinner {{1}\rangle }\):
where \(\mathinner {{\Omega }\rangle }\) denotes the vacuum state and \(a^\dag _i\) are the usual particle creation operators in the second quantisation formalism. We note that the dualrail encoding assumes the presence of a single particle in a given pair of paths \(\bar{B}_k\) for \(k=1,2,3\). In our scheme this will be guaranteed by postselection on a single particle in each dualrail qubit \(\bar{B}_k\).
The optical protocol is depicted in Fig. 1. It consists of a sequence of three unitary transformations on three independent particles injected in paths 1, 6 and 8. First, the particles undergo local unitaries U, H and U in each subsystem \(A_1\), \(A_2\) and \(A_3\). Second, the paths are rearranged according to some permutation \(\sigma \in \mathcal {S}_{10}\). Third, there are two local unitaries V and W on subsystems \(B_1\) and \(B_2\) implemented at the output. Finally, the protocol ends with postselection on a single particle in each pair of paths \(\bar{B}_1\), \(\bar{B}_2\) and \(\bar{B}_3\) which generates three dualrail encoded qubits.
Now, we can make the unitaries in Fig. 1 more precise. Let the first two transformations U and V produce symmetric superposition of the injected particles, which in the matrix notation amounts to
The permutation of modes \(\sigma \in \mathcal {S}_{10}\) is given as follows
The final unitaries V and W are defined in a nontrivial way by the following two matrices
with some parameters \(\kappa ,\delta ,\nu ,\mu ,\epsilon ,\xi\) and \(\tau\). In the above notation, the dots “\({\textbf {.}}\)” are left unspecified and chosen so that the matrices are unitary. Observe that this can always be done by augmenting the missing columns/rows to an orthonormal basis (note that the two upper rows of V are orthogonal at the outset). The only constraint on the parameters \(\kappa ,\delta ,\nu ,\mu ,\epsilon ,\xi\) and \(\tau\) is their respective normalisation, i.e.
For our purposes, the dotted entries “\({\textbf {.}}\)” will play no role in the argument (in the following, they contribute only to the terms that drop out upon postselection). All the remaining parameters \(\kappa ,\delta ,\nu ,\mu ,\epsilon ,\xi\) and \(\tau\) will be specified shortly.
Let us write out the state that results from the protocol in Fig. 1 after injecting three independent particles in paths 1, 6, 8 and postselecting on a single particle in each dualrail qubit \(\bar{B}_1\), \(\bar{B}_2\) and \(\bar{B}_3\). The evolution of the system is given by a sequence of steps as described in the following lines:
where the last equality holds for bosons in the dualrail encoding. This renders the desired state in Eq. (2) when
We observe that we can always choose matrices W and V to satisfy these equations by defining parameters \(\kappa ,\delta ,\nu ,\mu ,\epsilon ,\xi\) and \(\tau\) in the following way
(If \(\mu =0\), then \(\xi\) and \(\tau\) can be taken arbitrarily). It is straightforward to check that the conditions in Eqs. (7)–(9) are satisfied, since the constraint in Eq. (3) holds.
Note that the scheme works for fermions as well. In this case, the final state in Eq. (16) takes the form
and then the Eqs. (18)–(20) require a trivial modification \(\nu =\,d\) and \(\xi =\,\frac {\textstyle {c}}{\textstyle {\mu }}\) in order to recover the desired state in Eq. (2). In a similar manner it is straightforward to adjust Eq. (16) for any particle statistics (anyons).
Finally, we observe that the expression in Eq. (16) is unnormalised due to postselection. This allows to read off the success probability (efficiency) of the process which is equal to \(\big (\,\frac {1}{3\sqrt{2}}\,\big )^{\scriptscriptstyle 2}=\frac {1}{18}\approx 5\%\). Notably, the efficiency is the same for every threequbit state \(\mathinner {{\psi }\rangle }\).
Discussion
We remark that the abovedescribed protocol, based on dualrail encoded qubits, provides a readymade template that straightforwardly translates into any other physical implementation of qubits. This turns out to be a generic feature of the notouching designs in which the question of particle statistics becomes virtually irrelevant because of postselection. It is due to the fact that the latter projects on the sector where the evolution of the system features at most a single particle in each mode, which makes immaterial the distinction between the bunching and antibunching effects for bosons and fermions; see Refs.^{14,15,16,17,18,19} for a discussion.
From the fundamental point of view, it is interesting to note the significance of the inherent indistinguishability of particles as conveniently described in the second quantisation formalism. It appears that entanglement resulting from the symmetrization postulate can be treated as a genuine resource and transformed into other kinds of entanglement which can be directly observed and used for practical applications^{14,22,23,24}. This paper shows that arbitrary entanglement of three qubits can be extracted in this way. For an extension to some multiparticle entangled states see e.g. Refs.^{19,25,26,27,28,29}.
An important advantage of the proposed protocol is the minimal amount of resources employed to generate an arbitrary threequbit state compared to the existing techniques:

(a)
It requires only linear optics and works equally well for any particle statistics, cf. Refs.^{7,8,9,10}.

(b)
There is no need for auxiliary systems (particles) or measurements, cf. Refs.^{25,27}.

(c)
The protocol requires only three independent particles in the input, i.e., no prior entanglement is required.

(d)
It has the same efficiency for the generation of any desired threequbit state.
This distinguishes our proposal from the typical approach based on filtering via SLOCC operations which requires auxiliary entanglement from the outset, and its success probability for arbitrary threequbit states drops to zero; see Methods section for discussion. Moreover, the generation of states via SLOCC filtering generally demands different initial states depending on the SLOCC equivalence class of the target state. For optical proposals aimed at preparation of single representatives in the SLOCC classes for the purpose of filtering see Refs.^{14,26,28,30}. Notably, our protocol overcomes the division into SLOCC equivalence classes due to the presence of mode permutation \(\sigma\), which is a nonlocal operation from the point of view of subsystems defined by mode grouping.
We note that our scheme relies on a specific type of postselection which requires coincidence count in the output channels encoding dualrail qubits \(\bar{B}_1\), \(\bar{B}_2\) and \(\bar{B}_3\). A direct way to check the coincidence criterion involves the measurement of each qubit. Typically this destroys the state, but the recorded correlations can be still used for the extraction of some information relevant to a given experiment. The utility of such a direct postselection depends on the task at hand. For illustration see, e.g., the recent boson sampling experiments^{31} or the direct verification of the boson nature of photons^{32,33}. It was also shown to be safe for Belltype tests of nonlocality^{24}. We remark that many modern state generation schemes refer to postselection of the the coincidencetype, like e.g. entanglement by path identity^{9,34,35} or spatial overlap of indistinguishable particles^{22,23,36}. However, if the generated state needs to be further processed, then direct detection does not meet this requirement. In such a case, the solution is provided by nondemolition measurements carried out on each dualrail qubit \(\bar{B}_1\), \(\bar{B}_2\) and \(\bar{B}_3\). Such a measurement ascertains the presence of a particle without destroying it and not affecting its state. Therefore, a positive joint result of those three (nondemolition) measurements heralds the generation of the desired state in the signal modes. This turns the protocol into an eventready scheme. Notably, a few nondemolition measurement techniques have been developed in recent years. See e.g. Refs.^{37,38,39} for nondemolition detection of photons (noting that polarization and dualrail encoding of qubits transforms one into another via polarizing beam splitters).
In summary, the characteristic features of the proposed scheme for state generation are marked by simplicity (just linear optics and postselection of the coincidence type), limited initial resources (just three independent particles in the input), and universal efficiency (equal for any desired state). This makes the proposal an interesting technique for integrated quantum technologies motivating further research towards an extension to an arbitrary number of qubits; see the recent progress in the optical generation of certain multiparticle states within the notouching paradigm^{19,25,26,27,28,30}. We also indicate possible further improvements using a graphtheoretical approach to the analysis of linear optical schemes^{40}.
Methods
Comparison with the generation of arbitrary states via SLOCC operations
In this paper, we presented a universal interferometric protocol for generating an arbitrary threequbit state from an input product state of three particles, which prepares an arbitrary state with constant finite efficiency. Here, we compare this scheme with the generation of arbitrary states from a GHZ class starting from the GHZ input state via SLOCC operations. We will see that the lattr method of state generation has a vanishing efficiency for some states in this class.
As shown in the seminal paper by Dür et al.^{12} an arbitrary state from the GHZ class can be parametrised by five real parameters as
in which the normalisation constant reads \(K=(1+2\cos (\chi )\sin (\chi )\cos (\alpha _1)\cos (\alpha _2)\cos (\alpha _3)\cos (\theta ))^{1}\) and the states \(\mathinner {{s_i}\rangle }\) are given by \(\cos (\alpha _i)\mathinner {{0}\rangle }+\sin (\alpha _i)\mathinner {{1}\rangle }\). The ranges of the parameters are as follows: \(\chi \in (0,\frac{\pi }{4}]\), \(\alpha _i\in (0, \frac{\pi }{2}]\) and \(\theta \in [0,2\pi )\). This state can be obtained from the standard GHZ state \(\mathinner {{\psi _{\text {GHZ}}}\rangle }=\frac{1}{\sqrt{2}}(\mathinner {{000}\rangle }+\mathinner {{111}\rangle })\) via SLOCC filtering operations specified by
where the SLOCC operator M has the form^{12}
Such a filtering operation can be implemented as a twooutcome POVM measurement^{13}, with measurement operators defined by \(P=M/M\) and \(P'=\sqrt{\mathbbm{1}P^{\dagger }P}\). The outcome related to the measurement operator P indicates the success of the protocol, whereas the outcome related to \(P'\)—its failure. The norm has to be chosen to guarantee that \(P^{\dagger }P\le \mathbbm{1}\). One of the typical choices is the spectral norm of the operator M, defined as the largest singular value of M. This choice turns out to be optimal for the task of entanglement distillation of twoqubit states^{13}. However, other choices that guarantee the condition \(P^{\dagger }P\le \mathbbm{1}\), such as the Frobenius norm, are also correct. The success probability of filtering arbitrary state of the form Eq. (22) for SLOCC operator M is thus given by^{41}
where \(\rho _{\text {GHZ}}=\mathinner {{\psi _{\text {GHZ}}}\rangle }\mathinner {\langle {\psi _{\text {GHZ}}}}\), and the last equality follows from the fact that \(\mathinner {{\psi _{\text {GHZ}}}\rangle }\) is already properly normalised. Note that the operator M is not unitary, and therefore it does not preserve the normalisation of a general state it acts on—the state \(\rho _{\text {GHZ}}\) is an exception.
Let us assume that we choose the spectral norm in Eq. (25). For the clarity of presentation we will focus on a twoparameter subclass of states from the GHZ class Eq. (22) of the form \(\mathinner {{\psi _{\text {GHZ}}(\chi ,\pi ,\alpha ,\alpha ,\alpha )}\rangle }\). In Fig. 2 we present the success probability of obtaining this state from the GHZ state as a function of parameters \(\chi\) and \(\alpha\). We can see that the probability tends to zero for \(\chi =\frac{\pi }{4}\) and \(\alpha \rightarrow 0\), which stands in sharp contrast with our protocol that allows for the generation of these states with the fixed finite probability of success independently of the values of the parameters. One may argue that the effect of vanishing probability is related to a specific choice of the norm. However, it is easy to see that this effect holds for any choice of the norm consistent with the condition \(P^{\dagger }P\le \mathbbm{1}\). Indeed, it suffices to show that \(M(\tfrac{\pi }{4},\pi ,\alpha \rightarrow 0)\rightarrow \infty\) for any choice of the norm. Due to Eq. (24) we have
Now it can be easily verified that \(\left \sqrt{2K\left( \tfrac{\pi }{4},\pi ,\alpha \rightarrow 0\right) }\right \rightarrow \infty\). Therefore it suffices to show that \(\tilde{M}(\tfrac{\pi }{4},\pi ,\alpha \rightarrow 0)\) is strictly positive for any choice of the norm. For the spectral norm one has \(\tilde{M}(\tfrac{\pi }{4},\pi ,\alpha \rightarrow 0)=2\). However, all matrix norms for finite dimensional matrices of a fixed dimension are equivalent, which means that for any two norms \(\cdot _X\) and \(\cdot _Y\) there exist two positive numbers \(x,x'\) such that for any matrix A one has \(xA_X\le A_Y\le x'A_X\). From this property it follows that \(\tilde{M}(\tfrac{\pi }{4},\pi ,\alpha \rightarrow 0)\) must be strictly positive for any choice of the matrix norm, which implies \(M(\tfrac{\pi }{4},\pi ,\alpha \rightarrow 0)\rightarrow \infty\) and therefore the success probability for filtering the states in the neighbourhood of \(\chi =\tfrac{\pi }{4}\) and \(\alpha =0\), for any implementation of the SLOCC operation in Eq. (24), is arbitrarily close to zero.
This shows that our protocol overcomes the difficulties of state generation via SLOCC filtering operations, since in the latter: (i) the filtering probability can vanish, (ii) we are confined within one of the six entanglement classes depending on the initial state of the filtering. Both restrictions do not apply to our protocol, in which the success probability is constant for any state and we can reach an arbitrary state from the same trivial initial state.
Data availability
All data generated or analysed during this study are included in this published article.
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Acknowledgements
We thank YongSu Kim and Marek Żukowski for discussions and helpful comments. PB acknowledges support from the PolishU.S. Fulbright Commission. MM acknowledges partial support from the Foundation for Polish Science (IRAP project, ICTQT, contract no. MAB/2018/5, cofinanced by EU within Smart Growth Operational Programme).
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Blasiak, P., Borsuk, E. & Markiewicz, M. Arbitrary entanglement of three qubits via linear optics. Sci Rep 12, 21596 (2022). https://doi.org/10.1038/s41598022228354
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DOI: https://doi.org/10.1038/s41598022228354
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