Abstract
A transparent polarisation sensitive phase pattern makes a polarisation dependent transformation of quantum state of photons without absorbing them. Such an invisible pattern can be imaged with quantum entangled photons by making joint quantum measurements on photons. This paper shows a long path experiment to quantum image a transparent polarisation sensitive phase pattern with hyperentangled photon pairs involving momentum and polarisation degrees of freedom. In the imaging configuration, a single photon interacts with the pattern while the other photon, which has never interacted with the pattern, is measured jointly in a chosen polarisation basis and in a quantum superposition basis of its position which is equivalent to measure its momentum. Individual photons of each hyperentangled pair cannot provide a complete image information. The image is constructed by measuring the polarisation state and position of the interacting photon corresponding to a measurement outcome of the noninteracting photon. This paper presents a detailed concept, theory and free space long path experiments on quantum imaging of polarisation sensitive phase patterns.
Similar content being viewed by others
Introduction
A transparent polarisation sensitive phase pattern introduces a positiondependent change in the phase of transmitted light depending on the polarisation of incident light. A classical image of such a pattern can be obtained by measuring the positionwise polarisation shift of the transmitted classical electromagnetic field in the image plane by a method known as polarisation contrast imaging^{1,2,3,4,5,6,7}. However, an image formed by a single photon exposure of the pattern in each execution of the experiment is defined as a quantum image. In this way, one can gain the quantum mechanical advantage over the classical imaging. One such advantage is the quantum secure transfer of images. Furthermore, by incorporating quantum entangled photons, one can utilise properties of quantum entanglement and quantum measurements to construct an image of the pattern. Where a single photon of an entangled pair of photons interacts with the pattern. However, in contrast to the classical polarisation contrast imaging, complete information of the pattern is shared nonlocally by both photons as a consequence of quantum entanglement, even if they are separated by a large distance when a photon interacted with the pattern. Here, one cannot obtain complete pattern information just by measuring a single photon. Therefore, a joint measurement becomes necessary and a quantum image of the pattern can be constructed by correlating the measurement outcomes. Because of quantum entanglement, quantum images can be transferred to another location securely and directly.
This paper presents the first free space long path experiment of quantum imaging of a transparent polarisation sensitive phase pattern with hyperentangled photons. Where a hyperentangled state is a product of quantum entangled states involving different degrees of freedom^{8,9}. In the experiment, the hyperentangled state consists of a product of polarisation entanglement^{10} and momentum entanglement of two photons^{11,12,13,14,15,16}. Where the momentum entanglement corresponds to Einstein–Podolsky–Rosen type of quantum entangled state originating from a finite region. Each photon of a hyperentangled biphoton state carries information of polarisation and momentum of the other photon but an individual photon has no welldefined position, momentum and polarisation.
A nonbirefringent transparent phase object can be classically imaged with wellknown phasecontrast imaging methods where the phase information is converted to intensity^{17,18,19}. In the context of the development of imaging experiments, a phasecontrast imaging method is applied for a nondestructive detection of a Bose–Einstein condensate^{20,21}. Twophoton coincidence quantum imaging of absorptive objects has been studied theoretically and experimentally with spatially correlated photons from a perspective of foundations of quantum mechanics^{22,23,24,25,26,27,28,29,30,31}. Quantum imaging of an absorptive object has been realised experimentally without detecting a photon interacting with the object^{32,33}. Bell’s inequality violation experiments are performed with images^{34,35}. Twoatom ghost imaging of an absorptive pattern for atoms has been experimentally realised with metastable helium atoms^{36,37}. A polarisationsensitive metasurface is imaged in the near field with polarisation entangled photons^{38}.
In this paper, experiments involve a multidimensional entanglement in the form of a hyperentangled state, to quantum image a transparent polarisation sensitive phase pattern in free space, where the pattern is positioned at a distance 16.91 m from a coincidence imaging camera. However, this particular experiment is not aiming to close loopholes. In the experiment, polarisation as well as momentum degrees of freedom of the hyper entangled photons are utilised for quantum imaging.
Hyperentangled photons
Consider a hyperentangled photons pair emitted by a source in opposite directions as shown in a schematic diagram Fig. 1. Where photon2 is passed through a transparent polarisation sensitive phase pattern. Since photons are polarisation entangled and momentum entangled separately therefore, a polarisation sensitive phase pattern induces a positiondependent variation of the quantum entangled state of photons. Polarisation measurement outcomes of photon1 and photon2 are determined by a measurement setting (orientation of pass axis) of polariser1 and polariser2, respectively. After passing through polariser1, photon1 is focused by a lens \(L_{o}\) on a single photon detector after passing through a narrow aperture. A lens \(L_{o}\) permits detection in a quantum superposition basis of the position of photon1. A photon detection produces a pulse named an event signal, which is sent to a single photon detection camera to allow registration of photon2 corresponding to a selected measurement outcome. A quantum image is gradually formed by accumulating the photon registrations on camera for each repetition of the experiment with the same measurement setting. In this way, this is a coincidence imaging where the individual photon has no welldefined momentum and polarisation however, each photon is carrying momentum and polarisation information of the other photon by quantum entanglement. Therefore, measurement outcomes of both photons are required to construct a quantum image.
Consider Einstein–Rosen–Podolsky state (EPR)^{39} of two particles in a position space, \(\alpha \rangle =\int ^{\infty }_{\infty }x\rangle _{1}x+x_{o}\rangle _{2} \mathrm {d}x\), where subscripts 1 and 2 are the labels of particles. In this state, both particles are equally likely to exist at all points in the position space with a constant separation \(x_{o}\). In this way, they are spatially entangled. The EPR state in a momentum space can be written as \(\alpha \rangle =\int ^{\infty }_{\infty }e^{i \frac{p x_{o}}{\hslash }}p\rangle _{1}p\rangle _{2}\mathrm {d}p\), here both particles have opposite momenta and are equally likely to exist at all points in the momentum space such that they are momentum entangled. Where \(\hslash =h/2\pi\) is the reduced Planck’s constant. In this way, the position and momentum of each particle are completely unknown. Consider a source of a finite extension producing a pair of photons such that both photons are originating from the same position in the source. This is a case, if \(x_{o}=0\) in the onedimensional EPR state and in this paper, it is extended to three dimensions by including the polarisation of photons.
Quantum state of photons originating from a position vector \({\mathbf {r}}'\), in time independent case, leads to a finite amplitude to find a photon at a point \(o_{a}\) in regiona and another photon at a point \(o_{b}\) in regionb as shown in Fig. 1. Consider points \(o_{a}\) and \(o_{b}\) prior to any optical element from the source. A joint amplitude for photons to be at these points in threedimensions is \(\frac{e^{ip_{1}{\mathbf {r}}_{a}{\mathbf {r}}'/\hslash }}{{\mathbf {r}}_{a}{\mathbf {r}}'}\frac{e^{ip_{2}{\mathbf {r}}_{b}{\mathbf {r}}'/\hslash }}{{\mathbf {r}}_{b}{\mathbf {r}}'}\)^{40,41} where \(p_{1}\) and \(p_{2}\) are magnitudes of momentum of photon1 and of photon2, respectively. Position vectors of points \(o_{a}\) and \(o_{b}\) from origin are \({\mathbf {r}}_{a}\) and \({\mathbf {r}}_{b}\), respectively. Distances of \(o_{a}\) and \(o_{b}\) from \({\mathbf {r}}'\) are \({\mathbf {r}}_{a}{\mathbf {r}}'\) and \({\mathbf {r}}_{b}{\mathbf {r}}'\), respectively. Here, both photons are produced from a same location within the source. Consider, polarisation state of photon1 propagating in regiona is horizontal \(H\rangle _{a}\) and of photon2 propagating in regionb is vertical \(V\rangle _{b}\). A total amplitude to find photon1 at \(o_{a}\) and photon2 at \(o_{b}\) is a linear quantum superposition of amplitudes originating from all points within the source. Therefore, a combined twophoton quantum state can be written as
where \(A_{o}\) is a normalisation constant and \(\psi (x',y',z')\) is an amplitude of pair creation at a location \(r'(x',y',z')\) that is considered to be \(\frac{e^{\frac{x'^{2}}{2\sigma ^2_{x}}}}{(2\pi )^{1/2} \sigma _{x}} \frac{e^{\frac{y'^{2}}{2\sigma ^2_{y}}}}{(2\pi )^{1/2} \sigma _{y}} \frac{e^{\frac{z'^{2}}{2\sigma ^2_{z}}}}{(2\pi )^{1/2} \sigma _{z}}\).
For a source extension much smaller than distances of points \(o_{a}\) and \(o_{b}\) from origin, Eq. (1) is written as
where \(\Phi _{12}(r_{a};r_{b})\) is the amplitude to find photon1 at \(o_{a}\) and photon2 at \(o_{b}\), which is calculated by solving the integral in Eq. (1),
where \(p_{1x}=p_{1}\sin \theta _{a} \cos \phi _{a}\), \(p_{1y}=p_{1}\sin \theta _{a} \sin \phi _{a}\) and \(p_{1z}=p_{1}\cos \theta _{a}\) are the x, y and z components of momentum of photon1 in the spherical polar coordinate system. Similarly \(p_{2x}=p_{2}\sin \theta _{b} \cos \phi _{b}\), \(p_{2y}=p_{2}\sin \theta _{b} \sin \phi _{b}\) and \(p_{2z}=p_{2}\cos \theta _{b}\) are the x, y and z components of momentum of photon2.
Photons are momentum entangled due to inseparability of \(\Phi _{12}(r_{a};r_{b})\). Assume that photons have same energy therefore, magnitudes of their momenta are equal, \(p_{1}=p_{2}\). Since photons are identical particles and there exist different amplitudes that cannot be distinguished if a photon is detected at \(o_{a}\) and another photon is detected at \(o_{b}\). An amplitude to find photon1 at \(o_{a}\) and photon2 at \(o_{b}\) is indistinguishable from finding photon1 at \(o_{b}\) and photon2 at \(o_{a}\) after exchange of photons if their polarisation is not measured. Therefore, due to the Bosonic nature of identical photons, their symmetric quantum state is written as \(\Psi \rangle = \frac{1}{\sqrt{2}}(\Psi \rangle _{12}+\Psi \rangle _{21})\), where \(\Psi \rangle _{21}\) is a quantum state Eq. (1) after the exchange of photons.
After the exchange of photons, Eq. (2) becomes \(\Psi \rangle _{21}=\Phi _{21}(r_{a};r_{b})\otimes V\rangle _aH\rangle _b\). However, from Eq. (3), \(\Phi _{21}(r_{a};r_{b})=\Phi _{12}(r_{a};r_{b})\). Therefore, a combined quantum state becomes
This is a hyperentangled state since photons are momentum entangled due to inseparability of \(\Phi _{12}(r_{a};r_{b})\) and polarisation entangled due to inseparability of \(\frac{1}{\sqrt{2}} (H\rangle _aV\rangle _b+V\rangle _aH\rangle _b)\), where each quantum entangled state is symmetric. However, a combined quantum state is a product of each quantum entangled state. From here onwards, a photon in regiona is labeled as photon1 and a photon in regionb is labeled as photon2.
Imaging with hyperentangled photons
In a realistic experiment, a source emits entangled photons in particular directions. To incorporate this directional dependence, quantum state is multiplied by an additional directional function such that the highest probability of finding photons is around a point \(o_{a}\) in regiona and \(o_{b}\) in regionb. Let \(\psi _{a}(x_{1},y_{1}, z_{1})\) and \(\psi _{b}(x_{2},y_{2}, z_{2})\) are the envelops of wavefunctions for a photon around \(o_{a}\) and a photon around \(o_{b}\). From these considerations, a total symmetric quantum state of photons can be written as
where the phase \(\phi\) is not arbitrary, it is either zero or \(\pi\). The total quantum state is symmetrised with a plus sign if \(\phi =0\). For \(\phi =\pi\), the polarisation entangled state is antisymmetric after the exchange of photons therefore, the quantum state in the external degrees of freedom has to be antisymmetric. Here, \(a_{s}\) is a normalisation constant. In the experiment, a phase difference \(\phi\) between \(H\rangle\) and \(V\rangle\) quantum states of a photon is introduced either by placing a halfwave plate in the path of a photon or by tilting the nonlinear crystal source of entangled photons. In this paper, an antisymmetric polarisation entanglement is produced by the source. Since photons are propagating in different regions a and b such that \(\psi _{a}(x_{1},y_{1}, z_{1})\) and \(\psi _{b}(x_{2},y_{2}, z_{2})\) are nonoverlapping therefore, a second term \(\psi _{a}(x_{2},y_{2}, z_{2})\psi _{b}(x_{1},y_{1}, z_{1})a_{s}\Phi _{21}(r_{a};r_{b})\), in Eq. (5) is negligible.
To form an image with a hyperentangled state, consider photon2 in regionb is passed through a transparent polarisation sensitive phase pattern oriented perpendicular to zaxis as shown in Fig. 1. The pattern introduces a positiondependent phase difference between the horizontal and the vertical polarisation of a photon passing through it such that \(H\rangle _{2}\rightarrow e^{i\phi (x_{2}, y_{2})}H\rangle _{2}\) and \(V\rangle _{2}\rightarrow V\rangle _{2}\). In the experiment, a phase difference \(\phi (x_{2},y_{2})\) is either zero or \(\pi\). Consider photon2 of a hyperentangled state, with an antisymmetric polarisation entangled state \(\Psi ^\rangle _{p}=\frac{1}{\sqrt{2}}\left( H\rangle _1V\rangle _2V\rangle _1H\rangle _2\right)\), is incident on the pattern. A polarisation dependent phase is imprinted on photon2 in regionb. Assume that the pattern is located at \(z=d_{2}\) in regionb. An arbitrary location of photon2 on the pattern just after the phase imprint is represented by coordinates (\(x_{2}\), \(y_{2}\)) in the xy plane at \(z=d_{2}\). An arbitrary location of photon1 in a plane oriented perpendicular to zaxis at \(z=d_{1}\) in regiona is represented by coordinates (\(x_{1}\), \(y_{1}\)). Therefore, after the phase imprint and normalisation, the quantum state of photons is written as
A transparent polarisation sensitive phase pattern is imprinted in the phase of polarisation entangled state and a spread of a photon on the pattern is due to the momentum entangled part of the hyperentangled state. Photons are also spatially correlated due to their spatial entanglement in position space. The position dependent polarisation entangled state of photons is \(\Psi ^\rangle _{p}\) for \(\phi (x_{2}, y_{2})=0\) and \(\Psi ^+\rangle _{p}=\frac{1}{\sqrt{2}}\left( H\rangle _1V\rangle _2+V\rangle _1H\rangle _2\right)\) for \(\phi (x_{2}, y_{2})=\pi\). The location and polarisation information of each photon is carried by the other photon because of their quantum entanglement.
After the imprint of a pattern, the position coordinates (\(x_{2}\), \(y_{2}\)) at \(z=d_{2}\) of photon2 are measured by imaging with a lens on a single photon sensitive camera after its polarisation selection by polariser2 as shown in Fig. 1. The camera registers photon2 only if photon1 is detected by a single photon detector after passing through polariser1. Consider a lens \(L_{o}\) is not placed but a narrow aperture single photon detector is placed at a location \((x_{o1},y_{o1}, z=d_{1})\) and orientation of pass axis of polariser1 is vertical and of polariser2 is horizontal. This measurement setting corresponds to a coincidence detection when photon1 is detected at \((x_{o1},y_{o1}, z=d_{1})\) in the vertical polarisation and photon2 is detected in the horizontal polarisation state on the camera. The same experiment is repeated for a chosen measurement setting many times, a location of photon2 on camera varies each time and gradually an image is formed on the camera. A corresponding probability of coincidence detection is written as \(P_{V_{1},H_{2}}(x_{2}, y_{2})=\frac{1}{2} a_{s}\psi _{a}(x_{o1},y_{o1}, d_{1})\psi _{b}(x_{2},y_{2}, d_{2})\Phi _{12}(r_{a};r_{b})(e^{i\phi (x_{2}, y_{2})})^{2}\). Where subscripts of \(P_{V_{1},H_{2}}\) denote orientation of passaxes of polariser1 and polariser2. It is clear that the phase information is lost for this polarisation setting. Similarly, a polarisation sensitive phase information cannot be recovered for other combination of orientations of polarisers along horizontal and vertical directions.
Let the orientation of pass axes of polarisers is now changed to perform polarisation measurements in the diagonal basis that is \(d^{+}\rangle _{j}=\frac{H\rangle _{j}+V\rangle _{j}}{\sqrt{2}}\) and \(d^{}\rangle _{j}=\frac{H\rangle _{j}V\rangle _{j}}{\sqrt{2}}\), where a photon label j is 1 or 2. If both polarisers are oriented to pass quantum states \(d^{}\rangle _{j}\) and photon1 is detected at a location \((x_{o1},y_{o1}, z=d_{1})\), then the corresponding probability of coincidence detection is
which contains a phase information of the pattern. Since \(\phi (x_{2},y_{2})\) is either \(\pi\) or zero therefore, \(P_{d^{}_{1},d^{}_{2}}(x_{2},y_{2})\) is a two level image. Where an image of the transparent polarisation sensitive phase pattern is obtained by measuring coincidence detection probability. If on the other hand, polariser1 is aligned to pass \(d^{+}\rangle\) and polariser2 is aligned to pass \(d^{}\rangle\) then the corresponding probability of coincidence detection is written as
This image is exactly inverted as compared to Eq. (7), where the maximum and the minimum levels of the image are interchanged.
To make a measurement on photon1 in a quantum superposition basis of position \((x_{1}, y_{1})\), a convex lens \(L_{o}\) is placed at \(z=d_{1}\) and photon1 is detected close to its focal point by a narrow aperture single photon detector placed on zaxis. The lens transforms a particular quantum superposition of position (or an incident momentum state) in a plane at \(z=d_{1}\) to a single point in its focal plane. Therefore, probability of coincidence detection of photons for two different orientation \((d^{+}_{1},d^{}_{2})\) and \((d^{}_{1},d^{}_{2})\) of polarisers is succinctly written as
It is evident that opposite level images are formed when orientation of polarisers is changed from \((d^{}_{1},d^{}_{2})\) to \((d^{+}_{1},d^{}_{2})\). However, no image is formed if only photon2 is detected without considering the measurement outcome of photon1 or if photon1 is not measured at all.
Experiment and discussion
A schematic diagram of the experimental setup is shown in Fig. 2. Hyperentangled photons are produced by typeII spontaneous parametric down conversion (SPDC)^{42,43,44,45,46,47} in a betabariumborate (BBO) nonlinear crystal. A linearly polarised pump laser beam of wavelength 405 nm and narrow beam diameter is passed through a BBO crystal. Hyperentangled photons are produced at wavelength 810 nm in a first crystal, where a second crystal is placed to compensate transverse and longitudinal walkoffs. A polarisation sensitive phase pattern is produced by a reflection type spatial light modulator (SLM). After the collimation, photon2 is reflected from the spatial light modulator and a positiondependent phase is imprinted such that \(H\rangle _{2}\rightarrow e^{i\phi (x_{2},y_{2})}H\rangle _{2}\) and \(V\rangle _{2}\rightarrow V\rangle _{2}\). Photon2 is imaged on an intensifiedchargecoupleddevice (ICCD) camera, after passing through polariser2, with a three lens (\(L_{1}\), \(L_{2}\) and \(L_{3}\)) telescopic configuration. The telescope is aligned such that the object plane coincides with the reflecting surface of the spatial light modulator. In this way, a location of photon2 immediately after the phase imprint is measured by imaging it on the camera. The focal length of lens \(L_{1}\) of diameter 5 cm is 40 cm. The focal lengths of lenses \(L_{2}\) and \(L_{3}\) are 10 cm and 100 cm, respectively. Photon1 is passed through polariser1 to perform a polarisation measurement and a lens \(L_{o}\) to perform a measurement in the quantum superposition basis of position after detection by a narrow area single photon detector of very low dark counts. These are joint measurements. Passaxis of polariser1 is subtending an angle \(\delta _{1}\) and of polariser2 is subtending an angle \(\delta _{2}\) with the horizontal axis. These angles can be varied independently according to a measurement setting. An electrical signal is produced by a single photon detector corresponds to a measurement outcome for a chosen measurement setting for photon1. This signal is connected to a direct gate terminal of the ICCD camera. The direct gate terminal activates an electronic shutter of the camera that allows detection signal of photon2 produced by the imaging sensor of camera to reach the chargecoupleddevice (CCD) sensor of the camera after amplification. This process efficiently detects a coincidence event of photons with a 20 ns insertion delay. The distance of the imaging sensor surface of the ICCD camera from the spatial light modulator is 16.91 m. The spatial light modulator is placed at a distance 89 cm from the first BBO crystal. A first lens \(L_{1}\) of the telescope is placed at a distance 15.24 m from the spatial light modulator surface. This lens produces an inverted real image of the spatial light modulator surface, which acts as a real image for a second lens \(L_{2}\). A second lens is placed such that it produces a magnified virtual image in a virtual image plane as shown in Fig. 2. A third lens \(L_{3}\) of focal length f = 100 cm is positioned such that the photon detection plane of the ICCD camera and a virtual image plane are positioned at \(+2f\) and \(2f\), respectively from lens \(L_{3}\). In this 2f2f imaging configuration, an image can be finetuned on the ICCD camera by displacing the second lens \(L_{2}\) only and keeping other lenses stationary. The image demagnification of the telescope is 0.52 and its spatial resolution at the spatial light modulator surface is about \(\sim\) 0.3 mm. In the experiment, a structure size of the pattern is 1 mm, which is imaged by the ICCD camera from a distance 16.91 m.
Consider, photonj is detected after passing through a polariserj with its pass axis inclined at an angle \(\delta _{j}\) w.r.t. horizontal axis. Its measured state of polarisation is, \(H\rangle _{j}\) for \(\delta _{j}=0\), \(V\rangle _{j}\) for \(\delta _{j}=90^{\circ }\), \(d^{+}\rangle _{j}\) for \(\delta _{j}=45^{\circ }\) and \(d^{}\rangle _{j}\) for \(\delta _{j}=45^{\circ }\). Polarisation state of photon2 is measured once it is detected by ICCD camera at any location after passing through polariser2. If a single photon detector detects photon1 after passing through a polariser1 but without a lens \(L_{o}\), then it corresponds to a position measurement of photon1 \((x_{01}, y_{01})\) in a plane at \(z=d_{1}\) along with an outcome of measured state of polarisation of photon1. On the other hand, if a single photon detector detects a photon1 after passing through a polariser and a lens \(L_{o}\), then it corresponds to a measurement in the quantum superposition basis of position along with an outcome of a measured state of polarisation of photon1. For this measurement setting, a coincidence photon detection probability is given by Eq. (9).
A transparent polarisation sensitive phase pattern shown in Fig. 3a is displayed on the spatial light modulator, where a positiondependent grey level of the pattern determines a phase shift, which is either zero or \(\pi\). Lighter grey regions represent a \(\pi\) phase shift and since a source produces an antisymmetric polarisation entangled state therefore, polarisation entanglement of photons, after passing photon2 through this region, transformed to \(\Psi ^{+}\rangle _{p}=\frac{1}{\sqrt{2}} (H\rangle _1V\rangle _2+V\rangle _1H\rangle _2)\). Darker grey regions represents a zero phase shift and polarisation entangled state of photons remains same as produced by the source that is \(\Psi ^{}\rangle _{p}=\frac{1}{\sqrt{2}} (H\rangle _1V\rangle _2V\rangle _1H\rangle _2)\). Therefore, the information of a twophoton quantum image is contained by the momentum and the polarisation entanglement parts of \(\Psi \rangle _{I}\). In the first experiment, to produced a quantum image, both polarisers are aligned at \(\delta _{1}=45^{\circ }\) and \(\delta _{2}=45^{\circ }\) to detect a same state of polarisation of photons in the diagonal basis that is \(d^{}\rangle _{1}\) of photon1 and \(d^{}\rangle _{2}\) of photon2. Photon1 is also measured in the quantum superposition basis of position. The experiment is repeated for this setting and an image, in the form of gated photon counts of the pattern, is accumulated for 10 minutes exposure of the ICCD camera. A background image is captured by displaying a uniform grey level corresponding to \(\phi =0\) on the spatial light modulator with the same experimental setting. A coincidence photon image is constructed by subtracting a corresponding background image as shown in Fig. 3b. The ICCD camera also captures accidental counts in the coincidence window. These accidental counts are originated from the scattered photons and camera noise. These counts accumulate with the actual coincidence photon counts. A typical ratio of a coincidence to accidental counts is 0.35–0.45. This is why a background correction is necessary. The noise of accidental photon counts in the background image, which is defined as a ratio of standard deviation to an average of counts for twentyfive hundred pixels is typically 0.12. All images shown in this paper are background corrected. Each image on the ICCD camera is reduced by 0.52 image demagnification. In a similar experiment, polariser1 is aligned at \(\delta _{1}=+45^{\circ }\) to detect photon1 in \(d^{+}\rangle _{1}\) and polariser2 is kept at \(\delta _{2}=45^{\circ }\) to detect photon in \(d^{}\rangle _{2}\) . The coincidence image photon counts accumulated by the ICCD camera are shown in Fig. 3c, which corresponds to an image with inverted levels as compared to an image shown in Fig. 3b. This result is in agreement with Eq. (9) that shows an inversion of levels of images in the diagonal basis. These images are twolevel images corresponding to the twolevel phase shift of the pattern.
In another experiment, a different transparent polarisation sensitive phase pattern as shown in Fig. 4a is displayed on the spatial light modulator. Where the gray levels corresponding to the positiondependent phase shifts are the same as in the previous pattern. A backgroundcorrected image of this pattern shown in Fig. 4b is accumulated with the ICCD camera for 10 minutes time of exposure in the diagonal basis, for \(\delta _{1}=\delta _{2}=45^{\circ }\) and with a lens \(L_{o}\). This image is then compared with another backgroundcorrected image captured with a different setting of polariser1, \(\delta _{1}=+90^{\circ }\) as shown in Fig. 4c keeping all other settings the same. According to the theoretical analysis shown in the previous section, the coincidence probability corresponding to a measurement of \(H\rangle\) or \(V\rangle\) state of photon1 does not contain the phase information of the pattern therefore, no image should be formed. A measurement of photon1 polarisation state in \(V\rangle _{1}\) collapses photon2 polarisation state onto \(H\rangle _{2}\) and this polarisation state is transformed by the spatial light modulator such that \(H\rangle _{2}\rightarrow e^{i\phi (x_{2},y_{2})}H\rangle _{2}\). This is a pure phase pattern and it diffracts photons. However, a telescope is located at a far distance 15.24 m from the pattern and its spatial resolution at this distance is about \(\sim\) 0.3 mm, where the size of each square in the pattern is 1 mm \(\times\)1 mm. Due to the finite lens diameter, the telescope is not capturing all the diffracted photons carrying information of sharp edges and it leads to the fundamental diffraction limit of resolution. Thus, the edges or phase boundaries in the pattern lead to low twophoton coincidence counts. Therefore, the edges appear as lowlevel regions in the image. In this case, if all diffracted photons are also captured then no image of the pattern will result. This effect is exactly matching for all the sharp edges by a comparison of an image shown in Fig. 4c with a corresponding image shown in Fig. 4b. Another image is captured for setting, \(\delta _{1}=0\) to detect photon1 in \(H\rangle _{1}\) keeping all other settings the same as for the image shown in Fig. 4b. Since this setting collapses the polarisation state of photon2 to \(V\rangle _{2}\) and this quantum state remains unchanged by the spatial light modulator therefore, no pattern is formed on ICCD camera as shown in Fig. 4d. A similar experiment is repeated for \(\delta _{1}=90^{\circ }\) to detect \(V\rangle _{1}\) and \(\delta _{2}=45^{\circ }\) to detect \(d^{}\rangle _{2}\) for a pattern shown in Fig. 3a. A corresponding backgroundcorrected image is shown in Fig. 5a, where the sharp edges appear due to the diffraction limit of the telescope. As explained, for \(\delta _{1}=0\) and \(\delta _{2}=45^{\circ }\), no pattern is formed as shown in Fig. 5b. A single photon backgroundcorrected image of the same pattern is shown in Fig. 5c. In this case, photon1 is not measured and the ICCD camera shutter is kept open for continuous exposure of photon2 for 10 minutes. This image has low depth and only the sharp edges appear because of the diffraction limit of the telescope.
Conclusion
This paper presents quantum imaging experiments of transparent polarisation sensitive phase patterns with hyperentangled photons. The paper begins with the main concept of the experiment and then it is shown, how a hyperentangled state arises from the indistinguishability of identical photons. Furthermore, a detailed theoretical analysis of quantum imaging is presented. In the experiment, hyperentangled photons are produced by a typeII SPDC source and each polarisation sensitive phase pattern is imaged from a distance 16.91 m with the ICCD camera. In this type of coincidence imaging, polarisation entanglement and momentum entanglement of photons are involved. Images of patterns are constructed after background correction by accumulating coincidence photons on the ICCD camera for different measurement settings for both photons. In a diagonal basis, image levels are inverted if a measured outcome of polarisation state of photon1 is changed from \(d^{}\rangle _{1}\) to \(d^{+}\rangle _{1}\). Edges of the pattern are not captured because of the diffraction limit of the telescope. Eventually, lowlevel regions corresponding to edges appear in a twophoton captured image. Which is experimentally shown in detail. If photon1 is measured in a quantum state \(H\rangle _{1}\) then photon2 collapses to a quantum state \(V\rangle _{2}\), which is unaffected by the spatial light modulator and it leads to no pattern in the image. A single photon accumulation of photon2 on the camera by continuous exposure without considering photon1 produces a shallow image of the edges due to the diffraction limit of the telescope, which contains partial information of the pattern.
Methods
Experimental setup
Hyperentangled photons are produced by a typeII SPDC process in a first BBO crystal, which is a negative uniaxial crystal. A focused pump laser beam of extraordinary polarisation is incident on the crystal. Crystal is tuned such that the emission cones of ordinary and extraordinary polarised photons are intersecting. Hyperentanglement is produced in the intersection regions. Down converted photons at wavelength 810 nm are passed through a halfwave plate to interchange their linear polarisation. A second crystal of half thickness is placed parallel to the first crystal with a same orientation of its optic axis as the first crystal. This crystal compensates for transverse and longitudinal walkoffs of down converted photons. The source is aligned to produce an antisymmetric polarisation entangled state \(\Psi ^\rangle _{p}\) and a momentum entangled state. In a position basis, the momentum entangled photons are spatially entangled. Momentum entanglement is a result of the linear momentum conservation of photons. Photons are polarisation entangled and momentum entangled separately. Photon1 and photon2 of an entangled pair are passed through two polarisers aligned with their pass axes subtending angles \(\delta _{1}\) and \(\delta _{2}\) with the horizontal direction. The photons transmitted by the polarisers are passed through bandpass filters of peak transmission at 810 nm. To check polarisation entanglement, the photons are then detected by single photon detectors where single photon counts of each photon detector and coincidence photon counts are measured by a coincidence event counting module. However, to image the pattern the experimental setup is shown in Fig. 2.
Violation of CHSH inequality
Einstein’s locality condition strictly forbids the faster than light influence. Consider two polarisation entangled photons separated by a large distance. Any measurement performed on one photon should not affect the measurement outcome of the other photon immidiately if the locality condition is true. Consider two different observables \(A_{1}\) and \(A'_{1}\) of photon1 where any one of them is measured for a photon pair. Similarly, any one of the two different observables \(B_{2}\) and \(B'_{2}\) of photon2 is measured for a photon pair. A measured observable outcome corresponds to a polarisation measurement of a photon. A measurement outcome corresponds to one of the two orthogonal polarisations with measured value \(+1\) for one polarisation and \(1\) for the other. In the local realistic model, the values of all such observables are welldefined prior to any measurement. Consider a correlation function where each observable can have a value \(+\)1 or − 1, therefore
its value cannot exceed the bound \(\langle C_{l}\rangle \le 2\). However, quantum mechanical observables cannot always have a welldefined value and incompatible observables cannot be measured simultaneously. An observable value is obtained by the measurement as a possible outcome that depends on the quantum state and observable being measured. Quantum mechanics violates local realistic prediction expressed in quantum observables such that
Therefore, the following Clauser, Horne, Shimony and Holt (CHSH) inequality is violated by quantum mechanics^{48}
Expectation value of each term of product of observables in Eq. (11) can be evaluated from coincidence photon counts \(C(\delta _{1}, \delta _{2})\) measured for a corresponding orientation of pass axes of polarisers and from the coincidence photon counts \(C(\delta ^{\perp }_{1}, \delta ^{\perp }_{2})\) where \(\delta ^{\perp }_{j}=\delta _{j}+90^{\circ }\)^{10}. The CHSH inequality is violated for the polarisation entanglement. A plot of coincidence photon counts measurements is shown in Fig. 6 for different orientations of polarisers. The CHSH correlation parameter S, Eq. (11), is expressed in the form of angle of pass axes of polarisers as
which is evaluated from the coincidence photon measurements. Where \(E(\delta _{1},\delta _{2})\) represents an expectation value of the joint observable measurements performed on both photons, which is written as
A measured value of parameter \(S=2.66\) where \(0\le S\le 2\) for a local realistic model, thus CHSH inequality is violated. The CHSH inequality is also violated by taking coincidence photon measurements of observables with the ICCD camera gated by the single photon detector signal.
Spatial correlations
In the regions of the intersection of cones, the down converted photons are diverging and are spatially correlated in the transverse planes as a consequence of their spatial entanglement. These correlations are a result of momentum entanglement of photons which is represented by \(\Phi _{12}(r_{a};r_{b})\) in Eq. (4). Spatial entanglement correlates locations of photons. It is due to the spread of photons wavefunction the whole pattern is exposed by a single photon. Once a location of a photon is determined on the pattern its information is shared with the other photon due to their spatial correlations thus each photon carries the spatial location information of the other photon. Position correlations are measured in two planes oriented perpendicular to the mean direction of propagation of each photon. A singleslit of width 0.8 mm is placed at a distance \(d_{1}=1.247\) m, immediately in front of a convex lens \(L_{o}\), where the lens is placed in front of a narrow area single photon detector such that the detector is almost at its focal point. The length of the slit is very large as compared to its width. Polariser1 and polariser2 are removed from paths of photons and the remaining setup is the same as shown in Fig. 2.
If the singleslit is oriented horizontally and photon1 is passed through it and detected then a vertical position of photon1 is measured with a precision equals to the slit width because photon1 is detected only if it is transmitted by the slit. However, this measurement does not measure horizontal position because of large length of the slit in the horizontal direction. Similarly, a corresponding mean position of photon2 is measured on the ICCD camera, which corresponds to a measured mean position of photon2 on the spatial light modulator placed at \(d_{2}=0.89\) m reduced by 0.52 due to the image demagnification of the telescope. Mean vertical positions of photon1 and photon2 are measured after repeating the experiment for different vertical displacements of the singleslit. Correlation between the mean vertical positions of photon1 and of photon2 is shown in Fig. 7a. Similar measurements are performed when a singleslit is oriented vertically and displaced horizontally. This setting performs a horizontal position measurement of photon1 with a resolution equals to the slit width. Mean horizontal position of photon1 and of photon2 are measured by repeating the experiment for each horizontal displacement of the singleslit. A corresponding correlation of mean positions of photons is shown in Fig. 7b. The telescope demagnification is 0.52 and distances \(d_{1}\) and \(d_{2}\) are different in the position correlation plots. For \(d_{1}=d_{2}\) and after taking into account the demagnification, the measured mean position of photon1 is equal and opposite to the measured mean position of photon2 in the transverse planes.
Classical and quantum imaging
Most of the imaging methods in everyday applications are based on classical imaging. These methods utilise properties of classical fields such as intensity, polarisation, phase, frequency and coherence. In the case of optical imaging, classical fields are electromagnetic wave fields. If more than one electromagnetic wave fields are involved then a classical image can be constructed by correlating their classical observable properties. This type of imaging technique, which is known as classical coincidence imaging, has many applications in biomedical imaging and astronomy. A classical ghost imaging is also a coincidence imaging technique, where only one electromagnetic field interacts with the object and its intensity is measured positionwise while the other electromagnetic wave is detected by a bucket detector. Most of these imaging methods can image absorptive objects only. A pure phase object is transparent and cannot be imaged by such methods. However, a method of phasecontrast imaging, which transforms a phase variation to intensity variation across the object is used to image a pure phase object. A phasecontrast microscope can see transparent microorganisms and transparent objects. Such a method can also image a BoseEinstein condensate nondestructively. In addition, a transparent polarisation sensitive phase object can be imaged with a polarisationcontrast microscope^{1,6,7}, which measures the polarisation shift caused by the object. However, quantum imaging methods are based on the quantum mechanical properties of photons originating from their polarisation quantum states, their quantum entanglement and quantum coherence. Quantum entanglement enhanced resolution microscope can image microscopic structures beyond the diffraction limit^{49}. Quantum image construction also depends on how measurements are performed on each photon since incompatible observables can not be measured simultaneously. In experiments presented in this paper, two joint measurements of compatible observables are performed on each photon since they are hyper entangled in two different degrees of freedom. The first measurement is polarisation measurement in a chosen polarisation basis and the second measurement corresponds to a measurement of the momentum of the noninteracting photon and position for the interacted photon. The individual photon carries no complete image information and this method can be useful to send images of the polarisation sensitive phase pattern securely and directly over a large distance. The experiment shown in this paper is the first demonstration of quantum imaging with hyperentangled photons over a long path.
References
Oldenbourg, R. A new view on polarization microscopy. Nature 381, 811–812 (1996).
Gajdacz, M. et al. Nondestructive Faraday imaging of dynamically controlled ultracold atoms. Rev. Sci. Instrum. 84, 083105 (2013).
Baumann, B. Polarization sensitive optical coherence tomography: A review of technology and applications. Appl. Sci. (2017).
Zhang, Y. et al. Widefield imaging of birefringent synovial fluid crystals using lensfree polarized microscopy for gout diagnosis. Sci. Rep. 6, 28793 (2016).
Palmer, B. A. et al. Xray birefringence imaging. Science 344, 1013–1016 (2014).
Massoumian, F., Juškaitis, R., Neil, M. A. A. & Wilson, T. Quantitative polarized light microscopy. J. Microsc. 209, 13–22 (2003).
Wang, Z., Millet, L. J., Gillette, M. U. & Popescu, G. Jones phase microscopy of transparent and anisotropic samples. Opt. Lett. 33, 1270–1272 (2008).
Barreiro, J. T., Langford, N. K., Peters, N. A. & Kwiat, P. G. Generation of hyperentangled photon pairs. Phys. Rev. Lett. 95, 260501 (2005).
Graham, T. M., Bernstein, H. J., Wei, T.C., Junge, M. & Kwiat, P. G. Superdense teleportation using hyperentangled photons. Nat. Commun. 6, 7185 (2015).
Kwiat, P. G. et al. New highintensity source of polarizationentangled photon pairs. Phys. Rev. Lett. 75, 4337–4341 (1995).
Zeilinger, A. Experiment and the foundations of quantum physics. Rev. Mod. Phys. 71, S288–S297 (1999).
Horne, M. A., Shimony, A. & Zeilinger, A. Twoparticle interferometry. Phys. Rev. Lett. 62, 2209–2212 (1989).
Jaeger, G., Horne, M. A. & Shimony, A. Complementarity of oneparticle and twoparticle interference. Phys. Rev. A 48, 1023–1027 (1993).
Mandel, L. Quantum effects in onephoton and twophoton interference. Rev. Mod. Phys. 71, S274–S282 (1999).
Howell, J. C., Bennink, R. S., Bentley, S. J. & Boyd, R. W. Realization of the Einstein–Podolsky–Rosen paradox using momentum and positionentangled photons from spontaneous parametric down conversion. Phys. Rev. Lett. 92, 210403 (2004).
Kaur, M. & Singh, M. Quantum doubledoubleslit experiment with momentum entangled photons. Sci. Rep. 10, 11427 (2020).
Zernike, F. Phase contrast, a new method for the microscopic observation of transparent objects. Physica 9, 686–698 (1942).
Zernike, F. Phase contrast, a new method for the microscopic observation of transparent objects part ii. Physica 9, 983–986 (1942).
Zernike, F. How I discovered phase contrast. Science 121, 345–349 (1955).
Andrews, M. R. et al. Nondestructive observation of a Bose condensate. Science 273, 84–87 (1996).
Andrews, M. R. et al. Direct nondestructive imaging of magnetization in a spin1 BoseEinstein gas. Phys. Rev. Lett. 95, 050401 (2005).
Pittman, T. B., Shih, Y. H., Strekalov, D. V. & Sergienko, A. V. Optical imaging by means of twophoton quantum entanglement. Phys. Rev. A 52, R3429–R3432 (1995).
Gatti, A., Brambilla, E., Bache, M. & Lugiato, L. A. Ghost imaging with thermal light: Comparing entanglement and classical correlation. Phys. Rev. Lett. 93, 093602 (2004).
Abouraddy, A. F., Saleh, B. E. A., Sergienko, A. V. & Teich, M. C. Role of entanglement in twophoton imaging. Phys. Rev. Lett. 87, 123602 (2001).
D’Angelo, M., Kim, Y.H., Kulik, S. P. & Shih, Y. Identifying entanglement using quantum ghost interference and imaging. Phys. Rev. Lett. 92, 233601 (2004).
Aspden, R. S., Tasca, D. S., Boyd, R. W. & Padgett, M. J. EPRbased ghost imaging using a singlephotonsensitive camera. New J. Phys. 15, 073032 (2013).
Gatti, A., Brambilla, E. & Lugiato, L. Quantum imaging. Prog. Opt. 51, 251–348 (2008).
Pittman, T. B., Shih, Y. H., Strekalov, D. V. & Sergienko, A. V. Optical imaging by means of twophoton quantum entanglement. Phys. Rev. A 52, R3429 (1995).
Shapiro, J. H. Computational ghost imaging. Phys. Rev. A 78, 061802(R) (2008).
Ghalaii, M., Afsary, M., Alipour, S. & Rezakhani, A. T. Quantum imaging as an ancillaassisted process tomography. Phys. Rev. A 94, 042102 (2016).
Gatti, A., Brambilla, E. & Lugiato, L. A. Entangled imaging and waveparticle duality: From the microscopic to the macroscopic realm. Phys. Rev. Lett. 90, 133603 (2003).
Lemos, G. B. et al. Quantum imaging with undetected photons. Nature 512, 409–412 (2014).
Lahiri, M., Lapkiewicz, R., Lemos, G. B. & Zeilinger, A. Theory of quantum imaging with undetected photons. Phys. Rev. A 92, 013832 (2015).
Moreau, P.A. et al. Imaging belltype nonlocal behavior. Sci. Adv. (2019).
Moreau, P.A., Toninelli, E., Gregory, T. & Padgett, M. J. Imaging with quantum states of light. Nat. Rev. Phys. 1, 367–380 (2019).
Khakimov, R. I. et al. Ghost imaging with atoms. Nature 540, 100–103 (2016).
Hodgman, S. S., Bu, W., Mann, S. B., Khakimov, R. I. & Truscott, A. G. Higherorder quantum ghost imaging with ultracold atoms. Phys. Rev. Lett. 122, 233601 (2019).
Altuzarra, C. et al. Imaging of polarizationsensitive metasurfaces with quantum entanglement. Phys. Rev. A 99, 020101 (2019).
Einstein, A., Podolsky, B. & Rosen, N. Can quantummechanical description of physical reality be considered complete?. Phys. Rev. 47, 777–780 (1935).
Horne, M. A. & Zeilinger, A. Microphysical Reality and Quantum Formalism (Kluwer Academic, Dordrecht, 1988).
Horne, M. A. Experimental Metaphysics (Kluwer Academic, Dordrecht, 1997).
Monken, C. H., Ribeiro, P. H. S. & Pádua, S. Transfer of angular spectrum and image formation in spontaneous parametric downconversion. Phys. Rev. A 57, 3123–3126 (1998).
Walborn, S. P., de Oliveira, A. N., Thebaldi, R. S. & Monken, C. H. Entanglement and conservation of orbital angular momentum in spontaneous parametric downconversion. Phys. Rev. A 69, 023811 (2004).
Walborn, S. P., Monken, C., Pádua, S. & Souto Ribeiro, P. Spatial correlations in parametric downconversion. Phys. Rep.495, 87–139 (2010).
Schneeloch, J. & Howell, J. C. Introduction to the transverse spatial correlations in spontaneous parametric downconversion through the biphoton birth zone. J. Opt. 18, 053501 (2016).
Joobeur, A., Saleh, B. E. A., Larchuk, T. S. & Teich, M. C. Coherence properties of entangled light beams generated by parametric downconversion: Theory and experiment. Phys. Rev. A 53, 4360–4371 (1996).
Hong, C. K. & Mandel, L. Theory of parametric frequency down conversion of light. Phys. Rev. A 31, 2409 (1985).
Clauser, J. F., Horne, M. A., Shimony, A. & Holt, R. A. Proposed experiment to test local hiddenvariable theories. Phys. Rev. Lett. 23, 880–884 (1969).
Ono, T., Okamoto, R. & Takeuchi, S. An entanglementenhanced microscope. Nat. Commun. 4, 2426 (2013).
Acknowledgements
Mandip Singh acknowledges research funding by the Department of Science and Technology, Quantum Enabled Science and Technology grant for project No. Q.101 of theme title “Quantum Information Technologies with Photonic Devices”, DST/ICPS/QuST/Theme1/2019 (General).
Author information
Authors and Affiliations
Contributions
M.S. conceptualised the idea and setup the experiment. Both authors performed the experiment. M.K. took data. M.S. wrote the manuscript and supervised the project.
Corresponding author
Ethics declarations
Competing interests
The authors declare no competing interests.
Additional information
Publisher's note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.
About this article
Cite this article
Kaur, M., Singh, M. Quantum imaging of a polarisation sensitive phase pattern with hyperentangled photons. Sci Rep 11, 23636 (2021). https://doi.org/10.1038/s4159802102650z
Received:
Accepted:
Published:
DOI: https://doi.org/10.1038/s4159802102650z
This article is cited by

Subtomographic imaging of a polarisation sensitive phase pattern localised in phase space
Scientific Reports (2024)

Quantum ghost imaging of a transparent polarisation sensitive phase pattern
Scientific Reports (2022)
Comments
By submitting a comment you agree to abide by our Terms and Community Guidelines. If you find something abusive or that does not comply with our terms or guidelines please flag it as inappropriate.